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2020 年度 実績報告書

Fatigue behavior and underlying mechanism of tough and self-healing hydrogels

研究課題

研究課題/領域番号 19K23617
研究機関北海道大学

研究代表者

崔 昆朋  北海道大学, 化学反応創成研究拠点, 特任助教 (30843198)

研究期間 (年度) 2019-08-30 – 2021-03-31
キーワードTough and self-healing / hydrogels / fatigue resistance / phase contrast
研究実績の概要

In the past year, we studied the effect of phase contrast on the fatigue behavior of tough and self-healing polyampholyte (PA) hydrogels. We found that with a strong phase contrast, the stress singularity around the crack tip is gradually eliminated with the fatigue cycle, suppressing the fast crack growth; while stress concentration always exists in weak phase contrast samples, resulting in weak fatigue-resistance. The clarified role of mesoscale structure on fatigue resistance provides design principles for developing self-healing, tough, and fatigue resistant soft materials. In addition, we also used hydrogels to achieve dynamic memories with spontaneous but learning-strength-dependent forgetting ability by using nonequilibrium structure transformation, in analogy to the human brain.

  • 研究成果

    (10件)

すべて 2021 2020

すべて 雑誌論文 (8件) (うち国際共著 4件、 査読あり 8件) 学会発表 (2件) (うち招待講演 2件)

  • [雑誌論文] Effect of Mesoscale Phase Contrast on Fatigue-Delaying Behavior of Self-Healing Hydrogels2021

    • 著者名/発表者名
      Li Xueyu, Cui Kunpeng, Kurokawa Takayuki, Ye Ya Nan, Sun Tao Lin, Yu Chengtao, Creton Costantino, and Gong Jian Ping
    • 雑誌名

      Science Advance

      巻: - ページ: -

    • 査読あり / 国際共著
  • [雑誌論文] Molecular mechanism of abnormally large nonsoftening deformation in a tough hydrogel2021

    • 著者名/発表者名
      Ye Ya Nan、Cui Kunpeng、Hong Wei、Li Xueyu、Yu Chengtao、Hourdet Dominique、Nakajima Tasuku、Kurokawa Takayuki、Gong Jian Ping
    • 雑誌名

      Proceedings of the National Academy of Sciences

      巻: 118 ページ: --

    • DOI

      10.1073/pnas.2014694118

    • 査読あり / 国際共著
  • [雑誌論文] Aggregated structures and their functionalities in hydrogels2021

    • 著者名/発表者名
      Cui Kunpeng, Gong Jian Ping
    • 雑誌名

      Aggregate

      巻: - ページ: -

    • 査読あり
  • [雑誌論文] Constitutive modeling of bond breaking and healing kinetics of physical Polyampholyte (PA) gel2021

    • 著者名/発表者名
      Venkata Sairam Pamulaparthi、Cui Kunpeng、Guo Jingyi、Zehnder Alan T.、Gong Jian Ping、Hui Chung-Yuen
    • 雑誌名

      Extreme Mechanics Letters

      巻: 43 ページ: 101184~101184

    • DOI

      10.1016/j.eml.2021.101184

    • 査読あり / 国際共著
  • [雑誌論文] Constitutive modeling of strain-dependent bond breaking and healing kinetics of chemical polyampholyte (PA) gel2021

    • 著者名/発表者名
      Pamulaparthi Venkata Sairam、Cui Kunpeng、Guo Jingyi、Zehnder Alan T.、Gong Jian Ping、Hui Chung-Yuen
    • 雑誌名

      Soft Matter

      巻: - ページ: -

    • DOI

      10.1039/D1SM00110H

    • 査読あり / 国際共著
  • [雑誌論文] Stress Relaxation and Underlying Structure Evolution in Tough and Self-Healing Hydrogels2020

    • 著者名/発表者名
      Cui Kunpeng、Ye Ya Nan、Yu Chengtao、Li Xueyu、Kurokawa Takayuki、Gong Jian Ping
    • 雑誌名

      ACS Macro Letters

      巻: 9 ページ: 1582~1589

    • DOI

      10.1021/acsmacrolett.0c00600

    • 査読あり
  • [雑誌論文] Phase Separation Behavior in Tough and Self-Healing Polyampholyte Hydrogels2020

    • 著者名/発表者名
      Cui Kunpeng、Ye Ya Nan、Sun Tao Lin、Yu Chengtao、Li Xueyu、Kurokawa Takayuki、Gong Jian Ping
    • 雑誌名

      Macromolecules

      巻: 53 ページ: 5116~5126

    • DOI

      10.1021/acs.macromol.0c00577

    • 査読あり
  • [雑誌論文] Hydrogels as dynamic memory with forgetting ability2020

    • 著者名/発表者名
      Yu Chengtao、Guo Honglei、Cui Kunpeng、Li Xueyu、Ye Ya Nan、Kurokawa Takayuki、Gong Jian Ping
    • 雑誌名

      Proceedings of the National Academy of Sciences

      巻: 117 ページ: 18962~18968

    • DOI

      10.1073/pnas.2006842117

    • 査読あり
  • [学会発表] Tough and self-healing hydrogels composed of polyampholytes2020

    • 著者名/発表者名
      Cui Kunpeng, Gong Jian Ping
    • 学会等名
      35th Summer University in Hokkaido
    • 招待講演
  • [学会発表] Phase Separation Behavior in Tough Polyampholyte Hydrogels2020

    • 著者名/発表者名
      Cui Kunpeng, Kurokawa Takayuki, Gong Jian Ping
    • 学会等名
      第69回高分子討論会
    • 招待講演

URL: 

公開日: 2021-12-27  

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