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Behavior of marine originated bromine species in authentic aerosols collected in Okinawa, Japan

Research Project

Project/Area Number 15K12191
Research Category

Grant-in-Aid for Challenging Exploratory Research

Allocation TypeMulti-year Fund
Research Field Environmental dynamic analysis
Research InstitutionUniversity of the Ryukyus

Principal Investigator

ARAKAKI Takemitsu  琉球大学, 理学部, 教授 (80343375)

Project Period (FY) 2015-04-01 – 2018-03-31
Project Status Completed (Fiscal Year 2017)
Budget Amount *help
¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2017: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2016: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2015: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywords大気エアロゾル / 臭素 / 光化学反応 / 活性酸素 / 有機物 / エアロゾル
Outline of Final Research Achievements

Ozone in the atmosphere can be drastically destroyed by reaction with active bromine species. Origin and formation mechanisms of active bromine species are of special interest since ozone affects atmospheric oxidation capacity. We have investigated chemical forms of bromine in atmospheric aerosols collected in Okinawa, Japan. We found that nearly half of marine originated bromine was vaporized from the aerosols to gas phase by forming gaseous species. The rest was ca. 40% water-soluble Br species, mainly Br-, and 5% water-insoluble Br species. Further study is needed to better understand transformation mechanisms of Br in aerosols.

Report

(4 results)
  • 2017 Annual Research Report   Final Research Report ( PDF )
  • 2016 Research-status Report
  • 2015 Research-status Report
  • Research Products

    (11 results)

All 2017 2015 Other

All Int'l Joint Research (3 results) Journal Article (2 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 2 results,  Acknowledgement Compliant: 2 results,  Open Access: 1 results) Presentation (6 results) (of which Int'l Joint Research: 3 results)

  • [Int'l Joint Research] Univ. of Dar es Salaam(Tanzania)

    • Related Report
      2016 Research-status Report
  • [Int'l Joint Research] University of Dar es Salaam(Tanzania)

    • Related Report
      2015 Research-status Report
  • [Int'l Joint Research]

    • Related Report
      2015 Research-status Report
  • [Journal Article] Role of the Fenton Reaction in Coastal Seawater Samples Collected in Okinawa2017

    • Author(s)
      Hamdun, A.M., Y. Higaonna, H. Uehara, Arakaki T.
    • Journal Title

      Chemistry Letters

      Volume: 46 Issue: 1 Pages: 42-44

    • DOI

      10.1246/cl.160894

    • NAID

      130005308308

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Int'l Joint Research / Acknowledgement Compliant
  • [Journal Article] Analysis of ground level ozone and nitrogen oxides in the city of Dar es Salaam, and Rural area Bagamoyo, Tanzania2015

    • Author(s)
      Hamdun A. M. and T. Arakaki
    • Journal Title

      Open Journal of Air Pollution

      Volume: 4 Issue: 04 Pages: 224-238

    • DOI

      10.4236/ojap.2015.44019

    • Related Report
      2015 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research / Acknowledgement Compliant
  • [Presentation] 過酸化水素による次亜塩素酸、次亜臭素酸の濃度測定及びモル吸光係数の決定2017

    • Author(s)
      上原裕幸、新垣雄光
    • Organizer
      日本分析化学会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 沖縄県比謝川水中の界面活性剤様有機物質に関する研究2017

    • Author(s)
      亀川碧、笠羽知羽、上原裕幸、新垣結奈、五十嵐洋一、金城信之、新垣遼、新垣雄光
    • Organizer
      日本分析化学会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Determination of concentration and molar absorptivity of hypochlorous acid and hypobromous acid species by hydrogen peroxide titration2017

    • Author(s)
      Uehara H. and T. Arakaki
    • Organizer
      AGU Fall Meeting
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Study on the surfactants present in atmospheric aerosols collected in Okinawa Japan2017

    • Author(s)
      Kamegawa, A., T. Kasaba, W. Shimabukuro, N. Kinjo, R. Arakaki, H. Uehara, Y. Arakaki, T. Arakaki
    • Organizer
      AGU Fall Meeting
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Spectroscopic characteristics and organic carbon contents in the aerosols collected in Okinawa, Japan2015

    • Author(s)
      Kasaba, T., A. Tsuhako, H. Murayama and T. Arakaki
    • Organizer
      AGU Fall Meeting
    • Place of Presentation
      Moscone Center, San Francisco
    • Year and Date
      2015-12-14
    • Related Report
      2015 Research-status Report
    • Int'l Joint Research
  • [Presentation] 沖縄辺戸岬で採取した大気エアロゾル中の有機物の特徴に関する研究2015

    • Author(s)
      笠羽知葉、津波古愛、村山仁美、新垣雄光
    • Organizer
      第56回大気環境学会年会
    • Place of Presentation
      早稲田大学
    • Year and Date
      2015-09-15
    • Related Report
      2015 Research-status Report

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Published: 2015-04-16   Modified: 2019-03-29  

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