2007 Fiscal Year Final Research Report Summary
Control of Interaction Parameters and Quantum Phase Transitions under Extreme Conditions in Spin Gap Systems
Project/Area Number |
17204028
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Research Category |
Grant-in-Aid for Scientific Research (A)
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Allocation Type | Single-year Grants |
Section | 一般 |
Research Field |
Condensed matter physics II
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Research Institution | Tokyo Institute of Technology |
Principal Investigator |
TANAKA Hidekazu Tokyo Institute of Technology, Graduate School of Science, Professor (80188325)
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Co-Investigator(Kenkyū-buntansha) |
ONO Toshio Tokyo Institute of Technology, Graduate School of Science, Assistant Professor (40332639)
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Project Period (FY) |
2005 – 2007
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Keywords | Magnetism / Condensed matter experiment / Low-temperature Physics / High magnetic field / High pressure / Quantum spin systems / Spin gap / Quantum phase transition |
Research Abstract |
Spin gap system is a spin system that has a singlet ground state with an excitation gap. In the present project, we studied quantum phase transitions in the gapped spin system induced by external magnetic field, hydrostatic pressure and disorder due to nonmagnetic impurities or ion substitution. First, we performed magnetization measurements on TlCuCl_3 down to 77 mK and in magnetic fields up to 7 T. The critical density of magnons as a function of temperature and the magnetic phase diagram were obtained. The magnon-magnon interaction constant was estimated. The phase boundary is expressed by the power law and agrees almost perfectly with the magnon BEC theory based on the Hartree-Fock approximation with realistic dispersion relations and interaction constant obtained. The critical exponent converges to 3/2 that is derived from the magnon BEC theory with decreasing fitting temperature range. These results strongly support the BEC description of the field-induced magnetic ordering in Tl
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CuCl_3. We performed magnetization measurements and neutron scattering experiments on KCuCl_3 under a hydrostatic pressure. A pressure-induced quantum phase transition from a gapped state to an antiferromagnetic state occurs at the critical pressure P_c=8.2 kbar. Above P_c magnetic Bragg reflections were observed at reciprocal lattice points that are equivalent to those for the lowest magnetic excitation at zero pressure. We also performed neutron inelastic scattering under pressure using newly designed pressure cell, and succeeded in observing the softening of triplet excitations. These results confirm that the pressure-induced magnetic ordering observed arises from the closing of the spin gap. We performed magnetic susceptibility, specific heat and ESR measurements on the S=1/2 one-dimensional Heisenberg antiferromagnet KCuGaF6 with the large exchange interaction. Due to the DM interaction with alternating D-vectors and/or the staggered g-tensor, the staggered magnetic field is induced when external magnetic field is applied. The effective magnetic model in magnetic field can be expressed by the quantum sine-Gordon (SG) model. It was found that most experimental results in KCuGaF_6 were beautifully described by the quantum SG field theory. We have found a new S=1/2 Kagome antiferromagnet Rb_2Cu_3SnF_<12>, which has a singlet ground state with the spin gap, as predicted from a recent theory. Less
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Research Products
(169 results)
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[Journal Article] Magnetic-Field Induced Bose-Einstein Condensation of Magnons and Critical Behavior in Interacting Spin Dimer System TlCuCl_32008
Author(s)
F., Yamada, T., Ono, H., Tanaka, G, Misguich, M., Oshikawa, T., Sakakibara
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Journal Title
J. Phys. Soc. Jpn. 77
Pages: 013701(1-4)
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Singlet Ground State and Spin Gap in S=1/2 Kagome Antiferromagnet Rb_2Cu_3SnF_<12>2008
Author(s)
K., Morita, M., Yano, T., Ono, H., Tanaka, K., Fujii, H., Uekusa, Y., Narumi, K., Kindo
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Journal Title
J. Phys. Soc. Jpn. 77
Pages: 043707(1-4)
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Magnetic Field-Induced One-Magnon Raman Scattering in the Magnon Bose-Einstein Condensation Phase of TlCuCl_32008
Author(s)
H., Kuroe, K., Kusakabe, A., Oosawa, T., Sekine, F., Yamada, H., Tanaka, M., Matsumoto
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Journal Title
Phys. Rev. B 77
Pages: 134420(1-5)
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Softening of Magnetic Excitations Leading to Pressure-Induced Quantum Phase Transition in Gapped Spin System KCuCl_32007
Author(s)
K., Goto, T., Osakabe, K., Kakurai, Y., Uwatoko, A., Oosawa, J., Kawakami, H., Tanaka
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Journal Title
J. Phys. Soc. Jpn. 76
Pages: 053704(1-4)
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] The Effect of Randomness on the Ouantum Snin System Tl_<1-x>K_xCuCl_3 with x=0.44 Studied by the Zero-Field Muon-Spin-Relaxation (ZF-μSR) method2007
Author(s)
T., Suzuki, F., Yamada, I., Watanabe, T., Goto, A., Oosawa, H.,Tanaka
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Journal Title
J. Phys. Soc. Jpn 76
Pages: 074704(1-5)
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Thermodynamics of the Up-Up-Down Phase of the S=1/2 Triangular-Lattice Antiferromagnet Cs_2CuBr_42007
Author(s)
H., Tsujii, C., R., Rotundu, T., Ono, H., Tanaka, B., Andraka, K.Ingersent, Y., Takano
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Journal Title
Phys. Rev. B 76
Pages: 060406(R)(1-4)
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Magnetic Quantum Phase Transitions from Gapped Spin Liquid State in TlCuCl_32007
Author(s)
H., Tanaka, F., Yamada, T., Ono, T., Sakakibara, Y., Uwatoko, A., Oosawa, K., Kakurai, K., Goto
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Journal Title
J. Magn. & Magn. Mater. 310
Pages: 1343-1348
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Impurity- and Field-Induced Magnetic Orderings in Doped Quantum Antiferromagnet TlCu_<1-x>Mg_xCl_32007
Author(s)
M., Fujisawa, T., Ono, H., Fujiwara, H., Tanaka, V., Sikolenko, M., Meissner, P., Smeibidl, S., Gerischer, H. A., Graf
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Journal Title
J. Magn. & Magn. Mater. 310
Pages: 1357-1359
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Raman Sattering of TlCu_<1-x>Mg_xCl_32007
Author(s)
K., Kusakabe, H., Kuroe, A., Oosawa, T., Sekine, M., Fujisawa, H., Tanaka
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Journal Title
J. Magn. & Magn. Mater. 310
Pages: 1365-1367
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Thermodynamic Properties of the Field-Induced Neel Order of TlCuCl_32007
Author(s)
S., Stark, O., Heyer, A., Vasiliev, A., Oosawa, H., Tanaka, T., Lorenz
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Journal Title
J. Magn. & Magn. Mater. 310
Pages: 1374-1376
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Thermodynamics of the Coupled Spin-Dimer System TlCuCl_3 Close to a Quantum Phase Transition2007
Author(s)
T., Lorenz, S., Stark, O., Heyer, N., Hollmann, A., Vasiliev, A., Oosawa, H., Tanaka
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Journal Title
J. Magn. & Magn. Mater. 316
Pages: 291-297
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Pressure-Induced magnetic Quantum Phase Transition in KCuCl_32007
Author(s)
K., Goto, M., Fujisawa, A., Oosawa, T., Osakabe, K., Kakurai, Y., Uwatoko, H., Tanaka
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Journal Title
J. Phys. Soc. Jpn. 76
Pages: Suppl. A 162-163
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] ^<63/65>Cu-NMR Study of the Quantum Spin System NH_4CuCl_3 Showing Magnetization Plateaus2006
Author(s)
H. Inoue, T. Saito, S. Tani, S. Hosoya, A. Oosawa, T. Goto, M. Fujiwara, H. Tanaka, T. Sasaki, S. Awaji, K. Watanabe, N. Kobayashi
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Journal Title
J. Phys : Conf. Ser. 51
Pages: 103-106
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Cu-NMR Study on the Disordered Quantum Spin Magnet with the Bose-Glass Ground State2006
Author(s)
T. Fujiwara, H. Inoue, A. Oosawa, R. Tsunoda, T. Goto. T. Suzuki, Y. Shindo, H. Tanaka, T. Sasaki, N. Kobayashi, S. Awaji, K. Watanabe
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Journal Title
J. Phys : Conf. Ser. 51
Pages: 199-202
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Development and Application of High Field and High Pressure ESR System2006
Author(s)
T., Sakurai, A., Taketani, T., Tomita, S., Okubo, H., Ohta, H., Tanaka, Y., Uwatoko
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Journal Title
J. Phys : Conf. Ser 51
Pages: 565-568
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Phase Transitions and Disorder Effects in Pure and Doped Frustrated Qantum Antiferromagnet Cs_2CuBr_42005
Author(s)
T. Ono, H. Tanaka, T. Nakagomi, O. Kolomiyets, H. Mitamura, F. Ishikawa, T. Goto, K. Nakajima, A. Oosawa, Y. Koike, K. Kakurai, J. Klenke, P. Smeibidle, M. Meisner, H. Aruga Katori
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Journal Title
J. Phys. Soc. Jpn. 74 Suppl.)
Pages: 135-144
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Field-Induced Phase Transition Driven by Quantum Fluctuation in S=1/2 Anisotropic Triangular Antiferromagnet Cs_2CuBr_42005
Author(s)
T. Ono, H. Tanaka, O. Kolomiyets, H. Mitamura, F. Ishikawa, T. Goto, K. Nakajima, A. Oosawa, Y. Koike, K. Kakurai, J. Klenke, P. Smeibidle, M. Meisner, R. Coldea, A. D. Tennant, J. Olliver
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Journal Title
Prog. Theor. Phys. No. 159 Suppl.)
Pages: 217-221
Description
「研究成果報告書概要(欧文)」より
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[Journal Article] Cu-NMR Study on Field-Induced Phase Transitions in Quantum Spin magnet NH_4CuCl_32005
Author(s)
S. Tani, H. Inoue, T. Suzuki, S. Hosoya, K. Inokuchi, T. Fujiwara, T. Goto, H. Tnanaka, T. Sasaki, S. Awaji, K. Watanabe, N. Kobayashi
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Journal Title
Prog. Theor. Phys. No. 159 Suppl.)
Pages: 235-240
Description
「研究成果報告書概要(欧文)」より
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[Presentation] Pressure-Induced Magnetic Quantum Phase Transition In KCuCl_32006
Author(s)
K., Goto, M., Fujisawa, A., Oosawa, T., Osakabe, K., Kakurai, Y., Uwatoko, H., Tanaka
Organizer
Novel Pressure-Induced Phenomena In Condensed Matter Systems
Place of Presentation
Fukuoka, Japan.
Year and Date
20060826-29
Description
「研究成果報告書概要(欧文)」より
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[Presentation] Thermodynamic Properties of The Field-Induced Neel Order of TlCuCl_32006
Author(s)
T., Lorenz, S., Stark, N., Johannsen, T., Zabel, A., Vasiliev, A., Oosawa, H., Tanaka
Organizer
International Conference on Magnetism
Year and Date
20060820-25
Description
「研究成果報告書概要(欧文)」より
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[Presentation] The Phase Diagrams of Gapped Quantum Spin Systems Studied by Inelastic Neutron Scattering (Invited Talk)2006
Author(s)
Ch, Ruegg, D.F., McMorrow, A., Furrer, H.M., Ronnow, Ch., Niedermayer, B., Thielemann, M., Zyed, S., Gvasaliya, J., Mesot, K.W., Kramer, H.-U., Gidel, H., Tanaka, et. al.
Organizer
International Conference on Magnetism
Place of Presentation
Kyoto, Japan.
Year and Date
20060820-25
Description
「研究成果報告書概要(欧文)」より
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[Presentation] Magnetic Phase Diagram of the Frustrated Quasi-Two-Dimensional S=1/2 Heisenberg Antiferromagnet Cs2CuBr42006
Author(s)
Y., Takano, H., Tsujii, C. R., Rotunduu, T. E., Sherline, B., Andraka, N. A., Fortune, S. T., Hanahs, T., Ono, H., Tanaka
Organizer
International Conference on Magnetism
Place of Presentation
Kyoto, Japan.
Year and Date
20060820-25
Description
「研究成果報告書概要(欧文)」より
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[Presentation] Low-Energy Dynamics of The Spin Gap Magnet TlCuCl_3 at the Critical Field2006
Author(s)
V. N., Glazkov, A.I., Smirnov, A., Kolezhuk, H., Tanaka, A., Oosawa
Organizer
International Conference on Magnetism
Place of Presentation
Kyoto, Japan.
Year and Date
20060820-25
Description
「研究成果報告書概要(欧文)」より
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[Presentation] Raman Scattering of Tl(Cu_<1-x>Mg_x)Cl_32006
Author(s)
K., Kusakabe, H., Kuroe, A., Oosawa, T., Sekine, M., Fujisawa, H., Tanaka
Organizer
International Conference on Magnetism
Place of Presentation
Kyoto, Japan.
Year and Date
20060820-25
Description
「研究成果報告書概要(欧文)」より
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[Presentation] Magnetic Ordering Under Hydrostatic Pressure in Doped Spin Gap System ACu_<1-x>Mg_xCl_3 : A=Tl, K2006
Author(s)
H., Tanaka, H., Imamura, J., Kawakami, T., Ono, K., Goto
Organizer
International Conference on Magnetism
Place of Presentation
Kyoto, Japan.
Year and Date
20060820-25
Description
「研究成果報告書概要(欧文)」より
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[Presentation] ^<35/37>Cl, ^<63/65>Cu-NMR. Study of the Quantum Spin System NH_4CuCl_3 Showing Magnetization Plateaus2006
Author(s)
H., Inoue, T., Saito, S., Tani, S., Hosoya, A., Oosawa, T., Goto, M., Fujisawa, H., Tanaka, et. al.
Organizer
Yamada Conference LX on Research in High Magnetic Fields
Place of Presentation
Sendai, Japan
Year and Date
20060816-19
Description
「研究成果報告書概要(欧文)」より
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[Presentation] Cu-NMR study on disordered dimer system (Tl_<1-x>K_xCuCl_3 with the Bose-glass ground state2006
Author(s)
T., Fujiwara, A., Oosawa, R., Tsunoda, T., Goto, T., Suzuki, Y., Shindo, H., Tanaka
Organizer
Yamada Conference LX on Research in High Magnetic Fields
Place of Presentation
Sendai, Japan
Year and Date
20060816-19
Description
「研究成果報告書概要(欧文)」より
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[Presentation] Magnetic Field and Pressure Induced Quantum Phase Transition in the Spin Liquid TlCuCl_3 (Invited Talk)2005
Author(s)
Ch., Ruegg, A., Furrer, K., Kramer, H. -U., Gudel, H., Tanaka
Organizer
24th International Conference on Low Temperature Physics
Place of Presentation
Orland, Florida USA
Year and Date
20050810-17
Description
「研究成果報告書概要(欧文)」より
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[Presentation] NMR Studies on Magnetization Plateaus in Dimer Spin Systems (Invited Talk)2005
Author(s)
M., Takigawa, K., Kodama, M., Horvatic, C., Berthier, H., Kageyama, Y., Ueda, H., Tanaka
Organizer
24th International Conference on Low Temperature Physics
Place of Presentation
Orland, Florida USA
Year and Date
20050810-17
Description
「研究成果報告書概要(欧文)」より
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[Presentation] ^2D, ^<35/37>Cl,^<63/65>Cu-NMR study on quantum spin system NH_4CuCl_32005
Author(s)
H., Inoue, S., Tani, S., Hosova, T., Suzuki, T., Goto, H., Tanaka, T., Sasaki, N., Kobayashi
Organizer
24th International Conference on Low Temperature Physics
Place of Presentation
Orland, Florida USA
Year and Date
20050810-17
Description
「研究成果報告書概要(欧文)」より
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[Presentation] ESR Measurements of KCuCl3 under Multi Extreme Conditions2005
Author(s)
T., Sakurai A., Taketani, S., Kimura, M., Yoshida, S., Okubo, H., Ohta, H., Tanaka Y., Uwatoko
Organizer
24th International Conference on Low Temperature Physics
Place of Presentation
Orland, Florida USA
Year and Date
20050810-17
Description
「研究成果報告書概要(欧文)」より
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[Presentation] Magnetic Phase Diagram of the Quasi-Two-Dimensional S=1/2 Antiferromagnet Cs_2CuBr_42005
Author(s)
H., Tsujii, C. R., Rotundu, T., Ono, B., Andraka, H., Tanaka, Y., Takano
Organizer
24th International Conference on Low Temperature Physics
Place of Presentation
Orland Florida USA
Year and Date
20050810-17
Description
「研究成果報告書概要(欧文)」より
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