Development of minor-metal recovery technology using biovolatilization from waste and wastewater

• Project/Area Number: 22310047
• Research Category: Grant-in-Aid for Scientific Research (B)
• Allocation Type: Single-year Grants
• Section: 一般
• Research Field: Environmental technology/Environmental materials
• Research Institution: Osaka University
• Principal Investigator: IKE Michihiko 大阪大学, 大学院・工学研究科, 教授 (40222856)
• Co-Investigator(Kenkyū-buntansha): SODA Satoshi 大阪大学, 大学院・工学研究科, 准教授 (30322176) ; SEI Kazunari 大阪大学, 大学院・工学研究科, 助教 (80324177)
• Co-Investigator(Renkei-kenkyūsha): YAMASHITA Mitsuo 芝浦工業大学, 工学部, 教授 (40220347)
• Project Period (FY): 2010 – 2012
• Project Status: Completed (Fiscal Year 2012)
• Budget Amount: ¥18,330,000 (Direct Cost: ¥14,100,000、Indirect Cost: ¥4,230,000); Fiscal Year 2012: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000); Fiscal Year 2011: ¥6,890,000 (Direct Cost: ¥5,300,000、Indirect Cost: ¥1,590,000); Fiscal Year 2010: ¥8,320,000 (Direct Cost: ¥6,400,000、Indirect Cost: ¥1,920,000)
• Keywords: リサイクル技術 / レアメタル回収 / バイオボラタリゼーション / セレン / テルル / レアメタル / 排水 / 資源循環 / セレニウム

Research Abstract

The technology for minor-metal removal and recovery from waste and wastewater using minor-metal volatilizations by microbe was developed. Bioreactor using strain NT-I, capable of an efficient volatilization of selenium, successfully removed 66 % of initial selenium in water phase, and recovered it as selenium solution of high purity. Three tellurite-tolerant bacterial strains were isolated, and their capabilities of tellurium volatilization were revealed.

Research Products

• [Journal Article] Effective selenium volatilization under aerobic conditions and recovery from the aqueous phase by Pseudomonas stutzeriNT-I (2013)
  • Author(s): Kagami, T., Narita, T., Kuroda, M., Notaguchi, E., Yamashita, M., Sei, K., Soda, S., Ike, M
  • Journal Title: Water Research Volume: 47 Pages: 1361-1368
  • Peer Reviewed
• [Journal Article] Effective selenium volatilization under aerobic conditions and recovery from the aqueous phase by Pseudomonas stutzeri NT-I (2013)
  • Author(s): Kagami, T., Narita, T., Kuroda, M., Notaguchi, E., Yamashita, M., Sei, K., Soda, S., Ike, M.
  • Journal Title: Water Research Volume: 47 Pages: 1361-1368
  • DOI: 10.1016/j.watres.2012.12.001
  • Peer Reviewed
• [Journal Article] Isolation and characterization of bacteria capable of reducing tellurium oxyanions to insoluble elemental tellurium for tellurium recovery from wastewater (2012)
  • Author(s): Kagami, T., Fudemoto, A., Fujimoto, N., Notaguchi, E., Kanzaki, M., Kuroda, M., Soda, S., Yamashita, M., Ike, M
  • Journal Title: Waste and Biomass Val ori zati on Volume: 3 Pages: 409-418
  • Peer Reviewed
• [Journal Article] Biotreatment of selenium refinery wastewater using pilot-scale granular sludge and swim-bed bioreactors augmented with a selenium-reducing bacterium Pseudomonas stutzeriNT-I. (2012)
  • Author(s): Soda, S., Takahashi, H., Kagami, T., Miyake, M., Notaguchi, E., Sei, K., Iwasaki, N., Ike, M
  • Journal Title: Japanese Journal of Water Treatment Biology Volume: 48 Pages: 63-71
  • NAID: 10030809041
  • Peer Reviewed
• [Journal Article] Biotreatment of selenium refinery wastewater using pilot-scale granular sludge and swim-bed bioreactors augmented with a selenium-reducing bacterium Pseudomonas stutzeri NT-I (2012)
  • Author(s): Soda, S., Takahashi, H., Kagami, T., Miyake, M., Notaguchi, E., Sei, K., Iwasaki, N., Ike, M.
  • Journal Title: Japanese Journal of Water Treatment Biology Volume: 48 Pages: 63-71
  • NAID: 10030809041
  • Peer Reviewed
• [Journal Article] Isolation and characterization of bacteria capable of reducing tellurium oxyanions to insoluble elemental tellurium for tellurium recovery from wastewater (2012)
  • Author(s): Kagami, T., Fudemoto, A., Fujimoto, N., Notaguchi, E., Kanzaki, M., Kuroda, M., Soda, S., Yamashita, M., Ike, M.
  • Journal Title: Waste and Biomass Valorization Volume: 3 Pages: 409-418
  • DOI: 10.1007/s12649-012-9145-3
  • Peer Reviewed
• [Journal Article] Characterization of Pseudomonas stutzeriNT-I capable of removing soluble selenium from the aqueous phase under aerobic conditions (2011)
  • Author(s): Kuroda, M., Notaguchi, E., Sato, A., Yoshioka, M., Hasegawa, A., Kagami, T., Narita, T., Yamashita, M., Sei, K., Soda, S., Ike, M
  • Journal Title: Journal of Bioscience and Bioengineering Volume: 112 Pages: 259-264
  • NAID: 110008790452
  • Peer Reviewed
• [Journal Article] Characterization of Pseudomonas stutzeri NT-I capable of removing soluble selenium from the aqueous phase under aerobic conditions (2011)
  • Author(s): M.Kuroda, E.Notaguchi, A.Sato, M.Yoshioka, A.Hasegawa, T.Kagami, T.Narita, M.Yamashita, K.Sei, S.Soda, M.Ike
  • Journal Title: Journal of Bioscience and Bioengineering Volume: VOL.112 Issue: 3 Pages: 259-264
  • DOI: 10.1016/j.jbiosc.2011.05.012
  • NAID: 110008790452
  • ISSN: 1389-1723
  • Peer Reviewed
• [Presentation] 二種の高濃度セレン酸還元細菌の セレン酸還元関連遺伝子群の解析 (2013)
  • Author(s): 黒田真史
  • Organizer: 日本生物工学会メタルバイオテクノロジー研究部会ミニセミナー
  • Place of Presentation: 北里大学相模原キャンパス
  • Invited
• [Presentation] Pseudomonas stutzeri NT-Iによるセレン酸還元機構の解析 (2013)
  • Author(s): 黒田真史，三輪恵美子，清和成，惣田訓，山下光雄，池道彦
  • Organizer: 日本農芸化学会２０１３年度大会
  • Place of Presentation: 東北大学川内北キャンパス
• [Presentation] Pseudomonas stutzeri NT-Iによる亜セレン酸還元および揮発性セレン生成に及ぼす通気条件および培地成分の影響 (2012)
  • Author(s): 樋口靖典、三輪恵美子、黒田真史、惣田訓、池道彦
  • Place of Presentation: 北里大学
  • Year and Date: 2012-11-25
• [Presentation] Pseudomonas stutzeriNT-Iを用いた水相からのセレン揮発化除去・回収プロセスの試行 (2012)
  • Author(s): 黒田真史、成田尚宣、三輪恵美子、鏡つばさ、惣田訓、山下光雄、池道彦
  • Place of Presentation: 神戸国際会議場
  • Year and Date: 2012-10-25
• [Presentation] Pseudomonas stutzeri NT-Iを用いた水相からのセレン揮発化除去・回収プロセスの 試行 (2012)
  • Author(s): 黒田真史，成田尚宣，三輪恵美子，鏡つばさ，惣田訓，山下光雄，池道彦
  • Organizer: 第６４回日本生物工学会大会
  • Place of Presentation: 神戸国際会議場
• [Presentation] 二種のセレン酸 還元菌のセレン酸還元関連遺伝子群の解析 (2012)
  • Author(s): 黒田真史，三輪恵美子，清和成，惣田訓，山下光雄，池道彦
  • Organizer: 日本水処理生物学会第49 回大会
  • Place of Presentation: 北里大学白金キャンパス
• [Presentation] Pseudomonas stutzeri NT-Iによる亜セレン酸還元および揮発性セレン生成に及ぼす通気条件および培地成分 の影響 (2012)
  • Author(s): 樋口靖典，三輪恵美子，黒田真史，惣田訓，池道彦
  • Organizer: 日本水処理生物学会第49 回大会
  • Place of Presentation: 北里大学白金キャンパス
• [Presentation] Isolation and characterization of bacteria capable of reducing tellurium oxyanions to insoluble elemental tellurium (2011)
  • Author(s): Kagami, T., Fudemoto, A., Fujimoto, N., Notaguchi, E., Kanzaki, M., Soda, S., Yamashita, M., Ike, M.
  • Organizer: Eco-mates 2011
  • Place of Presentation: ホテル阪急エキスポパーク
  • Year and Date: 2011-11-28
• [Presentation] セメント工場から発生するKパウダーからのセレン回収方法の基礎検討 (2011)
  • Author(s): 長谷川愛, 黒田真史, 花田晶子, 惣田訓, 山下光雄, 池道彦
  • Organizer: 第22回廃棄物資源循環学会研究発表会
  • Place of Presentation: 東洋大学白山第2キャンパス(東京都)
  • Year and Date: 2011-11-05
• [Presentation] Pseudomonas stutzeriNT-I capable of reducing selenate/selenite into elemental selenium and volatilizing them as methylated selenium; a versatile microbial agent for biotreatment/ bioremediation of selenium contamination (2011)
  • Author(s): Miwa, E., Kuroda, M., Notaguchi, E., Sato, A., Yoshioka, M., Hasegawa, A., Kagami, T., Sei, K., Soda, S., Yamashita, M., Ike, M.
  • Organizer: International Union of Microbiological Societies 2011 Congress
  • Place of Presentation: 札幌市産業振興センター
  • Year and Date: 2011-09-07
• [Presentation] Pseudomonas stutzeri NT-I capable of reducing selenate/selenite into elemental selenium and volatilizing them as methylated selenium ; a versatile microbial agent for biotreatment/bioremediation of selenium contamination (2011)
  • Author(s): E.Miwa, M.Kuroda, E.Notaguchi, A.Sato, M.Yoshioka, A.Hasegawa, T.Kagami, K.Sei, S.Soda, M.Yamashita, M.Ike
  • Organizer: International Union of Microbiological Societies 2011 Congress
  • Place of Presentation: 札幌市産業振興センター(北海道)
  • Year and Date: 2011-09-07
• [Presentation] Isolation and characterization of bacteria capable of reducing tellurium oxyanions to insoluble elemental tellurium (2011)
  • Author(s): T.Kagami, A.Fudemoto, N.Fujimoto, E.Notaguchi, M.Kanzaki, S.Soda, M.Yamashita, M.Ike
  • Organizer: Eco-mates 2011
  • Place of Presentation: ホテル阪急エキスポパーク(大阪府)
• [Presentation] Pseudomonas stutzeri NT-Iのセレン酸還元能変異株の取得とその解析 (2010)
  • Author(s): 三輪恵美子, 黒田真史, 柏雅美, 清和成, 惣田訓, 池道彦, 山下光雄
  • Organizer: 日本水処理生物学会第47回大会
  • Place of Presentation: 筑波大学会館(つくば市)
  • Year and Date: 2010-11-17
• [Presentation] Pseudomonas stutzeri NT-Iのセレン酸還元関連遺伝子群の単離および解析 (2010)
  • Author(s): 黒田真史, 三輪恵美子, 柏雅美, 清和成, 惣田訓, 山下光雄, 池道彦
  • Organizer: 第62回日本生物工学会大会
  • Place of Presentation: 宮崎シーガイアワールドコンベンションセンターサミット (宮崎市)
  • Year and Date: 2010-10-27
• [Presentation] The characterization of the selenium volatilization by Pseudomonas stutzeri NT-I (2010)
  • Author(s): Tsubasa Kagami, Mitsuo Yamashita, Masashi Kuroda, Kazunari Sei, Satoshi Soda, Michihiko Ike
  • Organizer: 第62回日本生物工学会大会
  • Place of Presentation: 宮崎シーガイアワールドコンベンションセンターサミット (宮崎市)
  • Year and Date: 2010-10-27