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Improvement of polymer electrolyte fuel cell performance using gas diffusion layer with wettability distribution for water distribution control

Research Project

Project/Area Number 23360097
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Thermal engineering
Research InstitutionYokohama National University

Principal Investigator

UTAKA Yoshio  横浜国立大学, 工学(系)研究科(研究院), 教授 (50114856)

Co-Investigator(Kenkyū-buntansha) MATSUMOTO Hiroaki  横浜国立大学, 大学院工学研究院, 教授 (10251753)
ARAKI Takuto  横浜国立大学, 大学院工学研究院, 准教授 (90378258)
DAITOKU Tadafumi  秋田県立大学, システム科学技術部, 助教 (40452049)
CHIN Shigo  横浜国立大学, 大学院工学研究院, 研究教員 (60611275)
Project Period (FY) 2011-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥18,330,000 (Direct Cost: ¥14,100,000、Indirect Cost: ¥4,230,000)
Fiscal Year 2014: ¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2013: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2012: ¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2011: ¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Keywords燃料電池 / ガス拡散層 / 物質伝達 / 表面張力 / ぬれ性 / 拡散 / X線ラジオグラフィー / 熱物質伝達
Outline of Final Research Achievements

The objective of the study was to improve the PEFC performance with newly proposed hybrid GDL, in which different wettability areas were alternately arranged. It was shown that the apparent oxygen diffusivity was increased by using hybrid GDL in comparison with the normal GDL, elucidating the characteristics by the simultaneous measurement of oxygen diffusivity and visualization of water distribution by X-ray tomography. On the basis of those results, the improvement of the actual PEFC with parallel gas channels of 200 mm long was achieved with the combination of hybrid GDL and microgrooves in gas channels.

Report

(5 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (28 results)

All 2015 2014 2013 2012 2011

All Journal Article (12 results) (of which Peer Reviewed: 12 results,  Acknowledgement Compliant: 5 results) Presentation (14 results) (of which Invited: 1 results) Book (1 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] Proposal and Examination of Method of Water Removal from Gas Diffusion Layer by Applying Slanted Microgrooves inside Gas Channel in Separator to Improve Polymer Electrolyte Fuel Cell Performance2015

    • Author(s)
      Utaka, Y., Okabe, A. and Omori, Y.
    • Journal Title

      Journal of Power Sources

      Volume: 279 Pages: 533-579

    • DOI

      10.1016/j.jpowsour.2015.01.050

    • NAID

      120005553865

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Improvement of performance of polymer electrolyte fuel cell due to addition of micro-grooves as water removal mechanism2015

    • Author(s)
      是澤亮,宇高義郎
    • Journal Title

      Transactions of the JSME (in Japanese)

      Volume: 81 Issue: 824 Pages: 14-00537-14-00537

    • DOI

      10.1299/transjsme.14-00537

    • NAID

      130005066570

    • ISSN
      2187-9761
    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Water control by employing microgrooves inside gas channel for performance improvement in polymer electrolyte fuel cells2015

    • Author(s)
      Koresawa,R. and Utaka, Y.
    • Journal Title

      International Journal of Hydrogen Energy

      Volume: 0 Pages: 0-0

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Precise measurement of effective oxygen diffusivity for microporous media containing moisture by review of galvanic cell oxygen absorber configuration2014

    • Author(s)
      Koresawa,R. and Utaka, Y.
    • Journal Title

      International Journal of Heat and Mass Transfer

      Volume: 76 Pages: 549-558

    • DOI

      10.1016/j.ijheatmasstransfer.2014.05.005

    • NAID

      120005553862

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Improvement of Oxygen Diffusion Characteristics in Gas Diffusion Layer with Planer-distributed Wettability for Polymer Electrolyte Fuel Cell2014

    • Author(s)
      Koresawa,R. and Utaka, Y.
    • Journal Title

      Journal of Power Sources

      Volume: 271 Pages: 16-24

    • DOI

      10.1016/j.jpowsour.2014.05.151

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Numerical Analysis Considering the Effects of Liquid Water on PEMFC Unsteady Performance2014

    • Author(s)
      Fukuda, T. and Araki, T.
    • Journal Title

      ECS Transaction

      Volume: 64 Issue: 3 Pages: 581-592

    • DOI

      10.1149/06403.0581ecst

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 固体高分子形燃料電池内の液水分布状態可視化と非定常発電特性2014

    • Author(s)
      荒木拓人
    • Journal Title

      燃料電池

      Volume: 13 Pages: 9-13

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] ぬれ性分布を有するPEFC用ガス拡散層における酸素拡散促進と撥水材PTFE含有量の影響2013

    • Author(s)
      是澤 亮,大徳忠史,宇高義郎
    • Journal Title

      日本機械学会論文集(B編)

      Volume: 79 Pages: 1038-1050

    • NAID

      130003374798

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 固体高分子形燃料電池における壁面傾斜マイクログルーブを用いたガス拡散層からガスチャネルへの排水性向上2013

    • Author(s)
      岡部晃,宇高義郎
    • Journal Title

      日本機械学会論文集(B編)

      Volume: 79 Pages: 1866-1874

    • NAID

      130004555270

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Numerical Analysis of PEMFC Unsteady Performance Considering Water and Thermal Transport2013

    • Author(s)
      Takanori Fukuda, Akira Sato, Takuto Araki
    • Journal Title

      ECS Transaction

      Volume: 58 Pages: 9-13

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] ガルバニ電池式酸素吸収体を用いた多孔質体における酸素拡散係数測定の高精度化2011

    • Author(s)
      是澤亮, 大徳忠史, 宇高義郎
    • Journal Title

      日本機械学会論文集(B編)

      Volume: 77 Pages: 2191-2199

    • NAID

      130001433054

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Journal Article] ぬれ性分布を利用した固体高分子形燃料電池用ガス拡散層における液水分布の可視化と酸素拡散係数の同時計測2011

    • Author(s)
      是澤亮, 大徳忠史, 宇高義郎, 上杉健太朗
    • Journal Title

      日本機械学会論文集(B編)

      Volume: 77 Pages: 2019-2027

    • NAID

      130001433031

    • Related Report
      2011 Annual Research Report
    • Peer Reviewed
  • [Presentation] Effects Of Water Distribution Modes on Gas Diffussivity in PEMFC Gas Diffusion Layer2014

    • Author(s)
      Watanabe, K. and Araki, T.
    • Organizer
      The 25th International Symposium on Transport Phenomena (ISTP-25)
    • Place of Presentation
      Thailand
    • Year and Date
      2014-11-05 – 2014-11-07
    • Related Report
      2014 Annual Research Report
  • [Presentation] Development of Water Management Techniques for Each Component of a PEMFC2014

    • Author(s)
      Utaka, Y., Araki, T., Matsumoto, H., Munakata, T., Ito, H., Someya, S., Nakano, A., Zhang, J., Wang, S.
    • Organizer
      The 25th International Symposium on Transport Phenomena (ISTP-25)
    • Place of Presentation
      Thailand
    • Year and Date
      2014-11-05 – 2014-11-07
    • Related Report
      2014 Annual Research Report
  • [Presentation] PEFC内in-situ測定用マイクロ湿度センサの開発2014

    • Author(s)
      荒木拓人
    • Organizer
      公益財団法人 水素エネルギー製品研究試験センター 平成26年度 公開セミナー
    • Place of Presentation
      福岡
    • Year and Date
      2014-08-29
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Effect of Hydrophobic Polymer Concentration of Hydrophobic Region in Hybrid Type Gas Diffusion Layer on Apparent Oxygen Diffusivity2014

    • Author(s)
      Koresawa, R. Hozumi, Y. and Utaka, Y.,
    • Organizer
      JSSUME2014
    • Place of Presentation
      Yokohama
    • Year and Date
      2014-08-15 – 2014-08-16
    • Related Report
      2014 Annual Research Report
  • [Presentation] Control of Effective Oxygen Transfer Characteristics in Gas Diffusion Layer with Moisture for PEFC2014

    • Author(s)
      Koresawa,R. and Utaka, Y.
    • Organizer
      International Symposium on Convective Heat and Mass Transfer, CONV-14
    • Place of Presentation
      Turkey
    • Year and Date
      2014-06-08 – 2014-06-13
    • Related Report
      2014 Annual Research Report
  • [Presentation] Improvement of effective oxygen diffusivity measurement in micro porous media with moisture using a galvanic cell oxygen absorber2013

    • Author(s)
      Koresawa, R., Daitoku, T. and Utaka, Y.
    • Organizer
      8th World Conference on Experimental Heat Transfer, Fluid Mechanics, and Thermodynamics
    • Place of Presentation
      Lisbon, Portgul
    • Related Report
      2013 Annual Research Report
  • [Presentation] PEFCにおける傾斜マイクログルーブを用いた微細多孔体からガスチャネルへの排水性向上2013

    • Author(s)
      岡部晃,宇高義郎
    • Organizer
      第50回日本伝熱シンポジウム
    • Place of Presentation
      仙台
    • Related Report
      2013 Annual Research Report
  • [Presentation] ガルバニ電池酸素吸収体を用いた微細多孔質体の有効酸素拡散係数の測定精度の向上2013

    • Author(s)
      是澤亮,大徳忠史,宇高義郎
    • Organizer
      第50回日本伝熱シンポジウム
    • Place of Presentation
      仙台
    • Related Report
      2013 Annual Research Report
  • [Presentation] 固体高分子形燃料電池用ガス拡散層内液水移動制御による物質移動促進とガス拡散層内の液水分布の可視化2013

    • Author(s)
      是澤亮、宇高義郎
    • Organizer
      日本機械学会2013年度年次大会
    • Place of Presentation
      岡山
    • Related Report
      2013 Annual Research Report
  • [Presentation] Visualization of water droplets distributions inside PEMFC GDL2013

    • Author(s)
      Takuto Araki
    • Organizer
      Japan-Korea Joint Seminar on Heat Transfer VII
    • Place of Presentation
      福岡
    • Related Report
      2013 Annual Research Report
  • [Presentation] 固体高分子形燃料電池用ガス拡散層内液水移動制御による酸素移動促進2012

    • Author(s)
      宇高義郎
    • Organizer
      第49回日本伝熱シンポジウム
    • Place of Presentation
      富山
    • Related Report
      2012 Annual Research Report
  • [Presentation] ぬれ性分布を利用したマイクロポーラス層付きガス拡散層内の液水制御2012

    • Author(s)
      宇高義郎
    • Organizer
      第49回日本伝熱シンポジウム
    • Place of Presentation
      富山
    • Related Report
      2012 Annual Research Report
  • [Presentation] High precision measurement of apparent oxygen diffusion coefficient in gas diffusion layer of polymer electrolyte fuel cell using galvanic cell type oxygen absorber2011

    • Author(s)
      Koresawa, R., Daitoku, T., Utaka
    • Organizer
      Proc.of 22^<nd> International Conference on Transport Phenomena
    • Place of Presentation
      Delft, Netherland
    • Year and Date
      2011-11-10
    • Related Report
      2011 Annual Research Report
  • [Presentation] Simultaneous measurement of oxygen diffusivity and visualization of moisture distribution in gas diffusion layer with wettability distribution for improvement of polymer electrolyte fuel cell performance2011

    • Author(s)
      Koresawa, R., Daitoku, T., Utaka, Y., Uesugi
    • Organizer
      Proc.of 22^<nd> International Conference on Transport Phenomena
    • Place of Presentation
      Delft, Netherland
    • Year and Date
      2011-11-09
    • Related Report
      2011 Annual Research Report
  • [Book] Spring-8の高輝度放射光を利用したグリーンエネルギー分野における電池材料開発,第3章燃料電池,5固体高分子形燃料電池のイメージング2014

    • Author(s)
      宇高義郎,大徳忠史,是澤 亮
    • Total Pages
      259
    • Publisher
      シーエムシー出版
    • Related Report
      2013 Annual Research Report
  • [Patent(Industrial Property Rights)] 固体高分子型燃料電池2014

    • Inventor(s)
      宇高義郎、是澤亮
    • Industrial Property Rights Holder
      宇高義郎、是澤亮
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2014-162935
    • Filing Date
      2014-08-08
    • Related Report
      2014 Annual Research Report

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Published: 2011-04-06   Modified: 2019-07-29  

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