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2012 Fiscal Year Final Research Report

Measurement of spin transport properties and spin coherence in molecular semiconductors

Research Project

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Project/Area Number 22360008
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Applied materials science/Crystal engineering
Research InstitutionOsaka University

Principal Investigator

SHIRAISHI Masashi  大阪大学, 基礎工学研究科, 教授 (30397682)

Co-Investigator(Renkei-kenkyūsha) DR. VALENTIN Alek Dediu  イタリア ISMN-CNR研究所
Project Period (FY) 2010 – 2012
Keywordsスピントロニクス / 分子性半導体 / スピンコヒーレンス / 酸化物強磁性 / スピン緩和 / スピン輸送
Research Abstract

The purpose of this project is to estimate spin coherence in molecular semiconductors precisely. In the first stage of the project, I was provided a molecular spin valve device from a collaborator in Italy (Dr. V. Dediu) and tried to measure spin precession of propagating spins in molecular semiconductors, which is called as Hanle effect. However, no such effect was observed due to less reliability of spin injection into molecules in the device. He nce, in the second stage, experimental investigations of an interfacial electronics structures between molecular semiconductor single crystal and ferromagnetic metals and modulation of the electronic structure were implemented, in addition to a search for a new oxide ferromagnet as a good spin source for molecular semiconductors. Both were successfully carried out. In the final stage, a new spin injection method, dynamical spin pumping, was introduced, and spin injection into a zero-gap molecular semiconductor, single-layer graphene, was successfully demonstrated and spin coherence was precisely measured. This project revealed serious problems in earlier studies of molecular spintronics, and enabled an establishment of a novel spin injection method into molecular semiconductors.

  • Research Products

    (10 results)

All 2013 2012 2011 Other

All Journal Article (6 results) Presentation (4 results)

  • [Journal Article] Dynamically-generated pure spin current in graphene2013

    • Author(s)
      Z. Tang, H. Ago, E. Shikoh, Y. Ando, T. Shinjo and M. Shiraishi
    • Journal Title

      Phys. Rev

      Volume: B87 Pages: 140401

  • [Journal Article] Realization of ohmic-like contact between ferromagnet and rubrene single crystal2012

    • Author(s)
      Y. Kitamura, E. Shikoh, K. Sawabe, T. Takenobu and M. Shiraishi
    • Journal Title

      Appl. Phys. Lett

      Volume: 101 Pages: 073501

  • [Journal Article] Electrical investigation of an interface band structure in a rubrene single-crystal/nickel junction2011

    • Author(s)
      Y. Kitamura, E. Shikoh, T. Shinjo, S.Z. Bisri, T. Takenobu and M. Shiraishi
    • Journal Title

      Appl. Phys. Lett.

      Volume: 99 Pages: 043505

  • [Journal Article] Observation of a tunneling magnetoresistance effect in magnetic tunnel junctions with a high resistance magnetic oxide Fe_2.5Mn_0.5O electrode2011

    • Author(s)
      E. Shikoh, T. Kanki, H. Tanaka, T. Shinjo and M. Shiraishi
    • Journal Title

      Solid State Comm

      Volume: 151 Pages: 1296

  • [Journal Article] Molecular spintronics2011

    • Author(s)
      M. Shiraishi and T. Ikoma
    • Journal Title

      Physica E

      Volume: 43 Pages: 1295

  • [Journal Article] Vertical spin transport in Al with Pd/Al/Ni_80Fe_20 trilayer films at room temperature by spin pumping

    • Author(s)
      Y.Kitamura, Y. Ando, E. Shikoh, T. Shinjo and M. Shiraishi
    • Journal Title

      Scientific Reports

      Volume: (in press)

  • [Presentation] グラフェンへの電気的・動力学的スピン注入2012

    • Author(s)
      白石誠司
    • Organizer
      グラフェンの材料応用にむけた基礎と応用研究会
    • Place of Presentation
      筑波大
    • Year and Date
      20120800
  • [Presentation] 分子を介したスピン依存伝導と巨大磁気抵抗効果の発現2012

    • Author(s)
      白石誠司
    • Organizer
      日本化学会・特別企画講演
    • Place of Presentation
      慶應義塾大
    • Year and Date
      20120300
  • [Presentation] Spin-transport-induced phenomena in molecules2011

    • Author(s)
      M. Shiraishi
    • Organizer
      International workshop of Carbon-based spintronics
    • Place of Presentation
      MPI-PKS Dresden
    • Year and Date
      20111000
  • [Presentation] Spintronics using group-IV elements2011

    • Author(s)
      M. Shiraishi
    • Organizer
      International Workshop on Spin Currents 2011
    • Place of Presentation
      Sendai
    • Year and Date
      20110300

URL: 

Published: 2014-08-29  

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