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2005 Fiscal Year Final Research Report Summary

The assessment of emission mechanism in GaN-based nano-structures by scanning near-field optical microscopy

Research Project

Project/Area Number 15206033
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Electronic materials/Electric materials
Research InstitutionKyoto University

Principal Investigator

KAWAKAMI Yoichi  Kyoto University, Department of Electronic Science and Engineering, Associate Professor, 工学研究科, 助教授 (30214604)

Co-Investigator(Kenkyū-buntansha) FUNATO Mitsuru  Kyoto University, Department of Electronic Science and Engineering, Lecturer, 工学研究科, 講師 (70240827)
Project Period (FY) 2003 – 2005
KeywordsNear Field Spectroscopy / Photoluminescence / Emission Dynamics / Multi-probe Technique / Advanced Photo-sensing / GaN-based semiconductors / Quantum nano-structures / Highly Efficient Emission
Research Abstract

The purpose of this project is to assess and/or control the radiative recombination processes in InGaN/GaN-based quantum wells by employing photoluminescence (PL) mapping with scanning near field optical microscopy (SNOM), by which dramatic improvement of emission efficiency as well as the extension of operatable wavelength can be achieved in emitters such as light emitting diodes (LEDs), laser diodes (LDs) and new phosphors. Our approach is to fabricate micro/nano structures for multi-wavelength lighting, to elucidate fundamental optical properties, and to make a positive feedback to future device structures. Main results are summarized as shown below.
(1)We have developed the experimental technique by combining the SNOM-PL with atomic force microscopy (AFM), where the correlation was clearly revealed between dislocations and weak emission regions. Moreover, time-resolved PL measurements with this method showed the dynamical behavior of photo-generated carriers and/or excitons in potential fluctuations. It was found that the pathway to nonradiative recombination centers is effectively hindered by the compositional modulation around the dislocations, so that the carrier diffusion is spatially unisotropic process.
(2)We have proposed the re-growth technique, where well-established c-oriented GaN is used as a seed. It has been demonstrated that the growth on c-oriented GaN patterned with a stripe along the [11^^-00] direction forms (0001), <112^^-2>, and <112^^-0> facets and that the QW on the <112^^-2> facet involves weaker electric fields and has a higher PL efficiency, compared with conventional c-oriented InGaN/GaN QWs. Moreover, rainbow color PL covering the entire visible range has been achieved from InGaN/GaN QWs on the <112^^-2> facets with a few micron-width.

  • Research Products

    (36 results)

All 2006 2005 2004 2003

All Journal Article (30 results) Book (6 results)

  • [Journal Article] The fabrication of an Atomic Resolution Low Cost STM-SNOM Hybrid Probe2006

    • Author(s)
      R.Micheletto, M.Yokokawa, S.Okazaki, Y.Kawakami
    • Journal Title

      Journal of Nanoscience and Nanotechnology 6

      Pages: 72-76

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Observation of a nanometer size confined transient phenomenon at the gold STM tip interface under UV illumination2006

    • Author(s)
      R.Micheletto, M.Yokokawa, Y.Ding, D.Hobara, T.Kakiuchi, Y.Kawakami
    • Journal Title

      Colloid and Surfaces A : Physicochem. Eng. Aspects 273

      Pages: 189-192

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Observation of optical instabilities in the photoluminescence of InGaN quantum well2006

    • Author(s)
      R.Micheletto, M.Abiko, A.Kaneta, Y.Kawakami
    • Journal Title

      Applied Physics Letters 88

      Pages: 61118-61120

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Observation of a nanometer size confined transient phenomenon at the gold STM tip interface under UV illumination2006

    • Author(s)
      R.Micheletto, M.Yokokawa, Y.Ding, D.Hobara, T.Kakiuchi, Y.Kawakami
    • Journal Title

      Colloid and Surfaces A : Physicochem.Eng.Aspects 273

      Pages: 189-192

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Confined waveguide behaviour of Distributed Bragg Reflectors probed by polarization-controlled Near Field Optical Microscopy2005

    • Author(s)
      P.G.Gucciardi, M.Allegrini, R.Micheletto, T.Kotani, Y.Hatada, Y.Kawakami
    • Journal Title

      Journal of the Korean Physical Society 47

      Pages: S100-S107

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Fabrication and characterization of GaN-based distributed Bragg reflector mirrors for low lasing threshold and integrated photonics2005

    • Author(s)
      T.Kotani, Y.Hatada, M.Funato, Y.Narukawa, T.Mukai, Y.Kawakami, S.Fujita
    • Journal Title

      Physica Status Solidi (c) 2

      Pages: 2895-2898

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Near-field photoluminescence study in violet light emitting InGaN single quantum well structures2005

    • Author(s)
      A.Kaneta, D.Yamada, G.Marutsuki, Y.Narukawa, T.Mukai, Y.Kawakami
    • Journal Title

      Physica Status Solidi (c) 2

      Pages: 2728-2731

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Nano probing of the membrane dynamics of rat pheochromocytoma by near field optics2005

    • Author(s)
      R.Piga, R.Micheletto, Y.Kawakami
    • Journal Title

      Biophysical Chemistry 117

      Pages: 40-45

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Dynamical polarization filtering in anisotropically strained M-plane GaN films2005

    • Author(s)
      K.Omae, T.Fissikowski, P.Misra, O.Brandt, H.T.Grahn, K.Kojima, Y.Kawakami
    • Journal Title

      Applied Physics Letters 86

      Pages: 191909/1-3

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Efficient rainbow color luminescence from In_xGa_<1_x>N single quantum wells fabricated on {1122} microfacets2005

    • Author(s)
      K.Nishizuka, M.Funato, Y.Kawakami, Y.Narukawa, T.Mukai
    • Journal Title

      Applied Physics Letters 87

      Pages: 231901/1-3

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Near-field scanning optical microscopic transient lens for carrier dynamics study in InGaN/GaN2005

    • Author(s)
      K.Okamoto, A.Sherer, Y.Kawakami
    • Journal Title

      Applied Physics Letters 87

      Pages: 161104/1-3

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Surface plasmon enhanced spontaneous emission rate of InGaN/GaN quantum wells probed by time-resolved photoluminescence spectroscopy2005

    • Author(s)
      K.Okamoto, I.Niki, A.Sherer, Y.Narukawa, T.Mukai, Y.Kawakami
    • Journal Title

      Applied Physics Letters 87

      Pages: 071102/1-3

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Efficient rainbow color luminescence from In_xG_<1_x>N single quantum wells fabricated on {112^^-2} microfacets2005

    • Author(s)
      K.Nishizuka, M.Funato, Y.Kawakami, Y.Narukawa, T.Mukai
    • Journal Title

      Applied Physics Letters 87

      Pages: 231901/1-231901/3

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Indium Concentration on PL Spatial Inhomogeneity in InGaN Single Quantum Well Structures Detected by Original Low Cost Near-field Probes2004

    • Author(s)
      R.Micheletto, N.Yoshimatsu, A.Kaneta, Y.Kawakami, S.Fujita
    • Journal Title

      Applied Surface Science 229

      Pages: 338-345

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Submicron-scale photoluminescence of InGaN/GaN probed by confocal scanning laser microscopy2004

    • Author(s)
      K.Okamoto, J.Choi, Y.Kawakami, M.Terazima, T.Mukai, S.Fujita
    • Journal Title

      Japanese Journal of Applied Physics 43

      Pages: 839-840

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Optically pumped lasing and gain formation properties in blue In_xGa_<1_x>N MQWs2004

    • Author(s)
      K.Kojima, A.Shikanai, K.Omae, M.Funato, Y.Kawakami, Y.Narukawa, T.Mukai, S.Fujita
    • Journal Title

      physica status solidi (b) 241

      Pages: 2676-2680

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Efficient radiative recombination from <1122> -oriented InGaN multiple quantum wells fabricated by the re-growth technique2004

    • Author(s)
      K.Nishizuka, M.Funato Y.Kawakami, Y.Narukawa, T.Mukai, S.Fujita
    • Journal Title

      Applied Physics Letters 85

      Pages: 3122-3124

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Optically pumped lasing and gain formation properties in blue In_xGa_<1-x>N MQWs2004

    • Author(s)
      K.Kojima, A.Shikanai, K.Omae, M.Funato, Y.Kawakami, Y.Narukawa, T.Mukai, S.Fujita
    • Journal Title

      Physica Status Solidi (b) 241

      Pages: 3676-2680

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Efficient radiative recombination from <112^^-2> -oriented InGaN multiple quantum wells fabricated by the re-growth technique2004

    • Author(s)
      K.Nishizuka, M.Funato, Y.Kawakami, Y.Narukawa, T.Mukai, S.Fujita
    • Journal Title

      Applied Physics Letters 85

      Pages: 3122-3124

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Optical properties of Si-, Ge- and Sn-doped GaN2003

    • Author(s)
      A.Shikanai, H.Fukahori, Y.Kawakami, K.Hazu, T.Sota, T.Mitani, T.Mukai, S.Fujita
    • Journal Title

      Physica. Status. Solidi (b) 235

      Pages: 26-30

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Nonradiative recombination processes of carriers in InGaN/GaN probed by the microscopic transient lens spectroscopy2003

    • Author(s)
      K.Okamoto, K.Inoue, Y.Kawakami, M.Terazima, A.Tsujimura, I.Kidoguchi, S.Fuiita
    • Journal Title

      Review of Scientific Instruments 74

      Pages: 575-577

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Recombination dynamics in low-dimensional nitride semiconductors2003

    • Author(s)
      Y.Kawakami, A.Kaneta, K.Omae, A.Shikanai, K.Okamoto, G.Marutsuki, Y.Narukawa, T.Mukai, S.Fujita
    • Journal Title

      Physica Status Solidi (b) 240

      Pages: 337-343

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Sub-microscopic transient lens spectroscopy of InGaN/GaN quantum wells2003

    • Author(s)
      K.Okamoto, Y.Kawakami, S.Fujita, A.Scherer
    • Journal Title

      Physica Status Solidi (b) 240

      Pages: 368-371

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] The hot carrier dynamics in InGaN multi-quantum well structure2003

    • Author(s)
      A.Shikanai, K.Kojima, K.Omae, Y.Kawakami, Y.Narukawa, T.Mukai, S.Fujita
    • Journal Title

      Physica Status Solidi (b) 240

      Pages: 392-395

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Effects of internal electric field on transient absorption in In_xGa_1-_xN thin layers and quantum wells with different thickness by pump and probe spectroscopy2003

    • Author(s)
      K.Omae, Y.Kawakami, S.Fujita, Y.Narukawa, T.Mukai
    • Journal Title

      Physical Review B 68

      Pages: 085303/1-5

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Discrimination of local radiative and nonradiative recombination processes in an InGaN/GaN single-quantum-well structure by a time-resolved multimode scanning near-field optical microscopy2003

    • Author(s)
      A.Kaneta, T.Mutoh, G.Marutsuki, Y.Narukawa, T.Mukai, Y.Kawakami, S.Fujita
    • Journal Title

      Applied Physics Letters 83

      Pages: 3462-3464

    • Description
      「研究成果報告書概要(和文)」より
  • [Journal Article] Optical properties of Si-,Ge- and Sn-doped GaN2003

    • Author(s)
      A.Shikanai, H.Fukahori, Y.Kawakami.K.Hazu, T.Sota, T.Mitani, T.Mukai, S.Fujita
    • Journal Title

      Physica.Status.Solidi (b) 235

      Pages: 26-30

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Nonradiative recombination processes of carriers in InGaN/GaN probed by the microscopic transient lens spectroscopy2003

    • Author(s)
      K.Okamoto, K.Inoue, Y.Kawakami.M.Terazima, A.Tsujimura, I.Kidoguchi, S.Fujita
    • Journal Title

      Review of Scientific Instruments 74

      Pages: 575-577

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Recombination dynamics in low-dimensional nitride semiconductors2003

    • Author(s)
      Y.Kawakami.A.Kaneta, K.Omae, A.Shikanai, K.Okamoto, G.Marutsuki, Y.Narukawa, T.Mukai, S.Fujita
    • Journal Title

      Physica Status Solidi (b) 240

      Pages: 337-343

    • Description
      「研究成果報告書概要(欧文)」より
  • [Journal Article] Effects of internal electric field on transient absorption in In_xGa_<1-x>N thin layers and quantum wells with different thickness by pump and probe spectroscopy2003

    • Author(s)
      K.Omae, Y.Kawakami, S.Fujita, Y.Narukawa, T.Mukai
    • Journal Title

      Physical Review B 68

      Pages: 085303/1-085303/5

    • Description
      「研究成果報告書概要(欧文)」より
  • [Book] Recombination dynamics in In_xGa_<1_x>N-based nanostructures in Progress in Nano-Electro-Optics IV2005

    • Author(s)
      Y.Kawakami, A.Kaneta, K.Omae, Y.Narukawa, T.Mukai (分担執筆)
    • Total Pages
      83-125
    • Publisher
      Springer-Verlag Berlin Heidelberg
    • Description
      「研究成果報告書概要(和文)」より
  • [Book] Polarization-Modulation Techniques in Near-Field Optical Microscopy for Imaging of Polarization Anisotropy in Photonic Nanostructures in Applied Scanning Probe Methods II : Scanning Probe Microscopy Techniques2005

    • Author(s)
      P.Gucciardi, R.Micheletto, Y.Kawakami, M.Allegrini(分担執筆)
    • Total Pages
      317-356
    • Publisher
      Springer-Verlag Berlin Heidelberg
    • Description
      「研究成果報告書概要(和文)」より
  • [Book] O Plus E 2005年12月号 特集 近接場光とナノデバイス(分担執筆) 「近接場分光によってInGaNナノ構造の発光機構に迫る」2005

    • Author(s)
      金田昭男, 船戸充, 川上養一, 成川幸男, 向井孝志(分担執筆)
    • Total Pages
      1410-1417
    • Publisher
      新技術コミュニケーションズ
    • Description
      「研究成果報告書概要(和文)」より
  • [Book] Recombination dynamics in In_x/Ga_<1-x>N-based nanostructures, Progress in Nano-Electro-Optics IV2005

    • Author(s)
      Y.Kawakami, A.Kaneta, K.Omae, Y.Narukawa, T.Mukai
    • Total Pages
      83-125
    • Publisher
      Springer Verlag Berlin Heidelberg
    • Description
      「研究成果報告書概要(欧文)」より
  • [Book] Polarization-Modulation Techniques in Near-Field Optical Microscopy for Imaging of Polarization Anisotropy in Photonic Nanostructures, Applied Scanning Probe Methods II : Scanning Probe Microscopy Techniques2005

    • Author(s)
      P.Gucciardi, R.Micheletto, Y.Kawakami, M.Allegrini
    • Total Pages
      317-356
    • Publisher
      Springer Verlag Berlin Heidelberg
    • Description
      「研究成果報告書概要(欧文)」より
  • [Book] 新しいフォトニクス時代の材料とデバイス,第8章1節2003

    • Author(s)
      藤田茂夫(分担執筆)
    • Total Pages
      182-190
    • Publisher
      株式会社TIC
    • Description
      「研究成果報告書概要(和文)」より

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Published: 2007-12-13  

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