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Development of New Analyzing Method of Excited States Using Combination of Soft X-Rays and Laser

Research Project

Project/Area Number 17360022
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionSaga University

Principal Investigator

KAMADA Masao  Saga University, Synchrotron Light Application Center, Professor (60112538)

Co-Investigator(Kenkyū-buntansha) TAKAHASHI Kazutoshi  Saga University, Synchrotron Light Application Center, Lecturer (30332183)
AZUMA Junpei  Saga University, Synchrotron Light Application Center, Research Associate (40372768)
Project Period (FY) 2005 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥16,110,000 (Direct Cost: ¥15,000,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2007: ¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2006: ¥3,300,000 (Direct Cost: ¥3,300,000)
Fiscal Year 2005: ¥8,000,000 (Direct Cost: ¥8,000,000)
KeywordsSynchrotron Light / Time-Resolved Photoelectron Spectroscopy / Excited-State Spectroscopy / Excited-State Dynamics / Semiconductor Surface / Laser Combination Experiments / Two-Photon Excitation / Photo-Voltaic Effect / レーザー組合せ実験 / 超高速分光 / 内殻光電子分光 / 組合せ実験 / 軟X線
Research Abstract

In order to develop the new analyzing method for excited states, we have constructed the ultra-fast time-resolved photoelectron spectroscopy system based on the existing high energy and angle-resolved photoelectron spectrometer and the ultra-fast laser. Using this new system, we have carried out the measurement of the photoelectrons from the excited-states pumped by laser-light. The experimental results were compared with the calculation of the excited states, indicating the performance of the present new spectroscopy. The energy and angle-resolved photoelectron spectroscopy has been conducted on Ag/Si surfaces. The obtained energy dispersion curves of the bands indicate clearly the validity of the present new spectroscopy. We have also installed the planar undulator to obtain the higher brilliant synchrotron light and tuned up the monochromator system for combination experiments using synchrotron light and laser that have advantage in the high repetition frequency. We have constructed the new two-photon photoelectron spectroscopy system. Using this system we have successfully measured the ultra-fast time-resolved photoelectron spectra on n-and p-type GaAs. The result is very interesting and attractive to investigate the dynamics of the surface photo-voltage effect. A part of the results obtained in the present project has been reported in the international conference and Journals.

Report

(4 results)
  • 2007 Annual Research Report   Final Research Report Summary
  • 2006 Annual Research Report
  • 2005 Annual Research Report
  • Research Products

    (28 results)

All 2008 2007 2006 2005 Other

All Journal Article (18 results) (of which Peer Reviewed: 8 results) Presentation (8 results) Book (1 results) Remarks (1 results)

  • [Journal Article] Ultrafast Time Dependence of Surface Photo-Voltage Effect on p-type GaAs(100)Sufrace2008

    • Author(s)
      S. Tokudomi, J. Azuma, K. Takahashi, M. Kamada
    • Journal Title

      Journal of Physical Society of Japan 77

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Ultrafast Time Dependence of Surface Photo-Voltage Effect on p-type GaAs(100) Surface2008

    • Author(s)
      S., Tokudomi, J., Azuma, K., Takahashi, M., Kamada
    • Journal Title

      Journal of Physical Society of Japan 77

    • NAID

      110006594917

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Ultrafast Time Dependence of Surface Photo-Voltage Effect on p-type GaAs(100) Surface2008

    • Author(s)
      S.Tokudomi, J.Azuma, K.Takahashi and M.Kamada
    • Journal Title

      Journal of Physical Society of Japan 77

    • NAID

      110006594917

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ultrafast Decay of Surface Photo-Voltage Effect on n-type GaAs(100)Surface2007

    • Author(s)
      S. Tokudomi, J. Azuma, K. Takahashi, M. Kamada
    • Journal Title

      Journal of Physical Society of Japan 76

    • NAID

      110006448324

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] 「研究成果報告書概要(和文)」より2007

    • Author(s)
      K. Takahashi, J. Azuma, S. Tokudomi, M. Kamada
    • Journal Title

      Proc.of Int.Conf.on Synchrotron Radiation Instrumentation 879

    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Ultrafast Decay of Surface Photo-Voltage Effect on n-type GaAs(100)Surface2007

    • Author(s)
      S., Tokudomi, J., Azuma, K., Takahashi, M., Kamada
    • Journal Title

      Journal of Physical Society of Japan 76

    • NAID

      110006448324

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Development of the Experimental System for Time- and Angle-resolved Photoemission Spectroscopy2007

    • Author(s)
      K., Takahashi, J., Azuma, S., Tokudomi, M., Kamada
    • Journal Title

      Proc. of Int. Conf. on Synchrotron Radiation Instrumentation 879

      Pages: 1218-1221

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Soft X-ray Beamlines for Industry application in Saga2007

    • Author(s)
      M., Kamada, et. al.
    • Journal Title

      Proc. of Int. Conf. on Synchrotron Radiation Instrumentation 879

      Pages: 623-626

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article]2007

    • Author(s)
      S.Tokudomi, J.Azuma, K.Takahashi and M.Kamada
    • Journal Title

      Journal of Physical Spciety of Japan 76

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Development of the Experimental System for Time-and Angle-resolved Photoemission Spectroscopy2007

    • Author(s)
      K.Takahashi, J.Azuma, S.Tokudomi, M.Kamada
    • Journal Title

      Proc.of Int.Conf.on Synchrotron Radiation Instrumentation 879

      Pages: 1218-1221

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Core exciton migration in Rb^<0.82>Cs^<0.18>Cl under excitation with synchrotron radiation and laser light2007

    • Author(s)
      T.Tsujibayashi, J.Azuma, Y.Inabe, K.Toyoda, M.Kamada, M. Itoh
    • Journal Title

      Journal of Luminescence 122/123

      Pages: 899-904

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Soft X-ray Beamlines for Industry application in Saga2007

    • Author(s)
      M.Kamada, et. al.
    • Journal Title

      Journal of Luminescence 879

      Pages: 623-626

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Infrared Absorption changein single-walled carbon nanotubes observed by combination spectroscopy of SR and laser2007

    • Author(s)
      Junpei Azuma, Minoru Itoh, Masahiro Koike, Masao Kamada, Morinobu Endo
    • Journal Title

      Journal of Synchrotron Radiation 13

      Pages: 464-464

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Laser-induced infrared absorption in lead tungstate observed by laser-SR combined spectroscopy2006

    • Author(s)
      M.Itoh, J.Azuma, T.Shimizu, M.Kamada, M.Kobayashi, Y.Usuki
    • Journal Title

      J. Luminescence 119/120

      Pages: 590-590

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Present Atatus and Future Prospect of Saga Synchrotron Light Project2006

    • Author(s)
      Masao Kamada, Kazutoshi Takashima, Jyunpei Azuma, Tooru Tanaka, Hiroshi Ogawa
    • Journal Title

      Proc. of Progress in Electromagnetics Research Symposium 2006 2006

      Pages: 164-164

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Beamline for high-resolution angle-resolved photoemission at Saga Light Source2005

    • Author(s)
      K.Takahashi, Y.Kondo, J.Azuma, M.Kamada
    • Journal Title

      Journal of Electron Spectroscopy and Related Phenomena, 144/147

      Pages: 1093-1093

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Two-Photon Spectroscopy of Core Excitons in Barium Fluoride Using Synchrotron Radiation and Laser Light2005

    • Author(s)
      Toru Tsujibayashi, Minoru Itoh, Junpei Azuma, Masayuki Watanabe, Osamu Arimoto, Shunsuke Nakanishi, Hiroshi Itoh, Masao Kamada
    • Journal Title

      Phys.Rev.Lett. 94

      Pages: 76401-76401

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Core exciton migration in Rb_<0.82>Cs_<0.18>Cl under excitation with synchrotron radiation and laser light

    • Author(s)
      T., Tsujibayashi, J., Azuma, Y., Inabe, K., Toyoda, M., Kamada, M., Itoh
    • Journal Title

      Journal of Luminescence

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Potoelectron Spectroscopy of L-Cystein2008

    • Author(s)
      M., Kamada, S., Kitagima, H., Sugiyama, J., Azuma, K., Takahashi, S., Fujimoto
    • Organizer
      Annual Meeting of Physical Society of Japan
    • Place of Presentation
      Osaka
    • Year and Date
      2008-03-24
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] アミノ酸システィシの光電子分析2008

    • Author(s)
      鎌田、 北島、 杉山、東、高橋、 隅本、 藤本
    • Organizer
      日本物理学会
    • Place of Presentation
      近畿大学
    • Year and Date
      2008-03-24
    • Related Report
      2007 Annual Research Report
  • [Presentation] Potoelectron Study of Butterfly Template ZnO2008

    • Author(s)
      M., Kamada, H., Sugiyama, J., Azuma, K., Takahashi, Di, Zhang, Q., Guo
    • Organizer
      Annual Meeting of Japanese Society of Synchrotron Radiation Research
    • Place of Presentation
      Kusatsu
    • Year and Date
      2008-01-12
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Excited Carrier Dynamics on Semiconductor Surfaces Using Multi-Photon Potoelectron Spectroscopy2007

    • Author(s)
      M., Kamada
    • Organizer
      Symposium of institute f Solid State Physics of the university of Tokyo
    • Place of Presentation
      Kashiwa
    • Year and Date
      2007-11-27
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Potoelectron Study of Butterfly Template ZnO2007

    • Author(s)
      M. Kamada, H. Sugiyama, J. Azuma, K. Takahashi, Di Zhang, Q. Guo
    • Organizer
      Int.Conf.on Vacuum Ultra-Violet Radiation Physics
    • Place of Presentation
      Berlin
    • Year and Date
      2007-08-04
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Potoelectron Study of Butterfly Template ZnO2007

    • Author(s)
      M., Kamada, H., Sugiyama, J., Azuma, K., Takahashi, Di, Zhang, Q., Guo
    • Organizer
      Int. Conf. on Vacuum Ultra-Violet Radiation Physics
    • Place of Presentation
      Berlin
    • Year and Date
      2007-08-04
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Ultrafast photoemission measurement for Surface Photo-Voltage effect on Cr/n・GaAs(100) surface2007

    • Author(s)
      J., Azuma, S., Nagao, S., Tokudomi, K., Takahashi, M., Kamada
    • Organizer
      Int. Conf. on Vacuum Ultra-Violet Radiation Physics
    • Place of Presentation
      Berlin
    • Year and Date
      2007-08-04
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Present and future programs using synchrotron light in Saga University2007

    • Author(s)
      M., Kamada
    • Organizer
      Joint Seminar between Saga University Synchrotron Light Application Center and State Key Lab of Metal Matrix Composites Shanghai Jiaotong University on Material Science and Synchrotron Light
    • Place of Presentation
      Shanghai
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Book] 光物性の基礎(放射光分光)2006

    • Author(s)
      鎌田 雅夫(分担)
    • Total Pages
      20
    • Publisher
      オプトロニクス社
    • Related Report
      2006 Annual Research Report
  • [Remarks] 「研究成果報告書概要(和文)」より

    • URL

      http://www.slc.saga-u.ac.jp/

    • Related Report
      2007 Final Research Report Summary

URL: 

Published: 2005-04-01   Modified: 2016-04-21  

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