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Study of high-performance porous carbon synthesis and application for energy storage

Research Project

Project/Area Number 26289379
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypePartial Multi-year Fund
Section一般
Research Field Energy engineering
Research InstitutionNational Institute of Advanced Industrial Science and Technology

Principal Investigator

Xu Qiang  国立研究開発法人産業技術総合研究所, 電池技術研究部門, 上級主任研究員 (50357232)

Project Period (FY) 2014-04-01 – 2017-03-31
Project Status Completed (Fiscal Year 2016)
Budget Amount *help
¥16,120,000 (Direct Cost: ¥12,400,000、Indirect Cost: ¥3,720,000)
Fiscal Year 2016: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2015: ¥6,760,000 (Direct Cost: ¥5,200,000、Indirect Cost: ¥1,560,000)
Fiscal Year 2014: ¥5,330,000 (Direct Cost: ¥4,100,000、Indirect Cost: ¥1,230,000)
Keywords炭素 / エネルギー / エネルギー貯蔵 / エネルギー変換 / 多孔質材料 / キャパシター / 電池 / 配位高分子
Outline of Final Research Achievements

In this study, we used MOFs as templates/precursors to prepare hierarchically porous carbon materials for energy storage and conversion. Hierarchically porous carbons with both micro- and mesopores synthesized by direct carbonization of assembled nanoparticles of ZIF-8 have been used as supports for highly active Pd electrocatalysts for methanol electrooxidation. Hierarchical graphitic porous carbon architectures with atomically dispersed Fe and N doping have been fabricated from a MOF composite by using a facile strategy, which show high specific surface areas, hierarchical pore structures with macro/meso/micro multimodal pore size distributions, abundant surface functionality with single-atom dispersed N and Fe doping, and improved hydrophilicity. Detailed analyses unambiguously disclosed the main active sites of doped N atoms and FeNx species in the catalyst. The resultant catalyst affords high catalytic performance for oxygen reduction reaction.

Report

(4 results)
  • 2016 Annual Research Report   Final Research Report ( PDF )
  • 2015 Annual Research Report
  • 2014 Annual Research Report

Research Products

(16 results)

All 2017 2016 2015 2014 Other

All Int'l Joint Research (2 results) Journal Article (4 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 4 results,  Acknowledgement Compliant: 4 results) Presentation (10 results) (of which Int'l Joint Research: 9 results,  Invited: 10 results)

  • [Int'l Joint Research] Peking University/Chinese Academy of Sciences (CAS)(China)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] Monash University(Australia)

    • Related Report
      2015 Annual Research Report
  • [Journal Article] Atomically Dispersed Fe/N-Doped Hierarchical Carbon Architectures Derived from a Metal-Organic Framework Composite for Extremely Efficient Electrocatalysis2017

    • Author(s)
      Qi-Long Zhu, Wei Xia, Li-Rong Zheng, Ruqiang Zou, Zheng Liu, Qiang Xu
    • Journal Title

      ACS Energy Lett.

      Volume: 2 Pages: 504-511

    • DOI

      10.1021/acsenergylett.6b00686

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Metal-Organic Frameworks for Energy Applications2017

    • Author(s)
      Hailong Wang, Qi-Long Zhu, Ruqiang Zou, Qiang Xu
    • Journal Title

      Chem

      Volume: 2 Pages: 52-80

    • DOI

      10.1016/j.chempr.2016.12.002

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Fabrication of carbon nanorods and graphene nanoribbons from a metal-organic framework2016

    • Author(s)
      Pradip Pachfule, Dhanraj Shinde, Mainak Majumder, Qiang Xu
    • Journal Title

      NATURE CHEMISTRY

      Volume: -

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Pd nanoparticles supported on hierarchically porous carbons derived from assembled nanoparticles of a zeolitic imidazolate framework (ZIF-8) for methanol electrooxidation2015

    • Author(s)
      Jun Li, Qi-Long Zhu, Qiang Xu
    • Journal Title

      Chem. Commun.

      Volume: 51 Pages: 10827-10830

    • DOI

      10.1039/c5cc03008k

    • Related Report
      2015 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] Metal-Organic Frameworks as a Platform for Energy Conversion and Storage2016

    • Author(s)
      Qiang Xu
    • Organizer
      The 2nd International Symposium on Renewable Energy Technologies
    • Place of Presentation
      University of Technology Sydney, Sydney, Australia
    • Year and Date
      2016-12-02
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Nanostructured Materials for Energy Storage and Conversion2016

    • Author(s)
      Qiang Xu
    • Organizer
      8th Asian Conference on Nanoscience and Nanotechnology (AsiaNANO 2016)
    • Place of Presentation
      Sapporo Convention Center, Sapporo, Japan
    • Year and Date
      2016-10-11
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Metal Nanoparticle@Metal-Organic Framework Composites for Catalysis2016

    • Author(s)
      Qiang Xu
    • Organizer
      The 5th International Conference on Metal-Organic Frameworks & Open Framework Compounds (MOF2016)
    • Place of Presentation
      Hilton Hotel, Long Beach, California, USA
    • Year and Date
      2016-09-13
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Metal-Organic Frameworks as a Platform for Energy Conversion and Storage2016

    • Author(s)
      Qiang Xu
    • Organizer
      1st Japan-Australia Joint Symposium on Coordination Chemistry
    • Place of Presentation
      Fukuoka University, Fukuoka, Japan
    • Year and Date
      2016-09-09
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Metal-Organic Frameworks as a Platform for Energy Conversion and Storage2016

    • Author(s)
      Qiang Xu
    • Organizer
      Energy Conversion and Storage Forum 2016
    • Place of Presentation
      Institute of Process Engineering, Beijing, China
    • Year and Date
      2016-06-29
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Metal nanoparticle@metal-organic framework composites as high-performance catalysts2015

    • Author(s)
      Qiang Xu
    • Organizer
      250th ACS National Meeting & Exposition
    • Place of Presentation
      Boston, MA, USA
    • Year and Date
      2015-08-16
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Metal-Organic Frameworks as Platforms for Energy Applications2015

    • Author(s)
      Qiang Xu
    • Organizer
      2015 International Conference on Nanospace Materials
    • Place of Presentation
      Taipei, Taiwan
    • Year and Date
      2015-06-24
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Applications of functional metal-organic frameworks2015

    • Author(s)
      Qiang Xu
    • Organizer
      The 1st International Conference on Microstructure and Property of Materials
    • Place of Presentation
      Hangzhou, China
    • Year and Date
      2015-05-28
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Metal-Organic Frameworks as Platforms for Energy Applications2015

    • Author(s)
      Qiang Xu
    • Organizer
      The 2nd SYSU International Symposium on MOF and Related Open Framework Materials
    • Place of Presentation
      Guangzhou, China
    • Year and Date
      2015-05-25
    • Related Report
      2015 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Towards the application of metal-organic frameworks2014

    • Author(s)
      Qiang Xu
    • Organizer
      4th International Conference on Metal-Organic Frameworks and Open Framework Compounds (MOF2014)
    • Place of Presentation
      Kobe, Japan
    • Year and Date
      2014-10-01
    • Related Report
      2014 Annual Research Report
    • Invited

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Published: 2014-04-04   Modified: 2018-03-22  

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