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2011 Fiscal Year Final Research Report

Quantum Frustration

Planned Research

  • PDF
Project AreaNovel States of Matter Induced by Frustration
Project/Area Number 19052004
Research Category

Grant-in-Aid for Scientific Research on Priority Areas

Allocation TypeSingle-year Grants
Review Section Science and Engineering
Research InstitutionKyoto University

Principal Investigator

KAGEYAMA Hiroshi  京都大学, 大学院・工学研究科, 教授 (40302640)

Co-Investigator(Kenkyū-buntansha) UEDA Yutaka  東京大学, 物性研究所, 教授 (20127054)
MASUDA Takatsugu  東京大学, 物性研究所, 教授 (90313014)
KAKURAI Kazuhisa  日本原子力研究開発機構, 量子ビーム応用研究部門, 副部門長・上級研究主席 (00204339)
KAWASHIMA Naoki  東京大学, 物性研究所, 准教授 (30242093)
Project Period (FY) 2007 – 2011
Keywordsフラストレーション / 量子スピン / 低次元 / 新物質 / 量子相転移
Research Abstract

We have found various exotic quantum phenomena in 1D, 2D and 3D quantum frustrated systems, derived from competing antiferromagnetic and ferromagnetic interactions. 2D systems (CuX)An-1BnO_<3n+1> show novel phases such as a ferromagnetic Shastry-Sutherland spin singlet state ((CuCl)LaNb2O7) and a quantized magnetization state ((CuBr)Sr_2Nb_3O_<10>), and quantum phase separation. 1D system LiCuVO_4 exhibits an unprecedented magnetic state related to nematic state. 3D K_2Cr_8O_<16> exhibits a ferromagnetic metal to ferromagnetic insulator transition that is explained in terms of Peierls mechanism, and a theoretically predicted random fan out state is realized in Sr(Fe,Mn)O_2.

  • Research Products

    (41 results)

All 2011 2010 2009 2008 2007 Other

All Journal Article (27 results) (of which Peer Reviewed: 23 results) Presentation (13 results) Remarks (1 results)

  • [Journal Article] Spin Density Wave in Insulating Ferromagnetic Frustrated Chain LiCuVO42011

    • Author(s)
      T. Masuda, (5名、1番目)
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 80 Pages: 113705/1-113705/4

    • DOI

      DOI:10.1143/JPSJ.80.113705.

    • Peer Reviewed
  • [Journal Article] Magnetic properties of frustrated pyrochlore fluorides Cd_2M_2F_6S (M = Fe, Co, and Ni)2011

    • Author(s)
      H. Ueda, Y. Ueda, (5名、5番目)
    • Journal Title

      Phys. Rev.

      Volume: B84 Pages: 214411/1-214411/7

    • DOI

      DOI:10.1103/PhysRevB.84.214411.

    • Peer Reviewed
  • [Journal Article] Peierls Mechanism of the Metal-Insulator Transition in Ferromagnetic Hollandite K2Cr_8O_162011

    • Author(s)
      T. Toriyama, Y. Ueda,(12名、7番目)
    • Journal Title

      Phys. Rev. Lett.

      Volume: 107 Pages: 266402/1-266402/5

    • DOI

      DOI:0.1103/PhysRevLett.107.266402.

    • Peer Reviewed
  • [Journal Article] Random fan-out state induced by site-random interlayer couplings2011

    • Author(s)
      Ryo Tamura, Naoki Kawashima, Hiroshi Kageyama(5名、2番目:川島、5番目:陰山)
    • Journal Title

      Phys. Rev.

      Volume: 84 Pages: 214408/1-214408/11

    • DOI

      DOI:10.1103/PhysRevB.84.214408.

    • Peer Reviewed
  • [Journal Article] ToF inelastic neutron scattering studies on quantum spin systems (CuCl)LaB_2O_7 (B = Nb, Ta)2011

    • Author(s)
      S. Ohira-Kawamura, H. Kageyama, K. Kakurai
    • Journal Title

      Journal of Physics: Conference Series

      Volume: 320 Pages: 012037/1-012037/5

    • DOI

      DOI:10.1088/1742-6596/320/1/012037.

    • Peer Reviewed
  • [Journal Article] First Single-Crystal Synthesis and Low Temperature Structural Determination of the Quasi-2D Quantum Spin Compound (CuCl)LaNb_2O_72011

    • Author(s)
      Olivier J. Hernandez, Hiroshi Kageyama(10名、9番目
    • Journal Title

      Dalton Trans

      Volume: 40 Pages: 4065-4613

    • DOI

      DOI:10.1039/C0DT01665A.

    • Peer Reviewed
  • [Journal Article] Ferromagnetically Coupled Shastry-Sutherland Quantum Spin Singlets in (CuCl)LaNb_2O_72011

    • Author(s)
      C. Tassel, H. Kageyama,(12名、11番目)
    • Journal Title

      Phys. Rev. Lett.

      Volume: 105 Pages: 167205/1-4

    • DOI

      DOI: 10.1103/PhysRevLett.105.167205.

  • [Journal Article] Two-Dimensional S=1 Quantum Antiferromagnet (NiCl)Sr_2Ta_3O_1O2010

    • Author(s)
      Atsushi Kitada, Hiroshi Kageyama (13名、13番目)
    • Journal Title

      Chem. Mater.

      Volume: 22 Pages: 4625-4631

    • DOI

      DOI: 10.1021/cm100660v.

    • Peer Reviewed
  • [Journal Article] Structural and Magnetic Properties of the Oxyborate Co_5Ti(O_2BO_3)2 D.2010

    • Author(s)
      C. Freitas, H. Kageyama,(12名、8番目)
    • Journal Title

      Phys. Rev.

      Volume: B81 Pages: 024432/1-024432/7

    • DOI

      DOI:10.1103/PhysRevB.81.024432.

  • [Journal Article] Instability of magnons in two-dimensional antiferromagnets at high magnetic fields2010

    • Author(s)
      T. Masuda,(9名、1番目)
    • Journal Title

      Phys. Rev.

      Volume: B81(10) Pages: 100402(R)/1-100402(R)/4

    • DOI

      DOI:10.1103/physRevB.81.100402.

    • Peer Reviewed
  • [Journal Article] Universal Magnetic Structure of the Half-Magnetization Phase in Cr-Based Spinels2010

    • Author(s)
      M. Matsuda, Y. Ueda
    • Journal Title

      Phys. Rev . Lett.

      Volume: 104 Pages: 047201/1-047201/4

    • DOI

      DOI:10.1103/PhysRevLett.104.047201.

    • Peer Reviewed
  • [Journal Article] Magnetic properties of the spin-1/2 XXZ model on the Shastry-Sutherland lattice: Effect of long-rangeinteractions2009

    • Author(s)
      Takahumi Suzuki, Naoki Kawashima (3名、3番目)
    • Journal Title

      Phys. Rev.

      Volume: B80 Pages: 180405(R)(1-4)

    • DOI

      DOI:10.1103/PhysRevB.80.180405.

    • Peer Reviewed
  • [Journal Article] Muon Spin Relaxation Studies of the FrustratedQuasi-Two-Dimensional Square-Lattice Spin System Cu(Cl, Br)La(Nb, Ta)_2O_7 : Evolution from Spin-Gap to Antiferromagnetic State2009

    • Author(s)
      Y. J. Uemura, H. Kageyama(18名、18番目)
    • Journal Title

      Phys. Rev.

      Volume: B80 Pages: 174408/1-174408/12

    • DOI

      DOI:10.1103/PhysRevB.80.174408

    • Peer Reviewed
  • [Journal Article] Discovery of Ferromagnetic-Half-Metal-to-Insulator Transition in K_2Cr_8O_<16>2009

    • Author(s)
      K. Hasegawa, Y. Ueda(9名、9番目)
    • Journal Title

      Phys. Rev. Lett.

      Volume: 103(14) Pages: 146403/1-146403/4

    • DOI

      DOI:10.1103/PhysRevLett.103.146403.

    • Peer Reviewed
  • [Journal Article] 15.Spin Transition in a Four-Coordinate Iron Oxide2009

    • Author(s)
      T. Kawakami, Y. Tsujimoto, H. Kageyama ,(18名、3番目)
    • Journal Title

      Nature Chemistry

      Volume: 1(August) Pages: 371-376

    • DOI

      DOI:10.1038/nchem.289

    • Peer Reviewed
  • [Journal Article] 16.Direct Mapping of the Finite Temperature Phase Diagram of Strongly Correlated Quantum Models2009

    • Author(s)
      Qi Zhou, Naoki Kawashima,(4名、3番目)
    • Journal Title

      Phys. Rev. Lett.

      Volume: 103(8) Pages: 085701/1-085701/4

    • DOI

      DOI:10.1103/PhysRevLett.103.085701.

    • Peer Reviewed
  • [Journal Article] Weakly Coupled s = 1/2 Quantum Spin Singlets in Ba_3Cr_2O_82009

    • Author(s)
      M. Kofu, Y. Ueda(8名、8番目)
    • Journal Title

      Phys. Rev. Lett.

      Volume: 102(3) Pages: 037206/1-037206/4

    • DOI

      DOI:10.1103/PhysRevLett.102.037206.

  • [Journal Article] Longitudinal Spin Density Wave Order in a Quasi-1DIsing-like Quantum Antiferro magnet2008

    • Author(s)
      S. Kimura, T. Masuda,(13名、3番目)
    • Journal Title

      Phys. Rev. Lett.

      Volume: 101(20) Pages: 207201/1-207201/4

    • DOI

      DOI:10.1103/PhysRevLett.101.207201.

    • Peer Reviewed
  • [Journal Article] First-Order Transition to Incommensurate Phase with Broken Lattice Rotation Symmetry in Frustrated Heisenberg Model2008

    • Author(s)
      R. Tamura and N. Kawashima
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 77(10) Pages: 103002(1-4)

    • DOI

      DOI:10.1143/JPSJ.77.103002.

    • Peer Reviewed
  • [Journal Article] 平面正方FeO_4ユニットが導く新しい酸化物-無限層構造から梯子構造まで-2008

    • Author(s)
      陰山洋, (3名、1番目)
    • Journal Title

      固体物理

      Volume: 43 Pages: 67-76

  • [Journal Article] Magnetic Excitation in Artificially Designed Oxygen Molecule Magnet2008

    • Author(s)
      T. Masuda, (4名、1番目)
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 77(8) Pages: 083703/1-083703/4

    • DOI

      DOI:10.1143/JPSJ.77.083703.

    • Peer Reviewed
  • [Journal Article] NMR Evidence for the Persistence of Spin-Superlattice above the 1/8 Magnetization Plateau in SrCu_2(BO_3)22008

    • Author(s)
      M. Takigawa, H. Kageyama, and Y. Ueda,(6名、5番目:陰山、6番目:上田)
    • Journal Title

      Phys. Rev. Lett.

      Volume: 101(3) Pages: 037202-1-037202-4

    • DOI

      DOI:10.1103/PhysRevLett.101.037202.

    • Peer Reviewed
  • [Journal Article] Sharp Peaks in the Momentum Distribution of Bosons in Optical Lattices in the Normal State2008

    • Author(s)
      Y. Kato, N. Kawashima, (4名、3番目)
    • Journal Title

      Nature Physics

      Volume: 4(August) Pages: 617-621

    • DOI

      DOI:10.1038/nphys983.

    • Peer Reviewed
  • [Journal Article] Pressure-EnhancedDirectExchangeCouplingsin Chromium Spinels2008

    • Author(s)
      H. Ueda and Y. Ueda
    • Journal Title

      Phys. Rev.

      Volume: B77(22) Pages: 224411/1-224411/6

    • DOI

      DOI:10.1103/PhysRevB.77.224411

    • Peer Reviewed
  • [Journal Article] Successive Phase Transitions of LuBaCo_4O_7 with Kagome and Triangular Lattices2007

    • Journal Title

      M. Soda, K. Kakurai(5名、5番目)

      Volume: 76(No.8) Pages: 084701/1-084701/6

    • DOI

      DOI:10.1143/JPSJ.76.084701.

    • Peer Reviewed
  • [Journal Article] Infinite-layer iron oxide with a square-planar coordination2007

    • Author(s)
      Y.Tsujimoto, H.Kageyama, (10名、5番目)
    • Journal Title

      Nature

      Volume: 450(Dec.13) Pages: 1062-1065

    • DOI

      DOI:10.1038/nature06382.

    • Peer Reviewed
  • [Journal Article] Magnetic and Structural Studies of the Quasi-Two-Dimensional Spin Gap System (CuCl)LaNb_2O_72007

    • Author(s)
      M.Yoshida, H.Kageyama,(9名、7番目)
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 76(10) Pages: 104703/1-104703/9

    • DOI

      DOI:10.1143/JPSJ.76.104703

    • Peer Reviewed
  • [Presentation]2011

    • Author(s)
      Naoki Kawashima
    • Organizer
      Quantum Monte Carlo and Non-Ginzburg-Landau Type Phase Transition NTU Colloquium
    • Place of Presentation
      NTU(台北)
    • Year and Date
      2011-12-27
  • [Presentation] Spin nematic correlation in frustrated ferromagnetic chain2011

    • Author(s)
      益田隆嗣
    • Organizer
      ICC-IMR Workshop on Novel Material Science by Neutron Scattering-Polarization Analysis &Cross-CorrelationMethod
    • Place of Presentation
      東北大学金属研究所(宮城県)
    • Year and Date
      2011-11-18
  • [Presentation] 酸素の通り道 : ペロブスカイトを舞台とした低温反応2011

    • Author(s)
      陰山洋
    • Organizer
      計算物質科学研究センター第1回シンポジウム~『京』と大型実験施設の連携に向けて~
    • Place of Presentation
      東京大学物性研究所(千葉県)
    • Year and Date
      2011-09-13
  • [Presentation] 計算物性物理学のいくつかのトピックス2011

    • Author(s)
      川島直輝
    • Organizer
      物性研究所計算物質科学研究センター第1回シンポジウム
    • Place of Presentation
      東京大学物性研究所(千葉県)
    • Year and Date
      2011-09-12
  • [Presentation] Hollandites: K2M8O16 (M = Ti, V, Cr, Mn)-a novel class of oxides with unusual properties2011

    • Author(s)
      Yutaka Ueda
    • Organizer
      Tokyo-Cologne Workshop on Strongly Correlated Transition-Metal Compounds
    • Place of Presentation
      ケルン(ドイツ)
    • Year and Date
      2011-09-09
  • [Presentation] ソフト化学による酸化物の構造・機能制御2011

    • Author(s)
      陰山洋
    • Organizer
      日本セラミックス協会関西支部第6回学術講演会
    • Place of Presentation
      イーグレ姫路(兵庫県)
    • Year and Date
      2011-07-29
  • [Presentation] Monte Carlo Simulations on Deconfined Critical Phenomena2011

    • Author(s)
      Naoki Kawashima
    • Organizer
      ICTP Workshop on Synergies between Field Theory and Exact Computational Methods in Strongly Correlated Quantum Matter
    • Place of Presentation
      トリエステ(イタリア)
    • Year and Date
      2011-07-25
  • [Presentation] Monte Carlo Simulations on Deconfined Critical Phenomena2011

    • Author(s)
      Naoki Kawashima
    • Organizer
      Komaba Seminar
    • Place of Presentation
      東京大学駒場キャンパス(東京都)
    • Year and Date
      2011-07-22
  • [Presentation] Mixed State and Novel Transitions in Quasi-2D Frustrated Magnets2011

    • Author(s)
      Naoki Kawashima
    • Organizer
      MEXT/CIFAR Program on Frustrated Magnetic and Other Systems
    • Place of Presentation
      Coast Plaza Hotel, Vancouver(カナダ)
    • Year and Date
      2011-05-31
  • [Presentation] 物性物理学における量子モンテカルロ法の応用2011

    • Author(s)
      川島直輝
    • Organizer
      計算分子科学研究拠点第1回研究会
    • Place of Presentation
      岡崎自然科学研究機構分子科学研究所
    • Year and Date
      2011-02-05
  • [Presentation] Sqaure Planar Coordination in Iron Oxide Explore the Old and Create2008

    • Author(s)
      陰山洋
    • Organizer
      the New International Institute for Advanced Studies
    • Year and Date
      2008-11-12
  • [Presentation] Polarized neutron scattering investigation of non-collinear magnetic ground State2007

    • Author(s)
      K. Kakurai, M. Takeda, M. Nakamura, A. Oosawa, M. Matsuda, S. Wakimoto, Y. Shimojo, E. Lelievre-Berna, F. Tasset, L.-P. Regnault
    • Organizer
      Nagoya International Symposium on Science of Molecular Assembly and Biomolecular Systems
    • Place of Presentation
      名古屋大学
    • Year and Date
      2007-11-30
  • [Presentation] 新しい低次元量子スピン系の合成と磁性研究2007

    • Author(s)
      陰山洋
    • Organizer
      日本物理学会秋季大会
    • Place of Presentation
      北海道大学
    • Year and Date
      2007-09-23
  • [Remarks]

    • URL

      http://www.frustration.jp/modules/contents/index.php?content_id=6

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Published: 2013-07-31   Modified: 2018-07-30  

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