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Development of scanning tunneling microscope under multiple extreme conditions and study of electronic phases in organic conductors

Research Project

Project/Area Number 24654095
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Condensed matter physics II
Research InstitutionHokkaido University

Principal Investigator

ICHIMURA Koichi  北海道大学, 工学(系)研究科(研究院), 准教授 (50261277)

Project Period (FY) 2012-04-01 – 2015-03-31
Project Status Completed (Fiscal Year 2014)
Budget Amount *help
¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Fiscal Year 2013: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2012: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywords走査トンネル顕微鏡 / 高圧 / 有機導体 / 電荷秩序 / 強相関電子系
Outline of Final Research Achievements

A scanning tunneling microscope (STM) under high pressure and low temperature was developed. The electronic state of organic conductors, which are materials with the highly correlated electron system, were studied by STM. The role of the long range Coulomb interaction was discussed.
STM measurements were performed on three organic conductors with the alpha-type donor arrangement, in which the system tends to undergo the charge ordering state. The charge disproportionation with a stripe structure was found at high temperature in three salts irrespective of its ground states. Moreover, the stripe pattern varied depending on the anisotropy of the electronic band structure. The results suggest that a dimerization has an important role in forming the charge ordering as well as the long range Coulomb interaction. The finding obtained by the present study contributes to elucidate the origin of the charge ordering state, which characterizes highly correlated electron systems.

Report

(4 results)
  • 2014 Annual Research Report   Final Research Report ( PDF )
  • 2013 Research-status Report
  • 2012 Research-status Report
  • Research Products

    (27 results)

All 2015 2014 2013 2012

All Journal Article (13 results) (of which Peer Reviewed: 13 results,  Open Access: 2 results,  Acknowledgement Compliant: 2 results) Presentation (14 results) (of which Invited: 4 results)

  • [Journal Article] STM observation of charge stripe in metallic phase of α-(BEDT-TTF)2I32015

    • Author(s)
      K. Katono, T. Taniguchi, K. Ichimura, Y. Kawashima, S. Tanda, and K. Yamamoto
    • Journal Title

      Physical Review B

      Volume: 91 Issue: 12 Pages: 125110-125110

    • DOI

      10.1103/physrevb.91.125110

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] STM/STS study of the superconducting gap in SmFeAsO1-xFx2015

    • Author(s)
      Y. Kawashima, K. Ichimura, K. Katono, T. Kurosawa, M. Oda, S. Tanda, Y. Kamihara, H. Hosono
    • Journal Title

      Solid State Communications

      Volume: 204 Pages: 33-36

    • DOI

      10.1016/j.ssc.2014.12.003

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Charge disproportionation in alpha-(BEDT-TTF)2X2015

    • Author(s)
      K. Katono, K. Ichimura, T, Taniguchi, K. Kawashima, K. Yamaya, S. Tanda
    • Journal Title

      Physica B

      Volume: 460 Pages: 64-67

    • DOI

      10.1016/j.physb.2014.11.041

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] STM spectroscopy on deuterated kappa-(ET-d[3,3])2Cu[N(CN)2]Br2015

    • Author(s)
      Y. Oka, H. Nobukane, N. Matsunaga, K. Nomura, K. Katono, K. Ichimura, A. Kawamoto
    • Journal Title

      Physica B

      Volume: 460 Pages: 93-95

    • DOI

      10.1016/j.physb.2014.11.047

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Metai-insulator transition in iron doped 2H-TaSe2: Suggestion of chiral unitary localization2015

    • Author(s)
      T. Kanno, T Matsumoto, K. Ichimura, T. Matsuura, S. Tanda
    • Journal Title

      Physica B

      Volume: 460 Pages: 165-167

    • DOI

      10.1016/j.physb.2014.11.061

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed
  • [Journal Article] STM Observation of Charge Disproportionation in Organic Conductors2014

    • Author(s)
      K. Katono, K. Ichimura, T. Taniguchi, Y. Kawashima, K. Yamaya and S. Tanda
    • Journal Title

      Topologica

      Volume: 3

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Discovery of Chiral CDW in 1T-VSe22014

    • Author(s)
      Y. Sugawara, J. Ishioka, Y.Toda, M. Oda, T. Kurosawa, T. Matsuura, K. Ichimura and S. Tanda
    • Journal Title

      Topologica

      Volume: 3

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Metal-Insulator Transition in the Chiral-Unitary System 2H-FexTa1-xSe22014

    • Author(s)
      T. Kanno, T. Matsumoto, S. K. Kataria, J. Ishioka, N. Matsunaga, K. Ichimura, T. Matsuura and S. Tanda
    • Journal Title

      Topologica

      Volume: 3

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Charge Stripe Structure in Fe1+xTe by STM2013

    • Author(s)
      Y. Kawashima, K. Ichimura, J. Ishioka, T. Kurosawa, M. Oda, K. Yamaya and S. Tanda
    • Journal Title

      Solid State Communications

      Volume: 167 Pages: 10-13

    • DOI

      10.1016/j.ssc.2013.04.033

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Charge Stripe Structure in FeTe2012

    • Author(s)
      Y. Kawashima, K. Ichimura, J. Ishioka, T. Kurosawa, M. Oda, K. Yamaya and S. Tanda
    • Journal Title

      Physica B

      Volume: 407 Issue: 11 Pages: 1796-1798

    • DOI

      10.1016/j.physb.2012.01.032

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Mixed Density Wave State in Quasi-2D Organic Conductor2012

    • Author(s)
      K. Katono, K. Ichimura, Y. Kawashima, K. Yamaya and S. Tanda
    • Journal Title

      Physica B

      Volume: 407 Issue: 11 Pages: 1827-1830

    • DOI

      10.1016/j.physb.2012.01.041

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Fluctuating superconductivity in the strongly correlated two-dimensional organic superconductor k-(BEDT-TTF)2Cu(NCS)2 in an in-plane magnetic field2012

    • Author(s)
      S. Tsuchiya et al.
    • Journal Title

      Phys. Rev. B

      Volume: 85 Issue: 22

    • DOI

      10.1103/physrevb.85.220506

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Journal Article] Reply to “Comment on ‘Charge-Parity Symmetry Observed through Friedel Oscillations in Chiral Charge-Density Waves’”2012

    • Author(s)
      J. Ishioka, T. Fujii, K. Katono, K. Ichimura, T. Kurosawa, M. Oda and S. Tanda
    • Journal Title

      Physical Review B

      Volume: 86 Issue: 24

    • DOI

      10.1103/physrevb.86.247102

    • Related Report
      2012 Research-status Report
    • Peer Reviewed
  • [Presentation] Charge disproportionation in alpha-(BEDT-TTF)2X2014

    • Author(s)
      K. Katono, K. Ichimura, T, Taniguchi, K. Kawashima, K. Yamaya, S. Tanda
    • Organizer
      International School and Workshop on Electronic Crystals 2014 (ECRYS-2014)
    • Place of Presentation
      カルジェス(フランス)
    • Year and Date
      2014-08-12 – 2014-08-22
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] STM spectroscopy on deuterated kappa-(ET-d[3,3])2Cu[N(CN)2]Br2014

    • Author(s)
      Y. Oka, H. Nobukane, N. Matsunaga, K. Nomura, K. Katono, K. Ichimura, A. Kawamoto
    • Organizer
      International School and Workshop on Electronic Crystals 2014 (ECRYS-2014)
    • Place of Presentation
      カルジェス(フランス)
    • Year and Date
      2014-08-12 – 2014-08-22
    • Related Report
      2014 Annual Research Report
  • [Presentation] Metai-insulator transition in iron doped 2H-TaSe2: Suggestion of chiral unitary localization2014

    • Author(s)
      T. Kanno, T Matsumoto, K. Ichimura, T. Matsuura, S. Tanda
    • Organizer
      International School and Workshop on Electronic Crystals 2014 (ECRYS-2014)
    • Place of Presentation
      カルジェス(フランス)
    • Year and Date
      2014-08-12 – 2014-08-22
    • Related Report
      2014 Annual Research Report
  • [Presentation] Charge disproportionation in organic conductors2014

    • Author(s)
      K. Ichimura
    • Organizer
      Collaborative Conference on Material Research Joint with CC3DR2014 (CC3DMR2014)
    • Place of Presentation
      仁川(韓国)
    • Year and Date
      2014-06-23 – 2014-06-27
    • Related Report
      2014 Annual Research Report
    • Invited
  • [Presentation] Charge Disproportionation in Organic Conductors2014

    • Author(s)
      K. Ichimura
    • Organizer
      Collaborative Conference on Material Research Joint with CC3DR 2014 (CC3DMR2014)
    • Place of Presentation
      仁川(韓国)
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] Charge Order Fluctuation in Organic Conductors2013

    • Author(s)
      K. Ichimura
    • Organizer
      Collaborative Conference on Material Research Joint with CC3DR 2013 (CC3DMR2013)
    • Place of Presentation
      済州島(韓国)
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] muSR Study of the Density Wave State in alpha-(BEDT-TTF)2MHg(SCN)4 (M=K, Rb)2013

    • Author(s)
      K. Ichimura and K. Katono
    • Organizer
      10th Program Advisory Committee Meeting for Materials and Life Science at RIKEN Nishina Center
    • Place of Presentation
      理化学研究所、和光市
    • Related Report
      2013 Research-status Report
  • [Presentation] Charge Order Fluctuation in alpha-(BEDT-TTF)2I3 Observed by STM2013

    • Author(s)
      K. Ichimura
    • Organizer
      International Symposium on Crystalline Organic Metals, Superconductors and Magnets (ISCOM2013)
    • Place of Presentation
      モントリオール(カナダ)
    • Related Report
      2013 Research-status Report
  • [Presentation] Density Wave State in alpha-(BEDTTTF)2KHg(SCN)4 Probed by STM2013

    • Author(s)
      K. Katono, K. Ichimura, T. Taniguchi, S. Tanda and K. Yamaya
    • Organizer
      International Symposium on Crystalline Organic Metals, Superconductors and Magnets (ISCOM2013)
    • Place of Presentation
      モントリオール(カナダ)
    • Related Report
      2013 Research-status Report
  • [Presentation] STM Observation of Charge Disproportionation in Organic Conductors2013

    • Author(s)
      K. Katono, K. Ichimura, T. Taniguchi, Y. Kawashima, K. Yamaya and S. Tanda
    • Organizer
      International Workshop on Phase Transition, Critical Phenomena and Related Topics in Complex Networks
    • Place of Presentation
      北海道大学、札幌市
    • Related Report
      2013 Research-status Report
  • [Presentation] Discovery of Chiral CDW in 1T-VSe22013

    • Author(s)
      Y. Sugawara, J. Ishioka, Y.Toda, M. Oda, T. Kurosawa, T. Matsuura, K. Ichimura and S. Tanda
    • Organizer
      International Workshop on Phase Transition, Critical Phenomena and Related Topics in Complex Networks
    • Place of Presentation
      北海道大学、札幌市
    • Related Report
      2013 Research-status Report
  • [Presentation] Metal-Insulator Transition in the Chiral-Unitary System 2H-FexTa1-xSe22013

    • Author(s)
      T. Kanno, T. Matsumoto, S. K. Kataria, J. Ishioka, N. Matsunaga, K. Ichimura, T. Matsuura and S. Tanda
    • Organizer
      International Workshop on Phase Transition, Critical Phenomena and Related Topics in Complex Networks
    • Place of Presentation
      北海道大学、札幌市
    • Related Report
      2013 Research-status Report
  • [Presentation] alpha-(BEDT-TTF)2KHg(SCN)4における密度波状態2013

    • Author(s)
      上遠野一広、市村晃一、河島祐樹、山谷和彦、丹田聡
    • Organizer
      日本物理学会第68回年次大会
    • Place of Presentation
      広島大学東広島キャンパス(東広島市)
    • Related Report
      2012 Research-status Report
  • [Presentation] STM observation of the density wave state in alpha-(BEDT-TTF)2KHg(SCN)42012

    • Author(s)
      K. Katono, K. Ichimura, Y. Kawashima, K. Yamaya and S. Tanda
    • Organizer
      International Symposium on Material Science Opened by Molecular Degree of Freedom (MDF2012)
    • Place of Presentation
      宮崎国際会議場(宮崎市)
    • Related Report
      2012 Research-status Report

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Published: 2013-05-31   Modified: 2020-05-15  

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