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Low-temperature synthesis of oxynitrides for development of new functional materials

Research Project

Project/Area Number 17H04950
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Inorganic materials/Physical properties
Research InstitutionHokkaido University

Principal Investigator

MIURA Akira  北海道大学, 工学研究院, 准教授 (10603201)

Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥24,310,000 (Direct Cost: ¥18,700,000、Indirect Cost: ¥5,610,000)
Fiscal Year 2019: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2018: ¥6,630,000 (Direct Cost: ¥5,100,000、Indirect Cost: ¥1,530,000)
Fiscal Year 2017: ¥15,730,000 (Direct Cost: ¥12,100,000、Indirect Cost: ¥3,630,000)
Keywords酸窒化物 / 窒化物 / 酸素還元触媒 / 半導体 / メタセシス反応 / 低温合成 / 電気化学触媒 / 電子構造 / 機能性 / 低温反応
Outline of Final Research Achievements

This reserch project aims to propose the new synthesis method for oxynitrides without long heat treatment, and to emerge new functional materials. Our achievement includes the combustion reaction from chloride, oxyhydride and amide to form BaNbO2N and BaTaO2N. Mn incorporation into Mo2N framework changed its electronic structure and improved the catalytic activity toward oxygen reduction reaction.

Academic Significance and Societal Importance of the Research Achievements

本研究では、新規機能性材料を生み出すための新たな合成手法の創出と、酸化物イオンと窒化物イオンを組み合わせた新規材料の創出を目指して研究を行った。その結果、ナトリウムアミドと塩化物、酸水化物の混合によって、光触媒として着目されている酸窒化物ペロブスカイト型を数秒で合成することに成功した。また、新規窒化物であるマンガン―モリブデン窒化物を発見し、マンガンが窒化物格子中にはいることで、電子構造が変化し酸素還元触媒能が向上した。さらに、液相を介した半導体薄膜の機能性向上を目指し、酸化インジウム薄膜の電子移動度の向上に成功した。

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • Research Products

    (29 results)

All 2020 2019 2018 2017 Other

All Int'l Joint Research (2 results) Journal Article (5 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 5 results,  Open Access: 2 results) Presentation (17 results) (of which Int'l Joint Research: 7 results,  Invited: 7 results) Remarks (5 results)

  • [Int'l Joint Research] UC Berkeley/Lawrence Berkeley National Laboratory/University of Michigan(米国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] lawrence berkeley national laboratory(米国)

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Selective metathesis synthesis of MgCr2S4 by control of thermodynamic driving forces2020

    • Author(s)
      Miura Akira、Ito Hiroaki、Bartel Christopher J.、Sun Wenhao、Rosero-Navarro Nataly Carolina、Tadanaga Kiyoharu、Nakata Hiroko、Maeda Kazuhiko、Ceder Gerbrand
    • Journal Title

      Materials Horizons

      Volume: - Issue: 5 Pages: 0-0

    • DOI

      10.1039/c9mh01999e

    • NAID

      120007032609

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Self-Combustion Synthesis of Novel Metastable Ternary Molybdenum Nitrides2019

    • Author(s)
      Jin Odahara, Wenhao Sun, Akira Miura, Nataly Carolina Rosero-Navarro, Masanori Nagao, Isao Tanaka, Gerbrand Ceder, and Kiyoharu Tadanaga
    • Journal Title

      ACS Materials Letters

      Volume: 1 Issue: 1 Pages: 64-70

    • DOI

      10.1021/acsmaterialslett.9b00057

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Synthesis, Crystal Structure and Optical Absorption of NaInS2-xSex2018

    • Author(s)
      Takahashia, Natsuumi; Ito, Hiroaki; Miura, Akira; Rosero-Navarro, Nataly Carolina;Goto, Yosuke; Mizuguchi, Yoshikazu; Moriyoshi, Chikako; Kuroiwa, Yoshihiro; Nagao, Masanori;Watauchi, Satoshi; Tanaka, Isao; Tadanaga, Kiyoharu
    • Journal Title

      Journal of Alloys and Compounds

      Volume: 750 Pages: 409-413

    • DOI

      10.1016/j.jallcom.2018.03.407

    • Related Report
      2018 Annual Research Report 2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Low-temperature synthesis and rational design of nitrides and oxynitrides for novel functional material development2017

    • Author(s)
      Miura, Akira
    • Journal Title

      Journal of the Ceramic Society of Japan

      Volume: 125 Issue: 7 Pages: 552-558

    • DOI

      10.2109/jcersj2.17055

    • NAID

      130006899954

    • ISSN
      1348-6535, 1882-0743
    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Explosive Reaction for Barium Niobium Perovskite Oxynitride2017

    • Author(s)
      Odahara Jin、Miura Akira、Rosero-Navarro Nataly Carolina、Tadanaga Kiyoharu
    • Journal Title

      Inorganic Chemistry

      Volume: 57 Issue: 1 Pages: 24-27

    • DOI

      10.1021/acs.inorgchem.7b02660

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Presentation] Preparation of Cu3N thin films on glass substrate by nitridation of solution process-derived CuO thin film with urea2019

    • Author(s)
      Y. Ohigashi, A. Miura, N. Rosero Navarro, K. Tadanaga
    • Organizer
      25th International Congress on Glasses (ICG2019), Abstract ICG-SI-120-2019 (2019. 6.9-14, Boston, USA).
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 液相法および尿素による窒化を用いたTaON薄膜の作製2019

    • Author(s)
      樋口亜門・三浦章・Nataly Carolina ROSERO NAVARO・鱒渕友治・忠永清治
    • Organizer
      日本化学会北海道支部2019年夏季研究発表会、講演要旨集A01 (2019.7.20).
    • Related Report
      2019 Annual Research Report
  • [Presentation] ナトリウムアミド融液を用いたスピネル型マンガン鉄酸窒化物の低温合成2019

    • Author(s)
      清藤太郎・三浦章・Nataly Carolina ROSERO NAVARO・忠永清治
    • Organizer
      日本化学会北海道支部2019年夏季研究発表会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Preparation of transition metal nitride and oxynitride thin films by nitridation of sol-gel derived oxide thin films with urea2019

    • Author(s)
      K. Tadanaga, Y. Ohigashi, A. Higuchi, N. C. Rosero Navarro and A. Miura
    • Organizer
      The 20th International Sol-Gel Conference
    • Related Report
      2019 Annual Research Report
  • [Presentation] Synthesis of Binary and Ternary Nitrides by Self-Combustion Synthesis using NaNH22019

    • Author(s)
      A. Miura, J. Odahara, N.C. Rosero Navarro, M. Nagao, I. Tanaka, K. Tadanaga
    • Organizer
      The 13th Pacific Rim Conference of Ceramic Societies(PACRIM13)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Molten Salt Synthesis of Chalcogenide Spinels MgIn2S4-2xSe2x (x=0 and 0.5)2019

    • Author(s)
      H. Ito, A. Miura, N.C. ROSERO-NAVARRO, Nataly Y. MIZUGUCHI, Y. GOTO, Y. KUROIWA, C. MORIYOSHI, K. TADANAGA
    • Organizer
      The 13th Pacific Rim Conference of Ceramic Societies(PACRIM13)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 自己燃焼反応による新規マンガンモリブデン窒化物の合成2019

    • Author(s)
      三浦 章・小田原 仁・Nataly Carolina Rosero-Navarro・忠永 清治・長尾 雅則・田中 功
    • Organizer
      日本セラミックス協会2019年年会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Explosive Synthesis of BaNbO2N2018

    • Author(s)
      Akira Miura
    • Organizer
      The 8th Advanced Functional Materials and Devices
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Low-Temperature Synthesis of Nitrides/Oxynitrides and Emerging New Functional Materials by Controlling Electronic Structure2018

    • Author(s)
      A. Miura, N. C. Rosero-Navarro, K. Tadanaga
    • Organizer
      4th Workshop for Materials-Informatics Classic, MSSJ
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] アミド溶液を介した酸化インジウム薄膜への窒素ドープ2018

    • Author(s)
      成瀬 雅浩・三浦 章・Rosero-Navarro Nataly Carolina・伊左治 忠之・前田 真一・藤本 修・忠永 清治
    • Organizer
      日本セラミックス協会第31回秋季シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] Synthesis of Nitrides and Oxynitrides using NaNH2 for Emerging New Functional Materials2018

    • Author(s)
      Akira Miura, Kiyoharu, Tadanaga
    • Organizer
      2018 International Conference of Young Researchers on Advanced Materials
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] BaM(O,N)3 (M=Nb, Ta)の爆発合成2018

    • Author(s)
      小田原仁・三浦章・Nataly Carolina Rosero-Navarro・忠永清治
    • Organizer
      化学系学協会北海道支部2018年冬季研究発表会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 室温窒素プラズマ照射による酸化インジウム薄膜への窒素ドープ手法の開発2017

    • Author(s)
      成瀬雅浩・三浦章・樋口幹雄・忠永清治
    • Organizer
      日本化学会北海道支部2017年夏季研究発表会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Hexane-Assisted Synthesis of BaNbO2N2017

    • Author(s)
      Akira Miura, Jin Odahara, N.C. Rosero-Navarro, Kiyoharu Tadanaga
    • Organizer
      9th International Symposium on Nitrides & International Symposium on SiAlONS and Non-oxides
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] NaNH2を用いたBaNbO2Nの合成2017

    • Author(s)
      小田原仁・三浦章・Nataly Carolina Rosero Navarro・忠永清治
    • Organizer
      平成29年度日本セラミックス協会東北北海道支部研究発表会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 酸化インジウム薄膜の室温プラズマ窒化と電気特性2017

    • Author(s)
      成瀬雅浩・三浦章・Nataly Carolina Rosero Navarro・樋口幹雄・忠永清治
    • Organizer
      平成29年度日本セラミックス協会東北北海道支部研究発表会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Liquid-Phase Synthesis of Energy Materials with Multiple Anions: Mn(O,N) Electrocatalyst and Li6PS5Br Electrolyte2017

    • Author(s)
      Akira Miura, Nataly Carolina Rosero-Navarro, Kiyoharu Tadanaga
    • Organizer
      The 7th Advanced Functional Materials and Devices
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Remarks] リサーチマップ

    • URL

      https://researchmap.jp/amiura/

    • Related Report
      2018 Annual Research Report 2017 Annual Research Report
  • [Remarks] Google Scholar

    • URL

      https://scholar.google.com/citations?hl=en&user=_vPBvrAAAAAJ&view_op=list_works

    • Related Report
      2018 Annual Research Report
  • [Remarks] 無機合成化学研究室

    • URL

      http://www.eng.hokudai.ac.jp/labo/inorgsyn/

    • Related Report
      2017 Annual Research Report
  • [Remarks] 北海道大学研究者総覧

    • URL

      https://researchers.general.hokudai.ac.jp/profile/ja.utqoGJX7-oVpr36A-zjM1Q==.html

    • Related Report
      2017 Annual Research Report
  • [Remarks] Google Scholar

    • URL

      https://scholar.google.co.jp/citations?user=_vPBvrAAAAAJ&hl=en

    • Related Report
      2017 Annual Research Report

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Published: 2017-04-28   Modified: 2021-02-19  

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