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The influence of land-surface reactivity on atmospheric carbon dioxide during past hyperthermals

研究課題

研究課題/領域番号 22K14137
研究種目

若手研究

配分区分基金
審査区分 小区分17050:地球生命科学関連
研究機関国立研究開発法人海洋研究開発機構

研究代表者

Sproson Adam  国立研究開発法人海洋研究開発機構, 海洋機能利用部門(生物地球化学センター), Young Research Fellow (40937728)

研究期間 (年度) 2022-04-01 – 2025-03-31
研究課題ステータス 中途終了 (2023年度)
配分額 *注記
4,550千円 (直接経費: 3,500千円、間接経費: 1,050千円)
2023年度: 2,210千円 (直接経費: 1,700千円、間接経費: 510千円)
2022年度: 2,340千円 (直接経費: 1,800千円、間接経費: 540千円)
キーワードSilicate weathering / Magnesium isotopes / Lithium isotopes / Paleoclimate / Paleoweathering / Hyperthermals / Beryllium isotopes
研究開始時の研究の概要

This project will determine the Li, Mg and Be isotope variation of marine sediments to understand how weathering in the Amazon River basin responds to a global warming of 2°C. This will help ascertain the capacity for weathering to reverse global warming in the future under increasing CO2 emissions.

研究実績の概要

In this study, marine sediments were analysed for magnesium and lithium isotopes to create a time-series of chemical and physical silicate weathering in the Earth’s geological past. The purpose is to elucidate the response of silicate weathering, which experts a major control on atmospheric CO2 concentration, to regional and global warming. A warmer, wetter climate should provide more energy and fluids for silicate weathering reaction at the Earth’s surface to occur, consuming atmospheric CO2 and reversing the global warming trend. However, if the products of silicate weathering remain in the surficial system for too long before being deposited in marine sediments, they are converted back to silicates (reverse weathering), remitting the consumed CO2 leading to no net change on climate.

During the past fiscal year, 200 sediment samples from several IODP cores collected from deep ocean basins as well as the Amazon margin were ordered, dried, crushed and chemically processed to extract the carbonate, iron oxide and silicate phase. Mg was purified from these phases and the Mg isotopic composition was measured by inductively coupled plasma mass spectrometry. This revealed that the carbonate and reactive phase of marine sediments could be used as a proxy for past seawater variation. Li has been purified and is awaiting measurement. This will provide records of past weathering during periods of regional and global warming over tens of thousands to millions of years to help understand the silicate weathering capacity to reverse global warming.

現在までの達成度 (区分)
現在までの達成度 (区分)

2: おおむね順調に進展している

理由

Marine sediments from the Amazon margin, Pacific Ocean, Indian Ocean and Atlantic Ocean were ordered and received from IODP. The samples were dried and crushed before undergoing a leaching technique to separate the carbonate, iron oxide and silicate phases. Major, minor and Rare Earth elements of these phases have been analysed successfully. Magnesium and lithium for the Pacific Ocean, Indian Ocean and Atlantic Ocean samples were purified and have undergone magnesium isotope measurement. Lithium isotopes are awaiting measurement. The Amazon samples will begin purification in the near future.

Findings from this project were presented at an international conference in France and domestic conference in Japan.

今後の研究の推進方策

The remaining marine sediment samples from the Pacific Ocean, Indian Ocean and Atlantic Ocean will be measured for lithium isotopes soon after already being purified. The remaining ~50 Amazon River samples will undergo purification of magnesium and lithium and measurement of magnesium and lithium isotopes and element concentrations.

報告書

(2件)
  • 2023 実施状況報告書
  • 2022 実施状況報告書
  • 研究成果

    (11件)

すべて 2023 2022

すべて 雑誌論文 (4件) (うち国際共著 4件、 査読あり 4件、 オープンアクセス 3件) 学会発表 (7件) (うち国際学会 4件、 招待講演 3件)

  • [雑誌論文] Deep submarine infiltration of altered geothermal groundwater on the south Chilean Margin2022

    • 著者名/発表者名
      Clementi Vincent J.、and the Expedition 379T scientists
    • 雑誌名

      Communications Earth & Environment

      巻: 3 号: 1 ページ: 1-9

    • DOI

      10.1038/s43247-022-00541-3

    • 関連する報告書
      2022 実施状況報告書
    • 査読あり / オープンアクセス / 国際共著
  • [雑誌論文] Beryllium isotope variations recorded in the Adelie Basin, East Antarctica reflect Holocene changes in ice dynamics, productivity, and scavenging efficiency2022

    • 著者名/発表者名
      Behrens Bethany C.、Yokoyama Yusuke、Miyairi Yosuke、Sproson Adam D.、Yamane Masako、Jimenez-Espejo Francisco J.、McKay Robert M.、Johnson Katelyn M.、Escutia Carlota、Dunbar Robert B.
    • 雑誌名

      Quaternary Science Advances

      巻: 7 ページ: 100054-100054

    • DOI

      10.1016/j.qsa.2022.100054

    • 関連する報告書
      2022 実施状況報告書
    • 査読あり / オープンアクセス / 国際共著
  • [雑誌論文] Holocene melting of the West Antarctic Ice Sheet driven by tropical Pacific warming2022

    • 著者名/発表者名
      Sproson Adam D.、Yokoyama Yusuke、Miyairi Yosuke、Aze Takahiro、Totten Rebecca L.
    • 雑誌名

      Nature Communications

      巻: 13 号: 1 ページ: 1-9

    • DOI

      10.1038/s41467-022-30076-2

    • 関連する報告書
      2022 実施状況報告書
    • 査読あり / オープンアクセス / 国際共著
  • [雑誌論文] Osmium and lithium isotope evidence for weathering feedbacks linked to orbitally paced organic carbon burial and Silurian glaciations2022

    • 著者名/発表者名
      Sproson Adam D.、Pogge von Strandmann Philip A.E.、Selby David、Jarochowska Emilia、Frida Jiri、Hladil Jindrich、Loydell David K.、Slavik Ladislav、Calner Mikael、Maier Georg、Munnecke Axel、Lenton Timothy M.
    • 雑誌名

      Earth and Planetary Science Letters

      巻: 577 ページ: 117260-117260

    • DOI

      10.1016/j.epsl.2021.117260

    • 関連する報告書
      2022 実施状況報告書
    • 査読あり / 国際共著
  • [学会発表] The impact of Antarctic ice sheet expansion (ca. 34 Ma) on silicate weathering, erosion and the carbon cycle: insights from Li and Mg isotopes2023

    • 著者名/発表者名
      Adam David Sproson, Toshihiro Yoshimura, Shigeyuki Wakaki, Takahiro Aze, Tsuyoshi Ishikawa, Yusuke Yokoyama, Naohiko Ohkouchi
    • 学会等名
      2023 Goldschmidt Conference
    • 関連する報告書
      2023 実施状況報告書
    • 国際学会
  • [学会発表] Orbital forcing paced Patagonian Ice Sheet extent and southern climate during the Last Glacial Period2023

    • 著者名/発表者名
      Adam David Sproson, Yusuke Yokoyama, Yosuke Miyairi, Takahiro Aze, Vincent J. Clementi, Hailey Riechelson, Samantha C. Bova, Yair Rosenthal, Laurel B. Childress
    • 学会等名
      JpGU 2023
    • 関連する報告書
      2023 実施状況報告書
    • 招待講演
  • [学会発表] Holocene climate change along the Chilean margin as determined by beryllium isotope analysis2023

    • 著者名/発表者名
      Karin Nemoto, Yusuke Yokoyama, Adam David Sproson, Yosuke Miyairi, Takahiro Aze, Matsuzaki Hiroyuki, Yair Rosenthal, Samantha Bova, Hailey Riechelson
    • 学会等名
      JpGU 2023
    • 関連する報告書
      2023 実施状況報告書
  • [学会発表] Adam Sproson, Yusuke Yokoyama, Yosuke Miyairi, Takahiro Aze, Vincent J Clementi, Hailey Riechelson, Samantha Claudia Bova, Yair Rosenthal, Laurel B Childress2022

    • 著者名/発表者名
      Southern Hemisphere pacing of global climate during the Late Pleistocene
    • 学会等名
      AGU Fall Meeting Abstracts 2022
    • 関連する報告書
      2022 実施状況報告書
    • 国際学会
  • [学会発表] Adam Sproson, Yusuke Yokoyama, Yosuke Miyairi, Takahiro Aze, Rebecca L Totten2022

    • 著者名/発表者名
      Holocene Ice Loss in the Amundsen Sea Embayment Linked to Tropical Pacific Warming
    • 学会等名
      AGU Fall Meeting Abstracts 2022
    • 関連する報告書
      2022 実施状況報告書
    • 国際学会 / 招待講演
  • [学会発表] Adam David Sproson, Toshihiro Yoshimura, Takahiro Aze, Shigeyuki Wakaki, Tsuyoshi Ishikawa, Yusuke Yokoyama, Nao Ohkouchi2022

    • 著者名/発表者名
      A novel application of Mg and Li isotopes reveals a link between erosion, chemical weathering, and atmospheric CO2 during the expansion of Antarctica’s ice sheets (ca. 34 Ma)
    • 学会等名
      2022 Goldschmidt Conference
    • 関連する報告書
      2022 実施状況報告書
    • 国際学会
  • [学会発表] Adam David Sproson, Toshihiro Yoshimura, Takahiro Aze, Shigeyuki Wakaki, Tsuyoshi Ishikawa, Yusuke Yokoyama, Naohiko Ohkouchi2022

    • 著者名/発表者名
      Can Mg and Li isotopes in the authigenic and detrital fractions of sediments be used to trace paleoweathering? Case study: The EOT
    • 学会等名
      JpGU 2022
    • 関連する報告書
      2022 実施状況報告書
    • 招待講演

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公開日: 2022-04-19   更新日: 2024-12-25  

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