• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Next Generation Thin Film Solar Cell Material SnS: Pursuit of Solid State Chemistry for Homojunction

Research Project

Project/Area Number 18KK0133
Research Category

Fund for the Promotion of Joint International Research (Fostering Joint International Research (B))

Allocation TypeMulti-year Fund
Review Section Medium-sized Section 26:Materials engineering and related fields
Research InstitutionUniversity of Yamanashi

Principal Investigator

Yanagi Hiroshi  山梨大学, 大学院総合研究部, 教授 (30361794)

Co-Investigator(Kenkyū-buntansha) 川西 咲子  東北大学, 多元物質科学研究所, 助教 (80726985)
鈴木 一誓  東北大学, 多元物質科学研究所, 助教 (60821717)
Project Period (FY) 2018-10-09 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥17,940,000 (Direct Cost: ¥13,800,000、Indirect Cost: ¥4,140,000)
Fiscal Year 2021: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Fiscal Year 2020: ¥6,630,000 (Direct Cost: ¥5,100,000、Indirect Cost: ¥1,530,000)
Fiscal Year 2019: ¥6,630,000 (Direct Cost: ¥5,100,000、Indirect Cost: ¥1,530,000)
Fiscal Year 2018: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
KeywordsSnS / 太陽電池 / コンビナトリアル製膜 / 薄膜 / n型伝導 / ホモ接合 / コンビナトリアル
Outline of Final Research Achievements

The n-type SnS thin film was realized by optimizing the film deposition conditions using a combinatorial sputtering method at NREL (USA). N-type SnS thin film was realized by supplying atomic sulfur, which reduces the number of in-gap states. It was found that SnS solar cells are expected to have a high open-circuit voltage of ~0.7 V if the interface defects at the p-n interface are suppressed, according to the XPS measurements performed at TU Darmstadt (Germany). A prototype homojunction solar cell was fabricated by forming a p-type thin film on an n-type single crystal. The conversion efficiency of 1.4% was lower than that of existing heterojunction solar cells, but the open-circuit voltage was as high as 0.36 V, demonstrating the effectiveness of homojunction solar cells.

Academic Significance and Societal Importance of the Research Achievements

n型SnS薄膜実現のために本質的に重要な制御因子を解明し、解決手法を実証した意義は大きい。これに加えてSnS太陽電池における高Vocの実現可能性の科学的根拠を与えた。これらにより環境親和性が高く資源制約の少ない高効率SnSホモ接合薄膜太陽電池への道を拓いたことで、次世代太陽電池材料に新たな選択肢を提供した。

Report

(5 results)
  • 2021 Annual Research Report   Final Research Report ( PDF )
  • 2020 Research-status Report
  • 2019 Research-status Report
  • 2018 Research-status Report
  • Research Products

    (28 results)

All 2022 2021 2020 2019 2018 Other

All Int'l Joint Research (2 results) Journal Article (2 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 2 results,  Open Access: 1 results) Presentation (21 results) (of which Int'l Joint Research: 7 results,  Invited: 1 results) Remarks (2 results) Patent(Industrial Property Rights) (1 results)

  • [Int'l Joint Research] National Renewable Energy Laboratory(米国)

    • Related Report
      2019 Research-status Report
  • [Int'l Joint Research] National Renewable Energy Laboratory(米国)

    • Related Report
      2018 Research-status Report
  • [Journal Article] n-type electrical conduction in SnS thin films2021

    • Author(s)
      Suzuki Issei、Kawanishi Sakiko、Bauers Sage R.、Zakutayev Andriy、Lin Zexin、Tsukuda Satoshi、Shibata Hiroyuki、Kim Minseok、Yanagi Hiroshi、Omata Takahisa
    • Journal Title

      Physical Review Materials

      Volume: 5 Issue: 12 Pages: 125405-125405

    • DOI

      10.1103/physrevmaterials.5.125405

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] SnS Homojunction Solar Cell with n‐Type Single Crystal and p‐Type Thin Film2021

    • Author(s)
      Kawanishi Sakiko、Suzuki Issei、Bauers Sage R.、Zakutayev Andriy、Shibata Hiroyuki、Yanagi Hiroshi、Omata Takahisa
    • Journal Title

      Solar RRL

      Volume: 5 Issue: 4 Pages: 2000708-2000708

    • DOI

      10.1002/solr.202000708

    • Related Report
      2020 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] キャリア濃度抑制を目指したSnS薄膜の製膜2022

    • Author(s)
      中川瞭、柳博
    • Organizer
      第60回セラミックス基礎科学討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] n型SnS単結晶/MoO3接合を用いた太陽電池の高変換効率化2022

    • Author(s)
      鈴木一誓、リンタクシン、野上大一、川西咲子、小俣孝久
    • Organizer
      2022年 第69回応用物理学会春季学術講演会
    • Related Report
      2021 Annual Research Report
  • [Presentation] n型SnS単結晶/MoO3接合を用いた太陽電池の変換効率の向上2022

    • Author(s)
      鈴木一誓、リンタクシン、野上大一、川西咲子、小俣孝久
    • Organizer
      日本セラミックス協会 2022年・年会
    • Related Report
      2021 Annual Research Report
  • [Presentation] N-Type SnS and Its Application to Homojunction PV2022

    • Author(s)
      Issei Suzuki, Sakiko Kawanishi, Sage Bauers, Andriy Zakutayev, Binxiang Huang, Zexin Lin, Hiroyuki Shibata, Andreas Klein, Hiroshi Yanagi, Takahisa Omata
    • Organizer
      2022 Virtual MRS Spring Meeting & Exhibit
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Solution growth of large single crystals of n-type tin monosulfide2021

    • Author(s)
      Sakiko Kawanishi, Issei Suzuki, Takahisa Omata, and Hiroyuki Shibata
    • Organizer
      22nd American Conference on Crystal Growth and Epitaxy (ACCGE-22
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] N-type conduction in Cl-doped SnS thin film2021

    • Author(s)
      I. Suzuki, S. Kawanishi, S.R. Bauers, A. Zakutayev, H. Shibata, M. Kim, H. Yanagi, T. Omata
    • Organizer
      Materials Research Meeting 2021
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] N-Type SnS Thin Films Applicable for Homojunction Solar Cells2021

    • Author(s)
      I. Suzuki, S. Kawanishi, S.R. Bauers, A. Zakutayev, H. Shibata, M. Kim, H. Yanagi, T. Omata
    • Organizer
      2021 Virtual MRS Spring Meeting & Exhibit
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Fabrication of pn Homojunction of SnS and Its Photovoltaic Properties2021

    • Author(s)
      I. Suzuki, S. Kawanishi, S.R. Bauers, A. Zakutayev, H. Shibata, H. Yanagi, T. Omata
    • Organizer
      2021 Virtual MRS Spring Meeting & Exhibit
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] SnS 単結晶/MoO3界面の電子構造と太陽電池への応用2021

    • Author(s)
      鈴木一誓、川西咲子、リンタクシン、小俣孝久、Binxiang Huang、Andreas Klein
    • Organizer
      第41回電子材料研究討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 大きなバンド屈曲を示すn型SnS/MoO3接合の太陽電池への応用2021

    • Author(s)
      リンタクシン、鈴木一誓、川西咲子、小俣孝久
    • Organizer
      日本セラミックス協会 第34回秋季シンポジウム
    • Related Report
      2021 Annual Research Report
  • [Presentation] n型SnS の作製とホモ接合太陽電池への展開2020

    • Author(s)
      鈴木一誓,川西咲子,Bauers Sage,Zakutayev Andriy,柴田浩幸,Kim Minseok,柳博,小俣 孝久
    • Organizer
      電子材料研究討論会
    • Related Report
      2020 Research-status Report
  • [Presentation] pnホモ接合SnSの作製と太陽電池特2020

    • Author(s)
      川西咲子,鈴木一誓,Bauers Sage,Zakutayev Andriy,柴田浩幸,柳博,小俣孝久
    • Organizer
      応用物理学会秋季学術講演会
    • Related Report
      2020 Research-status Report
  • [Presentation] スパッタリング法によるn型SnS薄膜の作製2020

    • Author(s)
      鈴木一誓,川西咲子,Bauers Sage,Zakutayev Andriy,柴田浩幸,Kim Minseok,柳博,小俣 孝久
    • Organizer
      応用物理学会秋季学術講演会
    • Related Report
      2020 Research-status Report
  • [Presentation] n型SnS薄膜のスパッタリング法による作製2020

    • Author(s)
      鈴木一誓,川西咲子,Bauers Sage,Zakutayev Andriy,柴田浩幸,Kim Minseok,柳博,小俣 孝久
    • Organizer
      資源・素材 2020
    • Related Report
      2020 Research-status Report
  • [Presentation] n型SnS薄膜の作製2020

    • Author(s)
      鈴木一誓,川西咲子,Bauers Sage,Zakutayev Andriy,柴田浩幸,Kim Minseok,柳博,小俣 孝久
    • Organizer
      日本セラミックス協会 第33回秋季シンポジウム
    • Related Report
      2020 Research-status Report
  • [Presentation] n 型SnS 単結晶の電子状態2019

    • Author(s)
      鈴木一誓、川西咲子、小俣孝久、柳博
    • Organizer
      応用物理学会
    • Related Report
      2019 Research-status Report
  • [Presentation] Growth of Halogen Doped n-Type SnS Single Crystals Using Self-Flux2019

    • Author(s)
      H. Yanagi, Y. Iguchi, K. Sato, K. Inoue, I. Suzuki, S. Kawanishi
    • Organizer
      MRM2019
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Growth of Cl-doped n-type SnS single crystals and their electrical properties2019

    • Author(s)
      Hiroshi Yanagi, Yuki Iguchi, Koichi Sato, Sakiko Kawanishi, and Issei Suzuki
    • Organizer
      ICAE2019
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Brドープn型SnS単結晶育成と物性評価2018

    • Author(s)
      井上 和俊、Rizky、椚 俊智、柳 博
    • Organizer
      太陽電池研究会年末講演会
    • Related Report
      2018 Research-status Report
  • [Presentation] 接昇華法により作製したSnS薄膜に対するBr添加の影響2018

    • Author(s)
      Rizky、柳 博
    • Organizer
      太陽電池研究会年末講演会
    • Related Report
      2018 Research-status Report
  • [Presentation] 近接昇華法を用いたSnS薄膜の作製と評価2018

    • Author(s)
      佐藤 孝一、井上 和俊、Rizky、大岩 正和、柳 博
    • Organizer
      太陽電池研究会年末講演会
    • Related Report
      2018 Research-status Report
  • [Remarks] 山梨大学応用化学科柳研究室

    • URL

      https://www.ccn.yamanashi.ac.jp/~hyanagi/index.html

    • Related Report
      2021 Annual Research Report
  • [Remarks] Materials Discovery Team@NREL

    • URL

      https://sites.google.com/view/materialsdiscovery/home

    • Related Report
      2019 Research-status Report
  • [Patent(Industrial Property Rights)] n型SnS薄膜、光電変換素子、太陽電池、n型SnS薄膜の製造方法、およびn型SnS薄膜の製造装置2020

    • Inventor(s)
      鈴木 一誓、川西 咲子、柳 博
    • Industrial Property Rights Holder
      山梨大学、東北大学
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2020-108143
    • Filing Date
      2020
    • Related Report
      2020 Research-status Report

URL: 

Published: 2018-10-12   Modified: 2023-01-30  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi