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Generation and catalysis of Bronsted acid site on the surface of ceramics

Research Project

Project/Area Number 21760627
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeSingle-year Grants
Research Field Catalyst/Resource chemical process
Research InstitutionKyoto University

Principal Investigator

SHISHIDO Tetsuya  Kyoto University, 大学院・工学研究科, 准教授 (80294536)

Project Period (FY) 2009 – 2010
Project Status Completed (Fiscal Year 2010)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2010: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2009: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Keywords固体酸触媒 / セラミックス / ブレンスレッド / ニオブ / タンタル / セラミック / ブレンステッド
Research Abstract

Nb_2O_5/Al_2O_3 and Ta_2O_5/Al_2O_3 catalysts calcined at high temperatures exhibited the Bronsted acid property. A monolayer of niobic acid- and tantalum acid-like compounds, which have distorted octahedral symmetry, was stabilized over Nb_2O_5/Al_2O_3 and Ta_2O_5/Al_2O_3 catalysts calcined at high temperatures. The two-dimensional Nb-O-Nb network and Ta-O-Ta network of stabilized niobic acid- and tantalum acid-like compounds account for the generation of Bronsted acid sites.

Report

(3 results)
  • 2010 Annual Research Report   Final Research Report ( PDF )
  • 2009 Annual Research Report
  • Research Products

    (43 results)

All 2011 2010 2009 Other

All Journal Article (4 results) (of which Peer Reviewed: 4 results) Presentation (38 results) Remarks (1 results)

  • [Journal Article] Generation of Bronsted Acid Over Alumina-Supported Niobia Calcined at High Temperatures2010

    • Author(s)
      Shishido, Tetsuya, Kitano, Tomoyuki, Teramura, Kentaro, Tanaka, Tsunehiro
    • Journal Title

      Topics in Catalysis 53(7-10)(有)

      Pages: 672-677

    • Related Report
      2010 Final Research Report
    • Peer Reviewed
  • [Journal Article] Generation of Bronsted Acid Over Alumina-Supported Niobia Calcined at High Temperatures.2010

    • Author(s)
      T.Shishido., T.kitano., K.Teramaura., T, Tanaka.
    • Journal Title

      Topics in Catalysis

      Volume: 52 Pages: 672-677

    • Related Report
      2010 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Generation of Bronsted Acid Over Alumina-Supported Niobia Calcined at High Temperatures2010

    • Author(s)
      T.Shishido, T.Kitano, K.Teramura, T.Tanaka
    • Journal Title

      Topics in Catalysis

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Bronsted Acid Generation over Alumina-Supported Niobia by Calcination at 1173K2009

    • Author(s)
      T.Shishido, T.Kitano, K.Teramura, T.Tanaka
    • Journal Title

      Catalysis Letters 128

      Pages: 1057-1061

    • NAID

      10026055417

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Presentation] アルミナ上のニオブ酸化物モノレイヤーの構造と酸性質2011

    • Author(s)
      北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      日本化学会第91春季年会
    • Place of Presentation
      横浜
    • Year and Date
      2011-03-27
    • Related Report
      2010 Final Research Report
  • [Presentation] アルミナ上のニオブ酸化物モノレイヤーの構造と酸性質2011

    • Author(s)
      北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      日本化学会第91春季年会
    • Place of Presentation
      神奈川大学
    • Year and Date
      2011-03-26
    • Related Report
      2010 Annual Research Report
  • [Presentation] アルミナ上にモノレイヤーで担持されたタンタル酸化物の構造と酸性質2011

    • Author(s)
      岡崎翔太, 北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      日本化学会第91春季年会
    • Place of Presentation
      神奈川大学
    • Year and Date
      2011-03-26
    • Related Report
      2010 Annual Research Report
  • [Presentation] Structure and acid property of tantalum oxide on alumina2011

    • Author(s)
      岡崎翔太, 北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      触媒学会西日本地区第1回触媒表面科学研究発表会
    • Place of Presentation
      大阪大学
    • Year and Date
      2011-01-17
    • Related Report
      2010 Annual Research Report
  • [Presentation] Structure and acid property of tantalum oxide on alumina2011

    • Author(s)
      岡崎翔太, 北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      触媒学会西日本地区第1回触媒表面科学研究発表会
    • Place of Presentation
      大阪
    • Year and Date
      2011-01-14
    • Related Report
      2010 Final Research Report
  • [Presentation] Structure and acid property of niobium oxide supported on alumina calcined at high temperatures2010

    • Author(s)
      Tomoyuki Kitano, Tetsuya Shishido, Kentaro Teramura, Tsunehiro Tanaka
    • Organizer
      Pacifichem
    • Place of Presentation
      Hawaii, USA
    • Year and Date
      2010-12-15
    • Related Report
      2010 Final Research Report
  • [Presentation] Bronsted acid generation over supported tungsten oxide by calcination at high temperautres2010

    • Author(s)
      Toshio Uesaka, Tomoyuki Kitano, Tetsuya Shishido, Kentaro Teramura, Tsunehiro Tanaka
    • Organizer
      Pacifichem
    • Place of Presentation
      Hawaii, USA
    • Year and Date
      2010-12-15
    • Related Report
      2010 Final Research Report
  • [Presentation] Structure and acid property of niobium oxide supported on alumina calcined at high temperature2010

    • Author(s)
      T.kitano., T, Shishido., K, Teramura., T.Tanaka.
    • Organizer
      The 2010 International Chemical Congress of Pacific Basin Societies
    • Place of Presentation
      Hawaii Convention Center, USA
    • Year and Date
      2010-12-15
    • Related Report
      2010 Annual Research Report
  • [Presentation] Bronsted acid generation over supported tungsten oxide by calcination at high temperautres2010

    • Author(s)
      T.Uesaka., T.Kitano., T.Shishido, K.Teramura., T, Tanaka.
    • Organizer
      The 2010 International Chemical Congress of Pacific Basin Societies
    • Place of Presentation
      Hawaii Convention Center, USA
    • Year and Date
      2010-12-15
    • Related Report
      2010 Annual Research Report
  • [Presentation] 高温焼成したアルミナ担時金属酸化物の酸性質2010

    • Author(s)
      宍戸哲也・北野友之・上坂登志夫・岡崎翔太・寺村謙太郎・田中庸裕
    • Organizer
      第40回石油・石油化学討論会
    • Place of Presentation
      神戸
    • Year and Date
      2010-11-25
    • Related Report
      2010 Final Research Report
  • [Presentation] 高温焼成したアルミナ担時金属酸化物の酸性質2010

    • Author(s)
      宍戸哲也・北野友之・上坂登志夫・岡崎翔太・寺村謙太郎・田中庸裕
    • Organizer
      第40回石油・石油化学討論会
    • Place of Presentation
      神戸国際会議場
    • Year and Date
      2010-11-25
    • Related Report
      2010 Annual Research Report
  • [Presentation] 高温で焼成したアルミナ担持タングステン酸化物の酸性質2010

    • Author(s)
      上坂登志夫, 北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      第3回触媒表面化学研究発表会
    • Place of Presentation
      大阪
    • Year and Date
      2010-10-15
    • Related Report
      2010 Final Research Report
  • [Presentation] 高温で焼成したアルミナ担持タングステン酸化物の酸性質2010

    • Author(s)
      上坂登志夫, 北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      第3回触媒表面化学研究発表会
    • Place of Presentation
      関西大学
    • Year and Date
      2010-10-15
    • Related Report
      2010 Annual Research Report
  • [Presentation] 高温で焼成したアルミナ担持タングステン酸化物の酸性質2010

    • Author(s)
      上坂登志夫, 北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      第106回触媒討論会
    • Place of Presentation
      山梨大学
    • Year and Date
      2010-09-17
    • Related Report
      2010 Annual Research Report
  • [Presentation] 単層担持されたニオブ酸化物の酸性質2010

    • Author(s)
      北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      第106回触媒討論会
    • Place of Presentation
      甲府
    • Year and Date
      2010-09-15
    • Related Report
      2010 Final Research Report
  • [Presentation] 高温で焼成したアルミナ担持タングステン酸化物の酸性質2010

    • Author(s)
      上坂登志夫, 北野友之, 宍戸 哲也,寺村 謙太郎, 田中庸裕
    • Organizer
      第106回触媒討論会
    • Place of Presentation
      甲府
    • Year and Date
      2010-09-15
    • Related Report
      2010 Final Research Report
  • [Presentation] 単層担持されたニオブ酸化物の酸性質2010

    • Author(s)
      北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      第106回触媒討論会
    • Place of Presentation
      ベルクラシック甲府
    • Year and Date
      2010-09-15
    • Related Report
      2010 Annual Research Report
  • [Presentation] Structure and acid property of niobium oxide over alumina calcined at high temperature2010

    • Author(s)
      Tomoyuki Kitano, Tetsuya Shishido, Kentaro Teramura, Tsunehiro Tanaka
    • Organizer
      6th International Conference on Environmental Catalysis
    • Place of Presentation
      Beijing, China
    • Year and Date
      2010-09-12
    • Related Report
      2010 Final Research Report
  • [Presentation] Structure and acid property of niobium oxide over alumina calcined at high temperature2010

    • Author(s)
      T.kitano., T, Shishido., K.Teramura., T, Tanaka.
    • Organizer
      6th International Conference on Environmental Catalysis
    • Place of Presentation
      北京大学 中国
    • Year and Date
      2010-09-12
    • Related Report
      2010 Annual Research Report
  • [Presentation] Structure and acid property of alumina-supported niobium oxide calcined at high temperatures2010

    • Author(s)
      北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      TOCAT6/APCAT5
    • Place of Presentation
      札幌コンベンションセンター
    • Year and Date
      2010-07-20
    • Related Report
      2010 Annual Research Report
  • [Presentation] Structure and acid property of alumina-supported niobium oxide calcined at high temperatures2010

    • Author(s)
      北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      TOCAT6/APCAT5
    • Place of Presentation
      札幌
    • Year and Date
      2010-07-18
    • Related Report
      2010 Final Research Report
  • [Presentation] Bronsted acid generation over alumina-supported niobia by calcination at 1173 K2010

    • Author(s)
      Tetsuya Shishido, Tomoyuki Kitano, Kentaro Teramura, Tsunehiro Tanaka
    • Organizer
      Scientific Bases for the preparation of Heterogeneous Catalysts
    • Place of Presentation
      Belgium
    • Year and Date
      2010-07-12
    • Related Report
      2010 Final Research Report
  • [Presentation] Bronsted acid generation over alumina-supported niobia by calcination at 1173 K2010

    • Author(s)
      T, Shishido., T.Kitano., K.Teramura., T.Tanaka.
    • Organizer
      Scientific Bases for the preparation of Heterogeneous Catalysts
    • Place of Presentation
      Louvain-la-Neuve, Belgium
    • Year and Date
      2010-07-12
    • Related Report
      2010 Annual Research Report
  • [Presentation] 高温で焼成したアルミナ担持タングステン酸化物の酸性質2010

    • Author(s)
      上坂登志夫, 北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      石油学会第59回研究発表会
    • Place of Presentation
      船堀
    • Year and Date
      2010-05-20
    • Related Report
      2010 Final Research Report
  • [Presentation] 高温で焼成したアルミナ担持タングステン酸化物の酸性質2010

    • Author(s)
      上坂登志夫, 北野友之, 宍戸哲也, 寺村謙太郎, 田中庸裕
    • Organizer
      石油学会 第59回研究発表会
    • Place of Presentation
      タワーホール船堀
    • Year and Date
      2010-05-20
    • Related Report
      2010 Annual Research Report
  • [Presentation] アルミナ上に担持されたタンタル酸化物の構造と酸性質2010

    • Author(s)
      岡崎翔太・北野友之・宍戸哲也・寺村謙太郎・田中庸裕
    • Organizer
      日本化学会第90回春季年会
    • Place of Presentation
      近畿大学
    • Year and Date
      2010-03-26
    • Related Report
      2009 Annual Research Report
  • [Presentation] アルミナ上に形成されたニオブ酸化物モノレイヤーの構造と酸性質2010

    • Author(s)
      北野友之・宍戸哲也・寺村謙太郎・田中庸裕
    • Organizer
      日本化学会第90回春季年会
    • Place of Presentation
      近畿大学
    • Year and Date
      2010-03-26
    • Related Report
      2009 Annual Research Report
  • [Presentation] アルミナ上に形成されたニオブ酸化物モノレイヤーの構造と酸性質2010

    • Author(s)
      北野友之・宍戸哲也・寺村謙太郎・田中庸裕
    • Organizer
      第105回触媒討論会
    • Place of Presentation
      京都テルサ
    • Year and Date
      2010-03-25
    • Related Report
      2009 Annual Research Report
  • [Presentation] 高温で焼成したNb_2O_5/Al_2O_3触媒の構造と酸性質2010

    • Author(s)
      宍戸哲也・北野友之・寺村謙太郎・田中庸裕
    • Organizer
      第105回触媒討論会
    • Place of Presentation
      京都テルサ
    • Year and Date
      2010-03-24
    • Related Report
      2009 Annual Research Report
  • [Presentation] セラミックス表面におけるブレンステッド酸性の発現とその構造2009

    • Author(s)
      宍戸哲也
    • Organizer
      触媒学会産学交流サロン
    • Place of Presentation
      東京
    • Year and Date
      2009-12-04
    • Related Report
      2010 Final Research Report
  • [Presentation] セラミックス表面におけるブレンステッド酸性の発現とその構浩2009

    • Author(s)
      宍戸哲也
    • Organizer
      触媒学会産学交流サロン
    • Place of Presentation
      日本教育会館
    • Year and Date
      2009-12-04
    • Related Report
      2009 Annual Research Report
  • [Presentation] Bronsted acid generation over alumina-supported niobia by calcinaned at 1173K2009

    • Author(s)
      T.Shishido, T.Kitano, K.Teramura, T.Tanaka
    • Organizer
      The 12th Japan-Korea Symposium on Catalysis
    • Place of Presentation
      秋田
    • Year and Date
      2009-10-15
    • Related Report
      2010 Final Research Report
  • [Presentation] Bronsted acid generation over alumina-supported niobia by calcinaned at 1173K2009

    • Author(s)
      T.Shishido, T.Kitano, K.Teramura, T.Tanaka
    • Organizer
      The 12th Japan-Korea Symposium on Catalysis
    • Place of Presentation
      秋田キャッスルホテル
    • Year and Date
      2009-10-15
    • Related Report
      2009 Annual Research Report
  • [Presentation] アルミナ担持ニオビアの構造と酸性質2009

    • Author(s)
      北野友之・宍戸哲也・寺村謙太郎・田中庸裕
    • Organizer
      第2回触媒表面化学研究発表会
    • Place of Presentation
      大阪
    • Year and Date
      2009-10-09
    • Related Report
      2010 Final Research Report
  • [Presentation] アルミナ上に担持されたニオブ酸化物の構造と酸性質2009

    • Author(s)
      北野友之・宍戸哲也・寺村謙太郎・田中庸裕
    • Organizer
      第104回触媒討論会
    • Place of Presentation
      宮崎大学工学部
    • Year and Date
      2009-09-30
    • Related Report
      2009 Annual Research Report
  • [Presentation] アルミナ上に担持されたニオブ酸化物の構造と酸性質2009

    • Author(s)
      北野友之・宍戸哲也・寺村謙太郎・田中庸裕
    • Organizer
      第104回触媒討論会
    • Place of Presentation
      宮崎
    • Year and Date
      2009-09-29
    • Related Report
      2010 Final Research Report
  • [Presentation] 高温焼成Nb2O5/Al2O3触媒のBronsted酸性2009

    • Author(s)
      宍戸哲也・北野友之・寺村謙太郎・田中庸裕
    • Organizer
      石油学会第58回研究発表会
    • Place of Presentation
      船堀
    • Year and Date
      2009-05-20
    • Related Report
      2010 Final Research Report
  • [Presentation] 高温焼成Nb_2O_5/Al_2O_3触媒のBronsted酸性2009

    • Author(s)
      宍戸哲也・北野友之・寺村謙太郎・田中庸裕
    • Organizer
      石油学会 第58回研究発表会
    • Place of Presentation
      タワーホール船堀
    • Year and Date
      2009-05-20
    • Related Report
      2009 Annual Research Report
  • [Remarks] ホームページ等

    • Related Report
      2010 Final Research Report

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Published: 2009-04-01   Modified: 2016-04-21  

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