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2021 年度 実施状況報告書

Designing high-performance thermoelectrics in low-dimensional materials

研究課題

研究課題/領域番号 20K15178
研究機関東北大学

研究代表者

NGUYEN TUANHUNG  東北大学, 学際科学フロンティア研究所, 助教 (10844425)

研究期間 (年度) 2020-04-01 – 2023-03-31
キーワードThermoelectricity / DFT calculations / 2D materials / Photovoltaics
研究実績の概要

In this fiscal year, we reported that the thermoelectric (TE) performance is enhanced by the unique density of states of a topological type-II nodal-line semimetal (NLS). We found that the Seebeck coefficient of the type-II NLS at the nodal-line region can be higher than the upper limit of the metal. On the other hand, the linear band of the type-II NLS also contributes to high electrical conductivity. Therefore, the type-II NLS shows a high-performance TE material among metals and semimetals, which are traditionally considered inadequate TE materials compared to semiconductors. We also reported other energy topics, such as the low-power consumption device based on the periodically doped graphene nanoribbon or the optical properties of two-dimensional materials.

現在までの達成度 (区分)
現在までの達成度 (区分)

2: おおむね順調に進展している

理由

Our progress is going on as planned, in which we have focused on the thermoelectricity of the topological semimetals for this fiscal year. There are two published papers on thermoelectricity. On the other hand, we also studied other energy topics for the two-dimensional materials, in which four related papers have been published.

今後の研究の推進方策

In the next fiscal year, we will study the generation of a transverse heat current upon applying an electric field in the presence of a magnetic field, so-called the thermoelectric Hall effect. Although thermoelectricity is promising for the Internet of Things (IoT) device by generating electricity from waste heat, room-temperature thermoelectricity has been a long-standing challenge to obtain high energy conversion efficiency. The thermoelectric Hall effect might offer a new avenue to obtaining high thermoelectric efficiency.

次年度使用額が生じた理由

In this fiscal year, some international conferences have been still canceled under the influence of Covid-19. Therefore, the travel expenses did not use. The incurring amount in the next fiscal year will be used to buy the workstation for calculations.

  • 研究成果

    (8件)

すべて 2022 2021

すべて 雑誌論文 (6件) (うち国際共著 6件、 査読あり 6件、 オープンアクセス 1件) 学会発表 (2件) (うち国際学会 1件)

  • [雑誌論文] Enhanced thermoelectric performance by van Hove singularities in the density of states of type-II nodal-line semimetals2022

    • 著者名/発表者名
      Nguyen T. Hung、Jyesta M. Adhidewata、Ahmad R. T. Nugraha、Riichiro Saito
    • 雑誌名

      Physical Review B

      巻: 105 ページ: 115142-1~5

    • DOI

      10.1103/PhysRevB.105.115142

    • 査読あり / 国際共著
  • [雑誌論文] Complex Raman tensor in helicity-changing Raman spectra of black phosphorus under circularly polarized light2022

    • 著者名/発表者名
      Shiyi Han、Yan Zhao、Nguyen T. Hung、Bo Xu、Riichiro Saito、Jin Zhang、Lianming Tong
    • 雑誌名

      The Journal of Physical Chemistry Letters

      巻: 13 ページ: 1241~1248

    • DOI

      10.1021/acs.jpclett.1c03826

    • 査読あり / 国際共著
  • [雑誌論文] Effects of strain and electric field on electronic and optical properties of monolayer γ-GeX (X = S, Se and Te)2022

    • 著者名/発表者名
      Vuong V. Thanh、Nguyen V. Duy、Do V. Truong、Nguyen T. Hung
    • 雑誌名

      Applied Surface Science

      巻: 582 ページ: 152321~152321

    • DOI

      10.1016/j.apsusc.2021.152321

    • 査読あり / 国際共著
  • [雑誌論文] Electronic, optical, and thermoelectric properties of bulk and monolayer germanium tellurides2021

    • 著者名/発表者名
      Wenny V. Sinambela、Sasfan A. Wella、Fitri S. Arsyad、Nguyen T. Hung、Ahmad R. T. Nugraha
    • 雑誌名

      Crystals

      巻: 11 ページ: 1290~1290

    • DOI

      10.3390/cryst11111290

    • 査読あり / オープンアクセス / 国際共著
  • [雑誌論文] Switching behavior of a heterostructure based on periodically doped graphene nanoribbon2021

    • 著者名/発表者名
      Sake Wang、Nguyen T. Hung、Hongyu Tian、Md Shafiqul Islam、Riichiro Saito
    • 雑誌名

      Physical Review Applied

      巻: 16 ページ: 024030-1~10

    • DOI

      10.1103/PhysRevApplied.16.024030

    • 査読あり / 国際共著
  • [雑誌論文] Selection rule for Raman spectra of two-dimensional materials using circularly-polarized vortex light2021

    • 著者名/発表者名
      Riichiro Saito、Muhammad S. Ukhtary、Sake Wang、Nguyen T. Hung
    • 雑誌名

      Physical Chemistry Chemical Physics

      巻: 23 ページ: 17271~17278

    • DOI

      10.1039/D1CP02209A

    • 査読あり / 国際共著
  • [学会発表] Thermoelectric energy conversion of 3D topological insulators2022

    • 著者名/発表者名
      Nguyen Tuan Hung
    • 学会等名
      The 62th FullerenesNanotubes-Graphene General Symposium
  • [学会発表] The origin of quantum effects in low‐dimensional thermoelectric materials2021

    • 著者名/発表者名
      Nguyen Tuan Hung
    • 学会等名
      NT21: International Conference on the Science and Application of Nanotubes and Low- Dimensional Materials, On-line by Zoom
    • 国際学会

URL: 

公開日: 2022-12-28  

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