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Application of hydrogen absorption/release characteristics of sulfur-poisoning nanoparticles to cancer detection

Research Project

Project/Area Number 26289255
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Structural/Functional materials
Research InstitutionNagoya University

Principal Investigator

Yagi Shinya  名古屋大学, 未来材料・システム研究所, 教授 (20284226)

Co-Investigator(Kenkyū-buntansha) 吉田 朋子  名古屋大学, エコトピア科学研究所, 准教授 (90283415)
Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥16,120,000 (Direct Cost: ¥12,400,000、Indirect Cost: ¥3,720,000)
Fiscal Year 2016: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2015: ¥5,980,000 (Direct Cost: ¥4,600,000、Indirect Cost: ¥1,380,000)
Fiscal Year 2014: ¥8,060,000 (Direct Cost: ¥6,200,000、Indirect Cost: ¥1,860,000)
Keywordsナノ粒子 / 水素吸放出 / ガン検知 / 硫黄被毒 / Rhナノ粒子 / 酸素被毒 / Pdナノ粒子 / XPS測定 / ガス中蒸発法 / 生体・医療・福祉材料 / がんスクリーニング / XAFS分析 / 金ナノ粒子 / 硫黄分子吸着 / XAFS測定
Outline of Final Research Achievements

We have fabricated the nanoparticles of Rh and Pd by gas evaporation method. The particle sizes of both Rh and Pd are estimated to be approximately 1-4 nm. Although a sulfur-containing molecules (mainly thiol-based molecules) adsorbed on the Rh nanoparticle surface chemically adsorbs but the adsorbed molecules does not show a dissociation reaction. Moreover the Rh nanoparticles does not show the hydrogen absorbing/releasing reaction. On the other hand, for the Pd nanoparticles, it is found that the hydrogen absorbing/releasing reaction rate is remarkably slow in comparison with the rate for without sulfur poisoning. Based on this result, we are planning to continue applying to cancer screening in the future.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Annual Research Report
  • 2014 Annual Research Report

Research Products

(21 results)

All 2017 2016 2015 2014 Other

All Int'l Joint Research (1 results) Journal Article (9 results) (of which Peer Reviewed: 9 results,  Open Access: 4 results,  Acknowledgement Compliant: 8 results) Presentation (11 results) (of which Int'l Joint Research: 5 results)

  • [Int'l Joint Research] Diamond Light Source(英国)

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Hydrogen Storage of Pd/Mg composite Nanoparticles Fabricated by Gas Evaporation Method2016

    • Author(s)
      Satoshi Ogawa, Hiroyuki Suzuki, Chie Tsukada, Tomoko Yoshida, Shinya Yagi
    • Journal Title

      e-J. Surf. Sci. Nanotech

      Volume: 14 Issue: 0 Pages: 150-153

    • DOI

      10.1380/ejssnt.2016.150

    • NAID

      130005151355

    • ISSN
      1348-0391
    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] 金属ナノ粒子を用いた水素吸蔵材料の分光学的手法による化学状態分析2015

    • Author(s)
      小川智史,内山直樹,藤本大志,金井友美,八木伸也
    • Journal Title

      日本金属学会誌

      Volume: 79 Pages: 118-123

    • NAID

      130004786489

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Hydrogen Storage Property of the Pd Nanoparticle with Clean Surfaces Studied by QCM2015

    • Author(s)
      Satoshi Ogawa, Taishi Fujimoto, Tomomi Kanai, Naoki Uchiyama, Chie Tsukada, Tomoko Yoshida, Shinya Yagi
    • Journal Title

      e-Journal of Surface Science and Nanotechnology

      Volume: 13 Pages: 343-346

    • NAID

      130005083978

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Hydrogen storage property of materials composed of Mg nanoparticles and Ni nanoparticles fabricated by gas evaporation method2015

    • Author(s)
      Taishi Fujimoto, Satoshi Ogawa, Tomomi Kanai, Naoki Uchiyama, Tomoko Yoshida, Shinya Yagi
    • Journal Title

      International Journal of Hydrogen Energy

      Volume: 40 Pages: 11890-11894

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Hydrogen storage of binary nanoparticles composed of Mg and Pd2015

    • Author(s)
      Satoshi Ogawa, Taishi Fujimoto, Tsuyoshi Mizutani, Masahiro Ogawa, Naoki Uchiyama, Kazuo Kato, Toshiaki Ohta, Tomoko Yoshida, Shinya Yagi
    • Journal Title

      International Journal of Hydrogen Energy

      Volume: 40 Pages: 11895-11901

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Spectroscopic and morphological studies on interaction between gold nanoparticle and liposome constructed with phosphatidylcholine2015

    • Author(s)
      C. Tsukada, T. Tsuji, K. Matsuo, T. Nomoto, G. Kutluk, M. Sawada, S. Ogawa, T. Yoshida, S. Yagi
    • Journal Title

      IOP Conference Series: Materials Science and Engineering

      Volume: 76 Pages: 012001-3

    • DOI

      10.1088/1757-899x/76/1/012001

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Vulcanization reaction of squalene and S8 powder studied by Sulfur K-edge NEXFAS under liquid phase2015

    • Author(s)
      S. Yagi, Y. Menjo, C. Tsukada, S. Ogawa, G. Kutluk, H. Namatame and M. Taniguchi
    • Journal Title

      IOP Conference Series: Materials Science and Engineering

      Volume: 76 Pages: 012004-6

    • DOI

      10.1088/1757-899x/76/1/012004

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] In situ ultraviolet-visible absorbance measurement during and after solution plasma sputtering for preparation of colloidal gold nanoparticles2014

    • Author(s)
      T. Mizutani, T. Murai, H. Nameki, T. Yoshida, S. Yagi
    • Journal Title

      Jpn. J. Appl. Phys.

      Volume: 53

    • NAID

      210000144617

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Preparation of gold nanoparticles included in anatase-phase titania by solution plasma method2014

    • Author(s)
      T. Mizutani, T. Murai, T. Nomoto, H. Nameki, T. Yoshida, S. Yagi
    • Journal Title

      Surf. Interface Anal.

      Volume: 46 Pages: 1125-1128

    • Related Report
      2014 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] 液中プラズマ法で作製したAuナノ粒子のCs吸着剤への応用検討2017

    • Author(s)
      塚田千恵、吉田光、小川智史、吉越章隆、八木伸也、矢板毅
    • Organizer
      第30回日本放射光学会
    • Place of Presentation
      神戸芸術センター(兵庫県神戸市)
    • Year and Date
      2017-01-07
    • Related Report
      2016 Annual Research Report
  • [Presentation] In-situ XAFSによるMg-Pdナノ粒子の水素吸放出時における局所状態変化分析2016

    • Author(s)
      小川智史、藤本大志、水谷剛士、小川雅裕、与儀千尋、加藤和男、太田俊明、吉田朋子、八木伸也
    • Organizer
      XAFS討論会
    • Place of Presentation
      名古屋大学
    • Year and Date
      2016-09-06
    • Related Report
      2016 Annual Research Report
  • [Presentation] Nanoparticles for Hydrogen Storage Application : Pd, Ni and Mg Nanoparticles2015

    • Author(s)
      Satoshi Ogawa, Hiroyuki Suzuki, Chie Tsukada, Tomoko Yoshida and Shinya Yagi
    • Organizer
      International Symposium on EcoTopia Science ’15
    • Place of Presentation
      Nagoya University, Nagoya, Aichi, Japan
    • Year and Date
      2015-11-27
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Preparation and photocatalytic activity of cholorine-free gold nanoparticles on titanium oxide by solution plasma method2015

    • Author(s)
      Tsuyoshi Mizutani, Satoshi Ogawa, Muneaki Yamamoto, Hirofumi Nameki, Tomoko Yoshida, and Shinya Yagi
    • Organizer
      International Symposium on EcoTopia Science ’15
    • Place of Presentation
      Nagoya University, Nagoya, Aichi, Japan
    • Year and Date
      2015-11-27
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 放射光XAFSによる水素吸蔵ナノ粒子の分析2015

    • Author(s)
      小川智史
    • Organizer
      第 7 回 SPring-8 萌芽的研究支援ワークショップ
    • Place of Presentation
      キャンパス・イノベーションセンター東京
    • Year and Date
      2015-10-28
    • Related Report
      2015 Annual Research Report
  • [Presentation] Spectroscopic characterization of Pd/Mg nanoparticles during hydrogen absorption2015

    • Author(s)
      Satoshi Ogawa, Chie Tsukada, Masahiro Ogawa, Toshiaki Ohta, Tomoko Yoshida, Shinya Yagi
    • Organizer
      10th International Symposium on Atomic Level Characterizations for New Materials and Devices ’15
    • Place of Presentation
      Kunibiki Messe, Matsue, Shimane, Japan
    • Year and Date
      2015-10-25
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Fabrication of Au nanorods by solution plasma method2015

    • Author(s)
      Chie Tsukada, Tsuyoshi Mizutani, Satoshi Ogawa, Hirofumi Nameki, Shinya Yagi
    • Organizer
      10th International Symposium on Atomic Level Characterizations for New Materials and Devices ’15
    • Place of Presentation
      Nagoya University, Nagoya, Aichi, Japan
    • Year and Date
      2015-10-25
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photocatalytic activity of gold nanoparticles on titanium oxide prepared by solution plasma method2015

    • Author(s)
      Tsuyoshi Mizutani, Satoshi Ogawa, Muneaki Yamamoto, Hirofumi Nameki, Tomoko Yoshida, and Shinya Yagi
    • Organizer
      European Conference on Surface Science (ECOSS 31)
    • Place of Presentation
      Barcelona, Spain
    • Year and Date
      2015-08-31
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Formation mechanism of nanoparticles prepared by electrode during solution plasma using pulsed high voltage2015

    • Author(s)
      T. Mizutani, T. Murai, T. Nomoto, H. Nameki, T. Yoshida, S. Yagi
    • Organizer
      7th International Symposium on Advanced Plasma Science and its Applications for Nitrides and Nanomaterials (ISPlasma 2015)
    • Place of Presentation
      日本(名古屋市)
    • Year and Date
      2015-03-02 – 2015-03-06
    • Related Report
      2014 Annual Research Report
  • [Presentation] Adsorption behavior between phosphatidylcholine(PC) and gold nanoparticle studied by XAFS and TEM2014

    • Author(s)
      C. Tsukada, T. Tsuji, K. Matsuo, T. Nomoto, G. Kutluk, M. Sawada, S. Ogawa, T. Yoshida, S. Yagi
    • Organizer
      International Conference on Solid Films and Surfaces (ICSFS17)
    • Place of Presentation
      ブラジル(リオデジャネイロ)
    • Year and Date
      2014-09-08 – 2014-09-11
    • Related Report
      2014 Annual Research Report
  • [Presentation] In-situ UV-Vis investigation of the formation of gold nanoparticles by the solution plasma spattering2014

    • Author(s)
      T. Mizutani, T. Murai, H. Nameki, T. Yoshida, S. Yagi
    • Organizer
      European Conference on Surface Science (ECOSS 30)
    • Place of Presentation
      トルコ(アンタルヤ)
    • Year and Date
      2014-08-31 – 2014-09-05
    • Related Report
      2014 Annual Research Report

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Published: 2014-04-04   Modified: 2022-01-31  

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