• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Dynamic Analysis of Fatigue Behavior in Lead-free Niobate Piezoceramics

Research Project

Project/Area Number 16H04495
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Inorganic materials/Physical properties
Research InstitutionNagoya Institute of Technology

Principal Investigator

KAKIMOTO Ken-ichi  名古屋工業大学, 工学(系)研究科(研究院), 教授 (40335089)

Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥17,810,000 (Direct Cost: ¥13,700,000、Indirect Cost: ¥4,110,000)
Fiscal Year 2018: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Fiscal Year 2017: ¥6,890,000 (Direct Cost: ¥5,300,000、Indirect Cost: ¥1,590,000)
Fiscal Year 2016: ¥7,670,000 (Direct Cost: ¥5,900,000、Indirect Cost: ¥1,770,000)
Keywords環境材料 / セラミックス / 電子・電気材料 / 無鉛圧電体 / 疲労
Outline of Final Research Achievements

Dynamic fatigue phenomena of niobium-based lead-free piezoelectric ceramics under harsh conditions mixing of temperature, electrical field, mechanical load, was characterized by using the inverse method incorporating the protocol in finite element analysis, high-power impedance spectroscopy capable of applying electric field over coercive field and soft X-ray spectroscopy capable of analyzing chemical bonding state. In addition to the effect by the grain/domain structure, it was also clarified that the reduction in the Nb-O bonding energy and the resultant ionic polarization contributed to the deterioration of the piezoelectric properties.

Academic Significance and Societal Importance of the Research Achievements

本研究では産業要請が強い圧電材料の無鉛化および高負荷耐性化に向けて、高負荷環境下での圧電諸物性における疲労特性やこれに及ぼす各構造階層の役割について、従前には報告例が乏しい新たな分析・解析手法によって、定性および定量的に精密評価した。その結果、環境対応の思想がまず先行した無鉛圧電材料において、実用化に繋がる本質的な基盤研究が進み、環境調和性を有する高性能無鉛圧電体の材料設計指針を得るなど重要な知見を得た。

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (39 results)

All 2019 2018 2017 2016 Other

All Int'l Joint Research (3 results) Journal Article (7 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 7 results,  Open Access: 2 results,  Acknowledgement Compliant: 4 results) Presentation (29 results) (of which Int'l Joint Research: 9 results,  Invited: 4 results)

  • [Int'l Joint Research] University of Erlangen-Nuremberg(ドイツ)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Univ. Erlangen-Nuremberg(ドイツ)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Univ. Erlangen-Nuremberg(ドイツ)

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Analyses for oxygen vacancies in (Na,K)NbO3-series piezoelectric ceramics by soft x-ray emission spectroscopy2019

    • Author(s)
      Tanaka Kiyotaka、Takatsuka Sayaka、Nishiyama Hiroshi、Kakimoto Ken-ichi
    • Journal Title

      AIP Advances

      Volume: 9 Issue: 4 Pages: 045102-045102

    • DOI

      10.1063/1.5089533

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] High-power impedance spectroscopy for lead-free alkali niobate piezoceramics2017

    • Author(s)
      Nishiyama Hiroshi、Kakimoto Ken-ichi、Hatano Keiichi、Konishi Yukihiro
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 56 Issue: 10S Pages: 10PD07-10PD07

    • DOI

      10.7567/jjap.56.10pd07

    • NAID

      210000148375

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ferroelastic behavior across the orthorhombic-to-tetragonal phase transition region of NKN-based lead-free ferroelectrics2017

    • Author(s)
      Martin Alexander、Kakimoto Ken-ichi、Hatano Keiichi、Doshida Yutaka、Webber Kyle G.
    • Journal Title

      Journal of Applied Physics

      Volume: 122 Issue: 20 Pages: 204102-204102

    • DOI

      10.1063/1.4989759

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Temperature Dependence of Mechanical Degradation in Lead-free Alkali Niobate Ceramics under Unipolar Loading2016

    • Author(s)
      A. Martin, K. Kakimoto, K. Hatano, Y. Doshida
    • Journal Title

      Mater. Lett.

      Volume: 175 Pages: 300-304

    • DOI

      10.1016/j.matlet.2016.03.103

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Temperature dependence of unipolar fatigue behavior of lead-free alkali niobate ceramics2016

    • Author(s)
      A. Martin, K. Kakimoto, K. Hatano, Y. Doshida
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: 124 Issue: 6 Pages: 730-736

    • DOI

      10.2109/jcersj2.15279

    • NAID

      130005155652

    • ISSN
      1348-6535, 1882-0743
    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Determination of Temperature Dependency of Material Parameters for Lead-free Alkali Niobate Piezoceramics by the Inverse Method2016

    • Author(s)
      K. Ogo, K. Kakimoto, M. Weiss, S. J. Rupitsch, R. Lerch
    • Journal Title

      AIP Advances

      Volume: 6 Issue: 6 Pages: 065101-065101

    • DOI

      10.1063/1.4953327

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Determination of Temperature Dependences of Material Constants for Lead-free (Na0.5K0.5)NbO3-Ba2NaNb5O15 Piezoceramics by Inverse Method2016

    • Author(s)
      K. Yoshida, K. Kakimoto, M. Weiss, S. J. Rupitsch, R. Lerch
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 55 Issue: 10S Pages: 10TD02-10TD02

    • DOI

      10.7567/jjap.55.10td02

    • NAID

      210000147189

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Presentation] 疲労したニオブ系圧電セラミックスにおける酸素欠陥の挙動2019

    • Author(s)
      前田晋朔、伊藤雄一朗、柿本健一
    • Organizer
      日本セラミックス協会2019年年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Defect Charge Behavior in the Vicinity of Domain Walls2018

    • Author(s)
      S. Maeda, H. Nishiyama, K. Kakimoto
    • Organizer
      2018 ISAF-FMA-AMF-AMEC-PFM Joint Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Ferroics and Electromechanical Coupling Property for NKN-Based Materials2018

    • Author(s)
      H. Nishiyama, K. Kakimoto, K. Hatano, Y. Konishi, A. Martin, K.G. Webber
    • Organizer
      2018 ISAF-FMA-AMF-AMEC-PFM Joint Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Stress-induced Tetragonal-to-orthorhombic Phase Transition in Lead-Free NKN-based Materials and the Implications for Future Material Design2018

    • Author(s)
      A. Martin, H. Nishiyama, K. Kakimoto, K. Hatano, Y. Doshida, K.G. Webber
    • Organizer
      2018 ISAF-FMA-AMF-AMEC-PFM Joint Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] PFM Observation in the Vicinity of Domain Walls for (Na,K)NbO3 Ceramics2018

    • Author(s)
      S. Maeda, Y. Ito, K. Kakimoto
    • Organizer
      12th Japan-Korea Conference on Ferroelectrics
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] (Li,Na,K)NbO3 圧電セラミックスの焼結組織と絶縁特2018

    • Author(s)
      永松野愛、柿本健一
    • Organizer
      日本セラミックス協会第31回秋季シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] 圧電応答顕微鏡によるドメイン構造評価と酸素欠陥2018

    • Author(s)
      前田晋朔、西山 拡、柿本健一
    • Organizer
      日本セラミックス協会第31回秋季シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] 繰り返し使用したニオブ系無鉛積層圧電材料の交流インピーダンス特性2018

    • Author(s)
      西山 拡、柿本健一、波多野 桂一、小西 幸宏、A. Martin、K. Webber
    • Organizer
      日本セラミックス協会第31回秋季シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] Zr4+ Acceptor Doped Alkari Niobate Piezoceramics and electrical Fatigue2018

    • Author(s)
      Y. Ito, H. Nishiyama, K. Kakimoto
    • Organizer
      10th Japan-China Symposium on Ferroelectric Materials and Their Applications
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] ユニポーラ電界駆動したニオブ系圧電セラミックスの疲労特性2018

    • Author(s)
      伊藤雄一朗、前田晋朔、柿本健一
    • Organizer
      第38回エレクトロセラミックス研究討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 圧電セラミックスのPFM観察と疲労現象2018

    • Author(s)
      前田晋朔、伊藤雄一朗、柿本健一
    • Organizer
      2018年度日本セラミックス協会東海支部学術研究発表
    • Related Report
      2018 Annual Research Report
  • [Presentation] ニオブ系無鉛圧電材料のフェロイクスと電気機械物性2018

    • Author(s)
      西山 拡、柿本健一、波多野桂一、小西幸宏、A. Martin、K. Webber
    • Organizer
      日本セラミックス協会2018年年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 圧電応答顕微鏡によるニオブ系圧電材料のChargedドメイン壁観察2018

    • Author(s)
      前田晋朔、西山 拡、柿本健一
    • Organizer
      日本セラミックス協会2018年年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 高負荷環境下におけるニオブ系無鉛圧電セラミックスの繰り返し電界疲労特性2018

    • Author(s)
      伊藤雄一朗、西山 拡、柿本健一
    • Organizer
      日本セラミックス協会2018年年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] アクセプタイオンを置換固溶させたニオブ系無鉛圧電セラミックスの疲労特性2017

    • Author(s)
      高塚清香、西山 拡、田中清高、渕上輝顕、柿本健一
    • Organizer
      日本セラミックス協会2017年年会
    • Place of Presentation
      東京
    • Year and Date
      2017-03-17
    • Related Report
      2016 Annual Research Report
  • [Presentation] Technical Challenges in Lead-free Alkali Niobate Piezoceramics2017

    • Author(s)
      K. Kakimoto
    • Organizer
      12th Pacific Rim Conference on Ceramic and Glass Technology
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] High-power Impedance Spectroscopy for Fatigued Alkali Niobate Piezoelectronics2017

    • Author(s)
      H. Nishiyama, K. Kakimoto, K. Hatano, Y. Konishi
    • Organizer
      8th International Conference on Electroceramics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] ニオブ系無鉛圧電セラミックスのハイパワーインピーダンス特性2017

    • Author(s)
      西山 拡、柿本健一、波多野桂一、小西幸宏
    • Organizer
      第34回強誘電体応用会議
    • Related Report
      2017 Annual Research Report
  • [Presentation] ニオブ系強誘電体セラミックスの特異な強弾性挙動2017

    • Author(s)
      西山 拡、柿本健一、波多野桂一、小西幸宏、A. Martin、K. Webber
    • Organizer
      日本セラミックス協会第30回秋季シンポジウム
    • Related Report
      2017 Annual Research Report
  • [Presentation] 圧縮応力下におけるニオブ系無鉛圧電セラミックスの強弾性挙動と誘電特性2017

    • Author(s)
      西山 拡、柿本健一、波多野桂一、小西幸宏、A. Martin、K. Webber
    • Organizer
      第37回エレクトロセラミックス研究討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Recent Progress in Lead-free Alkali Niobate Piezoceramics2017

    • Author(s)
      K. Kakimoto
    • Organizer
      JSPM International Conference on Powder and Powder Metallurgy - 60th Anniversary -
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] ニオブ系無鉛圧電セラミックスの電気的耐圧特性2017

    • Author(s)
      永松野愛、西山 拡、柿本健一
    • Organizer
      日本セラミックス協会平成29年度東海支部学術研究発表会
    • Related Report
      2017 Annual Research Report
  • [Presentation] ハイパワー駆動を想定したニオブ系無鉛圧電体材料のインピーダンス特性2017

    • Author(s)
      西山 拡、柿本健一、波多野桂一、小西幸宏
    • Organizer
      日本セラミックス協会平成29年度東海支部学術研究発表会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Material Design of Alkaline Niobate Piezoceramics for Sensor and Energy Application2016

    • Author(s)
      K. Kakimoto
    • Organizer
      8th Japan-China Symposium on Ferroelectric Materials and Their Applications
    • Place of Presentation
      Tsukuba, Japan
    • Year and Date
      2016-09-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] ニオブ系無鉛圧電材の構造制御およびエネルギー応用2016

    • Author(s)
      柿本健一
    • Organizer
      日本セラミックス協会第29回秋季シンポジウム
    • Place of Presentation
      広島
    • Year and Date
      2016-09-07
    • Related Report
      2016 Annual Research Report
    • Invited
  • [Presentation] ニオブ系無鉛圧電材料の高電界交流インピーダンス特性2016

    • Author(s)
      西山 拡、柿本健一、波多野桂一、小西幸宏
    • Organizer
      日本セラミックス協会第29回秋季シンポジウム
    • Place of Presentation
      広島
    • Year and Date
      2016-09-07
    • Related Report
      2016 Annual Research Report
  • [Presentation] インバース法を用いた(Na0.5K0.5)NbO3-Ba2NaNb5O15の圧電特性評価2016

    • Author(s)
      吉田克也、柿本健一
    • Organizer
      第33回強誘電体応用会議
    • Place of Presentation
      京都
    • Year and Date
      2016-05-25
    • Related Report
      2016 Annual Research Report
  • [Presentation] 疲労した圧電セラミックスのハイパワーインピーダンス測定2016

    • Author(s)
      西山 拡、柿本健一、波多野桂一、小西幸宏
    • Organizer
      平成28年度日本セラミックス協会東海支部学術研究発表会
    • Place of Presentation
      名古屋
    • Related Report
      2016 Annual Research Report
  • [Presentation] ニオブ系無鉛圧電セラミックスの元素置換と疲労特性2016

    • Author(s)
      高塚清香、西山 拡、渕上輝顕、柿本健一
    • Organizer
      平成28年度日本セラミックス協会東海支部学術研究発表会
    • Place of Presentation
      名古屋
    • Related Report
      2016 Annual Research Report

URL: 

Published: 2016-04-21   Modified: 2020-03-30  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi