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Study of quantum phase transition in antiferromagnetic alternating chain

Research Project

Project/Area Number 15K05150
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics II
Research InstitutionNational Institute for Materials Science

Principal Investigator

Hase Masashi  国立研究開発法人物質・材料研究機構, 先端材料解析研究拠点, グループリーダー (40281654)

Research Collaborator Kohno Masanori  
Project Period (FY) 2015-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2017: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2016: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2015: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywords反強磁性交替鎖 / 量子相転移 / 混晶 / スピンギャップ / 中性子非弾性散乱 / 磁化
Outline of Final Research Achievements

We investigated the magnetism of spin-3/2 antiferromagnetic alternating chain compounds RCrGeO5 (R = Ho, Er or Nd) and NdCrTiO5 using magnetization and neutron-scattering measurements. The compounds as well as already known R = Y or Sm compounds have a strongly dimerized ground state. We were not able to find a compound with a weakly dimerized ground state.
We also studied antiferromagnetic spin cluster compounds. We found a small magnetic moment in CuInVO5, reduction of the magnetic moment by quantum fluctuation in FeVMoO7 in spite of spin-5/2, and unstable ordered state in 0 T in Rb2Ni2Mo3O12 like an order in the vicinity of a quantum critical point.

Academic Significance and Societal Importance of the Research Achievements

RCrGeO5 (R = Y, Sm, Ho, Er, Nd)とNdCrTiO5の研究の結果、2つのCrスピン間に働く交換相互作用の大きさがCr-Cr距離にとても強く依存することが分かった。Cr-Cr距離が少しでも長くなると、交換相互作用が急激に小さくなるため、これらの物質の2種類の交換相互作用の大きさが大きく異なり、ボンド交替が弱いダイマー基底状態が実現できなかった。
量子臨界点近傍の秩序は通常、圧力や磁場を加えて初めて現れる。Rb2Ni2Mo3O12では、大気圧下のゼロ磁場でも、量子臨界点近傍の秩序が可能なことが分かった。

Report

(5 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (15 results)

All 2019 2018 2017 2016 Other

All Int'l Joint Research (2 results) Journal Article (6 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 6 results,  Open Access: 2 results,  Acknowledgement Compliant: 1 results) Presentation (7 results) (of which Int'l Joint Research: 4 results,  Invited: 1 results)

  • [Int'l Joint Research] Paul Scherrer Institut (PSI)(スイス)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] ANSTO(オーストラリア)

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Reduction of the ordered magnetic moment by quantum fluctuation in the antiferromagnetic spin-5/2 dimer compound FeVMoO72019

    • Author(s)
      (147)M. Hase, J. R. Hester, K. C. Rule, V. Yu. Pomjakushin, A. Matsuo, and K. Kindo
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 88 Issue: 3 Pages: 034711-034711

    • DOI

      10.7566/jpsj.88.034711

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Magnetic properties of the antiferromagnetic spin-1/2 tetramer compound CuInVO52018

    • Author(s)
      M. Hase, M. Matsumoto, A. Matsuo, and K. Kindo
    • Journal Title

      J. Phys.: Conference Series

      Volume: 969 Pages: 012100-012100

    • DOI

      10.1088/1742-6596/969/1/012100

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Erratum: Magnetism of the antiferromagnetic spin-3/2 dimer compound CrVMoO7 having an antiferromagnetically ordered state2018

    • Author(s)
      M. Hase, Y. Ebukuro, H. Kuroe, M. Matsumoto, A. Matsuo, K. Kindo, J. R. Hester, T. J. Sato, and H. Yamazaki
    • Journal Title

      Phys. Rev B

      Volume: 98 Issue: 13

    • DOI

      10.1103/physrevb.98.139901

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Magnetism of the antiferromagnetic spin-3/2 dimer compound CrVMoO7 having an antiferromagnetically ordered state2017

    • Author(s)
      M. Hase, Y. Ebukuro, H. Kuroe, M. Matsumoto, A. Matsuo, K. Kindo, J. R. Hester, T. J. Sato, and H. Yamazaki
    • Journal Title

      Physical Review B

      Volume: 95 Issue: 14 Pages: 144429-144429

    • DOI

      10.1103/physrevb.95.144429

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Magnetism of the spin-1 tetramer compound A2Ni2Mo3O12 (A = Rb or K)2017

    • Author(s)
      M. Hase, A. Matsuo, K. Kindo, and M. Matsumoto
    • Journal Title

      Phys. Rev B

      Volume: 96 Issue: 21 Pages: 214424-214424

    • DOI

      10.1103/physrevb.96.214424

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Magnetic excitations in antiferromagnetic alternating spin-3/2 chain compounds RCrGeO52016

    • Author(s)
      M. Hase, S. Asai, M. Soda, T. Masuda, D. Kawana, T. Yokoo, S. Itoh and M. Kohno
    • Journal Title

      J-PARC annual report

      Volume: 2 Pages: 30-31

    • NAID

      130007649105

    • Related Report
      2016 Research-status Report
    • Peer Reviewed
  • [Presentation] Magnetic excitations in antiferromagnetic alternating spin-3/2 chain compounds RCrGeO52018

    • Author(s)
      M. Hase
    • Organizer
      物性研短期研究会
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Magnetism of the spin-1 tetramer compound Rb2Ni2Mo3O122018

    • Author(s)
      M. Hase, A. Matsuo, K. Kindo, and M. Matsumoto
    • Organizer
      The 21st International Conference on Magnetism 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] High-Field Magnetization Measurements of Spin-Cluster Compounds2018

    • Author(s)
      M. Hase, A. Matsuo, K. Kindo, and M. Matsumoto
    • Organizer
      The 16th International Conference on Megagauss Magnetic Field Generation and Related Topics
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] スピン3/2反強磁性交替鎖物質RCrGeO5の磁気励起2018

    • Author(s)
      長谷正司、浅井晋一郎、左右田稔、益田隆嗣、川名大地、横尾哲也、伊藤晋一、河野昌仙
    • Organizer
      日本物理学会・第73回年次大会
    • Related Report
      2017 Research-status Report
  • [Presentation] スピン3/2反強磁性交替鎖物質RCrGeO5の磁気励起2018

    • Author(s)
      長谷正司、浅井晋一郎、左右田稔、益田隆嗣、川名大地、横尾哲也、伊藤晋一、河野昌仙
    • Organizer
      NIMS MI・計測合同シンポジウム2018
    • Related Report
      2017 Research-status Report
  • [Presentation] Magnetic excitations in antiferromagnetic alternating spin-3/2 chain compounds RCrGeO52017

    • Author(s)
      M. Hase, S. Asai, M. Soda, T. Masuda, D. Kawana, T. Yokoo, S. Itoh, and M. Kohno
    • Organizer
      28th International Conference on Low Temperature Physics (LT28)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Magnetic excitations in antiferromagnetic alternating spin-3/2 chain compounds RCrGeO52017

    • Author(s)
      M. Hase, S. Asai, M. Soda, T. Masuda, D. Kawana, T. Yokoo, S. Itoh, and M. Kohno
    • Organizer
      日本中性子科学会・第17回年会
    • Related Report
      2017 Research-status Report

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Published: 2015-04-16   Modified: 2020-05-15  

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