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Study of Long-range Trans-boundary Air Pollution of PM2.5 by Soft rime ice collected in Shikoku Island, Japan

Research Project

Project/Area Number 26340084
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Environmental risk control and evaluation
Research InstitutionThe University of Tokushima

Principal Investigator

IMAI Shoji  徳島大学, 大学院社会産業理工学研究部(理工学域), 教授 (50232591)

Project Period (FY) 2014-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2016: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2015: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2014: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Keywords越境汚染 / 石炭燃焼排出物 / 有機イオウ化合物 / 樹氷 / 重金属 / 石炭飛灰 / 環境分析 / 雪 / PM2.5 / 降水 / 起源解析 / 硫黄 / 大気エアロゾル / 環境化学 / 山岳研究 / 長距離輸送機構 / 越境大気汚染物質 / 長距離輸送物質 / 環境PM2.5粒子組成 / SEM-EDX
Outline of Final Research Achievements

Coal combustion exhausts transported from northeast Asia region were found in rime ice and snow collected on the summit of mountain (1400 m alt.) in Shikoku Island. The coal combustion with no exhaust purification specifically emits 1) aerosol particulates including cadmium and lead, 2) gaseous pollutants such as SO2 converting to sulfate, 3) products of incomplete combustion, and 4) inorganic small spherical particles (ISPs) from power plants. It was found in the rime and snow that organic sulfur species indicates to
a proof of the coal exhaust. A methodology for determination of generating area in northeast Asia was proposed by the chemical composition of the ISPs, heavy metals and sulfate ion concentration based on meteorological information. It can be concluded that the generating areas of air pollution were the region of Huabei of China and the south area of northeast China.

Report

(5 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • 2014 Research-status Report
  • Research Products

    (19 results)

All 2018 2017 2016 2015 2014 Other

All Journal Article (10 results) (of which Peer Reviewed: 10 results,  Open Access: 10 results,  Acknowledgement Compliant: 3 results) Presentation (8 results) (of which Invited: 3 results) Remarks (1 results)

  • [Journal Article] Sulfur Chemical State and Chemical Composition of Insoluble Substance in Soft Rime, Hard Rime, and Snow Collected in Remote and Rural Areas in Japan Using Wavelength-dispersive X-ray Fluorescence2018

    • Author(s)
      Shoji Imai, Yuhei Yamamoto, Takashi Yamamoto, Kenji KODAMA, NISHIMOTO Jun and KIKUCHI Yoichi
    • Journal Title

      Analytical Sciences

      Volume: 34 Issue: 5 Pages: 589-598

    • DOI

      10.2116/analsci.17P277

    • NAID

      130006733505

    • ISSN
      0910-6340, 1348-2246
    • Year and Date
      2018-05-10
    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Pb/Cd Ratios in Fresh Snow Derived from Cold Air Mass from Northern North Eastern China and Russian Maritime Province along the Coast of the Japan Sea in Honshu Island and a Long-range Transport Mechanism during Winter2018

    • Author(s)
      今井 昭二, 山本 祐平, 清水 魁人, 兼清 恵理, 西本 潤, 菊地 洋一
    • Journal Title

      BUNSEKI KAGAKU

      Volume: 67 Issue: 2 Pages: 95-101

    • DOI

      10.2116/bunsekikagaku.67.95

    • NAID

      130006417671

    • ISSN
      0525-1931
    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] WDXRFによる樹氷と雪の中の非水溶性イオウ化合物の化学形態別分析と東アジアの石炭燃焼排出物の冬期モンスーン下での長距離輸送機構2018

    • Author(s)
      今井昭二, 上村 健, 児玉憲治, 山本祐平
    • Journal Title

      X線分析の進歩

      Volume: 49 Pages: 125-142

    • NAID

      120006453346

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Long-range Transport Mechanism of Cadmium, Lead and Nonseasalt-sulfate Ion in Fresh Rime and Fresh Snow Collected on the Summit of Mt. Kajigamori, Kochi Prefecture, Japan during the 2008–2014 Winter Season2017

    • Author(s)
      今井 昭二, 山本 祐平, 佐名川 洋右, 耒見 祐哉, 黒谷 功, 西本 潤, 菊地 洋一
    • Journal Title

      BUNSEKI KAGAKU

      Volume: 66 Issue: 2 Pages: 95-113

    • DOI

      10.2116/bunsekikagaku.66.95

    • NAID

      130005465008

    • ISSN
      0525-1931
    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] 2008年から2014年における高知県梶ヶ森山頂の樹氷と降雪中のカドミウム、鉛、非海塩性硫酸イオンの長距離輸送機構2017

    • Author(s)
      今井 昭二, 山本 祐平, 佐名川 洋右, 耒見 祐哉, 黒谷 功, 西本 潤, 菊地 洋一
    • Journal Title

      分析化学

      Volume: 66 Pages: 95-113

    • NAID

      130005465008

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] 本州日本海沿いの遠隔地における降雪中の無機小球体粒子の組成と長距離輸送2016

    • Author(s)
      今井 昭二, 山本 祐平, 上村 健
    • Journal Title

      分析化学

      Volume: 65 Pages: 211-219

    • NAID

      130005150732

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Classification and Long-range Transport of Inorganic Small Spherical Particles in Snow Collected at Remote Area along Japan Sea in Honshu Island, Japan2016

    • Author(s)
      今井昭二、山本祐平、上村健
    • Journal Title

      BUNSEKI KAGAKU

      Volume: 65 Issue: 4 Pages: 211-219

    • DOI

      10.2116/bunsekikagaku.65.211

    • NAID

      130005150732

    • ISSN
      0525-1931
    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Classification of Inorganic Small Spherical Particles in Rime and Snow at the Summit of Mt. Kajigamori, Shikoku Island, Japan2014

    • Author(s)
      耒見 祐哉, 佐名川 洋右, 山本 祐平, 上村 健, 今井 昭二
    • Journal Title

      BUNSEKI KAGAKU

      Volume: 63 Issue: 10 Pages: 837-845

    • DOI

      10.2116/bunsekikagaku.63.837

    • NAID

      130004704066

    • ISSN
      0525-1931
    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Concentrations of Chemical Constituents in Glaze at the Summit of Mt. Kajigamori in Kochi Prefecture, Shikoku Region, Japan2014

    • Author(s)
      佐名川 洋右, 耒見 祐哉, 山本 祐平, 上村 健, 今井 昭二
    • Journal Title

      BUNSEKI KAGAKU

      Volume: 63 Issue: 4 Pages: 351-356

    • DOI

      10.2116/bunsekikagaku.63.351

    • NAID

      130004732527

    • ISSN
      0525-1931
    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] 四国の梶が森山頂における樹氷、降雪、冬期降雨中の粒子状物質と黒色浮遊性物質2014

    • Author(s)
      佐名川 洋右, 耒見 祐哉, 山本 祐平, 今井 昭二
    • Journal Title

      自然科学研究

      Volume: 28 Pages: 7-14

    • Related Report
      2014 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] 冬期の樹氷と雪の中の非水溶性成分と水溶性成分による東アジアの大気汚染物質の長距離輸送機構2017

    • Author(s)
      今井 昭二, 上村 健, 児玉憲治, 山本 祐平
    • Organizer
      日本分析化学会X線分析研究会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] 光X線分析法を用いた四国の樹氷と日本海沿いの遠隔地における降雪中の不溶性イオウのスペシエーション2017

    • Author(s)
      今井 昭二, 山本 祐平, 山本 孝, 児玉 憲治, 西本 潤, 菊地 洋一
    • Organizer
      日本分析化学会第66年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 本州の日本海沿いの山岳における降雪中のPb/Cd濃度比と石炭起源の影響2017

    • Author(s)
      今井 昭二, 清水 魁人, 兼清 恵理, 山本 祐平, 西本 潤, 菊地 洋一
    • Organizer
      日本分析化学会第66年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 日本海沿岸および四国の遠隔地における降雪中のPb/Cd比を用いた長距離輸送機構解明のためのバックグラウンド2016

    • Author(s)
      今井 昭二, 山本 祐平, 耒見 祐哉, 佐名川 洋右, 齋藤 あゆみ
    • Organizer
      日本分析化学会第65年会
    • Place of Presentation
      (北海道大学・北海道札幌市)
    • Year and Date
      2016-09-14
    • Related Report
      2016 Research-status Report
  • [Presentation] PM2.5粒子の東アジアからの冬季長距離輸送器項と起源評価2016

    • Author(s)
      今井昭二
    • Organizer
      山口機器分析研究会第85回学術講演会
    • Place of Presentation
      (山口大学・山口県山口市)
    • Related Report
      2016 Research-status Report
    • Invited
  • [Presentation] 自由大気層に位置する四国の冬期山岳を利用した越境汚染物質の評価2015

    • Author(s)
      今井昭二,山本祐平,耒見祐哉,斉藤あゆみ
    • Organizer
      日本分析化学会 第64年会
    • Place of Presentation
      九州大学・伊都キャンパス(福岡市西区)
    • Year and Date
      2015-09-09
    • Related Report
      2015 Research-status Report
    • Invited
  • [Presentation] 標高1400m四国の梶ヶ森山頂における冬期越境汚染物質2015

    • Author(s)
      耒見 祐哉 ・ 山本 祐平・ 児玉 憲治 ・ 上村 健 ・今井 昭二
    • Organizer
      第75回分析化学討論会
    • Place of Presentation
      山梨大学・甲府キャンパス(山梨県甲府市)
    • Year and Date
      2015-05-23
    • Related Report
      2015 Research-status Report
  • [Presentation] 本州と四国山岳での2013年度冬季降雪中のPM2.5相当の一次生成粒子の越境移流経路2014

    • Author(s)
      今井昭二、耒見祐哉、佐名川洋右、山本祐平、上村 健
    • Organizer
      日本分析化学会第63年会
    • Place of Presentation
      広島大学(広島県東広島市)
    • Year and Date
      2014-09-17 – 2014-09-19
    • Related Report
      2014 Research-status Report
  • [Remarks] 徳島大学機関リポジトリー

    • URL

      http://repo.lib.tokushima-u.ac.jp/ja/

    • Related Report
      2017 Annual Research Report

URL: 

Published: 2014-04-04   Modified: 2019-03-29  

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