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Wettability and release behaviour of fission products on solid nuclear fuels

Research Project

Project/Area Number 18H01918
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 31010:Nuclear engineering-related
Research InstitutionKyoto University

Principal Investigator

Kurosaki Ken  京都大学, 複合原子力科学研究所, 教授 (90304021)

Co-Investigator(Kenkyū-buntansha) 宇埜 正美  福井大学, 附属国際原子力工学研究所, 教授 (00232885)
橋本 直幸  北海道大学, 工学研究院, 教授 (50443974)
Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2022)
Budget Amount *help
¥17,420,000 (Direct Cost: ¥13,400,000、Indirect Cost: ¥4,020,000)
Fiscal Year 2020: ¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2019: ¥5,720,000 (Direct Cost: ¥4,400,000、Indirect Cost: ¥1,320,000)
Fiscal Year 2018: ¥7,150,000 (Direct Cost: ¥5,500,000、Indirect Cost: ¥1,650,000)
Keywords核燃料 / ぬれ性 / 核分裂生成物 / 原子力 / 二酸化ウラン / ヨウ素酸セシウム
Outline of Final Research Achievements

Focusing on the wettability between solid nuclear fuels and liquid fission product (FP) chemical species, the objective is to clarify the relationship between wettability and FP release behaviour from fuels through wettability evaluation tests between solids with fluorite-type crystal structures such as UO2 and various Cs halides such as CsI and FP release tests from simulated fuels. The objective of this study was to clarify the relationship between wettability and fission product release behaviour from fuels.
In this study, the wettability between solid and liquid was comprehensively verified using parameters such as the crystal orientation, crystal structure and surface roughness of the solid oxide, and the melt structure and bonding mode of the liquid caesium halides. Based on all the results obtained in this study, a new fission product (FP) release behaviour model was developed and proposed with the newly added effect of wettability.

Academic Significance and Societal Importance of the Research Achievements

1F事故以降、事故の原因究明や発電所を安定化させることを目的として、様々な基礎研究が行われているが、それらの中でも、高揮発性のFPであるCsとIの燃料からの放出挙動を評価することは優先度の高い重要な課題とされている。ところが、公開されているデータのばらつきは大きく、燃料からのFP放出挙動には多くの不確かさが残されている。本研究の着目点であるぬれ性とFP放出挙動を結びつけることができれば、多くの不確かさが残されているFP放出挙動の解明の一助となり、FP放出のソースターム評価や原子炉事故時の放射性物質の放出抑制技術の確立につながる。

Report

(4 results)
  • 2022 Final Research Report ( PDF )
  • 2020 Annual Research Report
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (13 results)

All 2022 2021 2020 2019 2018

All Journal Article (4 results) (of which Peer Reviewed: 3 results,  Open Access: 1 results) Presentation (9 results) (of which Int'l Joint Research: 3 results)

  • [Journal Article] DX application to the field of nuclear materials and its issues (1)2022

    • Author(s)
      黒﨑 健
    • Journal Title

      Journal of the Atomic Energy Society of Japan

      Volume: 64 Issue: 10 Pages: 569-571

    • DOI

      10.3327/jaesjb.64.10_569

    • ISSN
      1882-2606, 2433-7285
    • Related Report
      2020 Annual Research Report
  • [Journal Article] Phase behavior of oxidized Ce and Gd-doped (U,Zr)O22022

    • Author(s)
      Yifan Sun, Shiho Watanabe, Hiroaki Muta, Yuji Ohishi, and Ken Kurosaki
    • Journal Title

      J. Nucl. Sci. Technol.

      Volume: 60 Issue: 4 Pages: 425-434

    • DOI

      10.1080/00223131.2022.2112782

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Interaction of Liquid CsIO<sub>3</sub> with a Polycrystalline UO<sub>2</sub> Solid Surface2020

    • Author(s)
      石井 大翔, 大石 佑治, 牟田 浩明, 宇埜 正美, 黒崎 健
    • Journal Title

      Transactions of the Atomic Energy Society of Japan

      Volume: 19 Issue: 3 Pages: 147-151

    • DOI

      10.3327/taesj.J19.017

    • NAID

      130007889104

    • ISSN
      1347-2879, 2186-2931
    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Wettability of liquid cesium iodine and boron oxide on yttria-stabilized zirconia2018

    • Author(s)
      Hiroto Ishii, Ken Kurosaki, Yukihiro Murakami, Yuji Ohishi, Hiroaki. Muta, Masayoshi Uno, Shinsuke Yamanaka
    • Journal Title

      Journal of Nuclear Science and Technology

      Volume: 55 Issue: 8 Pages: 838-842

    • DOI

      10.1080/00223131.2018.1439413

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] 原子力材料におけるDX利用と課題 (1) 新材料開発とマテリアルズ・インフォマティクス2022

    • Author(s)
      黒﨑 健
    • Organizer
      日本原子力学会2022年春の年会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 核燃料の今後の展望2021

    • Author(s)
      黒﨑 健
    • Organizer
      日本原子力学会2021年秋の大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 多様な原子燃料の概念と基礎設計 -将来の原子炉のための燃料開発-2021

    • Author(s)
      黒﨑 健
    • Organizer
      日本原子力学会2021年春の年会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Wettability of liquid CsI on metal-oxide polycrystalline surfaces2019

    • Author(s)
      Hiroto Ishii, Yuji Ohishi, Hiroaki Muta, Masayoshi Uno, Ken Kurosaki
    • Organizer
      International Topical Workshop on Fukushima Decommissioning Research
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Wettability of liquid phase caesium compounds against metal oxides including UO2 and ThO22019

    • Author(s)
      Hiroto Ishii, Yuji Ohishi, Hiroaki Muta, Masayoshi Uno, Ken Kurosaki
    • Organizer
      The Minerals, Metals and Materials Society 2020
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 液体ヨウ化セシウムの酸化物多結晶固体表面 に対する濡れ性2019

    • Author(s)
      石 井 大 翔 , 大石佑治, 牟田浩明, 宇埜正美, 黒崎健
    • Organizer
      日本原子力学会 2019 年秋の大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] SUS316 固体表面における液体 CsI の濡れ性2019

    • Author(s)
      石 井 大 翔 , 大石佑治, 牟田浩明, 鈴木恵理子, 中島邦久, 三輪周平, 逢坂正彦, 宇埜正美, 黒崎健
    • Organizer
      日本原子力学会 2020 年春の年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Wettability of liquid-state caesium halides (CsCl, CsBr, CsI) on single crystalline oxides (YSZ, TiO2, MgO)2018

    • Author(s)
      Hiroto Ishii, Yuji Ohishi, Hiroaki Muta, Masayoshi Uno, Ken Kurosaki
    • Organizer
      The Nuclear Materials Conference 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 液体CsIの酸化物固体表面に対する濡れ挙動の評価2018

    • Author(s)
      石井大翔, 大石佑治, 牟田浩明, 宇埜正美, 黒崎健
    • Organizer
      次世代イニシアティブ廃炉技術カンファレンス(NDEC3)
    • Related Report
      2018 Annual Research Report

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Published: 2018-04-23   Modified: 2024-01-30  

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