2004 Fiscal Year Final Research Report Summary
Investigation of Tropospheric Ozone Production in Association with Biomass Burning in Southeast Asia
Project/Area Number |
13480153
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Research Category |
Grant-in-Aid for Scientific Research (B)
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Allocation Type | Single-year Grants |
Section | 一般 |
Research Field |
Environmental dynamic analysis
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Research Institution | Ibaraki University (2002-2004) The University of Tokyo (2001) |
Principal Investigator |
KITA Kazuyuki Ibaraki University, Faculty of Science, Associate professor, 理学部, 助教授 (30221914)
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Co-Investigator(Kenkyū-buntansha) |
WATANABE Takashi Ibaraki University, Faculty of Science, Professor, 理学部, 教授 (10023681)
NOZAWA Satoshi Ibaraki University, Graduate school of Sciences and Technology, Research Associate, 理工学研究科, 助手 (10261736)
KONDO Yutaka University of Tokyo, Research center for advanced science and technology, Professor, 先端科学技術研究センター, 教授 (20110752)
KOIKE Makoto University of Tokyo, Graduate school of Sciences, Associate Professor, 大学院・理学系研究科, 助教授 (00225343)
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Project Period (FY) |
2001 – 2004
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Keywords | ozone / biomass burning / Southeast Asia / El Nino / greenhouse effect / troposphere |
Research Abstract |
Tropospheric ozone is significant for global atmospheric environment because it can damage human health and vegetation including agricultural crops. It also affects climate because is one of significant greenhouse gases. However, the ozone distribution, its budget, and therefore, its influence on the environment have not been fully understood. In this study, the influence of the biomass burning in Southeast Asia on the production of the tropospheric ozone is discussed. This study consists of three parts : (I)ozone variation observed during the BIBLE aircraft observation campaigns and influence of biomass burning in the Indonesian region, (II)ozone increased layers observed during the TRACE-P aircraft observation campaign and influence of biomass burning in the Indochina region, and (III)ozone variation over Indochina observed by an intensive ozonezonde observation and influence of biomass burning in the Indochina region. During BIBLE, mixing ratios of O_3 and its precursor gases (OPG) w
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ere quite low over the tropical Pacific Ocean. In the upper troposphere, OPG gradually increased downwind in eastern and western Indonesia. While O_3 did not increased over Indonesia, it increased by 50 % in the air masses which passed over Indonesia and were observed in Indian Ocean and northern Australia. These results indicate that ozone was produced in the air masses affected by emissions and convection over Indonesia. Average O_3 production rate during transport is estimated to be about 2ppbv/day, being comparable with the photochemical model calculation. These results demonstrate that the convection over Indonesia in association with biomass burning and lightning influenced OPG amount over Indonesia, even when biomass burning was inactive, and that it caused 10-15 ppbv (about 50 %) increase of O_3 over Indian Ocean and northern Australia. During TRACE-P, increase of ozone and OPG was often observed at the altitude around 4 km over western and central Pacific in subtropical latitude at about 20N. Trajectory analyses and collation analyses between OPG and tracers indicate that this increase of ozone and OPG were attributed to the biomass burning in the Indochina region. An intensive ozonesonde observation was carried out at Sri Samrong (17N, 99E), Thailand, between March and June, 2003. Observed ozone mixing ratios generally exceeded 60 ppbv and sometimes exceeded 90 ppbv throughout the troposphere. There was a stable inversion layer at an altitude around 4 km over Thailand during the observation period, indicating that ozone precursors emitted from biomass burning and industrial activities were upwardly transported up to this layer. However, ozone mixing ratios did not show significant variation above and below this layer. Meteorological analyses combined with analyses of aerosol characteristics indicated that biomass burning in Southeast Asia was not only a dominant ozone source, but also the pollutant from South Asia and the transport from the middle latitude contributed to the high ozone concentrations, even below the inversion layer. Less
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Research Products
(16 results)
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[Journal Article] Carbonyl sulfide (OCS) and carbon disulfide (CS2) : Large scale distributions over the Western Pacific and emissions from Asia during TRACE-P2004
Author(s)
N.J.Blake, D.G.Streets, J.-H.Woo, I.J.Simpson, J.Green, S.Meinardi, K.Kita, E.Atlas, H.E.Huelberg, G.Sachse, M.A.Avery, S.A.Vay, R.W.Talbot, J.E.Dibb, A.R.Bandy, D.C.Thornton, F.S.Rowland, D.R.Blake
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Journal Title
J.Geophys.Res. 108
Pages: 8806, doi:10.1029/2003JD004259R
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Impacts of Biomass Burning in Southeast Asia on Ozone and Reactive Nitrogen over the Western Pacific in Spring2004
Author(s)
Y.Kondo, Y.Morino, N.Takegawa, M.Koike, K.Kita, Y.Miyazaki, G.W.Sachse, S.A.Vay, M.A.Avery, F.Flocke, A.J.Weinheimer, F.L.Eisele, M.A.Zondlo, R.J.Weber, H.B.Singh, G.Chen, J.Crawford, D.R.Blake, H.E.Fuelberg, A.D.Clarke, R.W.Talbot, S.T.Sandholm, E.V.Browell, D.G.Streets, B.Liley
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Journal Title
J.Geophys.Res. 109
Pages: 10.1029/2003JD004203
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Photochemical production of ozone in the upper troposphere in association with cumulus convection over Indonesia.2003
Author(s)
K.Kita, S.Kawakami, Y.Miyazaki, Y.Higashi, Y.Kondo, N.Nishi, M.Koike, D.R.Blake, T.Machida, T.Sano, W.Hu, M.Ko, T.Ogawa
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Journal Title
J.Geophys.Res. 108
Pages: 8400, doi:10.1029/2001JD000844
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Effects of biomass burning, lightning, and convection on O3, CO, and NOy over the tropical Pacific and Australia in August-October.2003
Author(s)
Y.Kondo, M.Koike, K.Kita, H.Ikeda, N.Takegawa, I.Bey, D.J.Jacob, S.Kawakami, D.Blake, S.C.Liu, M.Ko, H.Irie, Y.Miyazaki, Y.Higashi, B.Liley, N.Nishi, Y.Zhao, T.Ogawa
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Journal Title
J.Geophys.Res. 108
Pages: 8402, doi:10.1029/2001JD000820
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Reactive nitrogen over the tropical Western Pacific Influence from lightning and biomass burning2003
Author(s)
M.Koike, Y.Kondo, D.Akutagawa, K.Kita, N.Nishi, S.C.Liu, D.Blake, S.Kawakami, N.Takegawa, M.Ko, Y.Zhao, T.Ogawa
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Journal Title
J.Geophys.Res. 108
Pages: 8403, doi:10.1029/2001JD000823
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Black carbon in aerosol during BIBLE-B.2003
Author(s)
J.B.Liley, D.Baumgardner, Y.Kondo, K.Kita, D.R.Blake, M.Koike, T.Machida, N.Takegawa, S.Kawakami, T.Shirai, T.Ogawa
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Journal Title
J.Geophys.Res. 108
Pages: 8399, doi:10.1029/2001JD000845
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Removal of NOx and NOy in biomass burning plumes in the boundary layer over northern Australia.2003
Author(s)
N.Takegawa, Y.Kondo, M.Koike, M.Ko, K.Kita, D.R.Blake, N.Nishi, W.Hu, J.B.Liley, S.Kawakami, T Shirai, Y.Miyazaki, H.Ikeda, J.Russell-Smith, T.Ogawa
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Journal Title
Journal of Geophysical Research vol.108
Pages: 10.1029/ 2001JD002505
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Ozonesonde observation in the Indonesian maritime continent : a case study on ozone rich layer in the equatorial upper troposphere2003
Author(s)
M.Fujiwara, Y.Tomikawa, K.Kita, Y.Kondo, N.Komala, S.Saraspriya, T.Manik, A.Suripto, S.kawakami, T.Ogawa, E.Kelena, B.Suhardi, S.W.B.Harijono, M.Kudsy, T.Sribimawati, M.D.Yamanaka
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Journal Title
Atmos.Environ. 37
Pages: 353-362
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Effects of biomass burning and lightening on atmospheric chemistry over Austraria and South-east Asia2003
Author(s)
Y.Kondo, N.Takegawa, Y.Miyazaki, M.Ko, M.Koike, K.Kita, S.Kawakami, T.Shirai, T.Ogawa, D.R.Blake, B.Liley, J.Russel-Smith
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Journal Title
International Journal of Wildland Fire 12
Pages: 271-281
Description
「研究成果報告書概要(欧文)」より