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Study on hybrid nuclide separation method by using solid-type extractants combined with atmospheric-pressure non-thermal plasma chemical conversion method.

Research Project

Project/Area Number 23360423
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Nuclear engineering
Research InstitutionNagaoka University of Technology (2012-2015)
Tokyo Institute of Technology (2011)

Principal Investigator

Suzuki Tatsuya  長岡技術科学大学, 工学(系)研究科(研究院), 教授 (70323839)

Co-Investigator(Kenkyū-buntansha) NOGAMI Masanobu  近畿大学, 理工学部, 教授 (50415866)
NOMURA Masao  東京工業大学, 原子炉工学研究所, 助教 (60100997)
Co-Investigator(Renkei-kenkyūsha) ARAI Tsuyoshi  芝浦工業大学, 工学部, 准教授 (60415867)
KOYAMA Shin-ichi  独立行政法人日本原子力研究開発機構, 大洗研究開発センター, 副主任研究員 (70421782)
OHSAKA Masahiko  独立行政法人日本原子力研究開発機構, 大洗研究開発センター, 研究員 (10421471)
Research Collaborator TACHIBANA Yu  長岡技術科学大学, 大学院工学研究科, 助教 (40634928)
SATO Nobuhiro  京都大学, 原子炉実験所, 助教 (10303918)
KITAGAKI Toru  
YAMASAKI Yuki  
TOMOBUCHI Yusuke  
KANESHIKI Toshitaka  
HARATANI Tomohiro  
NISHIDA Tetsuhiro  
TAJIMA Shinya  
ISHII Ryota  
SAKAMOTO Hisanori  
Project Period (FY) 2011-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥17,810,000 (Direct Cost: ¥13,700,000、Indirect Cost: ¥4,110,000)
Fiscal Year 2015: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Fiscal Year 2014: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Fiscal Year 2013: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2012: ¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2011: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Keywords核燃料サイクル / 使用済み燃料 / 核種分離 / プラズマ化学 / 大気圧非平衡プラズマ / 固体抽出剤 / イオン交換 / 燃料再処理 / 放射能除染 / 固体抽出材 / クロマトグラフィ / 原子力エネルギー / 燃料サイクル / ピリジン樹脂 / クラウンエーテル樹脂 / イミノ二酢酸樹脂 / フェロシアン化物含浸吸着剤
Outline of Final Research Achievements

Many kinds of elements are contained in the nuclear spent fuel. Some of them are valuable elements. Some of them constitute a limitation factor of the amount of high-level waste in vitrified waste and the emplacement area for high-level waste disposal. Thus, the separation of these elements is required. For the development of nuclide separation method from the spent fuel, the basic study on the atmospheric-pressure non-thermal plasma chemical conversion and the dissolution of spent fuel was carried out, novel solid-type extractants were developed and the nuclide separation using the developed extractants was investigated.

Report

(6 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Annual Research Report
  • 2013 Annual Research Report
  • 2012 Annual Research Report
  • 2011 Annual Research Report
  • Research Products

    (29 results)

All 2016 2015 2014 2013 2012 2011 Other

All Journal Article (5 results) (of which Peer Reviewed: 5 results,  Acknowledgement Compliant: 5 results,  Open Access: 1 results) Presentation (23 results) (of which Int'l Joint Research: 3 results) Patent(Industrial Property Rights) (1 results)

  • [Journal Article] Uranium separation from a simulant fuel debris solution using a benzimidazole-type anion exchange resin2016

    • Author(s)
      Toru Kitagaki, Toshitaka Kaneshiki, Masao Nomura, Tatsuya Suzuki
    • Journal Title

      Journal of Nuclear Science and Technology

      Volume: 53 Issue: 10 Pages: 1639-1646

    • DOI

      10.1080/00223131.2016.1150219

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Application of atmospheric-pressure non-thermal plasma to chlorination of hardly soluble materials2015

    • Author(s)
      Toru Kitagaki, Tatsuya Suzuki, Toshitaka Kaneshiki, Masao Nomura
    • Journal Title

      Progress in Nuclear Energy

      Volume: 82 Pages: 122-125

    • DOI

      10.1016/j.pnucene.2014.07.039

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Effect of alcohols on separation behavior of rare earth elements using benzimidazole-type anion-exchange resin in nitric acid solutions2015

    • Author(s)
      Yusuke Tomobuchi, Yu Tachibana, Masao Nomura, Tatsuya Suzuki
    • Journal Title

      Journal of Radioanalytical and Nuclear Chemistry

      Volume: 303 Issue: 2 Pages: 1425-1428

    • DOI

      10.1007/s10967-014-3509-z

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Adsorptivity of Various Metal Ions onto Benzo-18-crown-6 and Dibenzo-18-crown-6 Resins2015

    • Author(s)
      M. Nogami, T. Haratani, Y. Tachibana, T. Kaneshiki, M. Nomura, T. Suzuki
    • Journal Title

      Journal of Radioanalytical and Nuclear Chemistry

      Volume: 303 Issue: 2 Pages: 1549-1553

    • DOI

      10.1007/s10967-014-3555-6

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Adsorption Behavior of Neptunium Ions on Pyridine-type Resin in Hydrochloric Acid Solutions2014

    • Author(s)
      Yu Tachibana, Tatsuya Suzuki, Tomoo Yamamura
    • Journal Title

      Journal of Ion Exchange

      Volume: 25 Pages: 228-233

    • NAID

      130004845692

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Presentation] Removal of Cesium by Heteropolyacid Salts from Radioactive Waste in HCl System2016

    • Author(s)
      T. Suzuki, Y. Tachibana, Y. Sakate, Son Nguyen An, Lanh Dang
    • Organizer
      9th International Conference on Nuclear and Radiochemistry
    • Place of Presentation
      Helsinki, Finland
    • Year and Date
      2016-08-29
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 多孔質PMMAを担体とするアンチモン酸吸着体の吸着特性2015

    • Author(s)
      田井毅、立花優、鈴木達也
    • Organizer
      第31回日本イオン交換研究発表会
    • Place of Presentation
      金沢工業大学
    • Year and Date
      2015-10-23
    • Related Report
      2015 Annual Research Report
  • [Presentation] Separation of Americium and Curium by using Anion Exchange Resin supported in High Porous Silica Beads in Alcoholic Nitric Acid System2015

    • Author(s)
      T. Suzuki, Y. Tachibana, Y. Tomobuchi, J. Katakura, T. Yamamura
    • Organizer
      Global 2015: International Nuclear Fuel Cycle Conference
    • Place of Presentation
      Paris, France
    • Year and Date
      2015-09-21
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of Inorganic Ion Exchanger Immobilized by Organic Support and Its Application to Radiochemical Separation2015

    • Author(s)
      Tsuyoshi Tai, Tatsuya Suzuki, Yu Tachibana
    • Organizer
      The 4th Intenational GIGAKU Conference in Nagaoka
    • Place of Presentation
      長岡技術科学大学
    • Year and Date
      2015-06-19
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Nuclide Separation Study using Actinide Facility at Oarai Center2014

    • Author(s)
      Tatsuya Suzuki, Yu Tachibana, Tomoo Yamamura
    • Organizer
      International Symposium on Utilization of Research Reactors for Material Studies
    • Place of Presentation
      東北大学、仙台市
    • Year and Date
      2014-12-11 – 2014-12-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] Adsorption Behavior of Neptunium Ions on Pyridine-Type Resin in Hydrochloric Acid Solutions2014

    • Author(s)
      Yu Tachibana, Yuki Yamazaki, Tatsuya Suzuki, Tomoo Yamamura
    • Organizer
      6th International Conference of Ion Exchange
    • Place of Presentation
      Okinawa ConventionCenter, Okinawa
    • Year and Date
      2014-11-09 – 2014-11-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] Adsorptivity of Various Metal Ions onto Benzo-15-crown-5 and Dibenzo-21-crown-7 Resins2014

    • Author(s)
      Masanobu Nogami, Tomohiro Haratani, Yu Tachibana, Toshitaka Kaneshiki, Masao Nomura, Tatsuya Suzuki
    • Organizer
      6th International Conference of Ion Exchange
    • Place of Presentation
      Okinawa ConventionCenter, Okinawa
    • Year and Date
      2014-11-09 – 2014-11-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] Adsorptivity of Various Metal Ions onto Benzo-18-crown-6 and Dibenzo-18-crown-6 Resins Irradiated by γ-ray2014

    • Author(s)
      Tetsuhiro Nishida, Shinya Tajima, Tomohiro Haratani, Masanobu Nogami, Nobuhiro Sato, Yu Tachibana, Tatsuya Suzuki
    • Organizer
      6th International Conference of Ion Exchange
    • Place of Presentation
      Okinawa ConventionCenter, Okinawa
    • Year and Date
      2014-11-09 – 2014-11-12
    • Related Report
      2014 Annual Research Report
  • [Presentation] Study on Mutual Separation of Minor Actinides using by benzimidazole-type Anion-Exchange Resin in Alcoholic Nitric Acid Solutions2014

    • Author(s)
      Yusuke Tomobuchi, Yu Tachibana, Masao Nomura, Tatsuya Suzuki, Jun-ichi Katakura
    • Organizer
      The 3rd Intenational GIGAKU Conference in Nagaoka
    • Place of Presentation
      長岡技術科学大学、長岡市
    • Year and Date
      2014-06-20 – 2014-06-21
    • Related Report
      2014 Annual Research Report
  • [Presentation] Reprocessing System with Nuclide Separation based on Chromatography in Hydrochloric Acid Solution2013

    • Author(s)
      Tatsuya Suzuki, Yu Tachibana, Shi-ichi Koyama
    • Organizer
      Global 2013: International Nuclear Fuel Cycle Conference
    • Place of Presentation
      Salt Lack City, Utah, USA
    • Related Report
      2013 Annual Research Report
  • [Presentation] Adsorptivity of Various Metal Ions onto Benzo-18-crown-6 and Dibenzo-18-crown-6 Resins2013

    • Author(s)
      Masanobu Nogami, Tomohiro Haratani, Yu Tachibana,Toshitaka Kaneshiki, Masao Nomura, Tatsuya Suzuki
    • Organizer
      The 5th Asia-Pacific Symposium on Radiochemistry ’13 (APSORC13)
    • Place of Presentation
      Kanazawa, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] Effect of alcohols on separation behavior of rare earth elements using benzimidazole-type anion-exchange resin in nitric acid solutions2013

    • Author(s)
      Yusuke Tomobuchi, Yu Tachibana, Masao Nomura, Tatsuya Suzuki
    • Organizer
      The 5th Asia-Pacific Symposium on Radiochemistry ’13 (APSORC13)
    • Place of Presentation
      Kanazawa, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] Adsorption Behavior of Neptunium Ions on Pyridine-type Resin in Hydrochloric Acid Solutions2013

    • Author(s)
      Yu Tachibana, Yuki Yamazaki, Yusuke Tomobuchi, Tatsuya Suzuki, Tomoo Yamamura
    • Organizer
      The 5th Asia-Pacific Symposium on Radiochemistry ’13 (APSORC13)
    • Place of Presentation
      Kanazawa, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] Application of Atmospheric-pressure Non-thermal Plasma to Chlorination for Hardly-Soluble Materials2013

    • Author(s)
      Toru Kitagaki, Tatsuya Suzuki, Toshitaka Kaneshiki, Masao Nomura
    • Organizer
      The 4th International Symposium on Innovative Nuclear Energy Systems
    • Place of Presentation
      Tokyo Institute of Technology, Japan
    • Related Report
      2013 Annual Research Report
  • [Presentation] Current Status of Reprocessing Process using Pyridine Resin in Hydrochloric Acid Solution2013

    • Author(s)
      Tatsuya Suzuki,, Yu Tachibana, Tomoo Yamamura, Masanobu Nogami, Shin-ichi Koyama
    • Organizer
      The 2nd China-Japan Academic Symposium on Nuclear Fuel Cycle (ASNFC 2013)
    • Place of Presentation
      Shanghai, China
    • Related Report
      2013 Annual Research Report
  • [Presentation] Dibenzo-21-crown-7樹脂の各種金属イオンに対する吸着特性2012

    • Author(s)
      原谷朋宏
    • Organizer
      日本原子力学会「2012年春の年会」
    • Place of Presentation
      福井大学(福井県)
    • Year and Date
      2012-03-20
    • Related Report
      2011 Annual Research Report
  • [Presentation] フェロシアン化物含有吸着剤を用いた汚染海水からのセシウムの除去2011

    • Author(s)
      鈴木達也
    • Organizer
      平成23年日本放射化学会年会・第55回放射化学討論会
    • Place of Presentation
      若宮ホール(長野県)
    • Year and Date
      2011-09-20
    • Related Report
      2011 Annual Research Report
  • [Presentation] BenzoおよびDibenzo-18-crown-6樹脂による金属イオンのクロマト分離挙動

    • Author(s)
      野上雅伸, 原谷朋宏, 野村雅夫, 金敷利隆, 立花優, 鈴木達也
    • Organizer
      東北大学 青葉山キャンパス
    • Place of Presentation
      東北大学青葉山キャンパス
    • Related Report
      2013 Annual Research Report
  • [Presentation] 大気圧非平衡プラズマを用いた難溶性核燃料の可溶化処理に関する基礎研究

    • Author(s)
      北垣徹、鈴木達也
    • Organizer
      日本原子力学会「2012年秋の大会」
    • Place of Presentation
      広島大学 東広島キャンパス
    • Related Report
      2012 Annual Research Report
  • [Presentation] Chloridization of hardly-soluble Nuclear Fuel Materials Using Non-Thermal Atmospheric-Pressure Plasma for Reprocessing

    • Author(s)
      Toru Kitagaki、Tatsuya Suzuki
    • Organizer
      11th Asia-Pacific Conference on Plasma Science and Technology and 25th Symposium on Plasma Science for Materials
    • Place of Presentation
      京都大学 桂キャンパス
    • Related Report
      2012 Annual Research Report
  • [Presentation] 硝酸/アルコール混合系における多孔質ベンゾイミダゾール型陰イオ ン交換樹脂を用いた希土類元素の相互分離

    • Author(s)
      友渕佑亮、立花優、野村雅夫、鈴木達也
    • Organizer
      2012年日本放射化学会年会・第56回放射化学討論会
    • Place of Presentation
      東京工業大学 大岡山キャンパス
    • Related Report
      2012 Annual Research Report
  • [Presentation] Benzo およびDibenzo-18-crown-6 樹脂の塩酸および硝酸系における金属イオン吸着特性

    • Author(s)
      原谷朋宏、野上雅伸、野村雅夫、金敷利隆、鈴木達也
    • Organizer
      2012年日本放射化学会年会・第56回放射化学討論会
    • Place of Presentation
      東京工業大学 大岡山キャンパス
    • Related Report
      2012 Annual Research Report
  • [Presentation] ベンゾイミダゾール型陰イオン交換樹脂を用いた希土類元素の相互分離

    • Author(s)
      友渕佑亮、立花優、野村雅夫、 鈴木達也
    • Organizer
      日本原子力学会 第8回再処理・リサイクル部会セミナー
    • Place of Presentation
      東京工業大学 大岡山キャンパス
    • Related Report
      2012 Annual Research Report
  • [Patent(Industrial Property Rights)] 難溶解性物質の可溶化処理方法および溶解方法2012

    • Inventor(s)
      鈴木達也、北垣徹、大岡靖典
    • Industrial Property Rights Holder
      国立大学法人長岡技術科学大学、原子燃料工業株式会社
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2012-226864
    • Filing Date
      2012-10-12
    • Related Report
      2012 Annual Research Report

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Published: 2011-04-06   Modified: 2019-07-29  

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