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Quantum transport phenomena of ferromagnetic two dimensional electron system by gas source MBE films

Research Project

Project/Area Number 18H01878
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 29020:Thin film/surface and interfacial physical properties-related
Research InstitutionInstitute of Physical and Chemical Research

Principal Investigator

Takahashi Kei  国立研究開発法人理化学研究所, 創発物性科学研究センター, 上級研究員 (90469932)

Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥17,550,000 (Direct Cost: ¥13,500,000、Indirect Cost: ¥4,050,000)
Fiscal Year 2020: ¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2019: ¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2018: ¥9,230,000 (Direct Cost: ¥7,100,000、Indirect Cost: ¥2,130,000)
Keywords分子線エピタキシー / 酸化物薄膜 / 量子伝導 / 強磁性 / スピン偏極電子 / 磁性半導体 / スピン偏極
Outline of Final Research Achievements

By fabricating high quality films of EuTiO3 using gas source molecular beam epitaxy, we tried to observe quantum transport phenomena and quantum Hall effect in the magnetic semiconductor.
Compressive strained films on LSAT substrate show peculiar anomalous Hall effect during the magnetization process from antiferromagnetic order to ferromagnetic one. The Weyl nodes path through the Fermi energy during the magnetization process. I found that such process causes the magnetic field dependence of anomalous Hall effect. On lattice matched substrate SrTiO3, the mobility of La doped EuTiO3 film reaches 3200 cm2V-1s-1 at 2 K, which is the record of this system. This is demonstrated by measuring the Shubnikov de Haas (SdH) oscillations in the ferromagnetic state. Using first-principles calculations, it is shown that the observed SdH oscillations originate genuinely from Ti 3d-t2g states which are fully spin-polarized due to their energetical proximity to the in-gap Eu 4f bands.

Academic Significance and Societal Importance of the Research Achievements

磁性半導体はスピントロニクス応用材料として期待されている。スピントロニクスは電子のスピン自由度をデバイスに応用するが、電子には量子効果、つまり電子の波の性質がある。この量子効果を使うことで電子に機能をさらに持たせることができる。通常、磁性半導体は磁性不純物をドープするためその不純物散乱により移動度が低下し、電子の波の性質を反映した量子干渉効果を観察することは困難であった。磁性半導体EuTiO3が量子常誘電体であり電子ドープしたときの移動度が高いことに注目し、スピン偏極電子の量子伝導の観察に成功した本研究は、今後スピントロニクスに量子効果を取り入れた応用研究への貢献が期待できる。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (6 results)

All 2021 2020 2019 2018

All Journal Article (2 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 2 results,  Open Access: 1 results) Presentation (4 results) (of which Int'l Joint Research: 3 results,  Invited: 3 results)

  • [Journal Article] Anisotropic Quantum Transport through a Single Spin Channel in the Magnetic Semiconductor EuTiO32020

    • Author(s)
      Kazuki Murahashi, Kei S. Takahashi, Mohammad Saeed Bahramy, Sunao Shimizu, Ryosuke Kurihara, Atushi Miyake, Masashi Tokunaga, Yoshinori Tokura, Masashi Kawasaki
    • Journal Title

      Advanced Materials

      Volume: - Issue: 24 Pages: 1908315-1908315

    • DOI

      10.1002/adma.201908315

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Anomalous Hall effect derived from multiple Weyl nodes in high-mobility EuTiO 3 films2018

    • Author(s)
      Takahashi Kei S.、Ishizuka Hiroaki、Murata Tomoki、Wang Qing Y.、Tokura Yoshinori、Nagaosa Naoto、Kawasaki Masashi
    • Journal Title

      Science Advances

      Volume: 4 Issue: 7

    • DOI

      10.1126/sciadv.aar7880

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Quantum transport of spin polarized electrons in EuTiO3 films grown by gas source MBE2021

    • Author(s)
      高橋圭
    • Organizer
      APS March Meeting 2021
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Quantum transport in magnetic semiconductor EuTiO3 films2019

    • Author(s)
      高橋圭
    • Organizer
      2019 MRS SPRING MEETING
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Quantum transport of spin polarized electrons in EuTiO3 films2019

    • Author(s)
      高橋圭
    • Organizer
      OSS (Oxide Superspin) Workshop 2019
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Quantum transport in the films of a magnetic semiconductor EuTiO32018

    • Author(s)
      高橋圭
    • Organizer
      25th International Workshop on Oxide Electronics
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research

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Published: 2018-04-23   Modified: 2022-01-27  

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