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Development of High-Performance Magnetic Refrigeration Materials by Numerical Simulations

Research Project

Project/Area Number 25420698
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Physical properties of metals/Metal-base materials
Research InstitutionNational Institute for Materials Science

Principal Investigator

Tamura Ryo  国立研究開発法人物質・材料研究機構, 理論計算科学ユニット, 研究員 (20636998)

Co-Investigator(Renkei-kenkyūsha) KITAZAWA Hideaki  国立研究開発法人・物質材料研究機構, 量子ビームユニット, ユニット長 (00195257)
TANAKA Shu  早稲田大学, 早稲田大学高等研究所, 助教 (40507836)
Project Period (FY) 2013-04-01 – 2016-03-31
Project Status Completed (Fiscal Year 2015)
Budget Amount *help
¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2015: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2014: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2013: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Keywords磁性材料 / 磁気冷凍 / 磁気エントロピー / 磁気構造 / 不純物効果 / 圧力効果 / 巨大磁気エントロピー変化 / 不純物ドープ / スケーリング則 / 断熱温度変化 / 熱吸収能力 / 反強磁性体 / 相転移
Outline of Final Research Achievements

In order to develop new high performance magnetic refrigeration materials, we established the method to obtain the maximum magnetic refrigeration efficiency and studied the control method of the magnetic refrigeration efficiency by numerical simulations. As a result, we found that the method where the magnetic refrigeration efficiency becomes maximum is different between ferromagnetic materials and non-ferromagnetic materials. We proposed new method to obtain the maximum magnetic refrigeration efficiency for all magnetic materials. Furthermore, we showed that the magnetic refrigeration efficiency can be controlled by the impurity effect and the pressure effect. In addition, we developed the magnetic refrigeration material Ho5Pd2 which is a candidate material for low-temperature magnetic refrigeration.

Report

(4 results)
  • 2015 Annual Research Report   Final Research Report ( PDF )
  • 2014 Research-status Report
  • 2013 Research-status Report

Research Products

(45 results)

All 2016 2015 2014 2013 Other

All Int'l Joint Research (1 results) Journal Article (8 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 8 results,  Open Access: 1 results,  Acknowledgement Compliant: 3 results) Presentation (31 results) (of which Int'l Joint Research: 6 results,  Invited: 1 results) Remarks (5 results)

  • [Int'l Joint Research] Universidad Autónoma de Madrid/Universidad de Sevilla(スペイン)

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Estimation of magnetocaloric properties by using Monte Carlo method for AMRR cycle2015

    • Author(s)
      R Arai, R Tamura, H Fukuda, J Li, A T Saito, S Kaji, H Nakagome, and T Numazawa
    • Journal Title

      IOP Conference Series: Materials Science and Engineering

      Volume: 101 Pages: 1-8

    • DOI

      10.1088/1757-899x/101/1/012118

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Magnetic structure of the frustrated antiferromagnetic spin-1/2 chain substance Cu3Mo2O9: appearance of a partial disordered state2015

    • Author(s)
      M. Hase, H. Kuroe, V. Y. Pomjakushin, L. Leller, R. Tamura, N. Terada, Y. Matsushita, A. Doenni, and T. Sekine
    • Journal Title

      Physical Review B

      Volume: 92

    • DOI

      10.1103/physrevb.92.054425

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Sample Dependence of Giant Magnetocaloric Effect in a Cluster-Glass System Ho5Pd22015

    • Author(s)
      Saori Toyoizumi, Hideaki Kitazawa, Yukihiko Kawamura, Hiroaki Mamiya, Noriki Terada, Ryo Tamura, Andreas Dönni, Kengo Morita, and Akira Tamaki
    • Journal Title

      Journal of Applied Physics

      Volume: 117

    • DOI

      10.1063/1.4906296

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Magnetic Ordered Structure Dependence of Magnetic Refrigeration Efficiency2014

    • Author(s)
      Ryo Tamura, Shu Tanaka, Takahisa Ohno, and Hideaki Kitazawa
    • Journal Title

      Journal of Applied Physics

      Volume: 116

    • DOI

      10.1063/1.4891803

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Phase Transitions with Discrete Symmetry Breaking in Antiferromagnetic Heisenberg Models on a Triangular Lattice2014

    • Author(s)
      Ryo Tamura, Shu Tanaka, and Naoki Kawashima
    • Journal Title

      JPS Conf. Proc. --- Proceedings of the 12th Asia Pacific Physics Conference (APPC12)

      Volume: 1

    • DOI

      10.7566/jpscp.1.012125

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] A Generalized Magnetic Refrigeration Scheme2014

    • Author(s)
      Ryo Tamura, Takahisa Ohno, and Hideaki Kitazawa
    • Journal Title

      Applied Physics Letters

      Volume: 104

    • DOI

      10.1063/1.4864161

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Second-order phase transition in the Heisenberg model on a triangular lattice with competing interactions2013

    • Author(s)
      Ryo Tamura, Shu Tanaka, and Naoki Kawashima
    • Journal Title

      Phys. Rev. B

      Volume: 87

    • DOI

      10.1103/physrevb.87.214401

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Journal Article] Interlayer-interaction dependence of latent heat in the Heisenberg mode 1 on a stacked triangular lattice with competing interactions2013

    • Author(s)
      Ryo Tamura and Shu Tanaka
    • Journal Title

      Physical Review E

      Volume: 88

    • DOI

      10.1103/physreve.88.052138

    • Related Report
      2013 Research-status Report
    • Peer Reviewed
  • [Presentation] 磁化過程を入力としたスピン間相互作用の推定手法2016

    • Author(s)
      田村亮,福島孝治
    • Organizer
      日本物理学会 第71回年次大会
    • Place of Presentation
      宮城
    • Year and Date
      2016-03-21
    • Related Report
      2015 Annual Research Report
  • [Presentation] クラスターグラス系Ho5-xErxPd2の磁気熱量効果2016

    • Author(s)
      豊泉沙織,Lukasz Zrodowski,北澤英明,田村亮,森田憲吾,田巻明
    • Organizer
      日本物理学会 第71回年次大会
    • Place of Presentation
      宮城
    • Year and Date
      2016-03-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] Multiple-q Phases in a Stacked Triangular Antiferromagnetic Heisenberg Model with Competing Interactions under Magnetic Field2015

    • Author(s)
      Shu Tanaka, Ryo Tamura, Kazuhiko Tanimoto, and Keisuke Totsuka
    • Organizer
      The International Chemical Congress of Pacific Basin Societies 2015
    • Place of Presentation
      Hawaii
    • Year and Date
      2015-12-17
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Magnetic Ordered Structure Dependence of Magnetocaloric Effect2015

    • Author(s)
      Ryo Tamura, Shu Tanaka, Takahisa Ohno, and Hideaki Kitazawa
    • Organizer
      The International Chemical Congress of Pacific Basin Societies 2015
    • Place of Presentation
      Hawaii
    • Year and Date
      2015-12-15
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Control of the Nature of the Phase Transition in Frustrated Systems2015

    • Author(s)
      Ryo Tamura and Shu Tanaka
    • Organizer
      STAC-9 & TOEO-9
    • Place of Presentation
      Ibaraki
    • Year and Date
      2015-10-20
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] ベイズ統計を用いた磁化過程からの相互作用推定2015

    • Author(s)
      田村亮,福島孝治
    • Organizer
      日本物理学会 2015年秋季大会
    • Place of Presentation
      大阪
    • Year and Date
      2015-09-19
    • Related Report
      2015 Annual Research Report
  • [Presentation] クラスターグラス系Ho5Pd2-xAx(A=Ni,Ag)の磁気熱量効果 II2015

    • Author(s)
      豊泉沙織,北澤英明,田村亮,寺田典樹,間宮広明,森田憲吾,田巻明
    • Organizer
      日本物理学会 2015年秋季大会
    • Place of Presentation
      大阪
    • Year and Date
      2015-09-18
    • Related Report
      2015 Annual Research Report
  • [Presentation] A Generalized Potts Model with Invisible States - Toward Applications to Information Science -2015

    • Author(s)
      Ryo Tamura and Shu Tanaka
    • Organizer
      New Horizons of Quantum and Classical Information 2015
    • Place of Presentation
      Tokyo
    • Year and Date
      2015-08-04
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Critical Phenomena in Two-Dimensional Frustrated Heisenberg Models2015

    • Author(s)
      Shu Tanaka, Ryo Tamura, and Naoki Kawashima
    • Organizer
      20th International Conference on Magnetism
    • Place of Presentation
      Barcelona
    • Year and Date
      2015-07-10
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] A New Method for Maximizing Magnetic Refrigeration Efficiency in Antiferromagnets2015

    • Author(s)
      Ryo Tamura, Shu Tanaka, Takahisa Ohno, and Hideaki Kitazawa
    • Organizer
      20th International Conference on Magnetism
    • Place of Presentation
      Barcelona
    • Year and Date
      2015-07-06
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] クラスターグラス系Ho5Pd2-xAxの磁気熱量効果2015

    • Author(s)
      北澤英明,豊泉沙織,M. Bochenek,田村亮,寺田典樹,間宮広明,田巻明
    • Organizer
      日本物理学会 第70回年次大会
    • Place of Presentation
      早稲田大学(東京都)
    • Year and Date
      2015-03-23
    • Related Report
      2014 Research-status Report
  • [Presentation] 複数の相互作用が競合する積層三角格子磁性模型の磁場中相図2015

    • Author(s)
      田村亮,田中宗,谷本和彦,戸塚圭介
    • Organizer
      日本物理学会 第70回年次大会
    • Place of Presentation
      早稲田大学(東京都)
    • Year and Date
      2015-03-22
    • Related Report
      2014 Research-status Report
  • [Presentation] 反強磁性体の磁気冷凍性能を最大限引き出す手法開発2015

    • Author(s)
      田村亮
    • Organizer
      第8回 三機関連携「量子複雑現象」研究会
    • Place of Presentation
      SPring-8(兵庫県)
    • Year and Date
      2015-01-05
    • Related Report
      2014 Research-status Report
  • [Presentation] 磁気秩序構造に依存した磁気熱量効果の理論研究2014

    • Author(s)
      田中宗,田村亮,大野隆央,北澤英明
    • Organizer
      第8回 物性科学領域横断研究会 (領域合同研究会)
    • Place of Presentation
      大阪大学(大阪府)
    • Year and Date
      2014-11-21
    • Related Report
      2014 Research-status Report
  • [Presentation] 積層三角格子反強磁性体における特異な潜熱変化2014

    • Author(s)
      田村亮
    • Organizer
      第8回 物性科学領域横断研究会 (領域合同研究会)
    • Place of Presentation
      大阪大学(大阪府)
    • Year and Date
      2014-11-21
    • Related Report
      2014 Research-status Report
  • [Presentation] 磁気冷凍における熱吸収能力と磁気構造の関係2014

    • Author(s)
      田村亮,田中宗,大野隆央,北澤英明
    • Organizer
      物性研究所計算物質科学研究センター 第4回シンポジウム・物性研スーパーコンピュータ共同利用報告会
    • Place of Presentation
      東京大学物性研究所(千葉県)
    • Year and Date
      2014-11-12
    • Related Report
      2014 Research-status Report
  • [Presentation] 磁気冷凍材料Ho5Pd2の磁場中中性子回折2014

    • Author(s)
      北澤英明,豊泉沙織,L. Keller,河村幸彦,田村亮,間宮広明,寺田典樹,A. Döenni,田巻明
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学(愛知県)
    • Year and Date
      2014-09-07
    • Related Report
      2014 Research-status Report
  • [Presentation] 磁気冷凍における磁気構造に依存した熱吸収能力の比較2014

    • Author(s)
      田村亮,田中宗,大野隆央,北澤英明
    • Organizer
      日本物理学会2014年秋季大会
    • Place of Presentation
      中部大学(愛知県)
    • Year and Date
      2014-09-07
    • Related Report
      2014 Research-status Report
  • [Presentation] Spatial Dimension Dependence of First-Order Phase Transition Nature in Stacked Triangular Lattice System2014

    • Author(s)
      Ryo Tamura and Shu Tanaka
    • Organizer
      International Conference on Highly Frustrated Magnetism 2014
    • Place of Presentation
      University of Cambridge (Cambridge)
    • Year and Date
      2014-07-08
    • Related Report
      2014 Research-status Report
  • [Presentation] Second-Order Phase Transition in Two-Dimensional Frustrated Systems2014

    • Author(s)
      Shu Tanaka, Ryo Tamura, and Naoki Kawashima
    • Organizer
      International Conference on Highly Frustrated Magnetism 2014
    • Place of Presentation
      University of Cambridge (Cambridge)
    • Year and Date
      2014-07-08
    • Related Report
      2014 Research-status Report
  • [Presentation] Second-Order Phase Transition in Antiferromagnetic Heisenberg Model on Triangular Lattice

    • Author(s)
      Ryo Tamura, Shu Tanaka, and Naoki Kawashima
    • Organizer
      The 12th Asia Pacific Physics Conference of AAPPS (APPC12)
    • Place of Presentation
      Chiba
    • Related Report
      2013 Research-status Report
  • [Presentation] Second-Order Phase Transition in Heisenberg Model on Triangular Lattice with Competing Interactions

    • Author(s)
      Ryo Tamura, Shu Tanaka, and Naoki Kawashima
    • Organizer
      XXV IUPAP International Conference on Statistical Physics (STATPHYS 25)
    • Place of Presentation
      Seoul
    • Related Report
      2013 Research-status Report
  • [Presentation] Toward an Alternative Method to Quantum Annealing - Quest for New Type of Fluctuation -

    • Author(s)
      Ryo Tamura and Shu Tanaka
    • Organizer
      Summer Workshop on "Physics, Mathematics, And All That Quantum Jazz"
    • Place of Presentation
      Osaka
    • Related Report
      2013 Research-status Report
    • Invited
  • [Presentation] 磁気冷凍材料Ho5Pd2における組成変化が及ぼす磁気熱量効果への影響

    • Author(s)
      北澤英明,豊泉沙織,河村幸彦,田村亮,間宮広明,寺田典樹,A. Doenni,田巻明
    • Organizer
      日本物理学会 2013年秋季大会
    • Place of Presentation
      徳島
    • Related Report
      2013 Research-status Report
  • [Presentation] 磁気熱量効果の磁気構造依存性

    • Author(s)
      田村亮,大野隆央,北澤英明
    • Organizer
      日本物理学会 2013年秋季大会
    • Place of Presentation
      徳島
    • Related Report
      2013 Research-status Report
  • [Presentation] 磁気冷凍材料に適した磁気構造の選定

    • Author(s)
      田村亮
    • Organizer
      第13回 NIMSフォーラム
    • Place of Presentation
      東京
    • Related Report
      2013 Research-status Report
  • [Presentation] 反強磁性体における磁気熱量効果の特徴

    • Author(s)
      田村亮,大野隆央,北澤英明
    • Organizer
      第4回 物性研スパコン共同利用・CMSI合同研究会
    • Place of Presentation
      千葉
    • Related Report
      2013 Research-status Report
  • [Presentation] Magnetic Structure Dependence of Magnetic Refrigeration Efficiency

    • Author(s)
      Ryo Tamura, Shu Tanaka, Takahisa Ohno, and Hideaki Kitazawa
    • Organizer
      RIKEN-APW joint workshop "Highlights in condensed matter physics"
    • Place of Presentation
      Saitama
    • Related Report
      2013 Research-status Report
  • [Presentation] Selection of Magnetic Structure Suited for Magnetic Refrigeration Material

    • Author(s)
      Ryo Tamura, Takahisa Ohno, and Hideaki Kitazawa
    • Organizer
      MANA International Symposium 2014
    • Place of Presentation
      Ibaraki
    • Related Report
      2013 Research-status Report
  • [Presentation] 磁気冷凍材料R5Pd2(R=Tb, Dy, Ho, Er)の磁気熱量効果

    • Author(s)
      北澤英明,M. Bochenek,豊泉沙織,河村幸彦,田村亮,間宮広明,寺田典樹,A. Doenni,L. Keller,田巻明
    • Organizer
      日本物理学会 第69回年次大会
    • Place of Presentation
      神奈川
    • Related Report
      2013 Research-status Report
  • [Presentation] 磁気冷凍性能の磁気構造依存性

    • Author(s)
      田村亮,田中宗,大野隆央,北澤英明
    • Organizer
      日本物理学会 第69回年次大会
    • Place of Presentation
      神奈川
    • Related Report
      2013 Research-status Report
  • [Remarks] 研究紹介webページ(田村亮個人ページ)

    • URL

      http://www.nims.go.jp/cmsc/fps1/ryo_tamura/tamura_home_j.html

    • Related Report
      2015 Annual Research Report
  • [Remarks] NIMSプレスリリース

    • URL

      http://www.nims.go.jp/news/press/2014/03/p201403100.html

    • Related Report
      2015 Annual Research Report 2014 Research-status Report
  • [Remarks] 研究紹介webページ(田村亮個人ページ)

    • URL

      http://www.nims.go.jp/icys/ryo_tamura/tamura_home_j.html

    • Related Report
      2014 Research-status Report
  • [Remarks] 研究紹介webページ(田村亮個人ページ)

    • URL

      http://www.nims.go.jp/icys/ryo_tamura/tamura_home_j.html

    • Related Report
      2013 Research-status Report
  • [Remarks] NIMSプレスリリース(反強磁性体の磁気冷凍性能を最大にする方法を発見)

    • URL

      http://www.nims.go.jp/news/press/2014/03/p201403100.html

    • Related Report
      2013 Research-status Report

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Published: 2014-07-25   Modified: 2019-07-29  

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