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Development of Waste Treatment Process by Water Plasmas

Research Project

Project/Area Number 23310052
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental technology/Environmental materials
Research InstitutionKyushu University (2012-2013)
Tokyo Institute of Technology (2011)

Principal Investigator

WATANABE Takayuki  九州大学, 工学(系)研究科(研究院), 教授 (40191770)

Co-Investigator(Kenkyū-buntansha) SHIGETA Masaya  大阪大学, 接合科学研究所, 准教授 (30431521)
Project Period (FY) 2011-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥19,630,000 (Direct Cost: ¥15,100,000、Indirect Cost: ¥4,530,000)
Fiscal Year 2013: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2012: ¥7,800,000 (Direct Cost: ¥6,000,000、Indirect Cost: ¥1,800,000)
Fiscal Year 2011: ¥10,270,000 (Direct Cost: ¥7,900,000、Indirect Cost: ¥2,370,000)
Keywords熱プラズマ / 水プラズマ / 大気圧プラズマ / 廃棄物処理 / 有機物分解 / エマルション / フェノール水溶液 / アーク変動 / OHラジカル / CHラジカル
Research Abstract

A DC arc water plasma torch which is operated at atmospheric pressure by using evaporated cooling water as plasma forming gas directly. Since a large amount of H, O, and OH radicals are generated in water plasma, decomposition of hazardous materials and waste are accelerated in the treatment of water-soluble organic compounds. Since there are many water-insoluble organic wastes as well as water soluble organic waste, their decomposition was attempted in the present work. Reaction mechanism was investigated in the decomposition region with high-temperature over 10,000 K and the recombination region with 1,000 K. The intermediate products of CH and CH3 radicals were identified, and their contribution on the decomposition mechanism was clarified.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (62 results)

All 2014 2013 2012 2011 Other

All Journal Article (16 results) (of which Peer Reviewed: 14 results) Presentation (44 results) (of which Invited: 6 results) Remarks (2 results)

  • [Journal Article] Decomposition of Glycerine by DC Water Plasmas at Atmospheric Pressure2013

    • Author(s)
      Takayuki Watanabe and Narengerile
    • Journal Title

      Plasma Science and Technology

      Volume: Vol.15 , No.4 Pages: 357-361

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Liquid Waste Decomposition by Long DC Arc under Atmospheric Pressure2013

    • Author(s)
      TianMing Li, Takayuki Watanabe, Kaoru Ochi, and Koji Otsuki
    • Journal Title

      Chemical Engieering Journal

      Volume: Vol.231 Pages: 152-162

    • Related Report
      2013 Annual Research Report 2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Numerical Analysis of Temperature Distribution in Long DC Arc Thermal Plasma for Waste Treatment2013

    • Author(s)
      Sooseok Choi, TianMing Li, Takashi Nakayama, Koji Otsuki, and Takayuki Watanabe
    • Journal Title

      Journal of Chemical Engineering Japan

      Volume: Vol.46 , No. 3 Pages: 201-208

    • NAID

      10031159965

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Numerical Study on Leading-Edge Receptivity to Freestream Vertical Vorticity2013

    • Author(s)
      Yu Nishio, Masaya Shigeta, Seiichiro Izawa, Yu Fukunishi
    • Journal Title

      Journal of Fluid Science and Technology

      Volume: Vol.8, No.1 Pages: 136-145

    • NAID

      130003366704

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Numerical Study on Leading-Edge Receptivity to Freestream Vertical Vorticity2013

    • Author(s)
      Yu Nishio, Masaya Shigeta, Seiichiro Izawa, Yu Fukunishi
    • Journal Title

      Journal of Fluid Science and Technology

      Volume: 8 Issue: 1 Pages: 136-145

    • DOI

      10.1299/jfst.8.136

    • NAID

      130003366704

    • ISSN
      1880-5558
    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Role of CH, CH_3 , and OH Radicals in Organic Compound Decomposition by Water Plasmas2012

    • Author(s)
      Takayuki Watanabe, Narengerile, and Hiroshi Nishioka
    • Journal Title

      Plasma Chemistry and Plasma Processing

      Volume: Vol.32, No.1 Pages: 123-140

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Decomposition of 1-Decanol Emulsion by Water Plasma Jet2012

    • Author(s)
      Sooseok Choi and Takayuki Watanabe
    • Journal Title

      Transactions of IEEE on Plasma Science

      Volume: Vol.40, No.11 Pages: 2831-2836

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Decomposition of 1-Decanol Emulsion by Water Plasma at Atmospheric Pressure2012

    • Author(s)
      Sooseok Choi and Takayuki Watanabe
    • Journal Title

      Journal of Physics : Conference Series

      Volume: Vol.406 Pages: 12003-12003

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Time-Dependent 3-D Simulation of an Argon RF Inductively Coupled Thermal Plasma2012

    • Author(s)
      Masaya Shigeta
    • Journal Title

      Plasma Sources Science and Technology

      Volume: Vol.2, No.5 Pages: 55029-55029

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 水プラズマによる有害物質の分解システム2012

    • Author(s)
      渡辺隆行
    • Journal Title

      日本伝熱学会誌

      Volume: Vol.51, No.216 Pages: 42-48

    • NAID

      10030975357

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
  • [Journal Article] 多彩な魅力を持つプラズマプロセッシング ~鶏ふんからエネルギーを取り出す~2012

    • Author(s)
      渡辺隆行
    • Journal Title

      畜産コンサルタント

      Volume: Vol.48, No.570 Pages: 40-41

    • Related Report
      2013 Final Research Report 2012 Annual Research Report
  • [Journal Article] Decomposition of 1-Decanol Emulsion by Water Plasma at Atmospheric Pressure2012

    • Author(s)
      Sooseok Choi and Takayuki Watanabe
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 406 Pages: 12003-12003

    • DOI

      10.1088/1742-6596/406/1/012003

    • Related Report
      2012 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Role of CH, CH_3, and OH Radicals in Organic Compound Decomposition by Water Plasmas2012

    • Author(s)
      Takayuki Watanabe, Narengerile, Hiroshi Nishioka
    • Journal Title

      Plasma Chemistry and Plasma Processing

      Volume: 32 Pages: 123-140

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Decomposition of Glycerine by DC Water Plasmas at Atmospheric Pressure2012

    • Author(s)
      Takayuki Watanabe, Narengerile
    • Journal Title

      Plasma Science and Technology

      Volume: (印刷中)

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Role of CH, CH_3, and OH Radicals in Organic Compound Decomposition by Water Plasmas2011

    • Author(s)
      Narengerile and Takayuki Watanabe
    • Journal Title

      Proceedings of 20th International Symposium on Plasma Chemistry

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Role of CH, CH_3, and OH Radicals in Organic Compound Decomposition by Water Plasmas2011

    • Author(s)
      Narengerile, Takayuki Watanabe
    • Journal Title

      Proceedings of 20th International Symposium on Plasma Chemistry

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] 水プラズマを用いた難水溶性有機物の分解機構2014

    • Author(s)
      渡辺隆行, 石井佑昌, 田中学
    • Organizer
      化学工学会第79年会
    • Place of Presentation
      岐阜
    • Year and Date
      2014-03-19
    • Related Report
      2013 Final Research Report
  • [Presentation] Numerical Simulation of Multiple Thermal Plasma Plumes from a Jet Array2013

    • Author(s)
      Masaya Shigeta
    • Organizer
      The 12th International Conference on Fluid Control, Measurements, and Visualization
    • Place of Presentation
      奈良
    • Year and Date
      2013-11-22
    • Related Report
      2013 Annual Research Report 2013 Final Research Report
  • [Presentation] Decomposition Mechanism of 1-Decanol Emulsion by Water Plasma at Atmospheric Pressure2013

    • Author(s)
      Yusuke Ishii, Manabu Tanaka, Sooseok Choi, and Takayuki Watanabe
    • Organizer
      26th Symposium on Plasma Science for Material
    • Place of Presentation
      福岡
    • Year and Date
      2013-09-02
    • Related Report
      2013 Final Research Report
  • [Presentation] Thermal Plasma Processing for Environmental Application2013

    • Author(s)
      Takayuki Watanabe
    • Organizer
      International Conference on Green Energy and Technology
    • Place of Presentation
      北九州
    • Year and Date
      2013-08-25
    • Related Report
      2013 Final Research Report
  • [Presentation] ロング DC アークによる液体廃棄物の分解2013

    • Author(s)
      李天明, 渡辺隆行, 越智馨, 大槻浩司
    • Organizer
      化学工学会第78年会
    • Place of Presentation
      大阪
    • Year and Date
      2013-03-17
    • Related Report
      2013 Final Research Report
  • [Presentation] 熱プラズマ流動の非定常3次元シミュレーション2013

    • Author(s)
      茂田正哉
    • Organizer
      平成 24年度電気学会北陸支部シンポジウム「高気圧高熱流プラズマ応用における先端測定・数値解析技術」
    • Place of Presentation
      金沢
    • Year and Date
      2013-03-06
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Thermal Plasma Processing for Environmental Application2013

    • Author(s)
      Takayuki Watanabe
    • Organizer
      International Conference on Green Energy and Technology
    • Place of Presentation
      北九州市立大学
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] 水プラズマを用いた難水溶性有機物の分解機構2013

    • Author(s)
      渡辺隆行, 石井佑昌, 田中学
    • Organizer
      化学工学会第79年会
    • Place of Presentation
      岐阜大学
    • Related Report
      2013 Annual Research Report
  • [Presentation] Decomposition Mechanism of 1-Decanol Emulsion by Water Plasma at Atmospheric Pressure2013

    • Author(s)
      Yusuke Ishii, Manabu Tanaka, Sooseok Choi, and Takayuki Watanabe
    • Organizer
      26th Symposium on Plasma Science for Material
    • Place of Presentation
      九州大学
    • Related Report
      2013 Annual Research Report
  • [Presentation] ロングDCアークによる液体廃棄物の分解2013

    • Author(s)
      李天明, 渡辺隆行, 越智馨, 大槻浩司
    • Organizer
      化学工学会第78年会
    • Place of Presentation
      大阪大学
    • Related Report
      2012 Annual Research Report
  • [Presentation] 熱プラズマ流動の非定常3次元シミュレーション2013

    • Author(s)
      茂田正哉
    • Organizer
      平成24年度電気学会北陸支部シンポジウム「高気圧高熱流プラズマ応用における先端測定・数値解析技術」
    • Place of Presentation
      金沢
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 水プラズマによる有機物の分解機構2012

    • Author(s)
      渡辺隆行
    • Organizer
      第16回オーガナイズド混相流フォーラム
    • Place of Presentation
      松山
    • Year and Date
      2012-12-07
    • Related Report
      2013 Final Research Report 2012 Annual Research Report
  • [Presentation] Liquid Waste Decomposition by Long Arc Plasma of Direct Current Discharge2012

    • Author(s)
      TianMing Li, Takayuki Watanabe, Kaoru Ochi, and Koji Otsuki
    • Organizer
      11th Asia-Pasific Conference on Plasma Science and Technology
    • Place of Presentation
      京都
    • Year and Date
      2012-10-02
    • Related Report
      2013 Final Research Report
  • [Presentation] PFCs Decomposition by Long-Arc Plasma under Atmospheric Pressure2012

    • Author(s)
      Koji Otsuki, Kaoru Ochi, TianMing Li, Sooseok Choi, and Takayuki Watanabe
    • Organizer
      11th Asia-Pasific Conference on Plasma Science and Technology
    • Place of Presentation
      京都
    • Year and Date
      2012-10-02
    • Related Report
      2013 Final Research Report
  • [Presentation] Numerical Investigation of DC Plasma Jet Effect on Thermofluid Field in a DC-RF Hybrid Plasma Torch by Three-Dimensional Simulation2012

    • Author(s)
      Masaya Shigeta
    • Organizer
      The Ninth International Conference on Flow Dynamics
    • Place of Presentation
      仙台
    • Year and Date
      2012-09-20
    • Related Report
      2013 Final Research Report
  • [Presentation] DC-RFハイブリッドプラズマ流の非定常3次元数値シミュレーション2012

    • Author(s)
      茂田正哉
    • Organizer
      日本機械学会 2012年度年次大会
    • Year and Date
      2012-09-10
    • Related Report
      2013 Final Research Report
  • [Presentation] Decomposition of 1-Decanol Emulsion by Water Plasma at Atmospheric Pressure2012

    • Author(s)
      Sooseok Choi and Takayuki Watanabe
    • Organizer
      12th European Plasma Conferenc
    • Place of Presentation
      Bologna, Italy
    • Year and Date
      2012-06-25
    • Related Report
      2013 Final Research Report
  • [Presentation] 熱プラズマによる廃棄物処理2012

    • Author(s)
      渡辺隆行
    • Organizer
      科学工学技術委員会特別講演会
    • Place of Presentation
      東京
    • Year and Date
      2012-04-21
    • Related Report
      2013 Final Research Report 2012 Annual Research Report
    • Invited
  • [Presentation] 大気圧直流放電による水プラズマを用いた難水溶性有機物の分解2012

    • Author(s)
      太田剛, 崔秀錫, 渡辺隆行
    • Organizer
      化学工学会第77年会
    • Place of Presentation
      東京
    • Year and Date
      2012-03-15
    • Related Report
      2013 Final Research Report
  • [Presentation] 大気圧直流放電による水プラズマを用いた難水溶性有機物の分解2012

    • Author(s)
      太田剛, 崔秀錫, 渡辺隆行
    • Organizer
      化学工学会第77年会
    • Place of Presentation
      工学院大学
    • Year and Date
      2012-03-15
    • Related Report
      2011 Annual Research Report
  • [Presentation] 気液二相噴流の混合過程に関するSPH シミュレーション2012

    • Author(s)
      和田康典, 茂田正哉, 伊澤精一郎, 福西祐
    • Organizer
      日本機械学会東北支部第47 期総会・講演
    • Place of Presentation
      仙台
    • Year and Date
      2012-03-13
    • Related Report
      2013 Final Research Report
  • [Presentation] Decomposition of 1-Decanol Emulsion by Water Plasma at Atmospheric Pressure2012

    • Author(s)
      Sooseok Choi and Takayuki Watanabe
    • Organizer
      12th European Plasma Conference
    • Place of Presentation
      Bologna, Italy
    • Related Report
      2012 Annual Research Report
  • [Presentation] Liquid Waste Decomposition by Long Arc Plasma of Direct Current Discharge2012

    • Author(s)
      TianMing Li, Takayuki Watanabe, Kaoru Ochi, and Koji Otsuki
    • Organizer
      11th Asia-Pasific Conference on Plasma Science and Technology
    • Place of Presentation
      京都大学
    • Related Report
      2012 Annual Research Report
  • [Presentation] PFCs Decomposition by Long-Arc Plasma under Atmospheric Pressure2012

    • Author(s)
      Koji Otsuki, Kaoru Ochi, TianMing Li, Sooseok Choi, and Takayuki Watanabe
    • Organizer
      11th Asia-Pasific Conference on Plasma Science and Technology
    • Place of Presentation
      京都大学
    • Related Report
      2012 Annual Research Report
  • [Presentation] Numerical Investigation of DC Plasma Jet Effect on Thermofluid Field in a DC-RF Hybrid Plasma Torch by Three-Dimensional Simulation2012

    • Author(s)
      Masaya Shigeta
    • Organizer
      The 9th International Conference on Flow Dynamics
    • Place of Presentation
      仙台
    • Related Report
      2012 Annual Research Report
  • [Presentation] DC-RFハイブリッドプラズマ流の非定常3次元数値シミュレーション2012

    • Author(s)
      茂田正哉
    • Organizer
      日本機械学会2012年度年次大会
    • Place of Presentation
      金沢
    • Related Report
      2012 Annual Research Report
  • [Presentation] Thermal Plasma Characterization on Long DC Arc Discharge for Waste Treatment2011

    • Author(s)
      Sooseok Choi, TianMing Li, Watanabe Takayuki
    • Organizer
      Plasma Conference 2011
    • Place of Presentation
      金沢
    • Year and Date
      2011-11-23
    • Related Report
      2013 Final Research Report
  • [Presentation] Characteristic of Water Plasmas Generated from O/W Emulsion by DC Discharge under Atmospheric Pressure2011

    • Author(s)
      Go Ohta, Sooseok Choi, and Takayuki Watanabe
    • Organizer
      Plasma Conference 2011
    • Place of Presentation
      金沢
    • Year and Date
      2011-11-23
    • Related Report
      2013 Final Research Report
  • [Presentation] Thermal Plasma Characterization on Long DC Arc Discharge for Waste Treatment2011

    • Author(s)
      Sooseok Choi, TianMing Li, Watanabe Takayuki
    • Organizer
      Plasma Conference 2011
    • Place of Presentation
      石川県立音楽堂
    • Year and Date
      2011-11-23
    • Related Report
      2011 Annual Research Report
  • [Presentation] Characteristic of Water Plasmas Generated from O/W Emulsion by DC Discharge under Atmospheric Pressure2011

    • Author(s)
      Go Ohta, Sooseok Choi, Takayuki Watanabe
    • Organizer
      Plasma Conference 2011
    • Place of Presentation
      石川県立音楽堂
    • Year and Date
      2011-11-23
    • Related Report
      2011 Annual Research Report
  • [Presentation] Decomposition Mechanism of Organic Compounds by DC Water Plasmas at Atmospheric Pressure2011

    • Author(s)
      Takayuki Watanabe
    • Organizer
      3rd Round Table on Thermal Plasma for Industrial Applications
    • Place of Presentation
      Muldersdrift, South Africa
    • Year and Date
      2011-11-04
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Decomposition Mechanism of Organic Compounds by DC Water Plasmas at Atmospheric Pressure2011

    • Author(s)
      Takayuki Watanabe
    • Organizer
      3^<rd> Round Table on Thermal Plasma for Industrial Applications
    • Place of Presentation
      南アフリカ・マルダーズドリフト(招待講演)
    • Year and Date
      2011-11-04
    • Related Report
      2011 Annual Research Report
  • [Presentation] 大気圧直流放電による水プラズマを用いた液体廃棄物の処理2011

    • Author(s)
      太田剛, 崔秀錫, 渡辺隆行
    • Organizer
      熱工学カンファレンス
    • Place of Presentation
      浜松
    • Year and Date
      2011-10-30
    • Related Report
      2013 Final Research Report
  • [Presentation] ロング DCアークの変動現象の解析2011

    • Author(s)
      李天明, 崔秀錫, 渡辺隆行
    • Organizer
      熱工学カンファレンス
    • Place of Presentation
      浜松
    • Year and Date
      2011-10-30
    • Related Report
      2013 Final Research Report
  • [Presentation] 大気圧直流放電による水プラズマを用いた液体廃棄物の処理2011

    • Author(s)
      太田剛, 崔秀錫, 渡辺隆行
    • Organizer
      熱工学カンファレンス
    • Place of Presentation
      静岡大学
    • Year and Date
      2011-10-30
    • Related Report
      2011 Annual Research Report
  • [Presentation] ロングDCアークの変動現象の解析2011

    • Author(s)
      李天明, 崔秀錫, 渡辺隆行
    • Organizer
      熱工学カンファレンス
    • Place of Presentation
      静岡大学
    • Year and Date
      2011-10-30
    • Related Report
      2011 Annual Research Report
  • [Presentation] ナレンゲルン, 大気圧の水プラズマによる有機物分解におけるラジカルの寄与2011

    • Author(s)
      渡辺隆行
    • Organizer
      化学工学会第43回秋季大会
    • Place of Presentation
      名古屋
    • Year and Date
      2011-09-15
    • Related Report
      2013 Final Research Report
  • [Presentation] 廃棄物処理用の水プラズマの放電特性2011

    • Author(s)
      李天明, 崔秀錫, 渡辺隆行
    • Organizer
      化学工学会第43回秋季大会
    • Place of Presentation
      名古屋
    • Year and Date
      2011-09-15
    • Related Report
      2013 Final Research Report
  • [Presentation] 大気圧の水プラズマによる有機物分解におけるラジカルの寄与2011

    • Author(s)
      渡辺隆行, ナレンゲルン
    • Organizer
      化学工学会第43回秋季大会
    • Place of Presentation
      名古屋工業大学
    • Year and Date
      2011-09-15
    • Related Report
      2011 Annual Research Report
  • [Presentation] 廃棄物処理用の水プラズマの放電特性2011

    • Author(s)
      李天明, 崔秀錫, 渡辺隆行
    • Organizer
      化学工学会第43回秋季大会
    • Place of Presentation
      名古屋工業大学
    • Year and Date
      2011-09-15
    • Related Report
      2011 Annual Research Report
  • [Presentation] Thermal Plasma Technology for Non-Degradable Greenhouse Gases Treatment2011

    • Author(s)
      Sooseok Choi, Sang Hee Hong, Dong-Wha Park, and Takayuki Watanabe
    • Organizer
      24th Symposium on Plasma Science for Materials
    • Place of Presentation
      大阪
    • Year and Date
      2011-07-20
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Spectroscopic Analysis for Organic Compound Decomposition Mechanism in Water Plasmas2011

    • Author(s)
      Narengerile and Takayuki Watanabe
    • Organizer
      24th Symposium on Plasma Science for Materials
    • Place of Presentation
      大阪
    • Year and Date
      2011-07-20
    • Related Report
      2013 Final Research Report
  • [Presentation] Thermal Plasma Technology for Non-Degradable Greenhouse Gases Treatment2011

    • Author(s)
      Sooseok Choi, Sang Hee Hong, Dong-Wha Park, Takayuki Watanabe
    • Organizer
      24th Symposium on Plasma Science for Materials
    • Place of Presentation
      大阪大学(招待講演)
    • Year and Date
      2011-07-20
    • Related Report
      2011 Annual Research Report
  • [Presentation] Spectroscopic Analysis for Organic Compound Decomposition Mechanism in Water Plasmas2011

    • Author(s)
      Narengerile, Takayuki Watanabe
    • Organizer
      24th Symposium on Plasma Science for Materials
    • Place of Presentation
      大阪大学
    • Year and Date
      2011-07-20
    • Related Report
      2011 Annual Research Report
  • [Remarks] 渡辺研究室の研究テーマ

    • URL

      http://www.chem-eng.kyushu-u.ac.jp/lab5/Pages/theme.html

    • Related Report
      2013 Annual Research Report
  • [Remarks] 渡辺研の研究テーマ

    • URL

      http://www.chem-eng.kyushu-u.ac.jp/lab5/Pages/theme.html

    • Related Report
      2012 Annual Research Report

URL: 

Published: 2011-04-06   Modified: 2019-07-29  

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