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Local fields in a colossal magnetoresistive manganite observed by a nuclear technique

Research Project

Project/Area Number 20612005
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Quantum beam science
Research InstitutionOsaka University

Principal Investigator

SATO Wataru  Osaka University, 物質化学系, 准教授 (90333319)

Co-Investigator(Kenkyū-buntansha) OHKUBO Yoshitaka  京都大学, 原子炉実験所, 教授 (70201374)
UENO Hideki  理化学研究所, 仁科加速器研究センター, 専任研究員 (50281118)
Co-Investigator(Renkei-kenkyūsha) IMAI Nobuaki  高エネルギー加速器研究機構, 素粒子原子核研究所, 助教 (80373273)
Project Period (FY) 2008 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2010: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2009: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2008: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Keywords超微細相互作用 / 超巨大磁気抵抗 / RIビーム / 摂動角相関 / ペロブスカイト / マンガン酸化物 / γ線摂動角相関 / ペロフスカイト / 核物性 / マンガナイト
Research Abstract

Perovskite manganese oxides are known to exhibit the effect of colossal magnetoresistance, a phenomenon that electrical resistivity undergoes a drastic change at the transition temperature. Because of this unique physical property, much attention has been given to these oxides aiming at wide industrial applications. In order to realize practical use of these compounds, it is of importance to obtain information on local fields in the material as well as macroscopic quantities such as resistivity and magnetization. From this point of view, we have applied the time-differential perturbed angular correlation (TDPAC) method to a study of a perovskite La_<0.7>Ca_<0.3>MnO_3 (T_c~245K). The TDPAC spectra show that Ce ions introduced into the La (Ca) site as impurities feel transferred field from Mn ions, whereas no internal field impinges on Cd ions at the substitutional La (Ca) site. These observations suggest that the magnetic field on the Ce nucleus arises from the spin polarization of a 4f electron as in the trivalent state.

Report

(4 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • 2008 Annual Research Report
  • Research Products

    (22 results)

All 2011 2010 2009 2008 Other

All Journal Article (14 results) (of which Peer Reviewed: 14 results) Presentation (8 results)

  • [Journal Article] Remarkable improvement of the signal-to-noise ratio of ^<57>Mn in-beam Mossbauer spectroscopy2011

    • Author(s)
      T.Nagatomo, Y.Kobayashi, M.K.Kubo, Y.Yamada, M.Mihara, W.Sato, J.Miyazaki, S.Sato, A.Kitagawa
    • Journal Title

      Nuclear Instruments and Methods in Physics Research B 269

      Pages: 455-459

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Electric field gradient at impunity sites in Ga-doped ZnO2011

    • Author(s)
      W.Sato, et al.
    • Journal Title

      Radiochimica Acta

      Volume: in Press

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Remarkable improvement of the signal-to-noise ratio of Mn^<57>/Fe^<57> in beam Mossbauers pectroscopy2011

    • Author(s)
      T.Nagatomo, et al.
    • Journal Title

      Nuclear Instruments and Methods in Physics Research B

      Volume: 269 Pages: 455-459

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Anticoincidence measurement of ^<57>Fe Mossbauer spectra obtained after ^<57>Mn implantation : Application to Fe in α-Al_2O_32010

    • Author(s)
      Y.Kobayashi, T.Nagatomo, Y.Yamada, M.Mihara, W.Sato, J.Miyazaki, S.Sato, A.Kitagawa, M.K.Kubo
    • Journal Title

      Hyperfine Interactions 198

      Pages: 173-178

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Anticoincidence measurement of Me^<57> mossbauer spectra obtained after Mn^<57> implantation : Apphcation to Fe in a-Al_2O_32010

    • Author(s)
      Y.Kobayashi, et al.
    • Journal Title

      Hyperfine Interactions

      Volume: 198 Pages: 173-178

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Anionic fluoro complex of element 105, Db2009

    • Author(s)
      Yoshitaka Kasamatsu, et al.
    • Journal Title

      Chemistry Letters 38

      Pages: 1084-1085

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Oxidation of element 102, nobelium, with flow electrolytic column chromatography on an atom-at-a-time scale2009

    • Author(s)
      Atsushi Toyoshima, et al.
    • Journal Title

      Journal of the American Chemical Society 131

      Pages: 9180-9181

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Adsorption of Db and its homologues Nb and Ta, and the pseudo-homologue Pa on anion-exchange resin in HF solution2009

    • Author(s)
      K.tsukada, et al.
    • Journal Title

      Radiochimica Acta 97

      Pages: 83-89

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Local fields and conduction-electron behavior at impurity sites in indium-doped ZnO2008

    • Author(s)
      W.Sato, Y.Itsuki, S.Morimoto, H.Susuki, S.Nasu, A.Shinohara, Y.Ohkubo
    • Journal Title

      Physical Review B 78

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Rattling motion of ^<140>Ce(←^<140>La)confined in the hexaboride cage2008

    • Author(s)
      W.Sato, A.Shinohara, Y.Ohkubo
    • Journal Title

      Physical Review B 78

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Temperature-dependent behavior of impurity atoms implanted in highly oriented pyrolytic graphite-An application of a new online TDPAC method2008

    • Author(s)
      Wataru Sato, Hideki Ueno, Hiroshi Watanabe, Hisanori Miyoshi, Akihiro Yoshimi, Daisuke Kameda, Takashi Ito, Kenzi Shimada, Jou Kaihara, Shinichi Suda, Yoshio Kobayashi, Atsushi Shinohara, Yoshitaka Ohkubo, Koichiro Asahi
    • Journal Title

      Journal of the Physical Society of Japan 77

    • NAID

      110006933502

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Local fields and conduction-electron behavior at impurity sites in indium-doped ZnO2008

    • Author(s)
      W. Sato
    • Journal Title

      Physical Review B 78

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Observation of local fields at^<111>・Cd(←^<111>In)sites in aluminum-doped ZnO2008

    • Author(s)
      W. Sato
    • Journal Title

      Journal of the Physical Society of Japan 77

    • NAID

      110006969316

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Electric field gradient at impurity sites in Ga-doped ZnO

    • Author(s)
      W.Sato, Y.Ohkubo, Y.Itsuki, S.Komatsuda, D.Minami, T.Kubota, S.Kawata, A.Yokoyama, T.Nakanishi
    • Journal Title

      Radiochimica Acta in press.

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Presentation] Local fields at impurity sites in ZnO observed by the TDPAC method2010

    • Author(s)
      W.Sato, S.Komatsuda, Y.Itsuki, Y.Ohkubo
    • Organizer
      2010 International Chemical Congress of Pacific Basin Societies
    • Place of Presentation
      Hilton Hawaiian Village(USA).
    • Year and Date
      2010-12-18
    • Related Report
      2010 Final Research Report
  • [Presentation] Local fields at impurity sites in ZnO observed by the TDPAC Method2010

    • Author(s)
      W.Sato
    • Organizer
      2010 International Chemical Congress of Pacific Basin Societies
    • Place of Presentation
      Hilto Hawaiian Village(U.S.A.)
    • Year and Date
      2010-12-18
    • Related Report
      2010 Annual Research Report
  • [Presentation] ^<111>Cdプローブを用いた酸化亜鉛の局所場観察2010

    • Author(s)
      佐藤渉、小松田沙也加、今川恵里、大久保嘉高、山田康洋
    • Organizer
      「短寿命核および放射線を用いた物性研究(III)」専門研究会
    • Place of Presentation
      京都大学原子炉実験所事務棟(大阪府)
    • Year and Date
      2010-11-25
    • Related Report
      2010 Final Research Report
  • [Presentation] ペロブスカイト型マンガン酸化物の超微細場測定2010

    • Author(s)
      佐藤渉、南大地、長明彦、佐藤哲也、大久保嘉高
    • Organizer
      2010日本放射化学会年会
    • Place of Presentation
      大阪大学銀杏会館(大阪府)
    • Year and Date
      2010-09-28
    • Related Report
      2010 Final Research Report
  • [Presentation] γ線摂動角相関法による酸化亜鉛中の局所場観察2010

    • Author(s)
      佐藤渉
    • Organizer
      第6回 停止・低速不安定核ビームを用いた核分光研究会
    • Place of Presentation
      東京工業大学 (東京)
    • Year and Date
      2010-03-01
    • Related Report
      2009 Annual Research Report
  • [Presentation] 第13族元素をドープした酸化亜鉛中の局所場観察2009

    • Author(s)
      佐藤渉、大久保嘉高、小松田沙也加、南大地、窪田瞳子、山田康洋、横山明彦、中西孝
    • Organizer
      「短寿命核および放射線を用いた物性研究(II)」専門研究会
    • Place of Presentation
      京都大学原子炉実験所事務棟(大阪府)
    • Year and Date
      2009-12-17
    • Related Report
      2010 Final Research Report
  • [Presentation] 不純物をドープした酸化亜鉛中の局所場観察2009

    • Author(s)
      佐藤渉、大久保嘉高、横山明彦、中西孝
    • Organizer
      2009日本放射化学会年会
    • Place of Presentation
      日本大学文理学部百周年記念館(東京都)
    • Year and Date
      2009-09-28
    • Related Report
      2010 Final Research Report
  • [Presentation] RIビームを用いた摂動角相関法による物性研究2008

    • Author(s)
      佐藤 渉
    • Organizer
      第5回 停止・低速不安定核ビームを用いた核分光研究会
    • Place of Presentation
      大阪大学(豊中)
    • Year and Date
      2008-12-25
    • Related Report
      2008 Annual Research Report

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Published: 2008-04-01   Modified: 2016-04-21  

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