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Intense investigation of the oxidation capacity of global atmosphere and its changes

Research Project

Project/Area Number 16H02937
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental dynamic analysis
Research InstitutionNagoya University

Principal Investigator

Sudo Kengo  名古屋大学, 環境学研究科, 准教授 (40371744)

Co-Investigator(Kenkyū-buntansha) 増永 浩彦  名古屋大学, 宇宙地球環境研究所, 准教授 (00444422)
Research Collaborator MIYAZAKI Kazuyuki  
ITO Akihiko  
Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥18,070,000 (Direct Cost: ¥13,900,000、Indirect Cost: ¥4,170,000)
Fiscal Year 2018: ¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000)
Fiscal Year 2017: ¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000)
Fiscal Year 2016: ¥7,150,000 (Direct Cost: ¥5,500,000、Indirect Cost: ¥1,650,000)
Keywords大気酸化能 / OHラジカル / 化学気候モデル / 化学輸送モデル / メタン / 対流圏オゾン / 光解離定数 / 物質循環 / 全球雲分布 / 化学気候モデリング
Outline of Final Research Achievements

This study improves the estimate of global distributions of hydroxy radical (OH) which controls oxidation and removal processes of various compounds in the atmosphere, and evaluates the recent change in the atmospheric oxidation capacity and its controlling mechanism. The estimate of OH distributions is improved by validating and elaborating the calculations of clouds, aerosols, and stratospheric ozone with combining a chemistry climate model simulation with the observational data as from satellite measurements. This study further investigates contributions of individual controlling factors of OH changes such as anthropogenic and natural emissions of nitrogen oxides (NOx), carbon monoxide (CO), volatile organic compounds (VOCs), in addition to the distributions of clouds, water vapor (H2O), and ozone.

Academic Significance and Societal Importance of the Research Achievements

本研究は、メタンをはじめ大気中の様々な物質の除去を担うOHラジカルの全球分布の推定を高精度化し、OH変動要因の定量的検討も行った。このような成果は、気候変動や大気環境変動の正確な予測・評価に大きく寄与し、今後の温室効果気体等の排出量削減シナリオの策定にも貢献が大である。また、次期IPCC報告書に向けたモデル間相互比較プロジェクトであるCMIP6、CCMI、およびAeroChem-MIPにも、本科研費課題の化学気候モデルを用いて参加しており、大気汚染が与える気候影響の理解の高精度化に寄与し、気候政策の策定にも大きく貢献する予定である。

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (38 results)

All 2019 2018 2017 2016 Other

All Int'l Joint Research (8 results) Journal Article (21 results) (of which Int'l Joint Research: 18 results,  Peer Reviewed: 21 results,  Open Access: 18 results,  Acknowledgement Compliant: 1 results) Presentation (9 results) (of which Int'l Joint Research: 2 results,  Invited: 2 results)

  • [Int'l Joint Research] University of Leeds(英国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] MIT/NCAR/NASA Goddard Space Flight Center(米国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Environment and Climate Change Canada/CCCMA, University of Victoria(カナダ)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] NIWA/Bodeker Scientific(ニュージーランド)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] University of Melbourne/University of New South Wales(オーストラリア)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research]

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] KNMI(オランダ)

    • Related Report
      2016 Annual Research Report
  • [Int'l Joint Research] NASA(米国)

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Quasi-Biennial Oscillations in Atmospheric Ozone from the Chemistry-Climate Model and Ozone Reanalysis2019

    • Author(s)
      Madhu Vazhathottathil、Sudo Kengo
    • Journal Title

      American Journal of Climate Change

      Volume: 08 Issue: 01 Pages: 110-136

    • DOI

      10.4236/ajcc.2019.81007

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] A new method (M<sup>3</sup>Fusion v1) for combining observations and multiple model output for an improved estimate of the global surface ozone distribution2019

    • Author(s)
      Chang Kai-Lan、Cooper Owen R.、West J. Jason、Serre Marc L.、Schultz Martin G.、Lin Meiyun、Mar?cal Virginie、Josse B?atrice、Deushi Makoto、Sudo Kengo、Liu Junhua、Keller Christoph A.
    • Journal Title

      Geoscientific Model Development

      Volume: 12 Issue: 3 Pages: 955-978

    • DOI

      10.5194/gmd-12-955-2019

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Balance of Emission and Dynamical Controls on Ozone During the Korea-United States Air Quality Campaign From Multiconstituent Satellite Data Assimilation2019

    • Author(s)
      Miyazaki K.、Sekiya T.、Fu D.、Bowman K. W.、Kulawik S. S.、Sudo K.、Walker T.、Kanaya Y.、Takigawa M.、Ogochi K.、Eskes H.、Boersma K. F.、Thompson A. M.、Gaubert B.、Barre J.、Emmons L. K.
    • Journal Title

      Journal of Geophysical Research: Atmospheres

      Volume: 124 Issue: 1 Pages: 387-413

    • DOI

      10.1029/2018jd028912

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Ozone sensitivity to varying greenhouse gases and ozone-depleting substances in CCMI-1 simulations2018

    • Author(s)
      Morgenstern O.、Stone K. A.、Schofield R.、Akiyoshi H.、Yamashita Y.、Kinnison D. E.、Garcia R. R.、Sudo K.、Plummer D. A.、Scinocca J.、Oman L. D.、Manyin M. E.、Zeng G.、Rozanov E.、Stenke A.、Revell L. E.、Pitari G.、Mancini E.、Di Genova G.、Visioni D.、Dhomse S. S.、Chipperfield M. P.
    • Journal Title

      Atmospheric Chemistry and Physics

      Volume: 18 Issue: 2 Pages: 1091-1114

    • DOI

      10.5194/acp-18-1091-2018

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Extremal dependence between temperature and ozone over the continental US2018

    • Author(s)
      Phalitnonkiat Pakawat、Hess Peter G. M.、Grigoriu Mircea D.、Samorodnitsky Gennady、Sun Wenxiu、Beaudry Ellie、Tilmes Simone、Deushi Makato、Josse Beatrice、Plummer David、Sudo Kengo
    • Journal Title

      Atmospheric Chemistry and Physics

      Volume: 18 Issue: 16 Pages: 11927-11948

    • DOI

      10.5194/acp-18-11927-2018

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Two-scale multi-model ensemble: is a hybrid ensemble of opportunity telling us more?2018

    • Author(s)
      Galmarini Stefano、Kioutsioukis Ioannis、Solazzo Efisio、Alyuz Ummugulsum、Balzarini Alessandra、Bellasio Roberto、Benedictow Anna M. K.、Bianconi Roberto、Bieser Johannes、Brandt Joergen、Christensen Jesper H.、Colette Augustin、Curci Gabriele、Davila Yanko、Dong Xinyi、Sudo Kengo、et al.
    • Journal Title

      Atmospheric Chemistry and Physics

      Volume: 18 Issue: 12 Pages: 8727-8744

    • DOI

      10.5194/acp-18-8727-2018

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Ultraviolet Radiation modelling using output from the ChemistryClimate Model Initiative2018

    • Author(s)
      Lamy K?vin、Sudo Kengo、Tanaka Taichu Y.、Visioni Daniele、Yoshida Kohei
    • Journal Title

      Atmospheric Chemistry and Physics Discussions

      Volume: 18 Pages: 1-34

    • DOI

      10.5194/acp-2018-525

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] The effects of intercontinental emission sources on European air pollution levels2018

    • Author(s)
      Jonson Jan Eiof、Schulz Michael、Emmons Louisa、Flemming Johannes、Henze Daven、Sudo Kengo、Tronstad Lund Marianne、Lin Meiyun、Benedictow Anna、Koffi Brigitte、Dentener Frank、Keating Terry、Kivi Rigel、Davila Yanko
    • Journal Title

      Atmospheric Chemistry and Physics

      Volume: 18 Issue: 18 Pages: 13655-13672

    • DOI

      10.5194/acp-18-13655-2018

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Multi-model study of HTAP?II on sulfur and nitrogen deposition2018

    • Author(s)
      Tan Jiani、Fu Joshua S.、Dentener Frank、Sun Jian、Emmons Louisa、Tilmes Simone、Sudo Kengo、Flemming Johannes、Jonson Jan Eiof、Gravel Sylvie、Bian Huisheng、Davila Yanko、Henze Daven K.、Lund Marianne T.、Kucsera Tom、Takemura Toshihiko、Keating Terry
    • Journal Title

      Atmospheric Chemistry and Physics

      Volume: 18 Issue: 9 Pages: 6847-6866

    • DOI

      10.5194/acp-18-6847-2018

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] HTAP2 multi-model estimates of premature human mortality due to intercontinental transport of air pollution and emission sectors2018

    • Author(s)
      Liang Ciao-Kai、West J. Jason、Silva Raquel A.、Bian Huisheng、Chin Mian、Davila Yanko、Dentener Frank J.、Emmons Louisa、Flemming Johannes、Folberth Gerd、Henze Daven、Sudo Kengo、et al.
    • Journal Title

      Atmospheric Chemistry and Physics

      Volume: 18 Issue: 14 Pages: 10497-10520

    • DOI

      10.5194/acp-18-10497-2018

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Estimates of ozone return dates from Chemistry-Climate Model Initiative simulations2018

    • Author(s)
      Dhomse Sandip S.、Kinnison Douglas、Chipperfield Martyn P.、Salawitch Ross J.、Cionni Irene、Hegglin Michaela I.、Abraham N. Luke、Akiyoshi Hideharu、Archibald Alex T.、Bednarz Ewa M.、Bekki Slimane、Sudo Kengo、Tilmes Simone、Visioni Daniele、Yamashita Yousuke、Zeng Guang, et al.
    • Journal Title

      Atmospheric Chemistry and Physics

      Volume: 18 Issue: 11 Pages: 8409-8438

    • DOI

      10.5194/acp-18-8409-2018

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Long-range transport impacts on surface aerosol concentrations and the contributions to haze events in China: an HTAP2 multi-model study2018

    • Author(s)
      Dong Xinyi、Fu Joshua S.、Zhu Qingzhao、Sun Jian、Tan Jiani、Keating Terry、Sekiya Takashi、Sudo Kengo、Emmons Louisa、Tilmes Simone、Jonson Jan Eiof、Schulz Michael、Bian Huisheng、Chin Mian、Davila Yanko、Henze Daven、Takemura Toshihiko、Benedictow Anna Maria Katarina、Huang Kan
    • Journal Title

      Atmospheric Chemistry and Physics

      Volume: 18 Issue: 21 Pages: 15581-15600

    • DOI

      10.5194/acp-18-15581-2018

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Review of the global models used within phase 1 of the Chemistry-Climate Model Initiative (CCMI)2017

    • Author(s)
      Morgenstern, O, M. I. Hegglin, E. Rozanov, F. M. O’Connor, N. L. Abraham, H. Akiyoshi, A. T. Archibald, S. Bekki, N. Butchart, M. P. Chipperfield et al.
    • Journal Title

      Geosci. Model Dev.

      Volume: 10 Issue: 2 Pages: 639-671

    • DOI

      10.5194/gmd-10-639-2017

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Investigation of global particulate nitrate from the AeroCom phase-III experiment2017

    • Author(s)
      Bian Huisheng、Chin Mian、Hauglustaine Didier A.、Schulz Michael、Myhre Gunnar、Bauer Susanne E.、Lund Marianne T.、Karydis Vlassis A.、Kucsera Tom L.、Pan Xiaohua、Pozzer Andrea、Skeie Ragnhild B.、Steenrod Stephen D.、Sudo Kengo、Tsigaridis Kostas、Tsimpidi Alexandra P.、Tsyro Svetlana G.
    • Journal Title

      Atmos. Chem. Phys.

      Volume: 17 Issue: 21 Pages: 12911-12940

    • DOI

      10.5194/acp-17-12911-2017

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Formaldehyde in the Tropical Western Pacific: Chemical Sources and Sinks, Convective Transport, and Representation in CAM-Chem and the CCMI Models2017

    • Author(s)
      Anderson Daniel C.、Nicely Julie M.、Wolfe Glenn M.、Hanisco Thomas F.、Kengo Sudo、et al.
    • Journal Title

      J. Geophs. Res.-Atmos.

      Volume: 122 Issue: 20

    • DOI

      10.1002/2016jd026121

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Corrigendum: Future global mortality from changes in air pollution attributable to climate change2017

    • Author(s)
      Silva Raquel A.、West J. Jason、Lamarque Jean-Fran?ois、Shindell Drew T.、Kengo Sudo、et al.
    • Journal Title

      Nat. Clim. Change

      Volume: 7 Issue: 11 Pages: 845-845

    • DOI

      10.1038/nclimate3427

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Long-term change in the source contribution to surface ozone over Japan2017

    • Author(s)
      Nagashima Tatsuya、Sudo Kengo、Akimoto Hajime、Kurokawa Junichi、Ohara Toshimasa
    • Journal Title

      Atmos. Chem. Phys.

      Volume: 17 Issue: 13 Pages: 8231-8246

    • DOI

      10.5194/acp-17-8231-2017

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Impact of intercontinental pollution transport on North American ozone air pollution: an HTAP phase 2 multi-model study2017

    • Author(s)
      Huang Min、Carmichael Gregory R.、Pierce R. Bradley、Jo Duseong S.、Park Rokjin J.、Flemming Johannes、Emmons Louisa K.、Bowman Kevin W.、Henze Daven K.、Davila Yanko、Sudo Kengo、Jonson Jan Eiof、Tronstad Lund Marianne、Janssens-Maenhout Greet、Dentener Frank J.、Keating Terry J.、Oetjen Hilke、Payne Vivienne H.
    • Journal Title

      Atmos. Chem. Phys.

      Volume: 17 Issue: 9 Pages: 5721-5750

    • DOI

      10.5194/acp-17-5721-2017

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] 化学気候モデルで探る大気微量成分の全球変動2017

    • Author(s)
      須藤健悟
    • Journal Title

      大気化学研究

      Volume: 36

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Journal Article] Decadal changes in global surface NOx emissions from multi-constituent satellite data assimilation2017

    • Author(s)
      Miyazaki, K., Eskes, H., Sudo, K., Boersma, K. F., Bowman, K., and Kanaya, Y
    • Journal Title

      Atmos. Chem. Phys

      Volume: 17 Issue: 2 Pages: 807-837

    • DOI

      10.5194/acp-17-807-2017

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Evolution of stratospheric sulfate aerosol from the 1991 Pinatubo eruption: Roles of aerosol microphysical processes2016

    • Author(s)
      T. Sekiya, K. Sudo
    • Journal Title

      J. Geophys. Res. Atmos.

      Volume: 121 Issue: 6 Pages: 2911-2938

    • DOI

      10.1002/2015jd024313

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed
  • [Presentation] 微量気体SLCPsの長期変動と気候影響2018

    • Author(s)
      須藤健悟, 長谷川晃一, 竹村俊彦
    • Organizer
      日本気象学会2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Improving estimation of global BVOCs emissions using ground-based VOCs observations and satellite data of atmospheric HCHO2018

    • Author(s)
      須藤健悟, 趙舒悦, 宮崎和幸, 伊藤昭彦
    • Organizer
      地球惑星科学連合大会(JPGU) 2018年5月22日、幕張
    • Related Report
      2018 Annual Research Report
  • [Presentation] Source attribution and budget analysis of black carbon in Antarctica2018

    • Author(s)
      大西貴都, 須藤健悟, 原圭一郎
    • Organizer
      地球惑星科学連合大会(JPGU) 2018年5月22日、幕張
    • Related Report
      2018 Annual Research Report
  • [Presentation] Interannual variability and long-term trends in global tropospheric chemistry and aerosols during recent decades and in the future2017

    • Author(s)
      Kengo Sudo
    • Organizer
      Chemistry-Climate Model Initiative Science Workshop 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] アジア・中国域からのエアロゾル流出量の季節・経年変動とその要因2017

    • Author(s)
      須藤健悟、山下剛史、竹村俊彦
    • Organizer
      日本気象学会2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Seasonal and interannual variation in aerosol outflow from Asia/China and its controlling factors2017

    • Author(s)
      須藤健悟、山下剛史、竹村俊彦
    • Organizer
      地球惑星科学連合大会(JPGU)
    • Related Report
      2017 Annual Research Report
  • [Presentation] Interannual variability and long-term trends in global tropospheric ozone and related chemistry during recent decades2016

    • Author(s)
      Kengo Sudo
    • Organizer
      Quadrennial Ozone Symposium 2016
    • Place of Presentation
      Edinburgh, United Kingdom
    • Year and Date
      2016-09-04
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 衛星観測・全球化学輸送モデルによるホルムアルデヒドの全球収支とBVOCSエミッション量の推定2016

    • Author(s)
      須藤健悟, 磯野結貴, 宮崎和幸
    • Organizer
      地球惑星科学連合大会(JPGU)2016
    • Place of Presentation
      幕張
    • Year and Date
      2016-05-26
    • Related Report
      2016 Annual Research Report
  • [Presentation] 中国域におけるエアロゾルの収支解析:濃度と流出量の経年変動2016

    • Author(s)
      山下剛史, 須藤健悟
    • Organizer
      地球惑星科学連合大会(JPGU)2016
    • Place of Presentation
      幕張
    • Year and Date
      2016-05-26
    • Related Report
      2016 Annual Research Report

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Published: 2016-04-21   Modified: 2022-10-07  

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