光合成アンテナをモデルとした超分子ナノデバイスの創製

• 研究課題/領域番号: 15350107
• 研究種目: 基盤研究(B)
• 配分区分: 補助金
• 応募区分: 一般
• 研究分野: 生体関連化学
• 研究機関: 立命館大学
• 研究代表者: 民秋 均 立命館大学, 理工学部, 教授 (00192641)
• 研究期間 (年度): 2003 – 2006
• 研究課題ステータス: 完了 (2006年度)
• 配分額: 11,900千円 (直接経費: 11,900千円); 2006年度: 3,100千円 (直接経費: 3,100千円); 2005年度: 2,800千円 (直接経費: 2,800千円); 2004年度: 2,800千円 (直接経費: 2,800千円); 2003年度: 3,200千円 (直接経費: 3,200千円)
• キーワード: 合成化学 / 自己組織化 / 超分子化学 / ナノ材料 / 表面・界面物性 / 超分化学 / 光合成 / 光収穫アンテナ / クロロフィル / 超分子 / 自己集積

研究概要

緑色光合成細菌の主たる光収穫アンテナ部であるクロロゾームにおける天然クロロフィルを模して、立体的に込み合っていない水酸基と水素結合能のあるカルボニル基を有する環状テトラピロール類の配位性金属(Mg・Zn・Cd)錯体を、天然産のクロロフィルや合成ポルフイリンを有機合成化学的手法で改変したり・生化学的に修飾したりして調製し、その自己会合体の構造と機能を解析した。天然型クロロゾームクロロフィル分子と同様に、今回合成した様々な置換基を有するモデル色素分子も自己会合性を有し、自己集積性クロロフィル化合物の多様性が広がった。またこのような化合物による自己会合体では、周辺置換基ばかりでなくπ電子系の飽和度を変化させることで、光収穫とエネルギー伝達能を幅広く調整することが可能であるという利点が見られた。
このようなクロロフィル分子の自己会合体の超分子構造を詳細に解明するために、従来の可視・円二色性吸収分光法ばかりでなく、^<18>Oで同位体標識を利用した振動分光法や^<13>Cで同位体標識を利用した核磁気共鳴法も使用し、「中心金属に配位結合した3^1位の水酸基が、13位のカルボニル基に水素結合しつつ、テトラピロール環同士がππ相互作用する」超分子構造を強く支持した。
安定なクロロフィル分子の自己集積体構築のために、シラノール基の縮重合(ゾルゲル法)を試み、化学的にも機械的にも安定なサブマイクロサイズの光収穫超分子系を調製できた。このような微粒子は、天然のクロロゾームと同様に水中では表面負電荷を有するために、正電荷を帯びた界面上に固定化できた。このような自己集積系と界面とのインターフェイスをうまく設計することで、高効率な光収穫・エネルギー移動型の超分子ナノデバイスの創製ができると考えている。

研究成果

• [雑誌論文] Self-aggregation of Synthetic Zinc 3^1-Hydroxy-13^1-Oxo-17,18-cis-Chlorin in a Non-Polar Organic Solvent (2007)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Res. Chem. Int. 33 ページ: 161-168
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] The 17-propionate function of (bacterio)chlorophylls : biological implication of their long esterifying chains in photosynthetic systems (2007)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Photochem. Photobiol. 83 ページ: 152-162
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Optical properties of synthetic porphyrins bearing or lacking an exo-five-membered ring and a keto carbonyl group on it, both of which are present in naturally occurring chlorophylls (2007)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: J. Photochem. Photobiol. A : Chem. 185 ページ: 321-330
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Crystal Structures of CbiL, a Methyltransferase Involved in Anaerobic Vitamin B_<12> Biosynthesis, and its Complex with S-Adenosylhomocysteine : Implications for the Reaction Mechanism (2007)
  • 著者名/発表者名: K.Wada, et al.
  • 雑誌名: FEBS J. 274 ページ: 563-573
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Self-aggregation of zinc chlorophylls possessing perfluoroalkyl chains in fluorous solvents : Selective extraction of the self-aggregates with fluorous phase and accelerated formation of the ordered supramolecules in this phase (2007)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Bioorg. Med. Chem. Lett. 17 ページ: 1920-1923
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Aqueous Self-Aggregates of Amphiphilic Zinc 3^1-Hydroxy- and 3^1-Methoxy-chlorins for Supramolecular Light-Harvesting Systems (2007)
  • 著者名/発表者名: T.Miyatake, et al.
  • 雑誌名: Tetrahedron Lett. 48 ページ: 2251-2254
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Regioisomerically controlled self-aggregation of zinc 3-hydroxymethyl-13-formyl-chlorin/porphyrin and their 3,13-inverted pigment (2007)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: J. Org. Chem. 72 ページ: 2443-2451
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Kinetic Analysis of Demetalation of Bacteriochlorophyll c and e Homologs Purified from Green Sulfur Photosynthetic Bacteria (2007)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: FEBS Lett. 581 ページ: 1847-1850
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] A dye-sensitized solar cells using pheophytin-carotenoid adduct : Enhancement of photocurrent by electron and singlet-energy transfer and by suppression of singlet-triplet annihilation due to the presence of the carotenoid moiety. (2007)
  • 著者名/発表者名: X.-F.Wang, et al.
  • 雑誌名: Chem. Phys. Lett. 439 ページ: 115-120
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Polarized Fluorescence of Aggregated Bacteriochlorophyll c and Baseplate Bacteriochlorophyll a in Single Chlorosomes Isolated from Chloroflexus aurantiacus (2007)
  • 著者名/発表者名: Y.Shibata, et al.
  • 雑誌名: Biochemistry 46(印刷中)
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] A facile synthetic method for conversion of chlorophyll-a to bacteriochlorophyll-c (2007)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: J. Org. Chem. 72(印刷中)
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Self-aggregation of synthetic zinc chlorophyll derivatives possessing multi-perfluoroalkyl chains in perfluorinated solvents (2007)
  • 著者名/発表者名: R.Shibata, et al.
  • 雑誌名: Photochem. Photobiol. Sci. 6(印刷中)
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Synthetic hydroxymethyl-porphyrins for protection of carboxy group (2007)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: J. Porphyrins Phthalocyanines 11(印刷中)
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Self-aggregation of Synthetic Zinc 31-Hydroxy-131-Oxo-17,18-cis-Chlorin in a Non-Polar Organic Solvent, (2007)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Res. Chem. Int. 33 ページ: 161-168
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] The 17-propionate function of (bacterio)chlorophylls : biological implication of their long esterifying chains in photosynthetic systems, (2007)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Photochem. Photobiol. 83 ページ: 152-162
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Optical properties of synthetic porphyrins bearing or lacking an exo-five-membered ring and a keto carbonyl group on it, both of which are present in naturally occurring chlorophylls, (2007)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: J. Photochem. Photobiol. A : Chem. 185 ページ: 321-330
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Crystal Structures of CbiL, a Methyltransferase Involved in Anaerobic Vitamin B12 Biosynthesis, and its Complex with S-Adenosylhomocysteine : Implications for the Reaction Mechanism, (2007)
  • 著者名/発表者名: K.Wada, et al.
  • 雑誌名: FEBS J. 274 ページ: 563-573
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Self-aggregation of zinc chlorophylls possessing perfluoroalkyl chains in fluorous solvents : Selective extraction of the self-aggregates with fluorous phase and accelerated formation of the ordered supramolecules in this phase, (2007)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Bioorg. Med. Chem. Lett. 17 ページ: 1920-1923
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Aqueous Self-Aggregates of Amphiphilic Zinc 31-Hydroxy-and 31-Methoxy-chlorins for Supramolecular Light-Harvesting Systems, (2007)
  • 著者名/発表者名: T.Miyatake, et al.
  • 雑誌名: Tetrahedron Lett. 48 ページ: 2251-2254
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Regioisomerically controlled self-aggregation of zinc 3-hydroxymethyl-13-formyl-chlorin/porphyrin and their 3,13-inverted pigments, (2007)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: J. Org. Chem. 72 ページ: 2443-2451
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Kinetic Analysis of Demetalation of Bacteriochlorophyll c and e Homologs Purified from Green Sulfur Photosynthetic Bacteria, (2007)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: FEBS Lett. 581 ページ: 1847-1850
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] A dye-sensitized solar cells using pheophytin-carotenoid adduct : Enhancement of photocurrent by electron and singlet-energy transfer and by suppression of singlet-triplet annihilation due to the presence of the carotenoid moiety, (2007)
  • 著者名/発表者名: X.-F.Wang, et al.
  • 雑誌名: Chem. Phys. Lett. 439 ページ: 115-120
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Polarized Fluorescence of Aggregated Bacteriochlorophyll c and Baseplate Bacteriochlorophyll a in Single Chlorosomes Isolated from Chloroflexus aurantiacus, (2007)
  • 著者名/発表者名: Y.Shibata, et al.
  • 雑誌名: Biochemistry 46(in press)
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] A facile synthetic method for conversion of chlorophyll-a to bacteriochlorophyll-c, (2007)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: J. Org. Chem. 72(in press)
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Self-aggregation of synthetic zinc chlorophyll derivatives possessing multi-perfluoroalkyl chains in perfluorinated solvents, (2007)
  • 著者名/発表者名: R.Shibata, et al.
  • 雑誌名: Photochem. Photobiol. Sci. 6(in press)
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Synthetic hydroxymethyl-porphyrins for protection of carboxy group, (2007)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: J. Porphyrins Phthalocyanines 11(in press)
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Self-aggregation of Synthetic Zinc 3^1-Hydroxy-13^1-Oxo-17,18-cis-Clorin in a Non-Polar Organic Solvent (2007)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Res.Chem.Int. 33 ページ: 161-168
• [雑誌論文] Optical properties of synthetic porphyrins bearing of lacking an exo-five-memberer ring and a keto carbonyl group on it, both of which are present in naturally occurring chlorophylls (2007)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: J.Photochem.Photobiol.A : Chem. 185 ページ: 321-330
• [雑誌論文] The 17-propionate function of(bakuterio) chlorophylls : biological implication of their long esterifying chains in photosynthetic systems (2007)
  • 著者名/発表者名: H.Tamaki, et al.
  • 雑誌名: Photochem.Photobiol. 83 ページ: 152-162
• [雑誌論文] Self-aggregation of zinc chlorophylls possessing perfluoroalkyl chains in fluorous solvents : Selective extraction of the self-aggregates with fluorous phase and accelerated formation of the ordered supramolecules in this phase (2007)
  • 著者名/発表者名: H.Tamaki, et al.
  • 雑誌名: Bioorg.Med.Chem.Lett. 17 ページ: 1920-1923
• [雑誌論文] Crystal Structure of CbiL, a Methyltransferase Involved in Anaerobic Vitamin B1_12 Biosynthesis, and its Complex with S-Adenosylhomocysteine : Implications for the Reaction Mechanism (2007)
  • 著者名/発表者名: K.Wada, et al.
  • 雑誌名: FEBS.J 274 ページ: 563-573
• [雑誌論文] Regioisomerically controlled self-aggregation of zinc 3-hydroxymethyl-13-formyl-chlorine/porphyrin and their 3, 13-invited pigments (2007)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: J.Org.Chem. 72 ページ: 2442-2451
• [雑誌論文] Aqueous Self-Aggregates of Amphiphilic Zinc 3~1-Hydroxy- and 3^1-Methoxy-chlorins for Supramolecular Light-Harvesting Systems (2007)
  • 著者名/発表者名: T.Miyatake, et al.
  • 雑誌名: Tetrahedron Lett. 48 ページ: 2251-2254
• [雑誌論文] Synthetic hydroxymethyl-porphyrins for protection of carboxy group (2007)
  • 著者名/発表者名: H.Tamaki, et al.
  • 雑誌名: J.Porphyrins Phthalocyanines 11(印刷中)
• [雑誌論文] Polarized Fluorescence of Aggregated Bacteriochlorophyll c and Baseplate Bacteriochlorophyll a in a Single Chlorosomes Isolates from Chloroflexus awantiacus (2007)
  • 著者名/発表者名: Y.Shibata, et al.
  • 雑誌名: Biochemistry 46(印刷中)
• [雑誌論文] A facile synthetic method for conversion of chlorophyll-a to bacteriochlorophyll-c (2007)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: J.Org Chem. 72(印刷中)
• [雑誌論文] Self-aggregation of synthetic zinc chlorophyll derivative possessing a perfluoroalkyl group in a fluorinated solvent (2006)
  • 著者名/発表者名: R.Shibata, et al.
  • 雑誌名: Bioorg. Med. Chem. 14 ページ: 2235-224
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Assembly of extramembranous light-harvesting complexes of green sulfur photosynthetic bacterium Chlorobium tepidum on glass surface by electrostatic layer-by-layer adsorption (2006)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Thin Solid Films 500 ページ: 278-282
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Gallium (III) complexes of methyl pyropheophorbide-a as synthetic models for investigation of diastereomerically controlled axial ligation towards chlorophylls (2006)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: Bioorg. Med. Chem. Lett. 16 ページ: 1168-1171
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Stereochemical determination of chlorophyll-d molecule from Acaryochloris marina and its modification to a self-aggregative chlorophyll as a model of green photosynthetic bacterial antennae (2006)
  • 著者名/発表者名: T.Mizoguchi, et al.
  • 雑誌名: Photochem. Photobiol. Sci. 5 ページ: 291-299
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Self-aggregation of synthetic zinc chlorins possessing 13-ester-carbonyl group as chlorosomal chlorophyll models (2006)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: Eur. J. Org. Chem. 2006 ページ: 2352-2361
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Synthesis and Optical Properties of Bacteriochlorophyll-a Derivatives Having Various C3-Substituents on the Bacteriochlorin π-System (2006)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: J. Org. Chem. 71 ページ: 2648-2654
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Single Supramolecule Spectroscopy of Natural and Alkaline-Treated Chlorosomes from Green Sulfur Photosynthetic Bacteria (2006)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: J. Nanosci. Nanotech. 6 ページ: 1750-1757
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] A Second Nitrogenase-like Enzyme for Bacteriochlorophyll Biosynthesis : Reconstitution of Chlorophyllide a Reductase with Purified X-protein (BchX) and YZ-protein (BchY BchZ) from Rhodobacter capsulatus (2006)
  • 著者名/発表者名: J.Nomata, et al.
  • 雑誌名: J. Biol. Chem. 281 ページ: 15021-15028
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Trifluoroacetyl-chlorin as a new chemosensor for alcohol/amine detection (2006)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: Tetrahedron Lett. 47 ページ: 4849-4852
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Synthesis of Cyclic Chlorophyll Oligomers (2006)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: Tetrahedron Lett. 47 ページ: 4965-4968
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Effects of plant carotenoid spacers on the performance of a dye-sensitized solar cell using a chlorophyll derivative : Enhancement of photocurrent determined by one electron-oxidation potential of each carotenoid (2006)
  • 著者名/発表者名: X.-F.Wang, et al.
  • 雑誌名: Chem. Phys. Lett. 423 ページ: 470-475
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Crystal Structures of BchU, a Methyltransferase Involved in Bacteriochlorophyll c Biosynthesis, and Its Complex with S-Adenosylhomocysteine : Implication for Reaction Mechanism (2006)
  • 著者名/発表者名: K.Wada, et al.
  • 雑誌名: J. Mol. Biol. 360 ページ: 843-853
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Transmission Electron Microscopic Study on Supramolecular Nanostructures of Bacteriochlorophyll Self-Aggregates in Chlorosomes of Green Photosynthetic Bacteria (2006)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: J. Biosci. Bioeng. 102 ページ: 118-123
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Self-assembly of natural light-harvesting bacteriochlorophylls of green sulfur photosynthetic bacteria in silicate capsules as stable models of chlorosomes (2006)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Bioconjugate Chem. 17 ページ: 988-994
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Analysis of photooxidized pigments in water-soluble chlorophyll protein complex isolated from Chenopodium album (2006)
  • 著者名/発表者名: H.Hirabayashi, et al.
  • 雑誌名: J. Photochem. Photobiol. A : Chem. 183 ページ: 121-125
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Low-temperature fluorescence from single chlorosomes, photosynthetic antenna complexes of green filamentous and sulfur bacteria (2006)
  • 著者名/発表者名: Y.Shibata, et al.
  • 雑誌名: Biophys. J. 91 ページ: 3787-3796
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Oligomethylene spacer length dependent interaction of synthetic galactolipids incorporated in phospholipid layers with ricin (2006)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Colloids Surf. B : Biointerfaces 53 ページ: 87-93
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Synthesis of self-aggregative zinc chlorophylls possessing polymerizable esters as a stable model for main light-harvesting antennas of green photosynthetic bacteria (2006)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: International J. Photoenergy 2006
  • 説明: 「研究成果報告書概要(和文)」より
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  • 雑誌名: J. Org. Chem. 70 ページ: 820-828
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] In vitro activity of C-20 methyltransferase, BchU, involved in bacteriochlorophyll c biosynthesis pathway in green sulfur bacteria, (2005)
  • 著者名/発表者名: J.Harada, et al.
  • 雑誌名: FEBS Lett. 579 ページ: 1983-1987
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Synthesis of Regioselectively 18O-Labelled Chlorophyll Derivatives at the 31-and/or 131-Positions through One-Pot Exchange of Carbonyl Oxygen Atoms, (2005)
  • 著者名/発表者名: H.Morishita, et al.
  • 雑誌名: Tetrahedron 61 ページ: 6097-61070
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Dye-sensitized solar cells using a chlorophyll a derivative as the sensitizer and carotenoids having different conjugation lengths as redox spacers, (2005)
  • 著者名/発表者名: X.-F.Wang, et al.
  • 雑誌名: Chem. Phys. Lett. 408 ページ: 409-414
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Excitation Energy Transfer in Individual Light-Harvesting Chlorosome from Green Photosynthetic Bacterium Chloroflexus aurantiacus at Cryogenic Temperature, (2005)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Chem. Phys. Lett. 409 ページ: 34-37
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Determination of Stereochemistry of Bacteriochlorophyll gF and 8^1-Hydroxy-Chlorophyll α_F from Heliobacterium modesticaldum, (2005)
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  • 雑誌名: Photochem. Photobiol. 81 ページ: 666-673
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Crystallization and preliminary X-ray diffraction study of BchU, methyltransferase from Chlorobium tepidum involved in bacteriochlorophyll c biosynthesis, (2005)
  • 著者名/発表者名: J.Harada, et al.
  • 雑誌名: Acta Crystal. F 61 ページ: 712-714
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Synthesis of Strapped Zinc Chlorophyll Derivatives and Their Complexation with a Single Axial Ligand, (2005)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: Tetrahedron 61 ページ: 8041-8048
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Bacteriochlorophyll-c Homolog Composition in Green Sulfur Photosynthetic Bacterium Chlorobium vibrioforme Dependent on the Concentration of Sodium Sulfide in Liquid Cultures, (2005)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Photosynth. Res. 86 ページ: 123-130
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Time-Dependent Self-Assembly of 31-Epimerically Pure and Mixed Zinc Methyl Bacteriopheophorbides-d in an Aqueous Tetrahydrofuran Solution, (2005)
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  • 雑誌名: Photosynth. Res. 86 ページ: 131-136
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Different sensitivities to oxygen between two strains of the photosynthetic green sulfur bacterium Chlorobium vibrioforme NCIB 8327 with bacteriochlorophyll c and d, (2005)
  • 著者名/発表者名: J.Harada, et al.
  • 雑誌名: Photosynth. Res. 86 ページ: 137-143
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Self-aggregates of natural and modified chlorophylls as photosynthetic light-harvesting antenna systems : Substituent effect on the B-ring, (2005)
  • 著者名/発表者名: H.Tamiaki
  • 雑誌名: Photochem. Photobiol. Sci. 4 ページ: 675-680
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Effects of peripheral substituents on diastereoselectivity of the fifth ligand binding to chlorophylls, and nomenclature of the asymmetric axial coordination sites, (2005)
  • 著者名/発表者名: T.Oba, et al.
  • 雑誌名: Bioorg. Med. Chem. 13 ページ: 5733-5739
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Chlorins Programmed for Self-Assembly, (2005)
  • 著者名/発表者名: T.S.Balaban, et al.
  • 雑誌名: Topics Curr. Chem. 258 ページ: 1-38
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Self-Aggregation of Synthetic Zinc 3-Hydroxymethyl-Purpurin-18 and N-Hexylimide Methyl Esters in an Aqueous Solution as Models of Green Photosynthetic Bacterial Chlorosomes, (2005)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Chem. Lett. 34 ページ: 1344-1345
  • NAID: 10019351724
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Synthesis of stereospecifically face-protected chlorophyll derivatives, (2005)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: Tetrahedron Lett. 46 ページ: 7687-7689
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Generation of carotenoid radical cation in the vicinity of a chlorophyll derivative bound to titanium oxide, upon excitation of the chlorophyll derivative to the Q_y state, as identified by time-resolved absorption spectroscopy, (2005)
  • 著者名/発表者名: X.-F.Wang, et al.
  • 雑誌名: Chem. Phys. Lett. 416 ページ: 229-233
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Self-aggregates of bacteriochlorophylls-c, d and e in a light-harvesting antenna system of green photosynthetic bacteria : Effect of stereochemistry at the chiral 3-(1-hydroxyethyl) group on the supramolecular arrangement of chlorophyllous pigments, (2005)
  • 著者名/発表者名: T.Miyatake, et al.
  • 雑誌名: J. Photochem. Photobiol. C : Photochem. Rev. 6 ページ: 89-107
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Self-aggregation of synthetic protobacteriochlorophyll-d derivatives (2005)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Photochem.Photobiol. 81 ページ: 170-176
• [雑誌論文] Self-aggregation of synthetic zinc oxo-bacteriochlorins bearing substituents characteristic of chlorosomal chlorophylls (2005)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: J.Org.Chem. 70 ページ: 820-828
• [雑誌論文] Self-aggregates of natural and modified chlorophylls as photosynthetic light-harvesting antenna systems : Substituent effect on the B-ring (2005)
  • 著者名/発表者名: H.Tamiaki
  • 雑誌名: Photochem.Photobiol.Sci. 4 ページ: 675-680
• [雑誌論文] Excitation energy transfer in individual light-harvesting chlorosome from green photosynthetic bacterium Chloroflexus aurantiacus at cryogenic temperatur (2005)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Chem.Phys.Lett 409 ページ: 34-37
• [雑誌論文] Determination of stereochemistry of bacteriochlorophyll g_F and 8^1-hydroxy-chlorophyll a_F from Heliobacterium modesticaldum (2005)
  • 著者名/発表者名: T.Mizoguchi, et al.
  • 雑誌名: Photochem.Photobiol. 81 ページ: 666-667
• [雑誌論文] Synthesis of regioselectively ^<18>O-labelled chlorophyll derivatives at the 3^1-and/or 13^1-positions through one-pot exchange of carbonyl oxygen atoms (2005)
  • 著者名/発表者名: H.Morishita, et al.
  • 雑誌名: Tetrahedron 61 ページ: 6097-6610
• [雑誌論文] Bacteriochlorophyll-c homolog composition in green sulfur photosynthetic bacterium Chlorobium vibrioforme dependent on the concentration of sodium sulfide in liquid cultures (2005)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Photosynth.Res. 86 ページ: 123-130
• [雑誌論文] Time-dependent self-assembly of 3^1-epimerically pure and mixed zinc methyl bacteriopheophorbides-d in an aqueous tetrahydrofuran solution (2005)
  • 著者名/発表者名: T.Miyatake, et al.
  • 雑誌名: Photosynth.Res. 86 ページ: 131-136
• [雑誌論文] Different sensitivities to oxygen between two strains of the photosynthetic green sulfur bacterium Chlorobium vibrioforme NCIB 8327 with bacteriochlorophyll c and d (2005)
  • 著者名/発表者名: J.Harada, et al.
  • 雑誌名: Photosynth.Res. 86 ページ: 137-143
• [雑誌論文] Synthesis of strapped zinc chlorophyll derivatives and their complexation with a single axial ligand (2005)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: Tetrahedron 61 ページ: 8041-8804
• [雑誌論文] Chlorins programmed for self-assembly (2005)
  • 著者名/発表者名: T.S.Balaban, et al.
  • 雑誌名: Topics Curr.Chem. 258 ページ: 1-38
• [雑誌論文] Self-aggregates of bacteriochlorophylls-c, d and e in a light-harvesting antenna system of green photosynthetic bacteria : Effect of stereochemistry at the chiral 3-(1-hydroxyethyl) group on the supramolecular arrangement of chlorophyllous pigments (2005)
  • 著者名/発表者名: T.Miyatake, et al.
  • 雑誌名: J.Photochem.Photobiol.C : Photochem.Rev. 6 ページ: 89-107
• [雑誌論文] Effects of peripheral substituents on diastereoselectivity of the fifth ligand binding to chlorophylls, and nomenclature of the asymmetric axial coordination sites (2005)
  • 著者名/発表者名: T.Oba, et al.
  • 雑誌名: Bioorg.Med.Chem. 13 ページ: 5733-5573
• [雑誌論文] Dye-sensitized solar cells using a chlorophyll a derivative as the sensitizer and carotenoids having different conjugation lengths as redox spacers (2005)
  • 著者名/発表者名: X.-F.Wang, et al.
  • 雑誌名: Chem.Phys.Lett. 408 ページ: 409-414
• [雑誌論文] Crystallization and preliminary X-ray diffraction study of BchU, methyltransferase from Chlorobium tepidum involved in bacteriochlorophyll c biosynthesis (2005)
  • 著者名/発表者名: J.Harada, et al.
  • 雑誌名: Acta Crystal.F 61 ページ: 712-771
• [雑誌論文] Self-aggregation of synthetic zinc 3-hydroxymethyl-purpurin-18 and N-hexylimide methyl esters in an aqueous solution as models of green photosynthetic bacterial chlorosome (2005)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Chem.Lett. 34 ページ: 1344-1345
  • NAID: 10019351724
• [雑誌論文] Generation of carotenoid radical cation in the vicinity of a chlorophyll derivative bound to titanium oxide, upon excitation of the chlorophyll derivative to the Qy state, as identified by time-resolved absorption spectroscopy (2005)
  • 著者名/発表者名: X.-F.Wang, et al.
  • 雑誌名: Chem.Phys.Lett. 416 ページ: 229-223
• [雑誌論文] Self-organization of BChl c in chlorosomes studied by MAS NMR of aggregated Cd-chlorins (2005)
  • 著者名/発表者名: I.de Boer, et al.
  • 雑誌名: Photosynthesis : Fundamental Aspects to Global Perspectives (Ed by A.van der Est & D.Bruce)(Allen Press, Lawrence, KS) ページ: 121-122
• [雑誌論文] Microscopic investigation of single chlorosomes from green photosynthetic bacteria at cryogenic temperature (2005)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Photosynthesis : Fundamental Aspects to Global Perspectives (Ed by A.van der Est & D.Bruce)(Allen Press, Lawrence, KS) ページ: 125-127
• [雑誌論文] Self-aggregation of synthetic zinc 17,18-cis-bacteriochlorophyll-d derivative (2005)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Photosynthesis : Fundamental Aspects to Global Perspectives (Ed by A.van der Est & D.Bruce)(Allen Press, Lawrence, KS) ページ: 127-128
• [雑誌論文] Self-aggregation of zinc oxo-bacteriochlorins as models of chlorosomal chlorophylls (2005)
  • 著者名/発表者名: M.Kunieda i, et al.
  • 雑誌名: Photosynthesis : Fundamental Aspects to Global Perspectives (Ed by A.van der Est & D.Bruce)(Allen Press, Lawrence, KS) ページ: 128-130
• [雑誌論文] Synthesis of ^<18>O-labelled (pyro)pheophytins including pheophytin-d (2005)
  • 著者名/発表者名: H.Morishita, et al.
  • 雑誌名: Photosynthesis : Fundamental Aspects to Global Perspectives (Ed by A.van der Est & D.Bruce)(Allen Press, Lawrence, KS) ページ: 796-797
• [雑誌論文] クロロフィルの固体表面への組織化とその光応答 (2005)
  • 著者名/発表者名: 佐賀佳央ら
  • 雑誌名: 化学工業 56・4 ページ: 272-276
• [雑誌論文] Self-aggregation of synthetitc zinc oxo-bacteriochlorins bearing substituents characteristic of chlorosomal chlorophylls (2005)
  • 著者名/発表者名: M.Kunieda, H.Tamiaki
  • 雑誌名: J.Org.Chem. 70 ページ: 820-828
• [雑誌論文] Self-aggregation of protobacteriochlorophyll-d derivatives (2005)
  • 著者名/発表者名: H.Tamiaki, H.Kitamoto, T.Watanabe, R.Shibata
  • 雑誌名: Photochem.Photobiol. 81 ページ: 170-176
• [雑誌論文] Fluorescence Spectroscopy of Single Photosynthetic Light-Harvesting Supramolecular Systems (2004)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Cell Biochem. Biophys 40 ページ: 149-166
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Effects of C8-substituents on spectroscopic and self-aggregation properties of synthetic bacteriochlorophyll-d analogues (2004)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: J. Photochem. Photobiol. A : Chem. 162 ページ: 307-315
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Facile Synthesis of Chlorophyll Analog Possessing a Disulfide Bond and Formation of Self-Assembled Monolayer on Gold Surface (2004)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: J. Photochem. Photobiol. B : Biol. 73 ページ: 29-34
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Diastereoselective self-aggregation of synthetic 3-(1-hydroxyethyl)-bacteriopyrochlorophyll-a as a novel photosynthetic antenna model absorbing near the infrared region (2004)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: Photochem. Photobiol. 79 ページ: 55-61
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Self-assembly of synthetic bacteriochlorophyll-f analogues possessing C8-formyl group (2004)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: Bull. Chem. Soc. Jpn. 77 ページ: 797-800
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Determination of 3^1-Stereochemistry in Synthetic Bacteriochlorophyll-d Homologs and Self-aggregation of Their Zinc Complexes (2004)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Bioorg. Med. Chem. 12 ページ: 1657-1666
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Synthesis of a novel cyclic chlorophyll hetero-dyad as a model compound for stacked chlorophylls found in photosynthetic systems (2004)
  • 著者名/発表者名: N.Kosaka, et al.
  • 雑誌名: Eur. J. Org. Chem. 2004 ページ: 2325-2330
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Coaggregation of Amphiphilic Zinc Chlorins with Synthetic Surfactants in Aqueous Medium to an Artificial Supramolecular Light-Harvesting Antenna (2004)
  • 著者名/発表者名: T.Miyatake, et al.
  • 雑誌名: Bioorg. Med. Chem. 12 ページ: 2173-2178
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Excitation Energy Transfer from Self-Aggregates of Zinc Chlorins to a Bacteriochlorin in a Silicate Nanocapsule (2004)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Chem. Lett. 33 ページ: 544-545
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Comparison between chlorosomes containing bacteriochlorophyll-c and chlorosomes containing bacteriochlorophyll-d isolated from two substrains of green sulfur photosynthetic bacterium Chlorobium vibrioforme NCIB 8327 (2004)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: J. Photochem. Photobiol. B : Biol. 75 ページ: 89-97
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] MAS NMR structures of aggregated cadmium chlorins reveal molecular control of self-assembly of chlorosomal bacteriochlorophylls (2004)
  • 著者名/発表者名: I.de Boer, et al.
  • 雑誌名: J. Phys. Chem. B 108 ページ: 16556-16566
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Syntheses of optical properties of stable 8-alkylidene-bacteriochlorins mimicking the molecular structures of natural bacteriochlorophyll-b and g (2004)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: Tetrahedron 60 ページ: 11349-11357
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Synthesis of 3,4,5-Tris(alkyloxy)benzyl Glycosides as Glycolipid Analogues (2004)
  • 著者名/発表者名: R.Sato, et al.
  • 雑誌名: J. Carbohydr. Chem. 23 ページ: 375-383
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Fluorescence Spectroscopy of Single Photosynthetic Light-Harvesting Supramolecular Systems, (2004)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Cell Biochem. Biophys. 40 ページ: 149-166
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Effects of C8-substituents on spectroscopic and self-aggregation properties of synthetic bacteriochlorophyll-d analogues, (2004)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: J. Photochem. Photobiol. A : Chem. 162 ページ: 307-315
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Facile Synthesis of Chlorophyll Analog Possessing a Disulfide Bond and Formation of Self-Assembled Monolayer on Gold Surface, (2004)
  • 著者名/発表者名: Y Saga, et al.
  • 雑誌名: J. Photochem. Photobiol. B : Biol. 73 ページ: 29-34
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Diastereoselective self-aggregation of synthetic 3-(1-hydroxyethyl)-bacteriopyrochlorophyll-a as a novel photosynthetic antenna model absorbing near the infrared region, (2004)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: Photochem. Photobiol. 79 ページ: 55-61
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Self-assembly of synthetic bacteriochlorophyll-f analogues possessing C8-formyl group, (2004)
  • 著者名/発表者名: S.Sasaki, et al.
  • 雑誌名: Bull. Chem. Soc. Jpn. 77 ページ: 797-800
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Determination of 3^1-Stereochemistry in Synthetic Bacteriochlorophyll-d Homologs and Self-aggregation of Their Zinc Complexes, (2004)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Bioorg. Med. Chem. 12 ページ: 1657-1666
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Synthesis of a novel cyclic chlorophyll hetero-dyad as a model compound for stacked chlorophylls found in photosynthetic systems, (2004)
  • 著者名/発表者名: N.Kosaka, et al.
  • 雑誌名: Eur. J. Org. Chem. ページ: 2325-2330
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Coaggregation of Amphiphilic Zinc Chlorins with Synthetic Surfactants in Aqueous Medium to an Artificial Supramolecular Light-Harvesting Antenna, (2004)
  • 著者名/発表者名: T.Miyatake, et al.
  • 雑誌名: Bioorg. Med. Chem. 12 ページ: 2173-2178
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Excitation Energy Transfer from Self-Aggregates of Zinc Chlorins to a Bacteriochlorin in a Silicate Nanocapsule, (2004)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Chem. Lett. 33 ページ: 544-545
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Comparison between chlorosomes containing bacteriochlorophyll-c and chlorosomes containing bacteriochlorophyll-d isolated from two substrains of green sulfur photosynthetic bacterium Chlorobium vibrioforme NCIB 8327, (2004)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: J. Photochem. Photobiol. B : Biol. 75 ページ: 89-97
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] MAS NMR structures of aggregated cadmium chlorins reveal molecular control of self-assembly of chlorosomal bacteriochlorophylls, (2004)
  • 著者名/発表者名: I.de Boer, et al.
  • 雑誌名: J. Phys. Chem. B 108 ページ: 16556-16566
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Syntheses of optical properties of stable 8-alkylidene-bacteriochlorins mimicking the molecular structures of natural bacteriochlorophyll-b and g, (2004)
  • 著者名/発表者名: M.Kunieda, et al.
  • 雑誌名: Tetrahedron 60 ページ: 11349-11357
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Synthesis of 3,4,5-Tris(alkyloxy)benzyl Glycosides as Glycolipid Analogues, (2004)
  • 著者名/発表者名: R.Sato, et al.
  • 雑誌名: J. Carbohydr. Chem. 23 ページ: 375-383
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Effects of C8-substituents on spectroscopic and self-aggregation properties of synthetic bacteriochlorophyll-d analogues (2004)
  • 著者名/発表者名: S.Sasaki, M.Omoda, H.Tamiaki
  • 雑誌名: J.Photochem.Photobiol.A : Chem. 162 ページ: 307-315
• [雑誌論文] Facile Synthesis of Chlorophyll Analog Possessing a Disulfide Bond and Formation of Self-Assembled Monolayer on Gold Surface (2004)
  • 著者名/発表者名: Y.Saga, H.Tamiaki
  • 雑誌名: J.Photochem.Photobiol.B : Biol. 73 ページ: 29-34
• [雑誌論文] Diastereoselective self-aggregation of synthetic 3-(1-hydroxyethyl)-bacteriopyrochlorophyll-a as a novel photosynthetic antenna model absorbing near the infrared region (2004)
  • 著者名/発表者名: M.Kunieda, T.Mizoguchi, H.Tamiaki
  • 雑誌名: Photochem.Photobiol. 79 ページ: 55-61
• [雑誌論文] Self-assembly of synthetic bacteriochlorophyll-f analogues possessing C8-formyl group (2004)
  • 著者名/発表者名: S.Sasaki, H.Tamiaki
  • 雑誌名: Bull.Chem.Soc.Jpn. 77 ページ: 797-800
• [雑誌論文] Determination of 3^1-Stereochemistry in Synthetic Bacteriochloro-phyll-d Homologs and Self-aggregation of Their Zinc Complexes (2004)
  • 著者名/発表者名: H.Tamiaki, H.Kitamoto, A.Nishikawa, T.Hibino, R.Shibata
  • 雑誌名: Bioorg.Med.Chem. 12 ページ: 1657-1666
• [雑誌論文] Coaggregation of Amphiphilic Zinc Chlorins with Synthetic Surfactants in Aqueous Medium to an Artificial Supramolecular Light-Harvesting Antenna (2004)
  • 著者名/発表者名: T.Miyatake, H.Tamiaki, M.Fujiwara, T.Matsushita
  • 雑誌名: Bioorg.Med.Chem. 12 ページ: 2173-2178
• [雑誌論文] Synthesis of a novel cyclic chlorophyll hetero-dyad as a model compound for stacked chlorophylls found in photosynthetic system (2004)
  • 著者名/発表者名: N.Kosaka, H.Tamiaki
  • 雑誌名: Eur.J.Org.Chem. 2004 ページ: 2325-2330
• [雑誌論文] Comparison between chlorosomes containing bacteriochlorophyll-c and chlorosomes containing bacteriochlorophyll-d isolated from two substrains of green sulfur photosynthetic bacterium Chlorobium vibrioforme NCIB 8327 (2004)
  • 著者名/発表者名: Y.Saga, H.Tamiaki
  • 雑誌名: J.Photochem.Photobiol.B : Biol. 75 ページ: 89-97
• [雑誌論文] Syntheses of optical properties of stable 8-alkylidene-bacteriochlorins mimicking the molecular structures of natural bacteriochlorophyll-b and g (2004)
  • 著者名/発表者名: M.Kunieda, T.Mizoguchi, H.Tamiaki
  • 雑誌名: Tetrahedron 60 ページ: 11349-11357
• [雑誌論文] MAS NMR structures of aggregated cadmium chlorins reveal molecular control of self-assembly of chlorosomal bacteriochlorophylls (2004)
  • 著者名/発表者名: I.de Boer, J.Matysik, K.Erkelens, S.Sasaki, T.Miyatake, S.Yagai, H.Tamiaki, A.R.Holzwarth, H.J.M.de Groot
  • 雑誌名: J.Phys.Chem., B 108 ページ: 16556-16566
• [雑誌論文] Synthesis of Homologously Pure Bacteriochlorophyll-e and f Analogues from BChls-c/d via Transformation of the 7-Methyl to Formyl Group and Self-Aggregation of Synthetic Zinc Methyl Bacteriopheophorbides-c/d/e/f in Non-Polar Organic Solvent (2003)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Tetrahedron 59 ページ: 4337-4350
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Synthesis of Specifically ^<18>O-Labelled Chlorophyll Derivatives at Carbonyl Oxygen Atoms by Acidic Hydrolysis of the Ethylene Ketal and Acetal (2003)
  • 著者名/発表者名: H.Morishita, et al.
  • 雑誌名: Bioorg. Med. Chem. 11 ページ: 4049-4057
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Self-aggregation of synthetic zinc 2^1-hydroxy-12^1/13^1-oxo-porphyrins (2003)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Tetrahedron 59 ページ: 7423-7435
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] MAS NMR Structure of a Microcrystalline Cd-bacteriochlorophyll d Analog (2003)
  • 著者名/発表者名: I.de Boer, et al.
  • 雑誌名: J. Am. Chem. Soc. 125 ページ: 13374-13375
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Presence of Exclusively Bacteriochlorophyll-c Containing Substrain in the Culture of Green Sulfur Photosynthetic Bacterium Chlorobium vibrioforme Strain NCIB 8327 Producing Bacteriochlorophyll-d (2003)
  • 著者名/発表者名: Y.Saga, et al.
  • 雑誌名: Anal. Sci 19 ページ: 1575-1579
  • 説明: 「研究成果報告書概要(和文)」より
• [雑誌論文] Synthesis of Homologously Pure Bacteriochlorophyll-e and f Analogues from BChls-c/d via Transformation of the 7-Methyl to Formyl Group and Self-Aggregation of Synthetic Zinc Methyl Bacteriopheophorbides-c/d/e/f in Non-Polar Organic Solvent, (2003)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Tetrahedron 59 ページ: 4337-4350
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Synthesis of Specifically ^<18>O-Labeled Chlorophyll Derivatives at Carbonyl Oxygen Atoms by Acidic Hydrolysis of the Ethylene Ketal and Acetal, (2003)
  • 著者名/発表者名: H.Morishita, et al.
  • 雑誌名: Bioorg. Med. Chem. 11 ページ: 4049-4057
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Self-aggregation of synthetic zinc 2^1-hydroxy-12^1/13^1-oxo-porphyrins, (2003)
  • 著者名/発表者名: H.Tamiaki, et al.
  • 雑誌名: Tetrahedron 59 ページ: 7423-7435
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] MAS NMR Structure of a Microcrystalline Cd-bacteriochlorophyll d Analog, (2003)
  • 著者名/発表者名: I.de Boer, et al.
  • 雑誌名: J. Am. Chem. Soc. 125 ページ: 13374-13375
  • 説明: 「研究成果報告書概要(欧文)」より
• [雑誌論文] Presence of Exclusively Bacteriochlorophyll-c Containing Substrain in the Culture of Green Sulfur Photosynthetic Bacterium Chlorobium vibrioforme Strain NCIB 8327 Producing Bacteriochlorophyll-d, (2003)
  • 著者名/発表者名: Y Saga, et al.
  • 雑誌名: Anal. Sci. 19 ページ: 1575-1579
  • 説明: 「研究成果報告書概要(欧文)」より
• [産業財産権] メチル基転移酵素、そのDNA、及び特定部位にメチル基が導入されたポルフィリン型化合物の製造方法 (2004)
  • 発明者名: 民秋 均, 原田二朗, 佐賀佳央
  • 権利者名: 学校法人立命館
  • 公開番号: 2006-005513
  • 出願年月日: 2004-08-23
  • 取得年月日: 2006-03-02
  • 説明: 「研究成果報告書概要(和文)」より
• [産業財産権] メチル基転移酵素、そのDNA、及び特定部位にメチル基が導入されたポルフィリン型化合物の製造方法 (2004)
  • 発明者名: 民秋 均, 原田 二朗, 佐賀 佳央
  • 権利者名: 学校法人立命館, 民秋 均, 原田 二朗, 佐賀 佳央
  • 産業財産権番号: 2004-242888
  • 出願年月日: 2004-08-23
• [文献書誌] Y.Saga, H.Oh-oka, T.Hayashi, H.Tamiaki: "Presence of Exclusively Bacteriochlorophyll-c Containing Substrain in the Culture of Green Sulfur Photosynthetic Bacterium Chlorobium vibrioforme Strain NCIB 8327 Producing Bacteriochlorophyll-d"Anal.Sci.. 19. 1575-1579 (2003)
• [文献書誌] H.Morishita, H.Tamiaki: "Synthesis of Specifically^<18>O-Labeled Chlorophyll Derivatives at Carbonyl Oxygen Atoms by Acidic Hydrolysis of the Ethylene Ketal and Acetal"Bioorg.Med.Chem.. 11. 4049-4057 (2003)
• [文献書誌] H.Tamiaki, S.Kimura, T.Kimura: "Self-aggregation of synthetic 2^1-hydroxy-12^1/13^1-oxo-porphyrins"Tetrahedron. 59. 7423-7435 (2003)
• [文献書誌] H.Tamiaki, H.Kitamoto, A.Nishikawa, T.Hibino, R.Shibata: "Diastereoselective Self-Aggregation of Synthetic Zinc Bacteriochlorophyll-d Homologs"BIOMOLECULAR CHEMISTRY-A Bridge for the Future-. 184-187 (2003)
• [文献書誌] S.Sasaki, M.Omoda, H.Tamiaki: "Effects of C8-substituents on spectroscopic and self-aggregation properties of synthetic bacteriochlorophyll-d analogues"J.Photochem.Photobiol. A: Chem.. 162. 307-315 (2004)
• [文献書誌] M.Kunieda, T.Mizoguchi H.Tamiaki: "Diastereoselective self-aggregation of synthetic 3-(1-hydroxyethyl)-bacteriopyrochlorophyll-a as a novel photosynthetic antenna model absorbing near the infrared region"Photochem.Photobiol.. 79. 55-61 (2004)
• [文献書誌] Y.Saga, H.Tamiaki: "Facile Synthesis of Chlorophyll Analog Possessing a Disulfide Bond and Formation of Self-Assembled Monolayer on Gold Surface"J.Photochem.Photobiol.B : Biol.. 73. 29-34 (2004)
• [文献書誌] S.Sasaki, H.Tamiaki: "Self-assembly of synthetic bacteriochlorophyll-f analogues possessing C8-formyl group"Bull.Chem.Soc.Jpn.. 77(In press). (2004)
• [文献書誌] H.Tamiaki, T.Watanabe, M.Kunieda: "Self aggregation of Synthetic Zinc 3^1-Hydroxy-13^1-Oxo-17, 18-cis-Chlorin in a Non-Polar Organic Solvent"Res.Chem.Int.. 30(In press). (2004)
• [文献書誌] T.Miyatake, H.Tamiaki, M.Fujiwara, T.Matsushita: "Coaggregation of Amphiphilic Zinc Chlorins with Synthetic Surfactants in Aqueous Medium to an Artifcial Supramolecular Light-Harvesting Antenna"Bioorg.Med.Chem.. 12(In press). (2004)
• [文献書誌] H.Tamiaki, H.Kitamoto, A.Nishikawa, T.Hibino, R.Shibata: "Determination of 3^1-Stereochemistry in Synthetic Bacteriochlorophyll-d Homologs and Self-aggregation of Their Zinc Complexes"Bioorg.Med.Chem.. 12(In press). (2004)
• [文献書誌] N.Kosaka, H.Tamiaki: "Synthesis of a novel cyclic chlorophyll hetero-dyad as a model compound for stacked chlorophylls found in photosynthetic apparatus"Eur.J.Org.Chem.. (In press). (2004)