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Study of ultrafast dynamics in graphene by using high-order haromonic photoelectron spectroscopy

Research Project

Project/Area Number 23310086
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Nanomaterials/Nanobioscience
Research InstitutionNTT Basic Research Laboratories

Principal Investigator

OGURI Katsuya  日本電信電話株式会社NTT物性科学基礎研究所, 量子光物性研究部, 主任研究員 (10374068)

Co-Investigator(Kenkyū-buntansha) NAKANO Hidetoshi  東洋大学, 理工学部, 教授 (90393793)
HIBINO Hiroki  日本電信電話株式会社NTT 物性科学基礎研究所, 機能物質科学研究部, 部長 (60393740)
KATO Keiko  日本電信電話株式会社NTT 物性科学基礎研究所, 量子光物性研究部, 研究主任 (40455267)
SEKINE Yoshiaki  日本電信電話株式会社NTT 物性科学基礎研究所, 機能物質科学研究部, 研究主任 (70393783)
Project Period (FY) 2011-04-01 – 2014-03-31
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥18,200,000 (Direct Cost: ¥14,000,000、Indirect Cost: ¥4,200,000)
Fiscal Year 2013: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2012: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2011: ¥12,090,000 (Direct Cost: ¥9,300,000、Indirect Cost: ¥2,790,000)
Keywordsグラフェン / 超高速ダイナミクス / 時間分解光電子分光 / 表面増強ラマン散乱 / 電子位相緩和 / 高次高調波 / 時間分解ARPES / エピタキシャルグラフェン
Research Abstract

To clarify ultrafast relaxation dynamics in high quality and large-area graphene which is grown on a silicon carbide substarate by sublimating silicon, we have developed femtosecond time-resolved surface photoelectron spectroscopy based on a high-order harmonics source. By using this system, we clarified the surfce transport of photoexcited electron and hole on a semiconductor surface, thus showing the potential of this system for measuring ultrafast relaxation dynamics in graphene. We have also studied the surface-enhanced Raman scattering (SERS)of graphene grown on SiC by depositing Ag. The enhancement of the Raman spectrum in graphene reached more than 60. Moreover, we have successfully estimated a electron dephasing time of monolayer graphene to be approxiamtely 50 fs by using a time-resolved transient diffraction technique.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (34 results)

All 2014 2013 2012 2011 Other

All Journal Article (6 results) (of which Peer Reviewed: 2 results) Presentation (25 results) (of which Invited: 7 results) Remarks (3 results)

  • [Journal Article] High-Order Harmonic Photoelectron Spectroscopy System Towards Measuring Attosecond Electron Dynamics on Solid Surfaces2013

    • Author(s)
      K. Oguri, H. Nakano, K. Kato, T. Nishikawa, A. Ishizawa, H. Gotoh, K. Tateno, and T. Sogawa
    • Journal Title

      Multiphoton Processes and Attosecond Physics, Springer Proceedings in Physics

      Volume: Vol.125 Pages: 373-378

    • DOI

      10.1007/978-3-642-28948-4_62

    • ISBN
      9783642289477, 9783642289484
    • Related Report
      2013 Final Research Report
  • [Journal Article] Surface-enhanced Raman scattering of graphene on SiC2013

    • Author(s)
      Yoshiaki Sekine, Hiroki Hibino, Katsuya Oguri, Tatsushi Akazaki, Hiroyuki Kageshima, Masao Nagase, Kenichi Sasaki, and Hiroshi Yamaguchi
    • Journal Title

      NTT technical review

      Volume: 11 Pages: 1-6

    • Related Report
      2013 Annual Research Report
  • [Journal Article] SiC上グラフェンの表面増強ラマン散乱2013

    • Author(s)
      関根佳明, 日比野浩樹, 小栗克也, 赤崎達志, 影島博之, 永瀬雅夫, 佐々木健一, 山口浩司
    • Journal Title

      NTT技術ジャーナル

      Volume: 6 Pages: 22-26

    • Related Report
      2013 Annual Research Report
  • [Journal Article] High-order harmonic photoelectron spectroscopy system towards measuring attosecond electron dynamics on solid surfaces2013

    • Author(s)
      K. Oguri, H. Nakano, K. Kato, T. Nishikawa, A. Ishizawa, H. Gotoh, K. Tateno, and T. Sogawa
    • Journal Title

      Multiphoton Processes and Attosecond Physics edited by K. Yamanouchi and K. Midorikawa, Springer Proceedings in Physics

      Volume: 125 Pages: 373-378

    • Related Report
      2012 Annual Research Report
  • [Journal Article] Time-Resolved Surface Photoelectron Spectroscopy of Photoexcited Electron and Hole Dynamics on GaAs Using 92 eV Laser Harmonic Source2012

    • Author(s)
      K. Oguri, K. Kato, T. Nishikawa, H. Gotoh, K. Tateno, Te. Sogawa and H. Nakano
    • Journal Title

      Japanese Journal Applied Physics

      Volume: Vol.51 Pages: 72401-72401

    • NAID

      40019351105

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Time-Resolved Surface Photoelectron Spectroscopy of Photoexcited Electron and Hole Dynamics on GaAs Using 92 eV Laser Harmonic Source2012

    • Author(s)
      Katsuya Oguri, Keiko Kato, Tadashi Nishikawa, Hideki Gotoh, Kouta Tateno, Tetsuomi Sogawa, Hidetoshi Nakano
    • Journal Title

      Japanese Journal Applied Physics

      Volume: (印刷中)

    • NAID

      40019351105

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] Ultrafast Spectroscopy Based on High-Order Harmonic Sources for Sub-Cycle Dynamics in Solids2014

    • Author(s)
      K. Oguri, H. Mashiko, K. Kato, T. Sogawa, and H. Gotoh
    • Organizer
      The 5th Shanghai-Tokyo Advanced ResearchSymposium on Ultrafast Intense LaserScience (STAR5)
    • Place of Presentation
      Miyazaki, Japan
    • Year and Date
      2014-05-23
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Manipulation of optical field emitted from autoionizing transition stimulated by isolated attosecond pulse2014

    • Author(s)
      Hiroki Mashiko, Tomohiko Yamaguchi, Katsuya Oguri, Akira Suda, and Hideki Gotoh
    • Organizer
      19th International Conference on Ultrafast Phenomena (UP2014)
    • Place of Presentation
      Okinawa Convention Center, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] Temporal characterization of emitted field from autoionization state stimulated by isolated attosecond pulse2014

    • Author(s)
      Hiroki Mashiko, Tomohiko Yamaguchi, Katsuya Oguri, Akira Suda, and Hideki Gotoh
    • Organizer
      the Conference on Lasers and Electro-Optics (CLEO2014)
    • Place of Presentation
      San Jose Convention Center, U.S.A.
    • Related Report
      2013 Annual Research Report
  • [Presentation] Ultrafast spectroscopy based on high-order haromonic sources for sub-cycle dynamics in solids2014

    • Author(s)
      Katsuya Oguri, Hiroki Mashiko, Keiko Kato, Tetsuomi Sogawa and Hideki Gotoh
    • Organizer
      The 5th Shanghai-Tokyo Advanced Research on Ultrafast Intense Laser (STAR5)
    • Place of Presentation
      Seagaia Convention Center, Miyazaki, Japan
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Lifetime measurement for autoionizing transition with isolated attosecond pulse2014

    • Author(s)
      Hiroki Mashiko, Tomohiko Yamaguchi, Katsuya Oguri, Akira Suda, and Hideki Gotoh
    • Organizer
      The 3rd Advanced Lasers and Photon Sources (ALPS’14)
    • Place of Presentation
      PACIFICO YOKOHAMA, Yokohama, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] 時間分解自己回折法によるCVD グラフェンの位相緩和時間測定2014

    • Author(s)
      玉城智啓,小栗克弥,増子拓紀,加藤景子, 中野秀俊
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学、相模原
    • Related Report
      2013 Annual Research Report
  • [Presentation] 単一アト秒パルスを用いたネオン原子における自動電離過程の遷移操作2014

    • Author(s)
      増子 拓紀、山口 量彦、小栗 克弥、須田 亮,後藤 秀樹
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学、相模原
    • Related Report
      2013 Annual Research Report
  • [Presentation] SiC 上グラフェンナノリボンの偏光ラマン散乱分光2014

    • Author(s)
      関根佳明, 日比野浩樹, 小栗克弥, 影島博之, 佐々木健一, 赤崎達志, 村田祐也
    • Organizer
      第61回応用物理学会春季学術講演会
    • Place of Presentation
      青山学院大学、相模原
    • Related Report
      2013 Annual Research Report
  • [Presentation] Properties of graphene nanoribbons embedded in SiC2013

    • Author(s)
      Yoshiaki Sekine, Hiroki Hibino, Katsuya Oguri, Hiroyuki Kageshima,Kenichi Sasaki, and Tatsushi Akazaki
    • Organizer
      5th International Conferencs on Recent Progress in Graphene Research (PRGR2013)
    • Place of Presentation
      東京工業大学、東京
    • Related Report
      2013 Annual Research Report
  • [Presentation] 炭素K端領域(284 eV)アト秒パルスのダブルオプティカルゲート法を用いた最適化2013

    • Author(s)
      増子拓紀、小栗克弥、寒川哲臣
    • Organizer
      第60 回応用物理学会春季学術講演会
    • Place of Presentation
      厚木
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] Ultrafast diagnostics of photo-excited processes in solid using femtosecondlaser-based soft x-ray2012

    • Author(s)
      K. Oguri, H. Nakano, Y. Okano, T. Nishikawa, K.Kato, A. Ishizawa, T. Tsunoi, H. Gotoh, K. Tateno, and T. Sogawa
    • Organizer
      8th International Conference on Photo-Excited Processes and Applications (ICPEPA-8)
    • Place of Presentation
      Rochester, USA. pulse sources
    • Year and Date
      2012-08-17
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] Surface Carrier dynamics onSemiconductor Studied with Femtosecond Core-Level Photoelectron Spectroscopy Using Extreme Ultraviolet High-OrderHarmonic Source2012

    • Author(s)
      K. Oguri, T. Tsunoi, K. Kato, H. Nakano, T. Nishikawa, H. Gotoh, K. Tateno, and T. Sogawa
    • Organizer
      XVIIIth International Conference on Ultrafast Phenomena (UP2012)
    • Place of Presentation
      Lausanne Switzerland
    • Year and Date
      2012-07-10
    • Related Report
      2013 Final Research Report
  • [Presentation] 液体ヘリウム温度におけるグラファイトのコヒーレントフォノンダイナミクス2012

    • Author(s)
      加藤景子、小栗克弥、眞田治樹、俵毅彦、後藤秀樹、西川正、寒川哲臣
    • Organizer
      第59回応用物理学関係連合講演会
    • Place of Presentation
      早稲田大学(東京都)
    • Year and Date
      2012-03-18
    • Related Report
      2011 Annual Research Report
  • [Presentation] 高次高調波を用いたフェムト秒時間分解表面光電子分光法による過渡表面光起電力効果の観測2012

    • Author(s)
      小栗克弥、角井貴信、加藤景子、中野秀俊、西川正、後藤秀樹、舘野功太、片山郁文、武田淳、寒川哲臣
    • Organizer
      第59回応用物理学関係連合講演会
    • Place of Presentation
      早稲田大学(東京都)
    • Year and Date
      2012-03-18
    • Related Report
      2011 Annual Research Report
  • [Presentation] 時間分解表面光電子分光法による半導体表面ダイナミクスの計測2012

    • Author(s)
      角井貴信、小栗克弥、加藤景子、中野秀俊、西川正、後藤秀樹、舘野功太、片山郁文、武田淳、寒川哲臣
    • Organizer
      第7回ナノテク交流シンポジウム
    • Place of Presentation
      横浜市立大学(神奈川県)
    • Year and Date
      2012-03-02
    • Related Report
      2011 Annual Research Report
  • [Presentation] 超短パルス軟X線で見る物質の超高速ダイナミクス2012

    • Author(s)
      小栗克弥、中野秀俊、岡野泰彬、西川正、加藤景子、石澤淳、後藤秀樹、舘野功太、寒川哲臣
    • Organizer
      平成23年度「多元技術融合光プロセス研究会」第5回研究交流会
    • Place of Presentation
      産業技術総合研究所臨海副都心センター別館(東京都)
    • Year and Date
      2012-02-16
    • Related Report
      2011 Annual Research Report
  • [Presentation] Ultrafast surface photoelectron spectroscopy of GaAs with high-order harmonic generation (invited)2012

    • Author(s)
      K. Oguri, K. Kato, T. Nishikawa, A. Ishizawa, H. Gotoh, K. Tateno, T. Sogawa, and H. Nakano
    • Organizer
      The 3rd Shanghai-Tokyo Advanced Research Symposium on Ultrafast Intense Laser Science (STAR3)
    • Place of Presentation
      Odawara, Japan
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] urface Carrier dynamics on Semiconductor Studied with Femtosecond Core-Level Photoelectron Spectroscopy Using Extreme Ultraviolet High-Order Harmonic Source2012

    • Author(s)
      K. Oguri, T. Tsunoi, K. Kato, H. Nakano*, T. Nishikawa, H. Gotoh, K. Tateno, and T. Sogawa
    • Organizer
      XVIIIth International Conference on Ultrafast Phenomena (UP2012)
    • Place of Presentation
      Lausanne, Switzerland
    • Related Report
      2012 Annual Research Report
  • [Presentation] Ultrafast diagnostics of photo-excited processes in solid using femtosecond laser-based soft x-ray pulse sources2012

    • Author(s)
      K. Oguri, H. Nakano, Y. Okano, T. Nishikawa, K. Kato, A. Ishizawa, T. Tsunoi, H. Gotoh, K. Tateno, and T. Sogawa
    • Organizer
      8th International Conference on Photo-Excited Processes and Applications (ICPEPA-8)
    • Place of Presentation
      Rochester, U.S. A.
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 高次高調波を用いた原子一層オーダー固体表面のフェムト秒ダイナミクス計測2012

    • Author(s)
      小栗克弥
    • Organizer
      電気学会「光・量子ビームによるナノダイナミクス応用技術調査専門委員会」第5回専門委員会
    • Place of Presentation
      東京
    • Related Report
      2012 Annual Research Report
    • Invited
  • [Presentation] 高次高調波を用いた時間分解光電子分光法による半導体表面ダイナミクス計測2011

    • Author(s)
      小栗克弥、加藤景子、石澤淳、西川正、後藤秀樹、舘野功太、寒川哲臣、中野秀俊
    • Organizer
      第6回レーザー学会専門委員会「レーザー駆動XUV~X線の産業応用専門委員会」
    • Place of Presentation
      東京八重洲ホール(東京都)(招待)
    • Year and Date
      2011-09-27
    • Related Report
      2011 Annual Research Report
  • [Presentation] Surface-enhanced Raman scattering of graphene on SiC2011

    • Author(s)
      Yoshiaki Sekine, Hiroki Hibino, Katsuya Oguri, Tatsushi Akazaki, Hiroyuki Kageshima, Masao Nagase, Hiroshi. Yamaguchi
    • Organizer
      6th International School and Conference on Spintronics and Quantum Information Technology (SPINTECH6)
    • Place of Presentation
      島根県立産業交流会館(くにびきメッセ)(島根県)
    • Year and Date
      2011-08-03
    • Related Report
      2011 Annual Research Report
  • [Presentation] High-order harmonic photoelectron spectroscopy system towards measuring attosecond electron dynamics on solid surfaces2011

    • Author(s)
      Katsuya Oguri, Hidetoshi Nakano, Keiko Kato, Tadashi Nishikawa, Atsushi Ishizawa, Hideki Gotoh, Kouta. Tateno, Tetsuomi Sogawa
    • Organizer
      The 3rd International Conference on Attosecond Physics (ATT03)
    • Place of Presentation
      北海道大学(北海道)
    • Year and Date
      2011-07-08
    • Related Report
      2011 Annual Research Report
  • [Presentation] SiC上グラフェンの表面増強ラマン散乱分光2011

    • Author(s)
      関根佳明、日比野浩樹、小栗克弥、赤崎達志、影島博之、永瀬雅夫、山口浩司
    • Organizer
      第30回電子材料シンポジウム
    • Place of Presentation
      ラフォーレ琵琶湖(滋賀県)
    • Year and Date
      2011-06-30
    • Related Report
      2011 Annual Research Report
  • [Presentation] Observation of photovoltage effect on GaAs surface with ultrafast high-order harmonic photoelectron spectroscopy2011

    • Author(s)
      Katsuya Oguri, Keiko Kato, Tadashi Nishikawa, Atsushi Ishizawa, Hideki Gotoh, Routa Tateno, Tetsuomi Sogawa, Hidetoshi Nakano
    • Organizer
      Joint Conference of The Fifth International Conference on the Science and Technology for Advanced Ceramics and The 2nd International Conference on Advanced Materials Development and Integration of Novel Structured Metallic and Inorganic Materials (STAC5-AMDI2)
    • Place of Presentation
      メルパルク横浜(神奈川県)
    • Year and Date
      2011-06-22
    • Related Report
      2011 Annual Research Report
  • [Remarks] ようこそ小栗 克弥のページへ

    • URL

      http://www.brl.ntt.co.jp/people/oguri/index.htm

    • Related Report
      2013 Annual Research Report
  • [Remarks] ようこそ小栗 克弥のページへ

    • URL

      http://www.brl.ntt.co.jp/people/oguri/index.htm

    • Related Report
      2012 Annual Research Report
  • [Remarks]

    • URL

      http://www.brl.ntt.co.jp/people/oguri/index.htm

    • Related Report
      2011 Annual Research Report

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Published: 2011-04-06   Modified: 2019-07-29  

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