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キラル分子干渉センシング向きの連続体における束縛状態を用いた円偏光レーザー

研究課題

研究課題/領域番号 23KF0107
研究種目

特別研究員奨励費

配分区分基金
応募区分外国
審査区分 小区分21030:計測工学関連
研究機関東京大学

研究代表者

J・J Delaunay  東京大学, 大学院工学系研究科(工学部), 准教授 (80376516)

研究分担者 XING DI  東京大学, 大学院工学系研究科(工学部), 外国人特別研究員
研究期間 (年度) 2023-07-26 – 2026-03-31
研究課題ステータス 交付 (2023年度)
配分額 *注記
3,000千円 (直接経費: 3,000千円)
2025年度: 100千円 (直接経費: 100千円)
2024年度: 1,400千円 (直接経費: 1,400千円)
2023年度: 1,500千円 (直接経費: 1,500千円)
キーワードmetasurface / emission / polarization
研究開始時の研究の概要

An optical functional structure sustaining coherent chiral light emission at a low threshold of energy is proposed, fabricated, and characterized. The proposed structure is applied in a chiral detection scheme for use in chiral molecules pharmaceutical research.

研究実績の概要

Structures that support a bound-state-in-the-continuum (BIC) lasing mode on a photonic crystal were designed by simulation. These structures made of dielectric materials were patterned into nanocylinder arrays to support a resonance mode with a high-quality factor (quasi-BIC mode). Solution-processed quantum dots (QDs) were integrated on top of the nanocylinder array to form an isolated cavity. Due to the existence of side edges, the lasing mode is better confined within the cavity and shows lower scattering losses in the lateral direction. In summary, a single-mode BIC laser using CsPbBr3 QDs having a narrow linewidth of around 0.1 nm and a small footprint (10 × 10 μm^2) was demonstrated. This lasing structure is the smallest among the existing solution-processed BIC laser.

現在までの達成度 (区分)
現在までの達成度 (区分)

2: おおむね順調に進展している

理由

Cavity structures supporting BIC lasing mode have been designed. Direct fabrication of well-defined patterns of quantum dots (QDs) via a solution process was proposed to take advantage of the pattern edges to reduce losses through the cavity edges. A miniaturized BIC laser (10 × 10 μm^2) with a low threshold has been demonstrated. The results were published in Advanced Functional Materials a leading journal in the field of nanotechnology.

今後の研究の推進方策

We will break the symmetry of the employed nanostructures to produce a high Q factor chiral lasing emission. For this purpose, simulations and experimental verifications will be used to design and optimize the chiral structure. To characterize the experimental result, an angle-resolved spectrometer will be built. This setup can characterize the polarization properties of the far field emission in off normal direction. Finally, a chiral emission with a high Q factor will be demonstrated.

報告書

(1件)
  • 2023 実施状況報告書
  • 研究成果

    (1件)

すべて 2024

すべて 雑誌論文 (1件) (うち国際共著 1件、 査読あり 1件、 オープンアクセス 1件)

  • [雑誌論文] Solution‐Processed Perovskite Quantum Dot Quasi‐BIC Laser from Miniaturized Low‐Lateral‐Loss Cavity2024

    • 著者名/発表者名
      Xing Di、Chen Mu‐Hsin、Wang Zhiyu、Deng Chih‐Zong、Ho Ya‐Lun、Lin Bo‐Wei、Lin Cheng‐Chieh、Chen Chun‐Wei、Delaunay Jean‐Jacques
    • 雑誌名

      Advanced Functional Materials

      巻: 2314953 号: 26 ページ: 1-8

    • DOI

      10.1002/adfm.202314953

    • 関連する報告書
      2023 実施状況報告書
    • 査読あり / オープンアクセス / 国際共著

URL: 

公開日: 2023-07-27   更新日: 2024-12-25  

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