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Study on electronic properties of two-dimensional layered materials under high electric field

Research Project

Project/Area Number 17K05500
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics I
Research InstitutionOkayama University

Principal Investigator

Goto Hidenori  岡山大学, 異分野基礎科学研究所, 准教授 (90322669)

Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2019: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2018: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2017: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Keywordsグラフェン / 電界効果 / 二次元層状物質 / バンド制御 / イオン液体 / 電子移動 / 自己組織化単分子膜 / 分子吸着 / 物性実験 / メゾスコピック系 / 低温物性 / マイクロ・ナノデバイス / 2次元電子系
Outline of Final Research Achievements

Purpose of this study is to investigate electronic properties of two-dimensional materials (2DMs) under perpendicular electric field. To produce large homogeneous electric field, we have combined electron transfer method and electrostatic gating method. Using mono-/bi-layer graphene, we found that electron-transfer molecules produced inhomogeneous electric field and degraded the mobility. These disadvantages were solved as follows. First, the ionic liquid gate enabled us to produce homogeneous electric field because the movable ions were arranged to suppress the inhomogeneity. Next, molecules with high symmetry and small size had a tendency not to decrease the mobility. Furthermore, unique electric-field effect was found in doped topological insulator in which the mobility depended on the direction of the electric field.
Our findings are useful for inducing novel electronic phenomena and producing multi-functional 2DM devices under electric field.

Academic Significance and Societal Importance of the Research Achievements

電界下における電子物性の研究には、トポロジカル物質における新規電磁現象のように、未踏の領域が広く残っている。その研究のためには、強く一様な電界の発生方法を開発することが必要である。電子移動および電界効果の2つの方法を用いたわれわれの研究成果により、この課題を解決する方針が見いだされた。これにより、二次元層状物質における新規電子物性の開拓や、自由度の高い電界制御による新たな多機能デバイスの創出が期待される。

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (32 results)

All 2020 2019 2018 2017

All Journal Article (15 results) (of which Int'l Joint Research: 13 results,  Peer Reviewed: 15 results,  Open Access: 7 results) Presentation (16 results) (of which Int'l Joint Research: 9 results,  Invited: 4 results) Book (1 results)

  • [Journal Article] Superconducting behavior of a new metal iridate compound, SrIr2, under pressure2020

    • Author(s)
      Xiaofan Yang, Huan Li, Tong He, Tomoya Taguchi, Yanan Wang, Hidenori Goto, Ritsuko Eguchi, Rie Horie, Kazumasa Horigane, Kaya Kobayashi, Jun Akimitsu, Hirofumi Ishii, Yen Fa Liao, Hitoshi Yamaoka, Yoshihiro Kubozono
    • Journal Title

      Journal of Physics Condensed Matter

      Volume: 32 Issue: 2 Pages: 025704-025704

    • DOI

      10.1088/1361-648x/ab4605

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Inhomogeneous superconductivity in thin crystals of FeSe1-xTex (x=1.0, 0.95, and 0.9)2020

    • Author(s)
      Ritsuko Eguchi, Megumi Senda, Eri Uesugi, Hidenori Goto, Akihiko Fujiwara, Yasuhiko Imai, Shigeru Kimura, Takashi Noji, Yoji Koike, Yoshihiro Kubozono
    • Journal Title

      Materials Research Express

      Volume: 7 Issue: 3 Pages: 036001-036001

    • DOI

      10.1088/2053-1591/ab7c85

    • NAID

      120006825998

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Fabrication of flexible high-performance organic field-effect transistors using phenacene molecules and their application toward flexible CMOS inverters2019

    • Author(s)
      Pompei Emanuela、Turchetti Claudio、Hamao Shino、Miura Akari、Goto Hidenori、Okamoto Hideki、Fujiwara Akihiko、Eguchi Ritsuko、Kubozono Yoshihiro
    • Journal Title

      Journal of Materials Chemistry C

      Volume: 印刷中 Issue: 20 Pages: 6022-6033

    • DOI

      10.1039/c8tc05824e

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Pressure-induced superconductivity in Bi2-xSbxTe3-ySey2019

    • Author(s)
      Tong He, Xiaofan Yang, Tomoya Taguchi, Teppei Ueno, Kaya Kobayashi, Jun Akimitsu, Hitoshi Yamaoka, Hirofumi Ishii, Yen-Fa Liao, Hiromi Ota, Hidenori Goto, Ritsuko Eguchi, Kensei Terashima, Takayoshi Yokoya, Harald O. Jeschke, Xianxin Wu, Yoshihiro Kubozono
    • Journal Title

      PHYSICAL REVIEW B

      Volume: 100 Issue: 9 Pages: 094525-094525

    • DOI

      10.1103/physrevb.100.094525

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Superconducting properties of (NH3) y Li x FeSe0.5Te0.5 under pressure2019

    • Author(s)
      Yang Xiaofan、He Tong、Taguchi Tomoya、Li Huan、Wang Yanan、Goto Hidenori、Eguchi Ritsuko、Miyazaki Takafumi、Yamaoka Hitoshi、Ishii Hirofumi、Liao Yen-Fa、Kubozono Yoshihiro
    • Journal Title

      New Journal of Physics

      Volume: 21 Issue: 11 Pages: 113010-113010

    • DOI

      10.1088/1367-2630/ab5034

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Preparation and characterization of superconducting Ba1-xCsxTi2Sb2O, and its pressure dependence of superconductivity2019

    • Author(s)
      Wang Yanan, Yang Xiaofan, Taguchi Tomoya, Li Huan, He Tong, Goto Hidenori, Eguchi Ritsuko, Miyazaki Takafumi, Liao Yen-Fa, Ishii Hirofumi, Kubozono Yoshihiro
    • Journal Title

      JAPANESE JOURNAL OF APPLIED PHYSICS

      Volume: 58 Issue: 11 Pages: 110603-110603

    • DOI

      10.7567/1347-4065/ab4ef5

    • NAID

      210000157392

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Synthesis of the extended phenacene molecules, [10]phenacene and [11]phenacene, and their performance in a field-effect transistor2019

    • Author(s)
      Okamoto Hideki、Hamao Shino、Eguchi Ritsuko、Goto Hidenori、Takabayashi Yasuhiro、Yen Paul Yu-Hsiang、Liang Luo Uei、Chou Chia-Wei、Hoffmann Germar、Gohda Shin、Sugino Hisako、Liao Yen-Fa、Ishii Hirofumi、Kubozono Yoshihiro
    • Journal Title

      Scientific Reports

      Volume: 9 Issue: 1 Pages: 4009-4009

    • DOI

      10.1038/s41598-019-39899-4

    • NAID

      120006777515

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Fermi level tuning of Ag-doped Bi2Se3 topological insulator2019

    • Author(s)
      Uesugi Eri、Uchiyama Takaki、Goto Hidenori、Ota Hiromi、Ueno Teppei、Fujiwara Hirokazu、Terashima Kensei、Yokoya Takayoshi、Matsui Fumihiko、Akimitsu Jun、Kobayashi Kaya、Kubozono Yoshihiro
    • Journal Title

      Scientific Reports

      Volume: 9 Issue: 1 Pages: 5376-5376

    • DOI

      10.1038/s41598-019-41906-7

    • NAID

      120006777514

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Preparation and characterization of a new metal-intercalated graphite superconductor2018

    • Author(s)
      Yang Xiaofan、Taguchi Tomoya、Wang Yanan、He Tong、Uchiyama Takaki、Takai Akihisa、Zhi Lei、Miyazaki Takafumi、Goto Hidenori、Eguchi Ritsuko、Ishii Hirofumi、Liao Yen-Fa、Yamaoka Hitoshi、Kubozono Yoshihiro
    • Journal Title

      Materials Research Express

      Volume: 6 Issue: 1 Pages: 016003-016003

    • DOI

      10.1088/2053-1591/aae9d2

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Pressure-induced superconductivity in AgxBi2-xSe32018

    • Author(s)
      Tong He, Xiaofan Yang, Takahiro Terao, Takaki Uchiyama, Teppei Ueno, Kaya Kobayashi, Jun Akimitsu, Takafumi Miyazaki, Takumi Nishioka, Koji Kimura, Kouichi Hayashi, Naohisa Happo, Hitoshi Yamaoka, Hirofumi Ishii, Yen-Fa Liao, Hiromi Ota, Hidenori Goto, and Yoshihiro Kubozono
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 10 Pages: 104503-104503

    • DOI

      10.1103/physrevb.97.104503

    • NAID

      120006523814

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Pressure dependence of superconductivity in low- and high-Tc phases of (NH3)yNaxFeSe2018

    • Author(s)
      Takahiro Terao, Xiaofan Yang, Xiao Miao, Lu Zheng, Hidenori Goto, Takafumi Miyazaki, Hitoshi Yamaoka, Hirofumi Ishii, Yen-Fa Liao, and Yoshihiro Kubozono
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 9 Pages: 094505-094505

    • DOI

      10.1103/physrevb.97.094505

    • NAID

      120006523813

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Transistor properties of exfoliated single crystals of 2H-Mo(Se1-xTex)2(0<=x<=1)2017

    • Author(s)
      Uesugi Eri、Miao Xiao、Ota Hiromi、Goto Hidenori、Kubozono Yoshihiro
    • Journal Title

      Physical Review B

      Volume: 95 Issue: 24 Pages: 245310-245310

    • DOI

      10.1103/physrevb.95.245310

    • NAID

      120006382535

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Preparation of new superconductors by metal doping of two-dimensional layered materials using ethylenediamine2017

    • Author(s)
      Xiao Miao, Takahiro Terao, Xiaofan Yang, Saki Nishiyama, Takafumi Miyazaki, Hidenori Goto, Yoshihiro Iwasa, Yoshihiro Kubozono
    • Journal Title

      Physical Review B

      Volume: 96 Issue: 1 Pages: 014502-014502

    • DOI

      10.1103/physrevb.96.014502

    • NAID

      120006382534

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Preparation and characterization of a new graphite superconductor: Ca0.5Sr0.5C62017

    • Author(s)
      Saki Nishiyama, Hidenori Fujita, Masatoshi Hoshi, Xiao Miao, Takahiro Terao, Takafumi Miyazaki, Hidenori Goto, Tomoko Kagayama, Katsuya Shimizu, Hitoshi Yamaoka, Hirofumi Ishii, Yen-Fa Liao and Yoshihiro Kubozono
    • Journal Title

      Scientific Reports

      Volume: 7 Issue: 1 Pages: 7436-7446

    • DOI

      10.1038/s41598-017-07763-y

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Difference in gating and doping effects on the band gap in bilayer graphene2017

    • Author(s)
      Uchiyama Takaki、Goto Hidenori、Akiyoshi Hidehiko、Eguchi Ritsuko、Nishikawa Takao、Osada Hiroshi、Kubozono Yoshihiro
    • Journal Title

      Scientific Reports

      Volume: 7 Issue: 1 Pages: 11322-11322

    • DOI

      10.1038/s41598-017-11822-9

    • NAID

      120007176805

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Electronic properties of bilayer graphene under an enormous electric field2020

    • Author(s)
      Lei Zhi, Hidenori Goto, Akihisa Takai, Ritsuko Eguchi, Takao NishikawaA, Shizuo TokitoA, Yoshihiro Kubozono
    • Organizer
      日本物理学会第75回年次大会, 名古屋大学, 現地開催中止, 2020/03/16-19
    • Related Report
      2019 Annual Research Report
  • [Presentation] Effects of molecular adsorption on carrier scattering in graphene2019

    • Author(s)
      Hidenori Goto, Akihisa Takai, Hidehiko Akiyoshi, Ritsuko Eguchi, Yoshihiro Kubozono
    • Organizer
      Superstripes 2019, Ischia, Naples, Italy, 2019/06/23-29
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Electronic properties of bilayer graphene under an enormous electric field2019

    • Author(s)
      Lei Zhi, Hidenori Goto, Akihisa Takai, Ritsuko Eguchi, Takao Nishikawa, Shizuo Tokito, Yoshihiro Kubozono
    • Organizer
      日本物理学会2019年秋季大会, 岐阜大学, 岐阜市, 2019/09/10-13
    • Related Report
      2019 Annual Research Report
  • [Presentation] 分子吸着によるグラフェンの散乱効果II2019

    • Author(s)
      高井彰久, 後藤秀徳, Zhi Lei, 岡本秀毅, 江口律子, 久保園芳博
    • Organizer
      日本物理学会2019年秋季大会, 岐阜大学, 岐阜市, 2019/09/10-13
    • Related Report
      2019 Annual Research Report
  • [Presentation] Semiconductor-metal transition in doped topological insulators2019

    • Author(s)
      Hidenori Goto, Takaki Uchiyama, Ritsuko Eguchi, Kaya Kobayashi, Jun Akimitsu, Yoshihiro Kubozono
    • Organizer
      Recent progress in graphene & 2D materials research (RPGR2019), Matsue, Shimane, Japan, 2019/10/06-10
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Carrier scattering in graphene caused byelectron-transfer molecules2019

    • Author(s)
      Akihisa Takai, Hidenori Goto, Hidehiko Akiyoshi, Ritsuko Eguchi, Yoshihiro Kubozono
    • Organizer
      Recent progress in graphene & 2D materials research (RPGR2019), Matsue, Shimane, Japan, 2019/10/06-10
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Effect of molecular adsorption on electronic properties in graphene2019

    • Author(s)
      Hidenori Goto, Akihisa Takai, Hidehiko Akiyoshi, Ritsuko Eguchi, Yoshihiro Kubozono
    • Organizer
      Carrier Doping in two-dimensional layered materials: toward novel physical properties and electronic device applications (CA2D), Naples, Italy, 2019/11/04-05
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Study on effect of impurity doping on transport properties in topological insulator Bi2Se32019

    • Author(s)
      Takaki Uchiyama, Hidenori Goto, Kaya Kobayashi, Jun Akimitsu, Ritsuko Eguchi, Yoshihiro Kubozono
    • Organizer
      The first international workshop on momentum microscopy & spectroscopy for materials science, IMS, 2019/02/22-23 (poster)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] 分子吸着によるグラフェンの 散乱効果2019

    • Author(s)
      高井彰久, 後藤秀徳, 内山貴生, Zhi Lei, 江口律子, 久保園芳博
    • Organizer
      日本物理学会第74回年次大会, 九州大学, 福岡, 2019/03/14-17
    • Related Report
      2018 Research-status Report
  • [Presentation] Carrier doping of graphene with electric-field effect and doping effect2018

    • Author(s)
      Hidenori Goto, Ritsuko Eguchi, Yoshihiro Kubozono
    • Organizer
      2018 EMRS Fall meeting, Warsaw, Poland, 2018/09/17-20
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Ag ドープBi2Se3における 特異な伝導特性2018

    • Author(s)
      内山貴生, 後藤秀徳, 上杉英里, He Tong, 太田弘道, 上野哲平,小林夏野,秋光純,久保園芳博
    • Organizer
      日本物理学会2018年秋季大会, 同志社大学, 京都, 2018/09/9-12
    • Related Report
      2018 Research-status Report
  • [Presentation] グラフェンの磁気散乱効果2018

    • Author(s)
      高井彰久, 後藤秀徳, 内山貴生, Zhi Lei, 江口律子, 久保園芳博
    • Organizer
      日本物理学会2018年秋季大会, 同志社大学, 京都, 2018/09/9-12
    • Related Report
      2018 Research-status Report
  • [Presentation] Bi2Se3へのAgドープの効果2018

    • Author(s)
      内山 貴生, 後藤 秀徳, 上杉 英里, He Tong, 太田 弘道, 上野 哲平, 小林 夏野, 秋光 純, 久保園 芳博
    • Organizer
      日本物理学会第73回年次大会(2018/3/22-25, 東京理科大学 野田キャンパス)
    • Related Report
      2017 Research-status Report
  • [Presentation] Doping effects on electronic properties of bilayer graphene2017

    • Author(s)
      Hidenori Goto, Takaki Uchiyama, Yoko Nakashima, Hidehiko Akiyoshi, Ritsuko Eguchi, Hiroshi Osada, Takao Nishikawa, Yoshihiro Kubozono
    • Organizer
      SUPERSTRIPES 2017, Quantum in Complex Matter: Superconductivity, Magnetism & Ferroelectricity (2017/6/4-10, Ischia, Naples, Italy)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Doping and gating methods to produce an electric field in bilayer graphene2017

    • Author(s)
      Hidenori Goto, Takaki Uchiyama, Hidehiko Akiyoshi, Ritsuko Eguchi, Yoshihiro Kubozono
    • Organizer
      Meeting on physics and chemistry of emerging superconductors and thermoelectric materials (PCST17) (2017/9/13-15 Sapienza University of Rome, Italy)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Bandgap opening of bilayer graphene doped with electron donor / acceptor molecules2017

    • Author(s)
      Takaki Uchiyama, Hidenori Goto, Yoshihiro Kubozono
    • Organizer
      International Conference on Chemistry and Materials Science (2017/11/4-5, Malang, Indonesia)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Book] Chap. 2 Physics of Graphene: Basic to FET Application in a book, "Physics and Chemistry of Carbon-Based Materials" edited by Yoshihiro Kubozono2019

    • Author(s)
      Hidenori Goto (one of authors of a book, "Physics and Chemistry of Carbon-Based Materials" edited by Yoshihiro Kubozono )
    • Total Pages
      35
    • Publisher
      Springer
    • ISBN
      9789811334177
    • Related Report
      2018 Research-status Report

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Published: 2017-04-28   Modified: 2021-02-19  

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