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2022 年度 実績報告書

Superfluorescence, free-induction decay, and four-wave mixing: experimental and numerical studies of the propagation of free-electron laser pulses through dense atomic/ionic media

研究課題

研究課題/領域番号 19K12636
研究機関国立研究開発法人量子科学技術研究開発機構

研究代表者

HARRIES JAMES  国立研究開発法人量子科学技術研究開発機構, 関西光科学研究所 放射光科学研究センター, 上席研究員 (30416383)

研究分担者 久間 晋  国立研究開発法人理化学研究所, 開拓研究本部, 専任研究員 (50600045)
研究期間 (年度) 2019-04-01 – 2023-03-31
キーワードFEL / 超蛍光 / ヘリウム / 量子光学
研究実績の概要

In the final year of this project we successfully carried out an experiment using soft X-ray free-electron laser pulses to ionise a dense sample of helium gas and directly observe the time profiles of pulses of superfluorescence at wavelengths of 469 nm and 164 nm following excitation of the dense sample of ions to the 3p state (164 nm emission only) and 4p state (emission at 469 nm followed by emission at 164 nm). The pulses at a wavelength of 469 nm were detected using a bandpass filter and a fast photodiode, those at a wavelength of 164 nm using a grazing-incidence monochromator and a fast micro-channel plate detector with a response time of around 100 ps. We were successful in confirming for the first time directly that the emission at 164 nm is indeed superfluorescence, and studied the dependence of the timing of the pulses on helium number density. We also studied the correlation between the emitted pulses at the two different wavelengths following excitation of the 4p ion state, revealing the longer delay of the emission for the 4p-3s-2p cascade. Due to the difficulty of aligning the system and the limited beamtime we were unable to conduct the measurements for the shorter wavelength transitions.

In parallel to the superfluorescence from helium ions experiment we continued to develop an apparatus for creating a beam of superfluid helium droplets, which will provide a sample of helium at densities equivalent to the bulk. Successful operation of the source was demonstrated, and attempts to observe superfluorescence from the droplets will be made in future experiments.

  • 研究成果

    (2件)

すべて 2022

すべて 学会発表 (2件) (うち国際学会 1件)

  • [学会発表] Photoionisation and excitation of dense samples of helium gas using an XFEL: superfluorescence at EUV wavelengths2022

    • 著者名/発表者名
      James Harries, Arisa Iguchi, Hiroshi Iwayama, Susumu Kuma
    • 学会等名
      IWP-RIXS 2022
    • 国際学会
  • [学会発表] A new superfluid liquid helium droplet machine2022

    • 著者名/発表者名
      James Harries, Arisa Iguchi, Susumu Kuma
    • 学会等名
      原子衝突学会第47回年会

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公開日: 2023-12-25  

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