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Study of magnetic dynamics on surfaces and interfaces by high frequency and atomic layer sensitive ESR

Research Project

Project/Area Number 17K18745
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Research Field Condensed matter physics and related fields
Research InstitutionTohoku University

Principal Investigator

NOJIRI HIROYUKI  東北大学, 金属材料研究所, 教授 (80189399)

Project Period (FY) 2017-06-30 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥6,500,000 (Direct Cost: ¥5,000,000、Indirect Cost: ¥1,500,000)
Fiscal Year 2018: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Fiscal Year 2017: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Keywords表面 / 界面 / ESR / 強磁場 / テラヘルツ
Outline of Final Research Achievements

Studies on X-ray magnetic circular dichroism(XMCD) detection type ESR has been performed to realize an atomic layer sensitive ESR. Such technique is expected to contribute to the understandings of functionalities of surface and interface of magnetic compounds. We have succeeded in the feasibility experiment by combining W-band frequency and sub-50 K cryostat. It enables us to examine paramagnetic compounds for the comparable range of Zeeman and thermal energies creating sizable XMCD signal. Various methods of signal modulations for the higher sensitivity enhancement have been examined and compared. A possibility of time dependent measurement has been also studies. It was turned out that 100 shots accumulation is required to perform such XMCD-ESR when it is combined with a X-ray free electron laser creating sub-ps X-ray pulses.

Academic Significance and Societal Importance of the Research Achievements

本研究は、表面や界面における磁性の動的な振る舞いを調べるために原子層感度を有する電子スピン共鳴手法を開発することを目的としている。物質表面の磁性を研究する方法は幾つかあるが、電子スピン共鳴のように、表面の磁性の安定性や動的な性質を低エネルギーで正確に求められる手法は少なく、また、対象物質や応用範囲が限られていた。今回、表面敏感なX線磁気円二色性と高周波を組合わせ、この手法の応用範囲を一般的な磁性体まで広げる可能性を実証したことは大きな意義がある。さらには、将来的に時間分解測定も可能であることを明らかにしたことで、磁性体の高速スイッチングなどの現象への応用を開く事が期待される。

Report

(3 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • Research Products

    (10 results)

All 2019 2018 2017 Other

All Int'l Joint Research (1 results) Journal Article (1 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 1 results) Presentation (7 results) (of which Int'l Joint Research: 4 results,  Invited: 3 results) Remarks (1 results)

  • [Int'l Joint Research] Paul Scherrer Institute/University of Zurich(スイス)

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Rationalization of single-molecule magnet behavior in a threecoordinate Fe(III) complex with a high-spin state (S=5/2)2018

    • Author(s)
      Ning Ge, Yuan-Qi Zhai, Yi-Fei Deng, You-Song Ding, Tao Wu, Zhen-Xing Wang, Zhongwen Ouyang, Hiroyuki Nojiri and Yan-Zhen Zheng
    • Journal Title

      Inorganic Chemistry Frontiers

      Volume: 5 Issue: 10 Pages: 2486-2492

    • DOI

      10.1039/c8qi00701b

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] OVAL実験:パルス磁石と高フィネス共振器を用いた真空複屈折の探索2019

    • Author(s)
      上岡修星, 成田佳奈香, 稲田聡明, 難波俊雄, 浅井祥仁, 吉岡孝高, 五神真, 松尾晶, 金道浩一, 野尻浩之
    • Organizer
      日本物理学会第74会年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Quantum Beam Experiments in Strong Magnetic Fields Generated by a Portable Capacitor Bank2018

    • Author(s)
      H. Nojiri
    • Organizer
      The 16th International Conference on Megagauss Magnetic Field Generation and Related Topics
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Development and Application of XMCD detection ESR2018

    • Author(s)
      S. Matsuzawa, H. Nojiri, Y. Kotani, T. Nakamura
    • Organizer
      International Conference on Coordination Chemistory 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] High Magnetic Field X-ray Experiments with Synchrotron Radiation and Free Electron Laser Sources2018

    • Author(s)
      Hiroyuki NOJIRI1, Satoshi MATSUZAWA1, Hiromasa YASUMURA, Yasuo NARUMI, Chi-Chang KAO, Diling ZHU and Jun-sik LEE
    • Organizer
      International Conference on Research in High Magentic Field 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Recent Progress in High Magnetic Field Science at SR and XFEL Sources2018

    • Author(s)
      H. Nojiri
    • Organizer
      X-ray Diffraction and Spectroscopy in Very High Magnetic Fields at the Helmholtz Beamline for Extreme Fields
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] XMCD 検出ESR の開発と応用2018

    • Author(s)
      野尻浩之
    • Organizer
      2017年度量子ビームサイエンスフェスタ
    • Related Report
      2017 Research-status Report
    • Invited
  • [Presentation] 軟X線XMCD検出法による高周波ESRの開発2017

    • Author(s)
      野尻浩之
    • Organizer
      第56回電子スピンサイエンス学会年会(SEST2017)
    • Related Report
      2017 Research-status Report
  • [Remarks] 磁気物理学部門ホームページ

    • URL

      http://www.hfpm.imr.tohoku.ac.jp

    • Related Report
      2017 Research-status Report

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Published: 2017-07-21   Modified: 2020-03-30  

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