Development of Surface plasmon excitation assited ultrafast all optical nanoswitching system

• Project/Area Number: 26286059
• Research Category: Grant-in-Aid for Scientific Research (B)
• Allocation Type: Partial Multi-year Fund
• Section: 一般
• Research Field: Optical engineering, Photon science
• Research Institution: Shizuoka University
• Principal Investigator: Sugita Atsushi 静岡大学, 工学部, 准教授 (20334956)
• Co-Investigator(Kenkyū-buntansha): 間瀬 暢之 静岡大学, 工学部, 教授 (40313936) ; 川田 善正 静岡大学, 電子工学研究所, 教授 (70221900)
• Project Period (FY): 2014-04-01 – 2017-03-31
• Project Status: Completed (Fiscal Year 2016)
• Budget Amount: ¥15,990,000 (Direct Cost: ¥12,300,000、Indirect Cost: ¥3,690,000); Fiscal Year 2016: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000); Fiscal Year 2015: ¥5,720,000 (Direct Cost: ¥4,400,000、Indirect Cost: ¥1,320,000); Fiscal Year 2014: ¥8,190,000 (Direct Cost: ¥6,300,000、Indirect Cost: ¥1,890,000)
• Keywords: 非線形光学 / 金属ナノ粒子 / 表面プラズモン / 非線形光学ポリマー / フェムト秒分光 / 量子エレクトロニクス / 光スイッチ / 光物性 / ナノ光工学 / 応用工学・量子光工学 / 表面・界面物性 / 光源技術

Outline of Final Research Achievements

Linear and second-order nonlinear optical properties were examined for Au nanoprisms at localized surface plasmon (LSP) resonances. The scattering and second harmonic (SH) spectroscopies demonstrated that the linear and second-order nonlinear optical (NLO) susceptibilities of the Au nanoprisms (AuNP) were independent of the polarization direction of the excitation light wave. The isotropic behaviors were consistent with the demands imposed from the C3v-point symmetry of the systems. The SH spectroscopies were also performed for the AuNP coated with NLO polymer thin films. The SH intensities from the NLO polymer coated AuNP were approximately 5 times as high as those of the polymer-noncoated ones. The nonlinearities of the AuNP were successfully enhanced with polymeric materials rich in nonlinearities. Finally, frequency-resolved optical gating spectroscopy were performed and the ultrafast dynamics of the LSP polarizations with ~10 fs dephasing times were resolved.

Research Products

• [Journal Article] The Role of Chemisorption for Push-Pull Chromophores on SiO2 Surfaces in Non-Electrically Poling Host-Guest NLO Polymers (2017)
  • Author(s): Atsushi Sugita, Kazuma Ito, Yasuaki Sato, Ryota Suzuki, Kohei Sato, Tetsuo Narumi, Nobuyuki Mase, Yasushi Takano, Tomonori Matsushita, Shigeru Tasaka, and Yoshimasa Kawata
  • Journal Title: Journal of Photochemistry and Photobiology A: Chemistry Volume: 340 Pages: 35-45
  • DOI: 10.1016/j.jphotochem.2017.03.007
  • Peer Reviewed / Acknowledgement Compliant
• [Journal Article] Melt-crystallizations of poly (L-lactic acid) under external DC electric fields (2016)
  • Author(s): Atsushi Sugita, Shota Masauji, Ryunosuke Yamaguchi, Atsushi Kubono, Shigeru Tasaka
  • Journal Title: Polymer Volume: 85 Pages: 185-188
  • DOI: 10.1016/j.polymer.2015.12.053
  • Peer Reviewed
• [Journal Article] Fabrication of bright and thin Zn2SiO4 luminescent film for electron beam excitation-assisted optical microscope (2015)
  • Author(s): Taichi Furukawa, Satoshi Kanamori, Masahiro Fukuta, Yasunori Nawa, Hiroko Kominami, Yoichiro Nakanishi, Atsushi Sugita, Wataru Inami, and Yoshimasa Kawata
  • Journal Title: Optics Express Volume: 23 Issue: 14 Pages: 18631-18637
  • DOI: 10.1364/oe.23.018630
  • Peer Reviewed
• [Journal Article] 電子線励起アシスト光学顕微鏡のためのナノ光源の開発 (2015)
  • Author(s): 古川太一、居波渉、守田智勇、杉田篤史、川田善正
  • Journal Title: レーザー研究 Volume: 43 Pages: 164-167
  • NAID: 130007957096
  • Peer Reviewed
• [Presentation] 金ナノ三角柱の局在表面プラズモン共鳴時における二次非線形光学効果 (2017)
  • Author(s): 杉田篤史, 余語宏文、小 篤史、川田善正
  • Organizer: 日本物理学会第72回年次大会
  • Place of Presentation: 大阪大学豊中キャンパス （大阪府豊中市）
  • Year and Date: 2017-03-17
• [Presentation] 局在表面プラズモン共鳴された金ナノ三角柱の偏光分解第二高調波分光 (2017)
  • Author(s): 余語宏文, 小野篤史, 川田善正, 杉田篤史
  • Organizer: 第64回応用物理学会春季学術講演会
  • Place of Presentation: パシフィコ横浜 （神奈川県横浜市）
  • Year and Date: 2017-03-14
• [Presentation] 金ナノ三角柱/非線形光学ポリマー複合系の局在表面プラズモン共鳴条件での第二高調波発生現象 (2017)
  • Author(s): 岸口光一, 余語宏文, 松井達也,、佐藤浩平, 小野篤史, 間瀬暢之, 川田善正, 杉田 篤史
  • Organizer: 第64回応用物理学会春季学術講演会
  • Place of Presentation: パシフィコ横浜 （神奈川県横浜市）
  • Year and Date: 2017-03-14
• [Presentation] 金ナノロッド/非線形光学ポリマー複合系の放射するSHG光の偏光特性 (2016)
  • Author(s): 松井達也、小野篤史、川田善正、杉田篤史
  • Organizer: 第77回応用物理学会秋季学術講演大会
  • Place of Presentation: 朱鷺メッセ （新潟県新潟市）
  • Year and Date: 2016-09-13
• [Presentation] 一次元・二次元金ナノロッド配列系の第二高調波発生 (2016)
  • Author(s): 二橋俊介、小野篤史、川田善正、杉田篤史
  • Organizer: 第77回応用物理学会秋季学術講演大会
  • Place of Presentation: 朱鷺メッセ 新潟県新潟市
  • Year and Date: 2016-09-13
• [Presentation] 局在表面プラズモン共鳴における金ナノ三角柱の偏光分解第二高調波分光 (2016)
  • Author(s): 余語宏文、二橋俊介、小野篤史、川田善正、杉田 篤史
  • Organizer: 第77回応用物理学会秋季学術講演大会
  • Place of Presentation: 朱鷺メッセ （新潟県新潟市）
  • Year and Date: 2016-09-13
• [Presentation] 一次元金ナノロッド配列系の表面プラズモン共鳴現象 (2016)
  • Author(s): 杉田篤史, 二橋俊介、小野篤史、川田善正
  • Organizer: 日本物理学会2016年秋季大会
  • Place of Presentation: 金沢大学 （石川県金沢市）
  • Year and Date: 2016-09-13
• [Presentation] Second Harmonic Generation From Au Nanoprisms at LSPR (2016)
  • Author(s): Hirofumi Yogo, Shunsuke Nihashi, Atsushi Ono, Yoshimasa Kawata, Atsushi Sugita
  • Organizer: NFO-14: The 14th International Conference of Near-Field Optics, Nanophotonics and Related Techniques
  • Place of Presentation: Act City （Hamamatsu, Japan）
  • Year and Date: 2016-09-04
  • Int'l Joint Research
• [Presentation] Second Order Nonlinear Optical Responses of Au Nanorods/NLO Polymer/Ag Films at LSP Resonances (2016)
  • Author(s): Daiki Ishii, Keiko Miyabayashi, Atsushi Ono, Yoshimasa Kawata, and Atsushi Sugita
  • Organizer: NFO-14: The 14th International Conference of Near-Field Optics, Nanophotonics and Related Techniques
  • Place of Presentation: Act City （Hamamatsu, Japan）
  • Year and Date: 2016-09-04
  • Int'l Joint Research
• [Presentation] Second-order Nonlinearities of 1D Arrays of Au Nanorods (2016)
  • Author(s): Shunsuke Nihashi, Atsusi Ono, Yoshimasa Kawata, Atsushi Sugita
  • Organizer: The 14th International Conference of Near-Field Optics, Nanophotonics and Related Techniques
  • Place of Presentation: Act City (Hamamatsu, Japan)
  • Year and Date: 2016-09-04
  • Int'l Joint Research
• [Presentation] Enhanced Second Order Nonlinearities of NLO Polymer-coated Au Nanorods at LSP Resonance (2016)
  • Author(s): Tatsuya Matsui, Atsushi Ono, Yoshimasa Kawata, Atsushi Sugita
  • Organizer: The 14th International Conference of Near-Field Optics, Nanophotonics and Related Techniques
  • Place of Presentation: Act City (Hamamatsu, Japan)
  • Year and Date: 2016-09-04
  • Int'l Joint Research
• [Presentation] Second-order nonlinearities of 2D periodic arrays of Au nanorods at surface plasmon resonances (2016)
  • Author(s): Atsushi Sugita, Shunsuke Nihashi, Atsushi Ono, and Yoshimasa Kawata
  • Organizer: SPIE.Optics+Photonics 2016 Plasmonics: Metallic Nanostructures and Their Optical Properties XIII, NanoScience + Engineering
  • Place of Presentation: San Diego Convention Center (San Diego, California U. S. A.)
  • Year and Date: 2016-08-28
  • Int'l Joint Research
• [Presentation] Ultrafast plasmonic dephasing dynamics studied by time-resolved spectroscopy based on SHG-FROG methods (2016)
  • Author(s): Atsushi Sugita, Sunsuke Nihashi, Atsushi Ono, Yoshimasa Kawata
  • Organizer: International Conference on Ultrafast Phenomena 2016
  • Place of Presentation: Santa Fe Community Center (Santa Fe, New Mexico, U.S.A.）
  • Year and Date: 2016-07-17
  • Int'l Joint Research
• [Presentation] Second harmonic generations in plasmonic 2D periodic arrays of Au nanorods (2016)
  • Author(s): Atsushi Sugita, Shunsuke Nihashi, Atsushi Ono, and Yoshimasa Kawata
  • Organizer: CLEO:2016
  • Place of Presentation: San Jose Convention Center （San Jose, CA. U.S.A.）
  • Year and Date: 2016-06-14
  • Int'l Joint Research
• [Presentation] 金ナノロッド/非線形光学ポリマー複合型微小非線形光学素子の励起光照射条件に対する熱耐性 (2016)
  • Author(s): 松井達也、小野篤史、川田善正、杉田篤史
  • Organizer: 第63回応用物理学会春季学術講演会
  • Place of Presentation: 東京工業大学(東京都目黒区)
  • Year and Date: 2016-03-22
• [Presentation] 一次元金ナノロッド配列系の散乱分光 (2016)
  • Author(s): 二橋俊介、小野篤史、川田善正、杉田篤史
  • Organizer: 第63回応用物理学会春季学術講演会
  • Place of Presentation: 東京工業大学(東京都目黒区)
  • Year and Date: 2016-03-19
• [Presentation] 金ナノ三角柱における局在表面プラズモン共鳴条件下での第二高調波発生現象 (2016)
  • Author(s): 余語宏文、二橋俊介、小野篤史、川田善正、杉田 篤史
  • Organizer: 第63回応用物理学会春季学術講演会
  • Place of Presentation: 東京工業大学(東京都目黒区)
  • Year and Date: 2016-03-19
• [Presentation] プッシュプル型NLO色素の無電界ポーリング現象における分子サイズ依存性 (2016)
  • Author(s): 北川顕磨、鳴海哲夫、間瀬暢之、川田善正、杉田 篤史
  • Organizer: 第63回応用物理学会春季学術講演会
  • Place of Presentation: 東京工業大学(東京都目黒区)
  • Year and Date: 2016-03-19
• [Presentation] 二次元金ナノロッド系における表面プラズモン共鳴条件での第二高調波発生現象 (2016)
  • Author(s): 杉田篤史、 二橋俊介、 小野篤史、 川田善正
  • Organizer: 第71回日本物理学会年次大会
  • Place of Presentation: 東北学院大学(宮城県仙台市)
  • Year and Date: 2016-03-19
• [Presentation] 二次元金属ナノ粒子配列系における第二高調波発生現象 (2015)
  • Author(s): 杉田篤史，二橋俊介，平林拓磨，小野篤史，川田善正
  • Organizer: 日本物理学会 2015年秋季大会
  • Place of Presentation: 関西大学(大阪府吹田市)
  • Year and Date: 2015-09-17
• [Presentation] ホストゲスト型非線形光学高分子におけるゲスト色素の界面分子配向動力学の研究 (2015)
  • Author(s): 鈴木 亮太、高須 亮佑、川田 善正、杉田 篤史
  • Organizer: 第9回分子科学討論会
  • Place of Presentation: 東京工業大学(東京都目黒区)
  • Year and Date: 2015-09-16
• [Presentation] 金属ナノ粒子表面の非線形性増大のための非線形光学ポリマーの開発 (2015)
  • Author(s): 北川 顕磨、小野 篤史、鳴海 哲夫、間瀬 暢之、川田 善正、杉田 篤史
  • Organizer: 76回応用物理学会秋季学術講演会
  • Place of Presentation: 名古屋国際会議場(愛知県名古屋市)
  • Year and Date: 2015-09-13
• [Presentation] 無電界ポーリングされたPMMA/DR1ホストゲスト型ポリマーにおけるゲスト色素の極性配向挙動に関する研究 (2015)
  • Author(s): 松井 達也、高須 亮佑、川田 善正、杉田 篤史
  • Organizer: 第76回応用物理学会秋季学術講演会
  • Place of Presentation: 名古屋国際会議場(愛知県名古屋市)
  • Year and Date: 2015-09-13
• [Presentation] 金ナノロッドの二次元周期配列系における第二高調波発生 (2015)
  • Author(s): 二橋 俊介、小野 篤史、川田 善正、杉田 篤史
  • Organizer: 第76回応用物理学会秋季学術講演会
  • Place of Presentation: 名古屋国際会議場(愛知県名古屋市)
  • Year and Date: 2015-09-13
• [Presentation] Enhancing second-order nonlinearity on Au-nanorods at localized surface plasmon resonance with nonlinear optical polymers (2015)
  • Author(s): Atsushi Sugita, Takuma Hirabayashi, Shunsuke Nihashi, Atsushi Ono, and Yoshimasa Kawata
  • Organizer: SPIE.Optics+Photonics 2015 Plasmonics: Metallic Nanostructures and Their Optical Properties XIII, NanoScience + Engineering
  • Place of Presentation: San Diego, California U. S. A.
  • Year and Date: 2015-08-09
  • Int'l Joint Research
• [Presentation] Molecular orientations of nonelectrically poled guest-host NLO polymers (2015)
  • Author(s): Atsushi Sugita, Yasuaki Sato, Tatsuya Matsui, Yoshimasa Kawata
  • Organizer: CLEO/Europe-EQEC 2015,
  • Place of Presentation: Munich, Germany
  • Year and Date: 2015-05-21
  • Int'l Joint Research
• [Presentation] Enhancing LSP-mediated SHG conversion efficiency with NLO polymer (2015)
  • Author(s): Atsushi Sugita, Takuma Hirabayashi, Shunsuke Nihashi, Atsushi Ono, and Yoshimasa Kawata
  • Organizer: CLEO/Europe-EQEC 2015
  • Place of Presentation: Munich, Germany
  • Year and Date: 2015-05-21
  • Int'l Joint Research
• [Presentation] Highly efficient SHG in NLO polymer-coated Au nanoparticles by doubly resonant excitations (2015)
  • Author(s): Atsushi Sugita, Takuma Hirabayashi, Shunsuke Nihashi, Atsushi Ono, and Yoshimasa Kawata
  • Organizer: CLEO 2015
  • Place of Presentation: San Jose Convention Center, CA. U.S.A.
  • Year and Date: 2015-05-11
  • Int'l Joint Research
• [Presentation] 二次元配列した金ナノロッドの線形光学応答 (2015)
  • Author(s): 杉田篤史，平林拓磨，棚倉悠史，二橋俊介，小野篤史，川田善正
  • Organizer: 日本物理学会第70回年次大会
  • Place of Presentation: 早稲田大学、東京都新宿区
  • Year and Date: 2015-03-21 – 2015-03-24
• [Presentation] 金ナノロッド/非線形光学ポリマー複合型非線形光学素子のポリマー積層条件による最適化 (2015)
  • Author(s): 棚倉悠史、平林拓磨、二橋俊介、小野篤史、川田善正、杉田篤史
  • Organizer: 第62回応用物理学会春季学術講演会
  • Place of Presentation: 東海大学、神奈川県平塚市
  • Year and Date: 2015-03-11 – 2015-03-14
• [Presentation] TCF-CF3アクセプターを含むNLO色素の合成 (2015)
  • Author(s): 鈴木亮太、北川顕磨、間瀬暢之、鳴海哲夫、杉田篤史
  • Organizer: 第62回応用物理学会春季学術講演会
  • Place of Presentation: 東海大学、神奈川県平塚市
  • Year and Date: 2015-03-11 – 2015-03-14
• [Presentation] DR1/PMMAホストゲストポリマーの無電界でのポーリング現象における分子配向性の調査 (2014)
  • Author(s): 杉田 篤史,佐藤 保彰,伊藤 一磨,間瀬 暢之,川田 善正
  • Organizer: 第8回分子科学討論会
  • Place of Presentation: 広島大学、広島県東広島市
  • Year and Date: 2014-09-21 – 2014-09-24
• [Presentation] 金ナノロッド/非線形光学ポリマー複合系からの局在型表面プラズモンにおける第二高調波発生 (2014)
  • Author(s): 平林拓磨，小野篤史，川田善正，杉田篤史、
  • Organizer: 第75回応用物理学会秋季学術講演会
  • Place of Presentation: 北海道大学、北海道札幌市
  • Year and Date: 2014-09-16 – 2014-09-19
• [Presentation] トリシアノフラン系色素を含むホスト/ゲストポリマーにおける二次非線形光学効果の界面吸着挙動に対する依存性 (2014)
  • Author(s): 高須亮佑，川田善正，間瀬暢之，杉田篤史
  • Organizer: 第75回応用物理学会秋季学術講演会
  • Place of Presentation: 北海道大学、北海道札幌市
  • Year and Date: 2014-09-16 – 2014-09-19
• [Presentation] 金ナノロッド/非線形光学ポリマー複合系からの第二高調波発生の励起条件に対する依存性 (2014)
  • Author(s): 棚倉悠史，平林拓磨，小野篤史，川田善正，杉田篤史
  • Organizer: 第75回応用物理学会秋季学術講演会
  • Place of Presentation: 北海道大学、北海道札幌市
  • Year and Date: 2014-09-16 – 2014-09-19
• [Presentation] TCF-CF3アクセプターを含むNLO色素の無電界ポーリング法 (2014)
  • Author(s): 鈴木亮太，伊藤一磨，間瀬暢之，鳴海哲夫，川田善正，杉田篤史
  • Organizer: 第75回応用物理学会秋季学術講演会
  • Place of Presentation: 北海道大学、北海道札幌市
  • Year and Date: 2014-09-16 – 2014-09-19
• [Presentation] PLD法で作製したY2O3:Eu3+蛍光体薄膜のカソードルミネッセンス特性 (2014)
  • Author(s): 守田智勇，豊嶋祐樹，福田真大，名和靖矩，居波渉，小南裕子，川田善正，中西洋一郎，堀田育志，杉田篤史
  • Organizer: 第75回応用物理学会秋季学術講演会
  • Place of Presentation: 北海道大学、北海道札幌市
  • Year and Date: 2014-09-16 – 2014-09-19
• [Presentation] NLOポリマー中での表面プラズモン増強光電場の第二高調波発生II (2014)
  • Author(s): 杉田篤史，平林拓磨，小野篤史，川田善正
  • Organizer: 日本物理学会 2014年秋季大会
  • Place of Presentation: 中部大学、愛知県春日井市
  • Year and Date: 2014-09-07 – 2014-09-10
• [Presentation] SP-enhanced SHG from NLO Polymer-coated Au nanorods (2014)
  • Author(s): Takuma Hirabayashi, Atsushi Ono, Yoshimasa Kawata, Atsushi Sugita
  • Organizer: Thirteenth International conference on near-field optics, nanophotonics and related technologies
  • Place of Presentation: Snowbird, Utah, U.S.A.
  • Year and Date: 2014-08-31 – 2014-09-04
• [Presentation] Enhancements of SP-mediated Nonlinearity with NLO Polymer (2014)
  • Author(s): Atsushi Sugita, Tomoyuki Sato, Kaname Suto, Atsushi Ono, and Yoshimasa Kawata
  • Organizer: Thirteenth International conference on near-field optics, nanophotonics and related technologies
  • Place of Presentation: Snowbird, Utah, U.S.A.
  • Year and Date: 2014-08-31 – 2014-09-04
• [Presentation] Second Harmonic Generations from Au Nanorods Coated with Nonelectrically Poled NLO polymer (2014)
  • Author(s): Atsushi Sugita, Takuma Hirabayashi, Atsushi Ono and Yoshimasa Kawata
  • Organizer: CLEO2014
  • Place of Presentation: San Jose Convention Center, San Jose, U. S. A.
  • Year and Date: 2014-06-09 – 2014-06-13