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2020 Fiscal Year Annual Research Report

Analysis and control of bubble generation in solid state nanopores

Research Project

Project/Area Number 20J22422
Research InstitutionThe University of Tokyo

Principal Investigator

PAUL SOUMYADEEP  東京大学, 工学系研究科, 特別研究員(DC1)

Project Period (FY) 2020-04-24 – 2023-03-31
KeywordsJoule heating / nanopore / bubble nucleation / microelectronic cooling
Outline of Annual Research Achievements

Control over nanobubble size and generation periodicity is key to realizing a bubble seed emitter for micro-electronic cooling applications. In the past year, the effects of changing nanopore diameter and bias voltages were studied on bubble size and periodicity. Bubble nucleation is actuated inside a solid state nanopore through localized Joule heating. As a bubble nucleates and grows at this hotspot to block the pore, we record transient current dips using a high bandwidth oscilloscope. A signal processing software was developed to analyze the bubble blockage events. Additionally, three theoretical models were constructed: (i) a continuum Joule heating model for nanopore temperature estimation, (ii) a 1D moving boundary model to capture bubble growth and collapse and (iii) a cluster competition model to explain the transition between nucleation modes. Our analysis indicates that as the pore diameter is increased, periodic and homogenous nucleation at the pore center transitions into predominantly heterogeneous nucleation on the pore walls, making the bubble generation stochastic. Also, with an increase in pore diameter, larger homogenous bubbles were generated. These results were summarized into two journal publications (Paul et al., Phys. Rev. Res. 2, 043400 (2020) and Paul et al., JTST 16, JTST0007 (2021)) and presented at two online conferences (57th NHTS (2020) and 73rd APS DFD meeting (2020)).

Current Status of Research Progress
Current Status of Research Progress

1: Research has progressed more than it was originally planned.

Reason

Our target for the first year was to understand the influence of pore diameter on periodic and non-periodic bubble generation in nanopores. Our investigation led us to the finding that transition between homogeneous and heterogeneous nucleation is responsible for the different bubble generation modes observed. This finding and the underlying analyses were well received by the thermal engineering and applied physics community, according to the response from conference audience and journal reviewers. Thus we reach the assessment of "above-expectation progress".

Strategy for Future Research Activity

In the following year, we plan to perform acoustic measurements of bubble dynamics using piezo-electric type hydrophones. In addition, we are working on
developing an optical thermometry experimental setup to measure superheat temperatures inside nanopore, caused as a result of Joule heating. Also, to better analyze the bubble signal data, we are working on adding a machine learning based binary classifier to our signal processing software for clear differentiation between homogeneous and heterogeneous bubbles.

  • Research Products

    (5 results)

All 2021 2020 Other

All Int'l Joint Research (1 results) Journal Article (2 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 2 results,  Open Access: 2 results) Presentation (2 results) (of which Int'l Joint Research: 1 results)

  • [Int'l Joint Research] Imperial College London/The Alan Turing Institute/University of Nottingham(英国)

    • Country Name
      UNITED KINGDOM
    • Counterpart Institution
      Imperial College London/The Alan Turing Institute/University of Nottingham
  • [Journal Article] Analysis and control of vapor bubble growth inside solid-state nanopores2021

    • Author(s)
      PAUL Soumyadeep、HSU Wei-Lun、MAGNINI Mirco、MASON Lachlan R.、ITO Yusuke、HO Ya-Lun、MATAR Omar K.、DAIGUJI Hirofumi
    • Journal Title

      Journal of Thermal Science and Technology

      Volume: 16 Pages: JTST0007

    • DOI

      10.1299/jtst.2021jtst0007

    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Single-bubble dynamics in nanopores: Transition between homogeneous and heterogeneous nucleation2020

    • Author(s)
      Paul Soumyadeep、Hsu Wei-Lun、Magnini Mirco、Mason Lachlan R.、Ho Ya-Lun、Matar Omar K.、Daiguji Hirofumi
    • Journal Title

      Physical Review Research

      Volume: 2 Pages: 043400

    • DOI

      10.1103/PhysRevResearch.2.043400

    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] A Study of Homogeneous and Heterogeneous Bubble Nucleation Inside Nanopores through Resistive Pulse Sensing2020

    • Author(s)
      Soumyadeep Paul, Wei-Lun Hsu, Mirco Magnini, Lachlan R. Mason, Ya-Lun Ho, Omar K. Matar and Hirofumi Daiguji
    • Organizer
      73rd Annual Meeting of the APS Division of Fluid Dynamics
    • Int'l Joint Research
  • [Presentation] Resistive pulse sensing of bubble generation inside solid-state nanopores2020

    • Author(s)
      Soumyadeep Paul, Wei-Lun Hsu, Ya-Lun Ho and Hirofumi Daiguji
    • Organizer
      57th National Heat Transfer Symposium

URL: 

Published: 2021-12-27  

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