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Study of metal-insulator transition in the 5d transition metal pyrochlore oxide Cd2Os2O7

Research Project

Project/Area Number 24540360
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionTokyo Institute of Technology

Principal Investigator

YAMAURA Jun-ichi  東京工業大学, 元素戦略研究センター, 特任准教授 (80292762)

Co-Investigator(Renkei-kenkyūsha) 廣井 善二 (筒井 智嗣)  東京大学, 物性研究所, 教授 (30192719)
長谷川 巧  広島大学, 総合科学研究科, 助教 (20508171)
堀場 律子  岡山大学, 自然科学研究科, 助教 (50415098)
大串 研也  東北大学, 理学部, 教授 (30455331)
Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2014: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2013: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2012: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Keywords金属絶縁体転移 / 反強磁性転移 / 磁気構造 / 共鳴X線散乱 / リフシッツ転移 / 磁気転移 / フラストレーション / パイロクロア / 国際情報交換(フランス)
Outline of Final Research Achievements

5d-transition metal pyrochlore oxide Cd2Os2O7 shows a metal-insulator transition at 227 K with magnetic ordering. The pyrochlore lattice is composed of the corner-shared tetrahedral Os network, in which the Os atoms have functions as the electric conduction and/or the magnetic moment. Since a geometrical frustration between localized spins prevents a long-range magnetic ordering, a peculiar magnetic structure is expected in the ordered state. We observed a commensurate magnetic peak of q = (0, 0, 0) by resonant x-ray scattering in a high-quality single crystal. We propose a noncollinear all-in/all-out spin arrangement on the pyrochlore lattice of Os atoms, in which all the spins point to (all-in) or away (all-out) from the centers of the tetrahedron. The magnetostriction, magnetocapacitance, Voigt magnetooptic effect, and magnetic susceptibility are expected to have a term linear to the external magnetic field.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Research-status Report
  • 2012 Research-status Report
  • Research Products

    (31 results)

All 2015 2014 2013 2012 Other

All Journal Article (15 results) (of which Peer Reviewed: 14 results,  Open Access: 1 results,  Acknowledgement Compliant: 1 results) Presentation (15 results) Remarks (1 results)

  • [Journal Article] Lifshitz metal-insulator transition induced by the all-in/all-out magnetic order in the pyrochlore oxide Cd2Os2O72015

    • Author(s)
      Zenji Hiroi, Jun-ichi Yamaura, Takahiro Hirose, Issei Nagashima, Yoshihiko Okamoto
    • Journal Title

      APL Materials

      Volume: 3 Issue: 4 Pages: 041501-041501

    • DOI

      10.1063/1.4907734

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] 5d遷移金属パイロクロア酸化物における低温磁気構造の研究2013

    • Author(s)
      山浦淳一, 大串研也,広井善二
    • Journal Title

      日本結晶学会誌

      Volume: 55 Pages: 116-120

    • NAID

      10031168500

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] 5d遷移金属パイロクロア酸化物における特異な磁気構造2013

    • Author(s)
      山浦淳一、有馬孝尚
    • Journal Title

      放射光

      Volume: 26 Pages: 283-290

    • NAID

      10031191830

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] パイロクロア酸化物Cd2Os2O7における全入全出型スピン配列と金属絶縁体転移2013

    • Author(s)
      広井善二, 山浦淳一, 播磨尚朝
    • Journal Title

      セラミックス

      Volume: 48 Pages: 453-458

    • Related Report
      2013 Research-status Report
  • [Journal Article] Complex orbital state stabilized by strong spin-orbit coupling in a2013

    • Author(s)
      Y. Hirata, K. Ohgushi, J. Yamaura, H. Ohsumi, S. Takeshita, M. Takata, T. Arima
    • Journal Title

      Phys. Rev. B

      Volume: 87 Issue: 16 Pages: 161111-161111

    • DOI

      10.1103/physrevb.87.161111

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Resonant X-ray Diffraction Study of the Strongly Spin-Orbit-Coupled Mott Insulator CaIrO32013

    • Author(s)
      K. Ohgushi, J. Yamaura, H. Ohsumi, K. Sugimoto, S. Takeshita, A. Tokuda, H. Takagi, M. Takata, and T. Arima
    • Journal Title

      Physical Review Letters

      Volume: 110 Issue: 21 Pages: 217212-217212

    • DOI

      10.1103/physrevlett.110.217212

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Pressure Effects on Rattling and Superconductivity in the Einstein Solids2013

    • Author(s)
      Y. Ikeda, Y. Kawasaki, T. Shinohara, S. Araki, T. C. Kobayashi, A. Onosaka, Y. Okamoto, J. Yamaura, Z. Hiroi
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 82 Issue: 6 Pages: 63707-63707

    • DOI

      10.7566/jpsj.82.063707

    • NAID

      210000132577

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Understanding of the Temperature-Pressure Phase Diagram of beta-Pyrochlore Oxides: A Role of Anhamonicity on Superconductivity2013

    • Author(s)
      T. Isono, D. Iguchi, T. Matsubara, Y. Machida, B. Salce, J. Flouquet, H. Ogusu, J. Yamaura, Z. Hiroi, K. Izawa
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 82 Issue: 11 Pages: 114708-114708

    • DOI

      10.7566/jpsj.82.114708

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Rattling and Superconducting Properties of the Cage Compound Ga_xV_2Al_202012

    • Author(s)
      Z. Hiroi, A. Onosaka, Y. Okamoto, J. Yamaura, H. Harima
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: 81 Issue: 12 Pages: 124707-124707

    • DOI

      10.1143/jpsj.81.124707

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Large Diamagnetism of AV2A20 (A=Y and La)2012

    • Author(s)
      A. Onosaka, Y. Okamoto, J. Yamaura, T. Hirose, and Z. Hiroi
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 81 Issue: 12 Pages: 123702-123702

    • DOI

      10.1143/jpsj.81.123702

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Orbital Switching in a Frustrated Magnet2012

    • Author(s)
      H. Yoshida. J. Yamaura, M. Isobe, Y. Okamoto, G J. Nilsen, Z. Hiroi
    • Journal Title

      Nature Communications

      Volume: 3 Issue: 1 Pages: 860-860

    • DOI

      10.1038/ncomms1875

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Large and homogeneous mass enhancement in the rattling-induced superconductor KOs2O62012

    • Author(s)
      T. Terashima, N. Kurita, A. Kiswandhi, E.-S. Choi, J. S. Brooks, K. Sato, J. Yamaura, Z. Hiroi, H. Harima, S. Uji
    • Journal Title

      Phys. Rev. B

      Volume: 85 Issue: 18 Pages: 180503-180503

    • DOI

      10.1103/physrevb.85.180503

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Crystal Chemistry and Magnetic Properties of Manganese Zinc Alloy "YMn2Zn20" Comprising a Mn Pyrochlore Lattice2012

    • Author(s)
      Y. Okamoto, T. Shimizu, J. Yamaura, Z. Hiroi
    • Journal Title

      Journal Solid State Chemistry

      Volume: 191 Pages: 246-246

    • DOI

      10.1016/j.jssc.2012.03.038

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] A novel crystal polymorph of volborthite, Cu_3V_2O_7(OH)_2・2H_2O2012

    • Author(s)
      H. Ishikawa, J. Yamaura, Y. Okamoto, H. Yoshida, G. J. Nilsen, Z.Hiroi
    • Journal Title

      Acta Crystal lographica Section C

      Volume: 68 Issue: 7 Pages: 141-141

    • DOI

      10.1107/s010827011202536x

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Tetrahedral Magnetic Order without Spatial Symmetry Breaking in the Pyrochlore Lattice of Cd2Os2O72012

    • Author(s)
      J. Yamaura, K. Ohgushi, H. Ohsumi, T. Hasegawa, I. Yamauchi, K. Sugimoto, S. Takeshita, A. Tokuda, M. Takata, M. Udagawa, M. Takigawa, H. Harima, T. Arima, and Z. Hiroi
    • Journal Title

      Phys. Rev. Lett.

      Volume: 108 Issue: 24 Pages: 247205-247205

    • DOI

      10.1103/physrevlett.108.247205

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] Cd2Os2O7における逆ファラデー効果の共鳴X線磁気散乱による検出2015

    • Author(s)
      大隅寛幸,高田昌樹,鈴木基寛,田中義人,長谷川尊之,白石龍太郎,松下龍樹,鳥本直隆,川瀬里美,西尾篤,有馬孝尚,山浦淳一,廣井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Annual Research Report
  • [Presentation] パイロクロア酸化物Cd2Os2O7の磁気ドメイン界面における伝導と磁性2015

    • Author(s)
      廣瀬峻啓,山浦淳一,廣井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Annual Research Report
  • [Presentation] Cd2Os2O7の磁歪・熱膨張2014

    • Author(s)
      三田村裕幸,山浦淳一,河野洋平,橘高俊一郎,榊原俊郎,廣井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      中部大学
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Annual Research Report
  • [Presentation] パイロクロア酸化物Cd2Os2O7における磁気ドメイン界面伝導の可能性2014

    • Author(s)
      廣瀬峻啓,山浦淳一,廣井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      中部大学
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Annual Research Report
  • [Presentation] Possible electric control of the‘all-in/all-out' magnetic domain distribution in Cd2Os2O72014

    • Author(s)
      Samuel Tardif,竹下聡史,大隅寛幸,奥山大輔,有馬孝尚,山浦淳一,広井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      東海大学
    • Related Report
      2013 Research-status Report
  • [Presentation] Cd2Os2O7の金属―絶縁体転移に対するRe置換効果2014

    • Author(s)
      長島一成,山浦淳一,後藤弘匡,岡本佳比古,廣井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      東海大学
    • Related Report
      2013 Research-status Report
  • [Presentation] 5dパイロクロア酸化物Cd2Os2O7およびCd2Re2O7に対する元素置換効果2013

    • Author(s)
      長島一成,山浦淳一,後藤弘匡,岡本佳比古,廣井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      徳島大学
    • Related Report
      2013 Research-status Report
  • [Presentation] AV2Al20 (A = Y, La)における巨大反磁性の起源2013

    • Author(s)
      廣瀬峻啓,岡本佳比古,山浦淳一,廣井善二,播磨尚朝
    • Organizer
      日本物理学会
    • Place of Presentation
      徳島大学
    • Related Report
      2013 Research-status Report
  • [Presentation] パイロクロア酸化物Cd2Os2O7単結晶のμSR法による磁気基底状態の研究II2013

    • Author(s)
      幸田章宏,宮崎正範,平石雅俊,山内一宏,小嶋健児,門野良典,山浦淳一,広井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      広島大学
    • Related Report
      2012 Research-status Report
  • [Presentation] パイロクロア酸化物Cd2Re2O7の圧力下における多彩な相と対称性2013

    • Author(s)
      山浦淳一,広井善二,武田圭生,中山友輝,池田陽一,桑名加奈子,小林達生,平尾直久,大石泰生
    • Organizer
      日本物理学会
    • Place of Presentation
      広島大学
    • Related Report
      2012 Research-status Report
  • [Presentation] パイロクロア酸化物Cd2Re2O7の圧力下における物性と結晶構造の関連2013

    • Author(s)
      広井善二,山浦淳一,武田圭生,中山友輝,池田陽一,桑名加奈子,小林達生,平尾直久,大石泰生
    • Organizer
      日本物理学会
    • Place of Presentation
      広島大学
    • Related Report
      2012 Research-status Report
  • [Presentation] パイロクロア酸化物Cd2Os2O7単結晶のμSR法による磁気基底状態の研究2012

    • Author(s)
      幸田章宏,宮崎正範,平石雅俊,小嶋健児,門野良典,山浦淳一,広井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      横浜国立大学
    • Related Report
      2012 Research-status Report
  • [Presentation] パイロクロア酸化物におけるオキソニウムイオンのダイナミクスの研究2012

    • Author(s)
      佐藤耕太,山浦淳一,岡本佳比古,古府麻衣子,山室修,広井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      横浜国立大学
    • Related Report
      2012 Research-status Report
  • [Presentation] 5d遷移金属酸化物AOsO4 (A=K,Rb,Cs)の構造と物性2012

    • Author(s)
      山浦淳一,大串研也,広井善二
    • Organizer
      日本物理学会
    • Place of Presentation
      横浜国立大学
    • Related Report
      2012 Research-status Report
  • [Presentation] Tetrahedral Magnetic Order and the Metal-Insulator Transition2012

    • Author(s)
      J. Yamaura, K. Ohgushi, H. Ohsumi, T. Hasegawa, I. Yamauchi, K. Sugimoto
    • Organizer
      International conference on highly frustrated magnetism
    • Place of Presentation
      MacMaster University
    • Related Report
      2012 Research-status Report
  • [Remarks] Xray Laboratory

    • URL

      http://www.issp.u-tokyo.ac.jp/labs/mdcl/lab/xsen/index2.html

    • Related Report
      2012 Research-status Report

URL: 

Published: 2013-05-31   Modified: 2020-05-15  

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