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Study on the mechanism of metal-insulator transition in the pyrochlore iridates

Research Project

Project/Area Number 23540417
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionKyushu Institute of Technology

Principal Investigator

KAZUYUKI Matsuhira  九州工業大学, 工学(系)研究科(研究院), 准教授 (40312342)

Co-Investigator(Kenkyū-buntansha) KAZUAKI Iwasa  東北大学, 大学院・理学研究科, 准教授 (00275009)
KEITARO Kuwahara  茨城大学, 理工学研究科, 准教授 (90315747)
TAKUMI Hasegawa  広島大学, 大学院・総合科学研究科, 助教 (20508171)
Project Period (FY) 2011 – 2013
Project Status Completed (Fiscal Year 2013)
Budget Amount *help
¥5,070,000 (Direct Cost: ¥3,900,000、Indirect Cost: ¥1,170,000)
Fiscal Year 2013: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2012: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2011: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Keywordsパイロクロア酸化物 / イリジウム酸化物 / 金属絶縁体転移 / 中性子散乱 / ラマン散乱 / X線回折 / イリジウム / 単結晶
Research Abstract

We investigated the mechanism of metal-insulator transition in the pyrochlore iridates by using neutron scattering, Raman scattering, X-ray diffraction, and thermal expansion measurements.
We revealed the magnetic structure of low temperature phase is "all-in all-out" for Nd2Ir2O7; this is first discovery. This magnetic structure has a unique character. There is no change of structural symmetry phase below transition temperature. Raman scattering and XRD measurements support this magnetic structure. Furthermore, we found the change of lattice parameter caused by the metal-insulator transition is small. On the other hand, the results of Raman scattering for Sm2Ir2O7 and Eu2Ir2O7 suggest structural change although cubic symmetry keeps. The structure in the low temperature phase is future subjects.
In addition, in this research process, we discovered giant magnetoresistance effect for Nd2Ir2O7.

Report

(4 results)
  • 2013 Annual Research Report   Final Research Report ( PDF )
  • 2012 Research-status Report
  • 2011 Research-status Report
  • Research Products

    (34 results)

All 2014 2013 2012 2011 Other

All Journal Article (12 results) (of which Peer Reviewed: 12 results) Presentation (20 results) (of which Invited: 4 results) Patent(Industrial Property Rights) (2 results)

  • [Journal Article] Metal-insulator Transition in Pyrochore Oxide (Nd1-xPrx)2Ir2O72014

    • Author(s)
      K. Matsuhira, K. Kuroda, T. Sakakibara, M. Wakeshima, Y. Hinatsu
    • Journal Title

      JPS Conference Proceedings (SECS2013)

      Volume: 3 Pages: 1-6

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Magnetic order in the pyrochlore iridate Nd2Ir2O7 probed by muon spin relaxation2013

    • Author(s)
      H. Guo, K. Matsuhira, I. Kawasaki, M. Wakeshima, Y. Hinatsu, I. Watanabe, Z. Xu
    • Journal Title

      Phys. Rev. B Rapid Commun

      Volume: Vol. 88

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Giant Magnetoresistance Effect in the Metal-Insulator Transition of Pyrochlore Oxide Nd2Ir2O72013

    • Author(s)
      K. Matsuhira, M. Tokunaga, M. Wakeshima, Y. Hinatsu, and S. Takagi
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: Vol. 82

    • NAID

      210000132393

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Magnetic order in the pyrochlore iridate Nd2Ir2O7 probed by muon spin relaxation2013

    • Author(s)
      H. Guo, K. Matsuhira, I. Kawasaki, M. Wakeshima, Y. Hinatsu, I. Watanabe, Z. Xu
    • Journal Title

      Physical Review B, Rapid Communication

      Volume: 88 Issue: 6 Pages: 60411-60411

    • DOI

      10.1103/physrevb.88.060411

    • Related Report
      2013 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Giant Magnetoresistance Effect in the Metal - Insulator Transition of Pyrochlore Oxide Nd_2Ir_2O_72013

    • Author(s)
      K. Matsuhira, M. Tokunaga, M. Wakeshima, Y. Hinatsu, and S. Takagi
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: 82 Issue: 2 Pages: 23706-23706

    • DOI

      10.7566/jpsj.82.023706

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Emergence of Magnetic Long-range Order in Frustrated Pyrochlore Nd2Ir2O7 with Metal-Insulator Transition2012

    • Author(s)
      K. Tomiyasu, K. Matsuhira, K. Iwasa, M. Watahiki, S. Takagi, M. Wakeshima, Y. Hinatsu, M. Yokoyama, K. Ohoyama, and K. Yamada
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: Vol. 81

    • NAID

      210000109450

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Emergence of Magnetic Long-range Order in Frustrated Pyrochlore Nd_2Ir_2O_7 with Metal-Insulator Transition2012

    • Author(s)
      K.Tomiyasu, K.Matsuhira, et al
    • Journal Title

      J.Phys.Soc.Jpn

      Volume: 81 Issue: 3 Pages: 34709-34709

    • DOI

      10.1143/jpsj.81.034709

    • Related Report
      2011 Research-status Report
    • Peer Reviewed
  • [Journal Article] Metal-Insulator Transition in Pyrochlore Oxides Ln2Ir2O72011

    • Author(s)
      K. Matsuhira, M. Wakeshima, Y. Hinatsu, and S. Takagi
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: Vol. 80

    • NAID

      120005764502

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Crystalline electric field study in the pyrochlore Nd2Ir2O7 with metal-insulator transition2011

    • Author(s)
      M. Watahiki, K. Tomiyasu, K. Matsuhira, K. Iwasa, M. Yokoyama, S. Takagi, M. Wakeshima, Y. Hinatsu
    • Journal Title

      J. Phys. : Conference Series

      Volume: Vol.320

    • Related Report
      2013 Final Research Report
    • Peer Reviewed
  • [Journal Article] Slow Dynamics in Dy Pyrohlore Oxides Dy_2Sn_2O_7 and Dy_2Ir_2O_72011

    • Author(s)
      K.Matsuhira, M.Wakeshima, Y.Hinatsu, C.Sekine, C.Paulsen, T.Sakakibara, S.Takagi
    • Journal Title

      J.Phys. : Conf.Series

      Volume: 320 Pages: 0120501-6

    • DOI

      10.1088/1742-6596/320/1/012050

    • Related Report
      2011 Research-status Report
    • Peer Reviewed
  • [Journal Article] Crystalline electric field study in pyrochlore-type iridate Nd_2Ir_2O_7 with metal-insulator transition2011

    • Author(s)
      M.Watahiki, K.Tomiyasu, K.Iwasa, K.Matsuhira, S.Takagi, M.Wakeshima, Y.Hinatsu
    • Journal Title

      J.Phys. : Conf.Series

      Volume: 320 Pages: 12080-12080

    • DOI

      10.1088/1742-6596/320/1/012080

    • Related Report
      2011 Research-status Report
    • Peer Reviewed
  • [Journal Article] Metal-insulator Transitions in Pyrochlore Oxides Ln_2Ir_2O_72011

    • Author(s)
      K.Matsuhira, M.Wakeshima, Y.Hinatsu, S.Takagi
    • Journal Title

      J.Phys.Soc.Jpn.

      Volume: 80 Issue: 9 Pages: 094701-094701

    • DOI

      10.1143/jpsj.80.094701

    • Related Report
      2011 Research-status Report
    • Peer Reviewed
  • [Presentation] Magnetic Properties of Pyrochlore Iridates Ln2Ir2O72014

    • Author(s)
      松平和之
    • Organizer
      International Workshop of frustration and topology in condensed matter physics
    • Place of Presentation
      国立成功大学(台南市, 台湾)
    • Year and Date
      2014-02-16
    • Related Report
      2013 Final Research Report
  • [Presentation] Pr-Substitution Effect in the Metal-Insulator Transition of Pyrochlore Oxide Nd2Ir2O72013

    • Author(s)
      K. Matsuhira, K.Kuroda, T. Sakakibara, M. Wakeshima, Y. Hinatsu
    • Organizer
      The International Conference on Strongly Correlated Electron Systems (SCES2013)
    • Place of Presentation
      東京大学(東京都)
    • Year and Date
      2013-08-08
    • Related Report
      2013 Final Research Report
  • [Presentation] パイロクロア型Ir酸化物におけるキャリアドープ効果2013

    • Author(s)
      松平和之, 水鳥雄斗, 後藤岳, 分島亮, 日夏幸雄, 徳永将史
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学(東広島市)
    • Year and Date
      2013-03-29
    • Related Report
      2013 Final Research Report
  • [Presentation] Metal-Insulator Transition in Pyrochore Oxide Nd2Ir2O72012

    • Author(s)
      松平和之
    • Organizer
      International Conference on Highly Frustrated Magnetism 2012 (HFM2012)
    • Place of Presentation
      McMaster Univ. (Hamilton, Canada)
    • Year and Date
      2012-06-04
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] 松平和之、分島亮、日夏幸雄、長谷川巧、荻田典夫、宇田川眞行、坂田雅文、 加賀山朋子、清水克哉、高木精志2012

    • Author(s)
      パイロクロア酸化物Ln2Ir2O7における金属絶縁体転移
    • Organizer
      特定領域研究「フラストレーションが創る新しい物性」最終成果報告会
    • Place of Presentation
      大阪大学吹田キャンパス(吹田市)
    • Related Report
      2011 Research-status Report
  • [Presentation] パイロクロア型Ir酸化物における金属絶縁体転移2012

    • Author(s)
      松平和之
    • Organizer
      KEK物構研・構造物性研究センター研究会「遍歴系における幾何学電子相関」(招待講演)
    • Place of Presentation
      つくば国際会議場(つくば市)
    • Related Report
      2011 Research-status Report
  • [Presentation] Nd2Ir2O7の金属絶縁体転移における強磁場効果2012

    • Author(s)
      松平和之, 徳永将史, 分島亮, 日夏幸雄, 高木精志
    • Organizer
      日本物理学会第67回年次大会
    • Place of Presentation
      関西学院大学(西宮市)
    • Related Report
      2011 Research-status Report
  • [Presentation] パイロクロア型Ir酸化物における金属絶縁体転移2011

    • Author(s)
      松平和之
    • Organizer
      KEK物構研・構造物性研究センター研究会「遍歴系における幾何学電子相関」
    • Place of Presentation
      つくば国際会議場(つくば市)
    • Year and Date
      2011-01-11
    • Related Report
      2013 Final Research Report
    • Invited
  • [Presentation] 金属絶縁体転移を示すパイロクロア型イリジウム酸化物Ln2Ir2O7の低温物性2011

    • Author(s)
      松平和之, 分島亮, 日夏幸雄, 高木精志
    • Organizer
      日本物理学会2011年秋季大会
    • Place of Presentation
      富山大学(富山市)
    • Related Report
      2011 Research-status Report
  • [Presentation] Pr-Substitution Effect in the Metal-Insulator Transition of Pyrochlore Oxide Nd2Ir2O7

    • Author(s)
      K. Matsuhira, K. Kuroda, T. Sakakibara, M. Wakeshima, Y. Hinatsu
    • Organizer
      The International Conference on Strongly Correlated Electron Systems (SCES2013)
    • Place of Presentation
      東京大学(東京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Transport Properties of Cu-Doped Pyrochlore Oxide Eu2Ir2O7

    • Author(s)
      G, Goto, K. Matsuhira, Y. Mizutori, Y. Koga, M. Wakeshima, Y. Hinatsu
    • Organizer
      The International Conference on Strongly Correlated Electron Systems (SCES2013)
    • Place of Presentation
      東京大学(東京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Effect of Cu-Doping in the Metal-Insulator Transition of Pyrochlore Oxide Nd2Ir2O7

    • Author(s)
      Y. Mizutori, K. Matsuhira, G, Goto, M. Tokunaga, M. Wakeshima, Y. Hinatsu
    • Organizer
      The International Conference on Strongly Correlated Electron Systems (SCES2013)
    • Place of Presentation
      東京大学(東京都)
    • Related Report
      2013 Annual Research Report
  • [Presentation] パイロクロア型イリジウム酸化物における巨大磁気抵抗効果

    • Author(s)
      松平和之、徳永将史,後藤岳,水鳥雄斗,分島亮、日夏幸雄
    • Organizer
      第119回日本物理学会九州支部例会
    • Place of Presentation
      久留米工業大学(福岡県久留米市)
    • Related Report
      2013 Annual Research Report
  • [Presentation] Magnetic Properties of Pyrochlore Iridates Ln2Ir2O7

    • Author(s)
      K. Matsuhira
    • Organizer
      International Workshop on frustration and topology in condensed matter physics
    • Place of Presentation
      国立成功大学(台南市,台湾)
    • Related Report
      2013 Annual Research Report
    • Invited
  • [Presentation] Metal-Insulator Transition in Pyrochlore Oxide Nd2Ir2O7

    • Author(s)
      松平和之
    • Organizer
      International Conference on Highly Frustrated Magnetism 2012 (HFM2012)
    • Place of Presentation
      Hamilton, Canada
    • Related Report
      2012 Research-status Report
    • Invited
  • [Presentation] 金属絶縁体転移を示すパイロクロア酸化物Nd2Ir2O7のPr置換効果

    • Author(s)
      松平和之、黒田耕平、分島亮、日夏幸雄、榊原俊郎、高木精志
    • Organizer
      日本物理学会2012年秋季大会
    • Place of Presentation
      横浜国立大学(横浜市)
    • Related Report
      2012 Research-status Report
  • [Presentation] キャリアドープされたパイロクロア型Ir酸化物の電子物性

    • Author(s)
      後藤岳,古賀佑司,水鳥雄斗,分島亮、日夏幸雄、徳永将史,松平和之
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学(東広島市)
    • Related Report
      2012 Research-status Report
  • [Presentation] パイロクロア型Ir酸化物におけるキャリアドープ効果

    • Author(s)
      松平和之、水鳥雄斗,後藤岳,分島亮、日夏幸雄、徳永将史
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学(東広島市)
    • Related Report
      2012 Research-status Report
  • [Presentation] 金属絶縁体転移を示すNd2Ir2O7におけるキャリアドープ効果

    • Author(s)
      水鳥雄斗,後藤岳,分島亮、日夏幸雄、徳永将史,松平和之
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学(東広島市)
    • Related Report
      2012 Research-status Report
  • [Presentation] muSR study on the pyrochlore iridate Nd2Ir2O7

    • Author(s)
      H. Guo, K. Matsuhira, M. Wakeshima, Y. Hinatsu, B. Adiperdana, I. A. Dharmawan, I. Watanabe
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学(東広島市)
    • Related Report
      2012 Research-status Report
  • [Patent(Industrial Property Rights)] 電気伝導性材料及びそれを用いた抵抗温度計2013

    • Inventor(s)
      松平和之, 分島亮, 徳永将史
    • Industrial Property Rights Holder
      松平和之, 分島亮, 徳永将史
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2013-093414
    • Filing Date
      2013-04-26
    • Related Report
      2013 Final Research Report
  • [Patent(Industrial Property Rights)] 電気伝導性材料およびそれを用いた抵抗温度計2013

    • Inventor(s)
      松平和之,徳永将史,分島亮
    • Industrial Property Rights Holder
      松平和之,徳永将史,分島亮
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2013-093414
    • Filing Date
      2013-04-26
    • Related Report
      2013 Annual Research Report

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Published: 2011-08-05   Modified: 2020-05-15  

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