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Exploring availability of plasma-induced solvated electrons: formation and transport

研究課題

研究課題/領域番号 22K14174
研究種目

若手研究

配分区分基金
審査区分 小区分19010:流体工学関連
研究機関東北大学

研究代表者

劉 思維  東北大学, 流体科学研究所, 助教 (60902228)

研究期間 (年度) 2022-04-01 – 2025-03-31
研究課題ステータス 交付 (2023年度)
配分額 *注記
4,030千円 (直接経費: 3,100千円、間接経費: 930千円)
2024年度: 1,300千円 (直接経費: 1,000千円、間接経費: 300千円)
2023年度: 1,430千円 (直接経費: 1,100千円、間接経費: 330千円)
2022年度: 1,300千円 (直接経費: 1,000千円、間接経費: 300千円)
キーワードsolvated electrons / plasma flow / homogeneous / time-resolved / solvated electron / plasma / formation / transport
研究開始時の研究の概要

This research innovatively proposes the plasma flow in the liquid as a potential high-effective source for solvated electrons. A real-time two-dimensional visualization using fluid dynamics methods is constructed to evaluate the formation and transport of plasma-induced solvated electrons. The systematic understanding of the coupling influence between solvated electrons and plasma flow will be elucidated. We expect to understand the coupling mechanism and promote the availability of plasma-induced solvated electrons as well as the controllability of plasma flow.

研究実績の概要

1. In FY 2023, the difficulty of transient measurement for charge distribution was overcome. Supplementary to the selection of indicators for solvated electrons(FY 2022), the applicant developed a plasma probe for the solvated electron by the behavior analysis of the plasma flow and the homogeneous low-energy plasma discharge. The results confirm the visualization of solvated electrons using fluid dynamics methods.
2. Time-resolved spectroscopy platform was constructed (FY 2022) and successfully achieved in detecting solvated electrons (FY 2023). The difficulties of synchronization, light intensity modulation, and emission line distinguishing were overcome. The spectral characteristics are also possible to be adopted for monitoring the chemical reactions and species involved in the studied transient phenomena.
3. Based on the previous plasma regulation techniques, the applicant succeeded in forming a pre-designed pathway (electric distortion, UV-VIS focusing, etc.) to change the behavior of plasma flow and enhance the local concentration of solvated electrons at the desired position. The generated solvated electrons have a usable concentration and were successfully adopted in environmental and biomedical fields.

現在までの達成度 (区分)
現在までの達成度 (区分)

1: 当初の計画以上に進展している

理由

1. Time-resolved spectroscopy was successfully achieved in FY 2022. In addition, we further analyzed the OES characteristics of the plasma in 2023 and it provided informative knowledge on the chemical species involved. These results are much beyond the original expectation.
2. The difficulty of transient measurement for charge distribution was overcome in FY 2023. The applicant developed a plasma probe for the detection of the solvated electron by the behavior analysis of the plasma flow. It was sufficiently improved compared to the indicators for solvated electrons in FY 2022.
3. The applicant is now able to form a pre-designed pathway to enhance the local concentration of solvated electrons at the desired position and adopt them in environmental and biomedical fields.

今後の研究の推進方策

In FY 2024, it is necessary to obtain a comprehensive understanding of the generation and regulation of solvated electrons. Three main works are planned:
1. I succeeded in detecting the chemical species involved in the studied case and I planned to monitor the chemical reactions with the plasma flow and solvated electrons. It is necessary to overcome the difficulty in distinguishing the spectral signals of solvated electrons from the strong emissions of plasma.
2. The interaction of the solvated electrons with the ambient substances should be clarified. I will study this topic in FY 2024 to promote the applications of solvated electrons in environmental and biomedical fields.
3. A conclusive summary of the results and achievements of this project is required and will be performed in FY 2024.

報告書

(2件)
  • 2023 実施状況報告書
  • 2022 実施状況報告書
  • 研究成果

    (11件)

すべて 2024 2023 2022 その他

すべて 国際共同研究 (2件) 雑誌論文 (1件) (うち国際共著 1件、 査読あり 1件) 学会発表 (8件) (うち国際学会 6件、 招待講演 1件)

  • [国際共同研究] ETH Zurich/EPFL(スイス)

    • 関連する報告書
      2023 実施状況報告書
  • [国際共同研究] ETH Zurich(スイス)

    • 関連する報告書
      2022 実施状況報告書
  • [雑誌論文] Plasma-based identification of gases in a laser-induced cavitation bubble2023

    • 著者名/発表者名
      Siwei Liu, Kaito Nitto, Outi Supponen, Sayaka Kamata, Tomoki Nakajima, Mohamed Farhat, Takehiko Sato
    • 雑誌名

      Applied Physics Letters

      巻: 123 号: 9 ページ: 094102-094102

    • DOI

      10.1063/5.0164732

    • 関連する報告書
      2023 実施状況報告書
    • 査読あり / 国際共著
  • [学会発表] Plasma Discharge Inside a Laser-Induced Cavitation Bubble2024

    • 著者名/発表者名
      Siwei Liu, Kaito Nitto, Outi Supponen, Sayaka Kamata, Tomoki Nakajima, Mohamed Farhat, Takehiko Sato
    • 学会等名
      The 13th Asia-Pacific International Symposium in the Basics and Applications of Plasma Technology (APSPT13)
    • 関連する報告書
      2023 実施状況報告書
    • 国際学会
  • [学会発表] Generation of spark-induced bubble and its dependence on conductivity2023

    • 著者名/発表者名
      Siwei Liu, Yijia Ren, Tomoki Nakajima, Yi Liu,Takehiko Sato
    • 学会等名
      The 7th International Symposium on Plasma & Fine Bubbles to Agriculture and Aquaculture (ISPFB 2023)
    • 関連する報告書
      2023 実施状況報告書
    • 国際学会
  • [学会発表] Plasma-enhanced Degradation of Chlorinated Compounds2023

    • 著者名/発表者名
      Siwei Liu, Tomoki Nakajima,Takehiko Sato
    • 学会等名
      25th International Symposium on Plasma Chemistry (ISPC25)
    • 関連する報告書
      2023 実施状況報告書
    • 国際学会
  • [学会発表] Observation of laser-induced optical breakdown and its application in biomedicine2023

    • 著者名/発表者名
      Siwei Liu, Keisuke Iwasawa, Airi Nakayama, Tomoki Nakajima, Takehiko Sato
    • 学会等名
      Twentieth International Conference on Flow Dynamics (ICFD2023)
    • 関連する報告書
      2023 実施状況報告書
    • 国際学会 / 招待講演
  • [学会発表] Effect of charge distribution on the plasma-induced fine bubble dynamics2023

    • 著者名/発表者名
      Siwei Liu, Outi Supponen, Tomoki Nakajima, Takehiko Sato
    • 学会等名
      Twenty-third International Symposium on Advanced Fluid Information (AFI2023)
    • 関連する報告書
      2023 実施状況報告書
    • 国際学会
  • [学会発表] Observation and modeling of laser-induced optical breakdown in water2023

    • 著者名/発表者名
      Siwei Liu, Tomoki Nakajima,Takehiko Sato
    • 学会等名
      第47回静電気学会全国大会
    • 関連する報告書
      2023 実施状況報告書
  • [学会発表] Degradation of Chlorinated Compounds by Treatment of Repetitive Plasma Discharges2022

    • 著者名/発表者名
      Siwei Liu, Tomoki Nakajima, Takehiko Sato
    • 学会等名
      12th International Symposium on Non-Thermal /Thermal Plasma for Pollution Control & Sustainable Energy(ISNTP-12) and International Symposium of Electrohydrodynamics (ISEHD)
    • 関連する報告書
      2022 実施状況報告書
    • 国際学会
  • [学会発表] Underwater Streamers Induced by Microsecond Pulsed Discharge with Bi-polarities2022

    • 著者名/発表者名
      Siwei Liu, Yi Liu, Takehiko Sato
    • 学会等名
      第23回静電気学会春期講演会
    • 関連する報告書
      2022 実施状況報告書

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公開日: 2022-04-19   更新日: 2024-12-25  

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