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Quantum spin liqid state in a frustrated magnetic system

Research Project

Project/Area Number 25400345
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionTokyo Metropolitan University

Principal Investigator

Kadowaki Hiroaki  首都大学東京, 理工学研究科, 准教授 (70194876)

Co-Investigator(Renkei-kenkyūsha) TAKATSU Hiroshi  首都大学東京, 理工学研究科, 助教 (60585602)
Project Period (FY) 2013-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2015: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2014: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2013: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Keywords磁性 / フラストレーション
Outline of Final Research Achievements

We have investigated the frustrated magnetic system Tb2Ti2O7, known as a candidate for a quantum spin-liquid state, by using high-quality single crystals of Tb2+xTi2-xO7+y, i.e., crystals with well-controlled compositions x and/or y of the order 0.001. To study interesting but puzzling behavior of this system it is very importatnt to grow high-quality single crystals. Although difficult, we have succeeded in growing high-quality crystals. By performing specific heat and magnetization measurements as well as inelastic neutron scattering experiments using these cryslals, we have found that this system has not only magnetic spin degrees of freedom but also frustated electric-multipole degrees of freedom, and that variation of x indudes a quantum phase transition between an electric-multipole ordered state and the quantum spin-liquid state.

Report

(5 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Research-status Report
  • 2014 Research-status Report
  • 2013 Research-status Report
  • Research Products

    (30 results)

All 2017 2016 2015 2014 2013 Other

All Int'l Joint Research (3 results) Journal Article (12 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 12 results,  Open Access: 3 results,  Acknowledgement Compliant: 5 results) Presentation (14 results) (of which Int'l Joint Research: 2 results,  Invited: 3 results) Remarks (1 results)

  • [Int'l Joint Research] Institut Laue-Langevin(France)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] Institut Laue-Langevin(France)

    • Related Report
      2015 Research-status Report
  • [Int'l Joint Research] NIST(米国)

    • Related Report
      2015 Research-status Report
  • [Journal Article] Thermodynamic properties of quadrupolar states in the frustrated pyrochlore magnet Tb2Ti2O72017

    • Author(s)
      H. Takatsu, T. Taniguchi, S. Kittaka, T. Sakakibara, H. Kadowaki
    • Journal Title

      Journal of Physics: Conf. Series

      Volume: 828 Pages: 012007-012007

    • DOI

      10.1088/1742-6596/828/1/012007

    • NAID

      120006305771

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Quantum spin liquid and electric quadrupolar states of single crystal Tb2+xTi2-xO7+y2016

    • Author(s)
      M. Wakita, T. Taniguchi, H. Edamoto, H. Takatsu and H. Kadowaki
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 683 Pages: 012023-012023

    • DOI

      10.1088/1742-6596/683/1/012023

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Quadrupole order in the frustrated pyrochlore magnet Tb2Ti2O72016

    • Author(s)
      H. Takatsu, T. Taniguchi S. Kittaka, T. Sakakibara, H. Kadowaki
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 683 Pages: 012022-012022

    • DOI

      10.1088/1742-6596/683/1/012022

    • NAID

      120006958102

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Quadrupole Order in the Frustrated Pyrochlore Tb2+xTi2-xO7+y2016

    • Author(s)
      H. Takatsu, S. Onoda, S. Kittaka, A. Kasahara, Y. Kono, T. Sakakibara, Y. Kato, B. Fak, J. Ollivier, J.W. Lynn, T. Taniguchi, M. Wakita, H. Kadowaki
    • Journal Title

      Phys. Rev. Lett.

      Volume: 0 Pages: 0-0

    • NAID

      120005848239

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Composite spin and quadrupole wave in the ordered phase of Tb2+xTi2-xO7+y2015

    • Author(s)
      H. Kadowaki, H. Takatsu, T. Taniguchi, B. Fak, J. Ollivier
    • Journal Title

      SPIN

      Volume: 05 Issue: 02 Pages: 154003-154003

    • DOI

      10.1142/s2010324715400032

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Comparative study of low-temperature x-ray diffraction experiments on R2Ir2O7 (R = Nd , Eu, and Pr)2014

    • Author(s)
      H. Takatsu, K. Watanabe, K. Goto, H. Kadowaki
    • Journal Title

      Phys. Rev. B

      Volume: 90 Issue: 23 Pages: 235110-235110

    • DOI

      10.1103/physrevb.90.235110

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Scaling ansatz for the ac magnetic response in two-dimensional spin ice2014

    • Author(s)
      H. Otsuka, H. Takatsu, K. Goto, H. Kadowaki
    • Journal Title

      Phys. Rev. B

      Volume: 90 Issue: 14 Pages: 144428-144428

    • DOI

      10.1103/physrevb.90.144428

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Stabilization of High-Tc Phase of BiS2-Based Superconductor LaO0.5F0.5BiS2 Using High-Pressure Synthesis2014

    • Author(s)
      Y. Mizuguchi, T. Hiroi, J. Kajitani, H. Takatsu, H. Kadowaki, O. Miura
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 83 Issue: 5 Pages: 053704-053704

    • DOI

      10.7566/jpsj.83.053704

    • NAID

      210000133063

    • Related Report
      2014 Research-status Report
    • Peer Reviewed
  • [Journal Article] Magnetic structure of the conductive triangular-lattice antiferromagnet PdCrO22014

    • Author(s)
      H. Takatsu, G. Nenert, H. Kadowaki, H. Yoshizawa, M. Enderle, S. Yonezawa, Y. Maeno, J. Kim, N. Tsuji, M. Takata, Y. Zhao, M. Green, and C. Broholm
    • Journal Title

      Physical Review B

      Volume: 89 Issue: 10 Pages: 104408-104408

    • DOI

      10.1103/physrevb.89.104408

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Correlation between crystal structure and superconductivity in LaO0.5F0.5BiS22014

    • Author(s)
      J. Kajitani, K. Deguchi, A. Omachi, T. Hiroi, Y. Takano, H. Takatsu, H. Kadowaki, O. Miura, Y. Mizuguchi
    • Journal Title

      Solid State Commun.

      Volume: 181 Pages: 1-4

    • DOI

      10.1016/j.ssc.2013.11.027

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] atsu, H., Goto, K., Otsuka, H., Higashinaka, R., Matsubayashi, K., Uwatoko, Y., Kadowaki, H. Two-dimensional monopole dynamics in the dipolar spin ice Dy 2Ti2O72013

    • Author(s)
      H. Takatsu, K. Goto, H. Otsuka, R. Higashinaka, K. Matsubayashi, Y. Uwatoko, and H. Kadowaki
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 82 Issue: 7 Pages: 73707-73707

    • DOI

      10.7566/jpsj.82.073707

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] AC susceptibility of the dipolar spin ice Dy2Ti 2O7: Experiments and Monte Carlo simulations2013

    • Author(s)
      H. Takatsu, K. Goto, H. Otsuka, R. Higashinaka, K. Matsubayashi, Y. Uwatoko, and H. Kadowaki
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 82 Issue: 10 Pages: 104710-104710

    • DOI

      10.7566/jpsj.82.104710

    • NAID

      210000132794

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Presentation] Thermodynamic properties of quadrupolar states in the frustrated pyrochlore magnet Tb2Ti2O72016

    • Author(s)
      H. Takatsu, T. Taniguchi, S. Kittaka, T. Sakakibara, H. Kadowaki
    • Organizer
      The 8th International Conference on Highly Frustrated Magnetism (HFM 2016)
    • Place of Presentation
      Taipei, Taiwan
    • Year and Date
      2016-09-07
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 量子スピン液体Tb2+xTi2-xO7+yの単結晶中性子非弾性散乱2016

    • Author(s)
      脇田美香, 高津浩, 門脇広明, B. Fak, J. Ollivier
    • Organizer
      日本物理学会
    • Place of Presentation
      東北学院大学 泉キャンパス
    • Year and Date
      2016-03-19
    • Related Report
      2015 Research-status Report
  • [Presentation] Quadrupole order and spin liquid state of Tb2+xTi2-xO7+y2015

    • Author(s)
      Hiroaki Kadowaki
    • Organizer
      International Chemical Congress of Pacific Basin Societies
    • Place of Presentation
      Honolulu, Hawaii
    • Year and Date
      2015-12-17
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] パイロクロアTb2+xTi2-xO7+yにおける4極子状態の研究2015

    • Author(s)
      門脇広明, 高津浩, 脇田美香, B. Fak, J. Ollivier
    • Organizer
      日本物理学会
    • Place of Presentation
      関西大学 千里山キャンパス
    • Year and Date
      2015-09-19
    • Related Report
      2015 Research-status Report
  • [Presentation] Tb2+xTi2-xO7+yにおけるスピン多極子複合励起の研究2015

    • Author(s)
      門脇広明, 高津浩, 谷口智洋, 脇田美香, B. Fak, J. Ollivier
    • Organizer
      日本物理学会
    • Place of Presentation
      関西大学 千里山キャンパス
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] 量子スピンアイスTb2+xTi2-xO7+yの研究2015

    • Author(s)
      脇田美香, 高津浩, 門脇広明
    • Organizer
      日本物理学会
    • Place of Presentation
      関西大学 千里山キャンパス
    • Year and Date
      2015-09-16
    • Related Report
      2015 Research-status Report
  • [Presentation] 低温磁化測定によるTb2+xTi2-xO7+yの長距離秩序の起源の検証2015

    • Author(s)
      高津浩,脇田美香,谷口智洋,門脇広明,笠原聡,河野洋平,橘高俊一郎,榊原俊郎
    • Organizer
      日本物理学会 第70回年次大会
    • Place of Presentation
      早稲田大学 早稲田キャンパス
    • Year and Date
      2015-03-21 – 2015-03-24
    • Related Report
      2014 Research-status Report
  • [Presentation] フラストレート磁性体Tb2+xTi2-xO7+yの純良単結晶とその物性2014

    • Author(s)
      脇田美香,谷口智洋,高津浩,門脇広明
    • Organizer
      日本物理学会 2014年秋季大会
    • Place of Presentation
      中部大学 春日井キャンパス
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] 極低温比熱測定からみたTb2+xTi2-xO7+yにおける隠れた秩序と磁場誘起相転移2014

    • Author(s)
      高津浩,谷口智洋,門脇広明,橘高俊一郎,榊原俊郎
    • Organizer
      日本物理学会 2014年秋季大会
    • Place of Presentation
      中部大学春日井キャンパス
    • Year and Date
      2014-09-07 – 2014-09-10
    • Related Report
      2014 Research-status Report
  • [Presentation] Dy2Ti2O7のカゴメアイス状態における磁気モノポールの二次元ダイナミクス

    • Author(s)
      後藤和基,高津浩,大塚博巳,東中隆二,門脇広明,J.W. Lynn,佐藤卓,松平和之,広井善二,松林和幸,上床美也
    • Organizer
      日本物理学会
    • Place of Presentation
      徳島大学 三島キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] Tb2+xTi2-xO7+yの長距離秩序と量子スピン液体状態

    • Author(s)
      門脇広明
    • Organizer
      日本物理学会
    • Place of Presentation
      徳島大学 三島キャンパス
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] パイロクロア磁性体Nd2Ir2O7の異常な負の熱膨張

    • Author(s)
      高津浩,渡邊邦彦,後藤和基,門脇広明
    • Organizer
      日本物理学会
    • Place of Presentation
      徳島大学 三島キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] 純良単結晶によるTb2+xTi2-xO7+yの長距離秩序の研究

    • Author(s)
      谷口智洋,脇田美香,東中隆二,後藤和基,高津浩,門脇広明,池田陽一,吉澤英樹,J.W. Lynn,J. Ollivier,B. Fak
    • Organizer
      日本物理学会
    • Place of Presentation
      東海大学 湘南キャンパス
    • Related Report
      2013 Research-status Report
  • [Presentation] Long-range order and spin-liquid state of Tb2+xTi2-xO7+y

    • Author(s)
      Hiroaki Kadowaki
    • Organizer
      International Workshop on Frustration and Topology in Condensed Matter Physics
    • Place of Presentation
      National Cheng Kung University, Tainan, Taiwan
    • Related Report
      2013 Research-status Report
    • Invited
  • [Remarks] 首都大学東京ニュース(報道発表)【研究成果発表】スピン液体の近くの“隠れた秩序”

    • URL

      http://www.tmu.ac.jp/news/topics/12819.html

    • Related Report
      2016 Annual Research Report

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Published: 2014-07-25   Modified: 2022-01-24  

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