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Laser flash Raman spectroscopy method and heat transfer performance of novel low-dimensional materials

Research Project

Project/Area Number 16H04280
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Thermal engineering
Research InstitutionKyushu University

Principal Investigator

Zhang Xing  九州大学, カーボンニュートラル・エネルギー国際研究所, 主任研究者 (40236823)

Co-Investigator(Kenkyū-buntansha) 高橋 厚史  九州大学, 工学研究院, 教授 (10243924)
Wang Haidong  九州大学, 工学研究院, 助教 (30729405)
Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥17,680,000 (Direct Cost: ¥13,600,000、Indirect Cost: ¥4,080,000)
Fiscal Year 2018: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Fiscal Year 2017: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2016: ¥10,790,000 (Direct Cost: ¥8,300,000、Indirect Cost: ¥2,490,000)
Keywordsナノマイクロ熱工学 / 熱伝導率 / ラマン分光 / 界面熱抵抗 / ナノフルイディクス / a
Outline of Final Research Achievements

A new method to measure the thermophysical property of nanomaterials was developed. This laser flash Raman spectroscopy method, using repetitive pulse heating, enabled us to determine the thermal conductivity, specific heat and thermal boundary resistance of graphene. Liquid in nanotube was also treated to create new composite materials and it was fond that the nano-confined water shows very stable state even in a very high-vacuum environment.

Academic Significance and Societal Importance of the Research Achievements

ナノ材料はフィラーとして用いることで熱伝導を大きく改善する可能性があるが、欠陥や環境因子によって熱伝導率が大きく変わりうることも知られている。その物理機構を解明し、工業的に再現性良く利用するためには、熱物性を精度よく計測する手法が不可欠である。そこで、本研究ではこれまでの計測法の問題点を解決する新しい計測法を開発するとともに、ナノ材料に液体を複合させるという新規材料についての基礎研究を行った。

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (52 results)

All 2019 2018 2017 2016 Other

All Int'l Joint Research (5 results) Journal Article (19 results) (of which Int'l Joint Research: 12 results,  Peer Reviewed: 19 results,  Open Access: 1 results,  Acknowledgement Compliant: 3 results) Presentation (28 results) (of which Int'l Joint Research: 23 results,  Invited: 5 results)

  • [Int'l Joint Research] Tsinghua University(中国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] The University of Edinburgh(英国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] 清華大学(中国)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] エジンバラ大学(英国)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] 清華大学(中国)

    • Related Report
      2016 Annual Research Report
  • [Journal Article] Dual-Wavelength Laser Flash Raman Spectroscopy Method for In-Situ Measurements of the Thermal Diffusivity: Principle and Experimental Verification2019

    • Author(s)
      Fan Aoran、Hu Yudong、Ma Weigang、Wang Haidong、Zhang Xing
    • Journal Title

      Journal of Thermal Science

      Volume: 28 Issue: 2 Pages: 159-168

    • DOI

      10.1007/s11630-019-1084-x

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Differential laser flash Raman spectroscopy method for non-contact characterization of thermal transport properties of individual nanowires2019

    • Author(s)
      Liu Jinhui、Liu Hao、Hu Yudong、Zhang Xing
    • Journal Title

      International Journal of Heat and Mass Transfer

      Volume: 135 Pages: 511-516

    • DOI

      10.1016/j.ijheatmasstransfer.2019.01.107

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Non-contact T-type Raman method for measurement of thermophysical properties of micro-/nanowires2019

    • Author(s)
      Liu Jinhui、Liu Hao、Ma Weigang、Zhang Xing
    • Journal Title

      Review of Scientific Instruments

      Volume: 90 Issue: 4 Pages: 044901-044901

    • DOI

      10.1063/1.5080728

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Measurement of thermal contact resistance between individual carbon fibers using a laser-flash Raman mapping method2019

    • Author(s)
      Li, Qin-Yi; Katakami, Koki; Ikuta, Tatsuya; Kohno, Masamichi; Zhang, Xing; Takahashi, Koji;
    • Journal Title

      Carbon

      Volume: 141 Pages: 92-98

    • DOI

      10.1016/j.carbon.2018.09.034

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Frequency-domain Raman method to measure thermal diffusivity of one-dimensional microfibers and nanowires2019

    • Author(s)
      Li, Qin-Yi; Takahashi, Koji; Zhang, Xing;
    • Journal Title

      International Journal of Heat and Mass Transfer

      Volume: 134 Pages: 539-546

    • DOI

      10.1016/j.ijheatmasstransfer.2019.01.057

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Unexpected Homogeneous Bubble Nucleation near a SolidィCLiquid Interface2018

    • Author(s)
      Tomo, Yoko; Li, Qin-Yi; Ikuta, Tatsuya; Takata, Yasuyuki; Takahashi, Koji;
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 122 Issue: 50 Pages: 28712-28716

    • DOI

      10.1021/acs.jpcc.8b09200

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Meniscus Motion and Void Generation Inside Carbon Nanotubes2018

    • Author(s)
      Yamada Yutaka、Taguchi Kanoko、Ikuta Tatsuya、Horibe Akihiko、Takahashi Koji
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 122 Issue: 38 Pages: 21910-21918

    • DOI

      10.1021/acs.jpcc.8b06406

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Variable-spot-size laser-flash Raman method to measure in-plane and interfacial thermal properties of 2D van der Waals heterostructures2018

    • Author(s)
      Li, Qin-Yi; Zhang, Xing; Takahashi, Koji;
    • Journal Title

      International Journal of Heat and Mass Transfer

      Volume: 125 Pages: 1230-1239

    • DOI

      10.1016/j.ijheatmasstransfer.2018.05.011

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Joule heating and laser flash tip-enhanced Raman spectroscopy method for characterizing the specific heat of a single nanoparticle2018

    • Author(s)
      Fan, Aoran; Li, Qinyi; Ma, Weigang; Zhang, Xing;
    • Journal Title

      Chinese Science Bulletin

      Volume: 63 Issue: 27 Pages: 2896-2903

    • DOI

      10.1360/n972018-00294

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Heater assisted Raman method to measure interfacial thermal conductance in van der Waals heterostructures2018

    • Author(s)
      Qinyi Li, Koji Takahashi, Xing Zhang
    • Journal Title

      Proceedings of the 16th International Heat Transfer Conference

      Volume: 1 Pages: 21756-21756

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Wettability of AFM tip influences the profile of interfacial nanobubbles2018

    • Author(s)
      Hideaki Teshima, Koji Takahashi, Yasuyuki Takata, Takashi Nishiyama
    • Journal Title

      Journal of Applied Physics

      Volume: 123 Issue: 5 Pages: 054303-054303

    • DOI

      10.1063/1.5010131

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Superstable Ultrathin Water Film Confined in a Hydrophilized Carbon Nanotube2018

    • Author(s)
      Tomo Yoko、Askounis Alexandros、Ikuta Tatsuya、Takata Yasuyuki、Sefiane Khellil、Takahashi Koji
    • Journal Title

      Nano Letters

      Volume: 18 Issue: 3 Pages: 1869-1874

    • DOI

      10.1021/acs.nanolett.7b05169

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Experimental study of thermal rectification in suspended monolayer graphene2017

    • Author(s)
      Wang Haidong、Hu Shiqian、Takahashi Koji、Zhang Xing、Takamatsu Hiroshi、Chen Jie
    • Journal Title

      Nature Communications

      Volume: 8 Issue: 1 Pages: 15843-15843

    • DOI

      10.1038/ncomms15843

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Measurement of specific heat and thermal conductivity of supported and suspended graphene by a comprehensive Raman optothermal method2017

    • Author(s)
      Li Qin-Yi、Xia Kailun、Zhang Ji、Zhang Yingying、Li Qunyang、Takahashi Koji、Zhang Xing
    • Journal Title

      Nanoscale

      Volume: 9 Issue: 30 Pages: 10784-10793

    • DOI

      10.1039/c7nr01695f

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Experimental study on thermal conductivity of free-standing fluorinated single-layer graphene2017

    • Author(s)
      Narasaki Masahiro、Wang Haidong、Nishiyama Takashi、Ikuta Tatsuya、Takahashi Koji
    • Journal Title

      Applied Physics Letters

      Volume: 111 Issue: 9 Pages: 093103-093103

    • DOI

      10.1063/1.5001169

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nanoscale pinning effect evaluated from deformed nanobubbles2017

    • Author(s)
      Hideaki Teshima, Takashi Nishiyama, Koji Takahashi
    • Journal Title

      The Journal of Chemical Physics

      Volume: 146 Issue: 1 Pages: 014708-014708

    • DOI

      10.1063/1.4973385

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Nanobubble nucleation studied using Fresnel fringes in liquid cell electron microscopy2017

    • Author(s)
      Yoko TOMO, Koji TAKAHASHI, Takashi NISHIYAMA, Tatsuya IKUTA, Yasuyuki TAKATA
    • Journal Title

      International Journal of Heat and Mass Transfer

      Volume: 108 Pages: 1460-1465

    • DOI

      10.1016/j.ijheatmasstransfer.2017.01.013

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Temperature-dependent specific heat of suspended platinum nanofilms at 80?380 K2016

    • Author(s)
      Li Qin-Yi、Narasaki Masahiro、Takahashi Koji、Ikuta Tatsuya、Nishiyama Takashi、Zhang Xing
    • Journal Title

      Chinese Physics B

      Volume: 25 Issue: 11 Pages: 114401-114401

    • DOI

      10.1088/1674-1056/25/11/114401

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Influence of ion beam scattering on the electrical resistivity of platinum hot films2016

    • Author(s)
      Masahiro Narasaki, Haidong Wang, Yasuyuki Takata, Koji Takahashi
    • Journal Title

      Microelectronic Engineering

      Volume: 166 Pages: 15-18

    • DOI

      10.1016/j.mee.2016.09.008

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] Thermophysical property measurements of two-dimensional sheets and ribbons2019

    • Author(s)
      Qin-Yi Li
    • Organizer
      Sendai "Plasma Forum"
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] TEM and AFM Studies of Bubble Nucleation and Growth Near Solid-Liquid Interfaces2019

    • Author(s)
      Koji Takahashi
    • Organizer
      Gordon Research Conference: Micro and Nanoscale Phase Change Heat Transfer
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 非定常ラマン光熱法とその応用2018

    • Author(s)
      李秦宜,張興,高橋厚史
    • Organizer
      第56回日本伝熱シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] カーボンナノチューブ内の純水液膜の安定性に関する実験的研究2018

    • Author(s)
      塘陽子, Askounis Alexandros, 生田竜也, 高田保之, Sefiane Khellil, 高橋厚史
    • Organizer
      第55回日本伝熱シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] Bubbles and droplets at the initial stage of nucleation: recent advances in experimental techniques2018

    • Author(s)
      Koji Takahashi
    • Organizer
      16th International Heat Transfer Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Influence of surface wettability and nanostructure on the generation of interfacial nanobubbles2018

    • Author(s)
      Hideaki Teshima,Takashi Nishiyama, Yasuyuki Takata, Koji Takahashi
    • Organizer
      16th International Heat Transfer Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Effective thermal rectification in suspended monolayer graphene2018

    • Author(s)
      Haidong Wang,Xing Zhang,Hiroshi Takamatsu,Koji Takahashi
    • Organizer
      16th International Heat Transfer Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Study on liquid-gas interface at nanoscale using transmission electron microscopy2018

    • Author(s)
      Yoko Tomo,Alexandros Askounis, Khellil Sefiane, Yasuyuki Takata, Koji Takahashi
    • Organizer
      16th International Heat Transfer Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Molecular dynamics simulation of the structure effect on interfacial thermal resistance between graphene and silicon2018

    • Author(s)
      Aoran Fan, Weigang Ma, Xing Zhang
    • Organizer
      16th International Heat Transfer Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Heater assisted Raman method to measure interfacial thermal conductance in van der Waals heterostructures2018

    • Author(s)
      Qin-Yi Li,Koji Takahashi,Xing Zhang
    • Organizer
      16th International Heat Transfer Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] T-type Raman method for non-contact characterization of thermal transport properties of individual nanowires2018

    • Author(s)
      Jinhui Liu, Yudong Hu, Xing Zhang
    • Organizer
      16th International Heat Transfer Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Size-dependent thermal conductivity of suspended monolayer graphene2018

    • Author(s)
      Ruixia Su, Weigang Ma, Xing Zhang
    • Organizer
      16th International Heat Transfer Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Frequency-domain Raman Optothermal Method to Measure Thermal and Optical Properties of 2D Materials and Heterostructures2018

    • Author(s)
      Qin-Yi Li,Koji Takahashi,Xing Zhang
    • Organizer
      19th International Conference on the Science and Application of Nanotubes and Low-Dimensional Materials
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Nanomaterials and Nanobubles for Heat Transfer2018

    • Author(s)
      Koji Takahashi
    • Organizer
      6th UK Japan Engineering Education League Workshop 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Bubble Generation and Growth in a Nano Liquid Cell and a Carbon Nanotube2018

    • Author(s)
      Yoko Tomo, Alexandros Askounis, Yasuyuki Takata, Koji Takahashi
    • Organizer
      5th European Conference on MicroFluidics 2018 (μFlu'18) , Feb.28 - March 2, Strasbourg, France
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Simultaneous measurement of thermal contact resistance between individual carbon fibers and their thermal diffusivity using a laser-flash Raman mapping method2018

    • Author(s)
      Koki Katakami, Qinyi Li, Tatsuya Ikuta, Koji Takahashi
    • Organizer
      3rd Thermal and Fluids Engineering Conference (TFEC) March 4-7, 2018, Ft. Lauderdale, FL, USA
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dual-mode Raman method to measure in-plane and interfacial thermophysical properties of 2D van der Waals heterostructures2017

    • Author(s)
      Li Q Y, Zhang X, Takahashi K.
    • Organizer
      2017 MRS Spring Meeting. Apr. 17-21, 2017, Phoenix, Arizona, US.
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 2次元材料のヘテロ構造の熱物性を計測するデュアルモードラマン分光法の開発2017

    • Author(s)
      李 秦宜, 張 興, 高橋 厚史
    • Organizer
      第54回伝熱シンポジウム. 2017年5月24日-26日,大宮市
    • Related Report
      2017 Annual Research Report
  • [Presentation] フッ化単層グラフェンの熱伝導率計測2017

    • Author(s)
      楢崎将弘、王海東、生田竜也、西山貴史、高橋厚史
    • Organizer
      第54回伝熱シンポジウム. 2017年5月24日-26日,大宮市
    • Related Report
      2017 Annual Research Report
  • [Presentation] Thermal Transport of Fluorinated Single-Layer Graphene2017

    • Author(s)
      Masahiro Narasaki, Haidong Wang, Tatsuya Ikuta, Takashi Nishiyama, Koji Takahashi
    • Organizer
      The 9th World Conference on Experimental Heat Tranfer, Fluid Mechanics and Thermodynamics, Foz do Iguacu, Brazil, 13th June, 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dual-mode Raman method to measure thermal transport properties of 2D materials and van der Waals heterostructures.2017

    • Author(s)
      Li Q Y, Zhang X, Takahashi K.
    • Organizer
      The 9th US-Japan Joint Seminar on Nanoscale Transport Phenomena, July 2-5, 2017, Tokyo, Japan.
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Direct Observation of Heterogeneous Bubble Nucleation in Nanoscale2017

    • Author(s)
      Yoko Tomo, Koji Takahashi, Tatsuya Ikuta, Yasuyuki Takata
    • Organizer
      International conference on nanochannels, microchannels, and minichannels, August 27-30, 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Experimental Approach to Control the Thermal Conductivity of Single-Layer Graphene by Fluorination2017

    • Author(s)
      Masahiro Narasaki, Haidong Wang, Yasuyuki Takata, Tatsuya Ikuta, Koji Takahashi
    • Organizer
      International Mechanical Engineering Congress and Exposition, Tampa, USA, 8th November, 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Highly sensitive charge mobility of suspended monolayer graphene2017

    • Author(s)
      Haidong Wang, Koji Takahashi, Hiroshi Takamatsu, Xing Zhang
    • Organizer
      The 6th International Symposium on Micro and Nano Technology, ISMNT-6, March 19-22, 2017, Fukuoka, Japan
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] IN SITU THERMAL CONDUCTANCE MEASUREMENT OF AN INDIVIDUAL CARBON NANOFIBER DEFECTED BY FOCUSED ION BEAM2016

    • Author(s)
      M. Narasaki, K. Takahashi, J. Miyawaki, Y. Takata
    • Organizer
      7th European Thermal-Sciences Conference, EUROTHERM 2016, 19-23 June 2016, Krakow, Poland
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Experimental Study of Nanobubbles and Nanodroplets on Hydrophilic/Hydrophobic Combined Surfaces2016

    • Author(s)
      Koji Takahashi, Takashi Nishiyama, Yutaka Yamada and Yasuyuki Takata
    • Organizer
      12th International Conference on Heat Transfer, Fluid Mechanics and Thermodynamics (HEFAT2016), 11 to 13 July 2016, Costa del Sol, Spain
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] TEM Study on Phase Change in a Nano Liquid Cell2016

    • Author(s)
      Yoko TOMO, Koji TAKAHASHI, Takashi NISHIYAMA, Tatsuya IKUTA, Yasuyuki TAKATA
    • Organizer
      5th Micro and Nano Flows Conference, Milan, Italy, 11-14 September 2016
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research
  • [Presentation] THERMAL TRANSPORT IN MULTI-WALLED CARBON NANOTUBE AND CARBON NANOFIBER DEFECTED BY FOCUSED ION BEAM2016

    • Author(s)
      M. Narasaki, J. Miyawaki, T. Ikuta, T. Nishiyama and K. Takahashi
    • Organizer
      The 27th International Symposium on Transport Phenomena, 20-23 September 2016, Honolulu, USA
    • Related Report
      2016 Annual Research Report
    • Int'l Joint Research

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Published: 2016-04-21   Modified: 2022-06-10  

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