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2004 Fiscal Year Final Research Report Summary

Proposal and theoretical investigation with optimization for nuclear spin-polarization using intense laser pulses

Research Project

Project/Area Number 14540262
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field 素粒子・核・宇宙線
Research InstitutionKyoto University

Principal Investigator

NAKAJIMA Takashi  Kyoto University, Institute of Advanced Energy, Associate Professor, エネルギー理工学研究所, 助教授 (50281639)

Project Period (FY) 2002 – 2004
KeywordsSpin-polarization / Autoionization resonance / ultrafast laser pulse / polarized source
Research Abstract

(1)We came to the idea that there may be a possibility to polarize electron-spin of residual ions if one can polarize spin of photoelectrons. Based on this assumption, we have pursued the possibility of the simultaneous production of spin-polarized electrons/ions upon photoionization. Alkaline-earth atoms are ideal for such investigation, and we have chosen Sr for a target atom. Two schemes are considered : The first one is one-photon resonant two-photon ionization, and the second one is one-photon resonant one-photon ionization. After the theoretical study, we have found that 66% spin-polarization is possible for the latter, while >90% spin polarization is possible for the former at the expense of more than few orders of magnitude smaller yield.
(2)Based on the theoretical result in (1), we have performed experimental study, and obtained 64% spin-polarization as we expected. This experimental result is an important cornerstone toward the construction of a spin-polarized source.
(3)In order to achieve a better performance as a spin-polarized source, it is essential to improve the degree of spin-polarization and yield. For that purpose, the use of autoionizing resonance seems to be a promising scheme. We have replaced a wavelength-fixed ionization laser (excimer laser) by a tunable dye-laser, and carried out experiments to find that the significant improvement of spin-polarization (64% to 78%) and two-orders of magnitude improvement in terms of yield. Furthermore, we have theoretically investigate a new scheme to polarize spin using short laser pulses.

  • Research Products

    (6 results)

All 2005 2004 2003 2002

All Journal Article (6 results)

  • [Journal Article] Modification of the photoelectron angular distribution through laser-induced continuum structure2005

    • Author(s)
      Takashi Nakajima, Gabriela Buica
    • Journal Title

      Physical Review A 71

      Pages: 013413

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Electron-spin polarization of photoions produced through photoionization from the laser-excited triplet state of Sr2004

    • Author(s)
      N.Yonekura, Takashi Nakajima, Y.Matsuo, T.Kobayashi, Y.Fukuyama
    • Journal Title

      Journal of Chemical Physics 120

      Pages: 1806-1812

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Control of the spin-polarization of photoelectrons/photoions using short laser pulses2004

    • Author(s)
      Takashi Nakajima
    • Journal Title

      Applied Physics Letters 84

      Pages: 3786-3789

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Role of spin-orbit interaction in the production of spin-polarized photoelectrons using a dressing laser2003

    • Author(s)
      Takashi Nakajima, L.A.A.Nikolopoulos
    • Journal Title

      Physical Review A 68

      Pages: 013413

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Simultaneous production of spin-polarized ions/electrons based on two-photon ionization of laser-ablated metallic atoms2003

    • Author(s)
      Takashi Nakajima, N.Yonekura, Y.Matsuo, T.Kobayashi, Y.Fukuyama
    • Journal Title

      Applied Physics Letters 83

      Pages: 2103-2105

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Electron spin-polarized alkali-earth ions produced by multiphoton ionization2002

    • Author(s)
      Takashi Nakajima, Nobuaki Yonekura
    • Journal Title

      Journal of Chemical Physics 117

      Pages: 2112-2119

    • Description
      「研究成果報告書概要(和文)」より

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Published: 2006-07-11  

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