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Demonstration of valley spin devices by coupling 2D semiconductors to chiral photonic crystal nanocavities

研究課題

研究課題/領域番号 22K14623
研究種目

若手研究

配分区分基金
審査区分 小区分30020:光工学および光量子科学関連
研究機関国立研究開発法人理化学研究所

研究代表者

Fong CheeFai  国立研究開発法人理化学研究所, 開拓研究本部, 基礎科学特別研究員 (30881544)

研究期間 (年度) 2022-04-01 – 2025-03-31
研究課題ステータス 交付 (2023年度)
配分額 *注記
4,680千円 (直接経費: 3,600千円、間接経費: 1,080千円)
2023年度: 2,080千円 (直接経費: 1,600千円、間接経費: 480千円)
2022年度: 2,600千円 (直接経費: 2,000千円、間接経費: 600千円)
キーワード2D materials device / Photonic crystal / Optics and photonics / photonic crystal / optics and photonics / Valley spin devices / semiconductor / layered material
研究開始時の研究の概要

In 2D semiconductors, the electron and holes possess coupled valley and spin properties which are referred to as valley spin. We propose the demonstration of valley spin devices by coupling 2D semiconductors to novel circularly polarized chiral photonic crystal nanocavities.

研究実績の概要

Using the photonic crystal (PhC) and 2D materials transfer technologies that we have developed previously, in this fiscal year, we have been focused on studying the self-aligned hybrid nanocavities. These hybrid nanocavities are formed by partially covering a photonic crystal waveguide post-fabrication with a suitably-sized 2D material flake. The presence of the flake increases the local refractive index causing a frequency mismatch of the optical fields in the regions with and without the flake results in the formation of a nanocavity. We successfully fabricated such hybrid nanocavity devices with hBN, WSe2 and MoTe2 flakes on silicon PhC waveguides.

現在までの達成度 (区分)
現在までの達成度 (区分)

1: 当初の計画以上に進展している

理由

In our hybrid nanocavity devices, we have obtained Q factors as high as 4.0×10^5. Remarkably, even monolayer flakes can provide sufficient local refractive index modulation to induce high Q nanocavity formation. We have also managed to observe cavity PL enhancement in a self-aligned MoTe2 cavity device, with a cavity Purcell enhancement factor of about 15. Our results highlight the potential of our devices to enhance light-matter coupling and to create functional optical devices.

今後の研究の推進方策

So far, we have fabricated hybrid nanocavities using a single flake per device. One of the key features of 2D materials is their amenability to heterogenous stacking i.e. stacking of 2D materials with different compositions and atomic lattices without having to worry about lattice matching. Such heterogeneous stacking has been used as encapsulation or passivation layer to sandwich and protect the 2D materials. Following from our results, our next step will be focused on coupling heterogenous stack of materials to the self-aligned hybrid nanocavities.

報告書

(2件)
  • 2023 実施状況報告書
  • 2022 実施状況報告書
  • 研究成果

    (5件)

すべて 2024 2023 2022

すべて 雑誌論文 (1件) (うち国際共著 1件、 査読あり 1件、 オープンアクセス 1件) 学会発表 (4件) (うち国際学会 3件)

  • [雑誌論文] Resonant exciton transfer in mixed-dimensional heterostructures for overcoming dimensional restrictions in optical processes2023

    • 著者名/発表者名
      Fang N.、Chang Y. R.、Yamashita D.、Fujii S.、Maruyama M.、Gao Y.、Fong C. F.、Otsuka K.、Nagashio K.、Okada S.、Kato Y. K.
    • 雑誌名

      Nature Communications

      巻: 14 号: 1 ページ: 8152-8159

    • DOI

      10.1038/s41467-023-43928-2

    • 関連する報告書
      2023 実施状況報告書
    • 査読あり / オープンアクセス / 国際共著
  • [学会発表] Emerging second-order nonlinearity in two-dimensional material functionalized silica microcavities2024

    • 著者名/発表者名
      Shun Fujii
    • 学会等名
      March Meeting of the American Physical Society
    • 関連する報告書
      2023 実施状況報告書
    • 国際学会
  • [学会発表] Intrinsically Circularly Polarized Modes Near Exceptional Points due to Symmetry Breaking in a H1 Photonic Crystal Cavity2023

    • 著者名/発表者名
      Chee Fai Fong
    • 学会等名
      International Conference on Nano-photonics and Nano-electronics (ICNN2023)
    • 関連する報告書
      2023 実施状況報告書
    • 国際学会
  • [学会発表] Nanocavity induced by atomically thin transition metal dichalcogenide in photonic crystal waveguide2023

    • 著者名/発表者名
      Chee Fai Fong
    • 学会等名
      JSAP-Optica Joint Symposia, the 84th JSAP Autumn Meeting 2023
    • 関連する報告書
      2023 実施状況報告書
    • 国際学会
  • [学会発表] Formation of heterocavity by deposition of hexagonal boron nitride flake on photonic crystal waveguide2022

    • 著者名/発表者名
      C.F. Fong, D. Yamashita, N. Fang, T. Taniguchi, K. Watanabe and Y. K. Kato
    • 学会等名
      JSAP-Optica Joint Symposia 2022
    • 関連する報告書
      2022 実施状況報告書

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公開日: 2022-04-19   更新日: 2024-12-25  

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