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Anomalous magnetic dynamics of spin systems with 2-dimensional honeycomb crystal structures

Research Project

Project/Area Number 15K05149
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionMeiji University

Principal Investigator

Yukio Yasui  明治大学, 理工学部, 専任教授 (80345850)

Co-Investigator(Kenkyū-buntansha) 菊地 淳  明治大学, 理工学部, 専任教授 (90297614)
Project Period (FY) 2015-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2018: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2017: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2016: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2015: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Keywordsハニカム格子 / 磁気特性 / 元素置換効果 / 中性子回折 / 磁気構造 / NMR / 磁化曲線 / 粉末中性子回折 / 磁気ダイナミクス / 反強磁性転移 / incommensurateな磁気構造
Outline of Final Research Achievements

In the present work, magnetic characteristics of the Ni2+ and Co2+ spin systems with the general formula of A3Ni2SbO6 and A3Co2SbO6 (A=Li, Na) with honeycomb crystal structures have been studied. Polycrystalline samples of these honeycomb spin systems were prepared, and measurements of the magnetic susceptibilities and specific heat have been carried out for these systems. Moreover, X-ray diffraction, neutron diffraction and Nuclear Magnetic Resonance (NMR) have been carried out to obtain microscopic information of the magnetic state of these systems. We have found various phase transitions and magnetic-field induced magnetic ones, and have clarified mechanism of magnetic anomalies and magnetic structures of these honeycomb spin systems.

Academic Significance and Societal Importance of the Research Achievements

磁性イオンが特徴的な形の格子を構成し、かつスピン間相互作用に競合やフラストレーションが生じている磁性体は、特異な磁気特性・磁気構造を取ることが期待され、多くの物質が研究対象になってきた。その点でハニカム格子磁性体も興味がもたれたが、パイロクロア格子・カゴメ格子・三角格子の磁性体と比べて物質例が少なく実験的な研究はあまり進んでいなかった。今回、数多くの種類のハニカム格子磁性体について試料を合成し、その磁気特性や磁性異常を実験的に明らかにすることができたので、ハニカム格子磁性体に特有の物理の解明が大きく進展したと考えている。

Report

(5 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (17 results)

All 2018 2017 2016 2015 Other

All Int'l Joint Research (6 results) Journal Article (3 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 3 results) Presentation (6 results) (of which Int'l Joint Research: 3 results,  Invited: 1 results) Remarks (2 results)

  • [Int'l Joint Research] Paul Scherrer Institut(スイス)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] University of Edinburgh(英国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] National Cheng Kung University(その他の国・地域)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] University of Warwick/University of Edinburgh(United Kingdom)

    • Related Report
      2017 Research-status Report
  • [Int'l Joint Research] National Cheng Kung University(Taiwan)

    • Related Report
      2017 Research-status Report
  • [Int'l Joint Research] University of Edinburgh(United Kingdom)

    • Related Report
      2016 Research-status Report
  • [Journal Article] Atomic structure study of the pyrochlore Yb2Ti2O7 and its relationship with low-temperature magnetic order2017

    • Author(s)
      Ali Mostaed, Geetha Balakrishnan, Martin Richard Lees, Yukio Yasui, Lieh-Jeng Chang, and Richard Beanland
    • Journal Title

      Phys. Rev. B.

      Volume: 95 Issue: 9 Pages: 094431-094431

    • DOI

      10.1103/physrevb.95.094431

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Comparison with Ground States of FrustratedQuantum Spin Chain Systems A2Cu2Mo3O12 (A=Rb and Cs)2016

    • Author(s)
      Akio Fujimura, Yukio Yasui, Yudai Yanagisawa, Ichiro Terasaki, Yohei Kono, Shunichiro Kittaka, and Toshiro Sakakibara
    • Journal Title

      IEEE Transactions on Magnetics

      Volume: 52 Issue: 7 Pages: 1-3

    • DOI

      10.1109/tmag.2016.2517091

    • Related Report
      2016 Research-status Report
    • Peer Reviewed
  • [Journal Article] First-order ferromagnetic transition of quantum spin ice system Yb2Ti2O72015

    • Author(s)
      Y. Yasui, N. Hamachi, Y. Kono, S. Kittaka, T. Sakakibara
    • Journal Title

      SPIN

      Volume: 5 Issue: 02 Pages: 1540002-1540002

    • DOI

      10.1142/s2010324715400020

    • Related Report
      2015 Research-status Report
    • Peer Reviewed
  • [Presentation] Magnetic Behavior of Quasi-One-dimensional Frustrated Quantum spin systems (Rb,Cs)2Cu2Mo3O122018

    • Author(s)
      Yukio Yasui, Shintaro Iguchi, Shota Nakamura, Yohei Kono, Shunichiro Kittaka, and Toshiro Sakakibara
    • Organizer
      International conference on Magnetism 2018 (ICM2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 超音波印加下でのY3Fe5O12の中性子散乱実験2018

    • Author(s)
      社本真一、松浦直人、赤津光洋、安井幸夫、伊藤孝、家田淳一、遠藤仁、小田達郎、L.-J.Chang、根本祐一、柴田薫
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Magnetic Properties of RCrTiO5 (R=Rare Earth Elements)2017

    • Author(s)
      Yukio Yasui, Takuma Miyamoto, Shunsuke Kori, Ichiro Terasaki, Daichi Yoshizawa, Mitsuru Akaki, Masayuki Hagiwara, Takeshi Matsukawa, Yukihiko Yoshida, Akinori Hoshikawa, Toru Ishigaki, and Naoki Igawa
    • Organizer
      SCES2017
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] J1 - J2モデルの一次元量子スピン系Cs2Cu2Mo3O12の磁気構造2017

    • Author(s)
      安井幸夫、藤村明央、大森喜由、井川直樹、松川健、吉田幸彦、星川晃範、石垣徹
    • Organizer
      日本中性子科学会第17回年会
    • Related Report
      2017 Research-status Report
  • [Presentation] フラストレートした一次元量子スピン系(Rb,Cs)2Cu2Mo3O12の多彩な磁気特性と誘電特性2016

    • Author(s)
      安井幸夫
    • Organizer
      日本物理学会2016年秋期大会
    • Place of Presentation
      金沢大学
    • Year and Date
      2016-09-15
    • Related Report
      2016 Research-status Report
    • Invited
  • [Presentation] Magnetic Properties and Crystal Structure of Honeycomb Lattice System Li3Ni2SbO62016

    • Author(s)
      Akito Fukui, Yukio Yasui, Naoki Igawa, Takeshi Matsukawa, Yukihiko Yoshida, Akinori Hoshikawa, Toru Ishigaki
    • Organizer
      13th Joint MMM-Intermag Conference
    • Place of Presentation
      San Diego, USA
    • Year and Date
      2016-01-12
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Remarks] 明治大学理工学部物理学科 量子固体物性研究室

    • URL

      http://www.isc.meiji.ac.jp/~yyasui/yasuilab.html

    • Related Report
      2018 Annual Research Report
  • [Remarks] 明治大学 理工学部 物理学科 量子固体物性研究室

    • URL

      http://www.isc.meiji.ac.jp/~yyasui/yasuilab.html

    • Related Report
      2017 Research-status Report

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Published: 2015-04-16   Modified: 2022-02-22  

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