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Fabrication of oxygen evolution anode for seawater electrolysis in acidic NaCl solution at about pH 1

Research Project

Project/Area Number 19760514
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Material processing/treatments
Research InstitutionTohoku Institute of Technology

Principal Investigator

KATO Zenta  Tohoku Institute of Technology, 工学部, 准教授 (40398491)

Project Period (FY) 2007 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥3,920,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥720,000)
Fiscal Year 2010: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2009: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2008: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2007: ¥800,000 (Direct Cost: ¥800,000)
Keywords電極活物質 / 海水電解 / 酸素発生 / 再生可能エネルギー / CO_2エネルギー / CO_2リサイクル / CO2エネルギー / 電極触媒 / 新エネルギー
Research Abstract

The oxygen evolution anode for seawater electrolysis was improved for the achievement of the energy system, that is, "Global CO_2 Recycling". The anodes were composed of the electrocatalyst oxide, the intermediate layer and the titanium substrate. Mn_<1-x>Mo_xSn_yO_<2+x> electrocatalyst oxide / Sn_<1-x>Ir_xO_2 intermediate layer/Ti anodes, whose the intermediate layer was prepared from 0.04 M Ir-0.06 M Sn solution, showed the oxygen evolution efficiency higher than 99.8% for more than 4300 h in electrolysis of 0.5 M NaCl solution of pH 1 at the current density of 1000 Am^<-2>.

Report

(6 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report   Self-evaluation Report ( PDF )
  • 2008 Annual Research Report
  • 2007 Annual Research Report
  • Research Products

    (34 results)

All 2011 2010 2009 2008 2007 2006

All Journal Article (11 results) (of which Peer Reviewed: 11 results) Presentation (18 results) Patent(Industrial Property Rights) (5 results)

  • [Journal Article] Durability enhancement and degradation of oxygen evolution anodes in seawater electrolysis for hydrogen production2011

    • Author(s)
      Z.Kato, J.Bhattarai, K.Izumiya, N.Kumaga, K.Hashimoto
    • Journal Title

      Applied Surface Science 257

      Pages: 8230-8236

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Durabitity enhancement and degradation of oxygen evotution anodes in seawater electrolysis for hydrogen production2010

    • Author(s)
      Z.Kato, J.Bhattarai, K.Izumiya, N.Kumaga, K.Hashimoto
    • Journal Title

      Applied Surface Science

      Volume: (In Press)

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Materials and Technology for supply of renewable energy and prevention of global warming2009

    • Author(s)
      K.Hashimoto, Z.Kato, N.Kumagai, K.Izumiya
    • Journal Title

      Journal of Physics : Conference Series 144

      Pages: 1-6

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] グローバル二酸化炭素リサイクル2009

    • Author(s)
      橋本功二、熊谷直和、加藤善大、泉屋宏一
    • Journal Title

      材料と環境 58巻

      Pages: 250-259

    • Related Report
      2010 Final Research Report 2009 Self-evaluation Report
    • Peer Reviewed
  • [Journal Article] Energy-saving seawater electrolysis for hydrogen production2009

    • Author(s)
      Z.Kato, K.Izumiya, N.Kumagai, K.Hashimoto
    • Journal Title

      J Solid State Elecrochemistry 13

      Pages: 219-224

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Energy-saving seawater electrolysis for hydrogen production2009

    • Author(s)
      Z. Kato, K. Izumiya, N. Kumagai, K. Hashimoto
    • Journal Title

      J Solid State Elecrochemistry 13

      Pages: 219-224

    • Related Report
      2009 Self-evaluation Report
    • Peer Reviewed
  • [Journal Article] Materials and Technology for Supply of Renewable Energy and Prevention of Global Warming2009

    • Author(s)
      K.Hashimoto, Z.Kato, N.Kumagai, K.Izumiya
    • Journal Title

      Journal of Physics : Conference Series 144

      Pages: 1-6

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] グローバル二酸化炭素リサイクル2009

    • Author(s)
      橋本功二、熊谷直和、加藤善大、泉屋宏一
    • Journal Title

      材料と環境 58

      Pages: 250-259

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Energy-saving seawater electrolysis for hydrogen production2009

    • Author(s)
      Z. Kato, K. Izumiya, N. Kumagai, K. Hashimoto
    • Journal Title

      J Solid State Elecrochemistry Volume 13

      Pages: 219-224

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] The effect of tungsten addition to the intermediate IrO2 layer of Mn-Mo-O/IrO2/Ti electrodes on the performance for oxygen evolution in seawater electrolysis2006

    • Author(s)
      Z. Kato, N. Kumagai, K. Asami, K. Hashimoto
    • Journal Title

      ECS Transactions / The Electrochemical Society Volume1

      Pages: 499-507

    • Related Report
      2009 Self-evaluation Report
    • Peer Reviewed
  • [Journal Article] The effect of tungsten addition to the intermediate IrO_2 layer of Mn-Mo-O/IrO_2/Ti electrodes on the performance for oxygen evolution in seawater electrolysis2006

    • Author(s)
      Z. Kato, N. Kumagai, K. Asami, K. Hashimoto
    • Journal Title

      ECS Transactions/The Electrochemical Society Volume1

      Pages: 499-507

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Presentation] Enhancement of durability of oxygen evolution anode in seawater electrolysis for hydrogen production2010

    • Author(s)
      Z.Kato, K.Izumiya, N.Kumaga, K.Hashimoto
    • Organizer
      European Materials Research Society
    • Place of Presentation
      Warsaw, Poland
    • Year and Date
      2010-09-14
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] Carbon dioxide, the feedstock for using renewable energy2010

    • Author(s)
      K.Hashimoto, N.Kumagai, K.Izumiya, Z.Kato
    • Organizer
      European Materials Research Society
    • Place of Presentation
      Warsaw, Poland
    • Year and Date
      2010-09-13
    • Related Report
      2010 Annual Research Report 2010 Final Research Report
  • [Presentation] Improvement of Intermediate Layer by Formation of Tin-iridium Dioxide in Oxygen Evolution Anodes for Seawater Electrolysis2009

    • Author(s)
      Z.Kato, J.Bhattarai, K.Izumiya, N.Kumaga, K.Hashimoto
    • Organizer
      The Electrochemical Society
    • Place of Presentation
      Vienna, Austria
    • Year and Date
      2009-10-07
    • Related Report
      2010 Final Research Report 2009 Annual Research Report 2009 Self-evaluation Report
  • [Presentation] Mn-Mo-Sn Oxide Anodes for Oxygen Evolution in Seawater Electrolysis for Hydrogen Production2009

    • Author(s)
      A.El-Moneim, J.Bhattarai, Z.Kato, K.Izumiya, N.Kumagai, K.Hashimoto
    • Organizer
      The Electrochemical Society
    • Place of Presentation
      Vienna, Austria
    • Year and Date
      2009-10-07
    • Related Report
      2010 Final Research Report 2009 Annual Research Report
  • [Presentation] Sn_<1-x>Ir_xO_2複酸化物の形成による海水電解用酸素発生陽極中間層の改良2009

    • Author(s)
      加藤善大、泉屋宏一、熊谷直和、橋本功二
    • Organizer
      第56回材料と環境討論会 (社)腐食防食協会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2009-09-30
    • Related Report
      2010 Final Research Report
  • [Presentation] 海水電解用酸素発生極の電気抵抗とアノード分極曲線2009

    • Author(s)
      A.El-Moneim、 J.Bhattarai、 加藤善大、泉屋宏一、熊谷直和、橋本功二
    • Organizer
      第56回材料と環境討論会 (社)腐食防食協会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2009-09-30
    • Related Report
      2010 Final Research Report
  • [Presentation] Sn_<1->Ir_xO_2複酸化物の形成による海水電解用酸素発生陽極中間層の改良2009

    • Author(s)
      加藤善大、泉屋宏一、熊谷直和、橋本功二
    • Organizer
      第56回材料と環境討論会(社)腐食防食協会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2009-09-30
    • Related Report
      2009 Annual Research Report
  • [Presentation] 海水電解用酸素発生極の電気抵抗とアノード分極曲線2009

    • Author(s)
      A.El-Moneim, J.Bhattarai, 加藤善大、泉屋宏一、熊谷直和、橋本功二
    • Organizer
      第56回材料と環境討論会(社)腐食防食協会
    • Place of Presentation
      大阪府立大学
    • Year and Date
      2009-09-30
    • Related Report
      2009 Annual Research Report
  • [Presentation] The Improvement of the Intermediate Layer by Substitution of Iridium with Tin in Mn-Mo-Sn Triple oxide/IrO_2/Ti Anodes for Oxygen Evolution in Seawater Electrolysis2008

    • Author(s)
      Z.Kato, J.Bhattarai, K.Izumiya, N.Kumagai, K.Hashimoto
    • Organizer
      214th Meeting of ECS-The Electrochemical Society
    • Place of Presentation
      Honolulu, Hawaii
    • Year and Date
      2008-10-16
    • Related Report
      2010 Final Research Report
  • [Presentation] The Improvement of the Intermediate Layer by Substitution of Iridium with Tin in Mn-Mo-Sn Triple oxide/IrO_2/Ti Anodes for Oxygen Evolution in Seawater Ele ctrolysis2008

    • Author(s)
      Z. Kato, J. Bhattarai, K. Izumiya, N. Kumagai, K. Hashimoto
    • Organizer
      214th Meeting of ECS-The Electrochemical Society
    • Place of Presentation
      Honolulu, Hawaii
    • Year and Date
      2008-10-16
    • Related Report
      2008 Annual Research Report
  • [Presentation] 海水電解のための酸素発生陽極の中間層の改良2008

    • Author(s)
      加藤善大、ジャガディシュ・バッタライ、泉屋宏一、熊谷直和、橋本功二
    • Organizer
      材料と環境2008 (社)腐食防食協会
    • Place of Presentation
      大宮ソニックシティー
    • Year and Date
      2008-09-17
    • Related Report
      2010 Final Research Report
  • [Presentation] 海水電解のための酸素発生陽極の改良2008

    • Author(s)
      加藤善大、泉屋宏一、熊谷直和、橋本功二
    • Organizer
      第55回材料と環境討論会 (社)腐食防食協会
    • Place of Presentation
      長崎大学工学部
    • Year and Date
      2008-09-17
    • Related Report
      2010 Final Research Report
  • [Presentation] 海水電解のための酸素発生陽極の改良2008

    • Author(s)
      加藤善大、泉屋宏一、熊谷直和、橋本功二
    • Organizer
      第55回材料と環境討論会(社)腐食防食協会
    • Place of Presentation
      長崎大学工学部
    • Year and Date
      2008-09-17
    • Related Report
      2008 Annual Research Report
  • [Presentation] 海水電解のための酸素発生陽極の中間層の改良2008

    • Author(s)
      加藤善大、ジャガディシュバッタライ、泉屋宏一、熊谷直和、橋本功二
    • Organizer
      材料と環境2008(社)腐食防食協会
    • Place of Presentation
      大宮ソニックシティー
    • Year and Date
      2008-05-13
    • Related Report
      2008 Annual Research Report
  • [Presentation] 強酸性海水電解による酸素発生のためのアノード電着MnO_2系複酸化物陽極の改良2007

    • Author(s)
      加藤善大、高野裕之、泉屋宏一、熊谷直和、橋本功二
    • Organizer
      第54回材料と環境討論会 (社)腐食防食協会
    • Place of Presentation
      RCC文化センター(広島)
    • Year and Date
      2007-11-01
    • Related Report
      2010 Final Research Report 2007 Annual Research Report
  • [Presentation] Energy-saving seawater electrolysis for hydrogen production2007

    • Author(s)
      Z.Kato, K.Izumiya, N.Kumagai, K.Hashimoto
    • Organizer
      European Materials Research Society
    • Place of Presentation
      Warsaw, Poland
    • Year and Date
      2007-09-19
    • Related Report
      2010 Final Research Report
  • [Presentation] Energy-saving seawater electrolysis for hydrogen production2007

    • Author(s)
      Z. Kato, K. Izumiya, N. Kumagai, K. Hashimoto
    • Organizer
      European Materials Research Society
    • Place of Presentation
      Warsaw (Poland)
    • Year and Date
      2007-09-19
    • Related Report
      2007 Annual Research Report
  • [Presentation] 中性海水電解におけるセル電圧上昇回避の試み2007

    • Author(s)
      加藤善大、高野裕之、泉屋宏一、熊谷直和、橋本功二
    • Organizer
      材料と環境2007 (社)腐食防食協会
    • Place of Presentation
      早稲田大学国際会議場
    • Year and Date
      2007-05-19
    • Related Report
      2010 Final Research Report 2007 Annual Research Report
  • [Patent(Industrial Property Rights)] 酸素発生用陽極2008

    • Inventor(s)
      橋本功二、加藤善大、泉屋宏一、熊谷直和
    • Industrial Property Rights Holder
      橋本功二、アタカ大機(株)
    • Filing Date
      2008-09-05
    • Related Report
      2010 Final Research Report
  • [Patent(Industrial Property Rights)] 酸素発生用陽極2008

    • Inventor(s)
      橋本功二、加藤善大、泉屋宏一、熊谷直和
    • Industrial Property Rights Holder
      橋本功二、アタカ大機(株)
    • Filing Date
      2008-09-05
    • Related Report
      2009 Self-evaluation Report
  • [Patent(Industrial Property Rights)] 酸素発生用陽極2008

    • Inventor(s)
      橋本功二、加藤善大、泉屋宏一、熊谷直和
    • Industrial Property Rights Holder
      橋本功二、アタカ大機(株)
    • Industrial Property Number
      2008-229124
    • Filing Date
      2008-09-05
    • Related Report
      2008 Annual Research Report
  • [Patent(Industrial Property Rights)] 炭素酸化物のメタン化触媒。その製造方法およびメタン化方法2007

    • Inventor(s)
      橋本功二、高野裕之、泉屋宏一、熊谷直和、加藤善大
    • Industrial Property Rights Holder
      橋本功二、アタカ大機(株)
    • Filing Date
      2007-08-03
    • Related Report
      2010 Final Research Report
  • [Patent(Industrial Property Rights)] 炭素酸化物のメタン化触媒。その製造方法およびメタン化方法2007

    • Inventor(s)
      橋本功二、高野裕之、泉屋宏一、熊谷直和、加藤善大
    • Industrial Property Rights Holder
      橋本功二、アタカ大機(株)
    • Industrial Property Number
      2007-203564
    • Filing Date
      2007-08-03
    • Related Report
      2007 Annual Research Report

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Published: 2007-04-01   Modified: 2016-04-21  

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