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Formation of highly-efficient photoenergy conversion fields by controlling configuration and orientation of anisotropic metal nanoparticles

Research Project

Project/Area Number 16H06120
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Structural/Functional materials
Research InstitutionKyushu University

Principal Investigator

Takahashi Yukina  九州大学, カーボンニュートラル・エネルギー国際研究所, 准教授 (10596076)

Project Period (FY) 2016-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥25,220,000 (Direct Cost: ¥19,400,000、Indirect Cost: ¥5,820,000)
Fiscal Year 2019: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Fiscal Year 2018: ¥3,510,000 (Direct Cost: ¥2,700,000、Indirect Cost: ¥810,000)
Fiscal Year 2017: ¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2016: ¥13,910,000 (Direct Cost: ¥10,700,000、Indirect Cost: ¥3,210,000)
Keywords金属ナノ粒子 / 局在表面プラズモン共鳴 / 光電気化学 / エネルギー全般 / マイクロ・ナノデバイス / ナノ材料
Outline of Final Research Achievements

In this study, I engaged to establish the novel and highly-efficient photoenergy conversion systems by controlling plasmonic metal nanoparticles.
First, I developed novel hydrophobization method of gold nanoparticles with larger size than before. I also succeeded in fabrication of monolayer films of the gold nanoparticles. I revealed that the diameter of gold nanoparticles can control their optical properties. Then, I applied the method to anisotropic metal nanoparticles. I also obtained their monolayer films which were controlled with the density and the orientation. Furthermore, I succeeded in the formation of the polymeric dyes located around the nanoparticles appropriately in nanoscale for highly effective photoenergy conversion systems.
These technologies should progress the field of photoenergy conversion systems with high efficiency.

Academic Significance and Societal Importance of the Research Achievements

本課題で確立した、金属ナノ粒子の光捕集効果を含む光学特性を制御する技術は、さまざまな光反応系に適用可能である。近赤外光まで利用可能であるため、従来系の光エネルギー利用において高効率化に大きく貢献し得る技術である。
また、デバイスの実現と機構の解明は両輪であるが、本課題の遂行を通して、詳細な機構にいまだ諸説があるプラズモン誘起電荷分離の、酸化力発生機構を提案するなど、新規な高効率光エネルギー変換システムの開発にも大いに役立つ知見が得られた。
以上のように、光エネルギーの高効率利用という課題に対して、社会的にも学術的にも大きなインパクトのある成果を上げることに成功した。

Report

(5 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • 2016 Annual Research Report
  • Research Products

    (36 results)

All 2020 2019 2018 2017 Other

All Journal Article (7 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 6 results,  Open Access: 1 results) Presentation (26 results) (of which Int'l Joint Research: 8 results,  Invited: 10 results) Remarks (2 results) Funded Workshop (1 results)

  • [Journal Article] Oxidation Reaction Energy in Photopolymerization Inspired by Plasmon-Induced Charge Separation2020

    • Author(s)
      Y. Takahashi, Y. Sota, T. Ishida, Y. Furukawa, S. Yamada
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 124 Issue: 7 Pages: 4202-4205

    • DOI

      10.1021/acs.jpcc.9b09738

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] プラズモニックナノ粒子の 熱力学的安定性の制御2020

    • Author(s)
      髙橋幸奈
    • Journal Title

      伝熱

      Volume: 59 Pages: 22-26

    • Related Report
      2019 Annual Research Report
  • [Journal Article] Development and Analytical Application of Nanosystems for Photoenergy Storage and Localization2019

    • Author(s)
      高橋幸奈
    • Journal Title

      BUNSEKI KAGAKU

      Volume: 68 Issue: 10 Pages: 777-782

    • DOI

      10.2116/bunsekikagaku.68.777

    • NAID

      130007742411

    • ISSN
      0525-1931
    • Year and Date
      2019-10-05
    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Space Optimization for Utilization of Plasmonic Effect on a P3HT-Gold Nanoparticle Photoelectrode2017

    • Author(s)
      Takuya Ishida, Miho Katagishi, Yukina Takahashi, and Sunao Yamada
    • Journal Title

      Chem. Lett.

      Volume: 46 Issue: 11 Pages: 1612-1615

    • DOI

      10.1246/cl.170707

    • NAID

      130006837431

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Structural characterization and plasmonic properties of two-dimensional arrays of hydrophobic large gold nanoparticles fabricated by Langmuir-Blodgett technique2017

    • Author(s)
      Takuya Ishida, Yuki Tachikiri, Takayuki Sako, Yukina Takahashi, Sunao Yamada
    • Journal Title

      Applied Surface Science

      Volume: 404 Pages: 350-356

    • DOI

      10.1016/j.apsusc.2017.01.304

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 金属ナノ構造の局在表面プラズモン共鳴を用いた光エネルギー変換2017

    • Author(s)
      高橋幸奈, 山田 淳
    • Journal Title

      Journal of the Japan Society of Colour Material

      Volume: 90 Pages: 426-430

    • NAID

      130006301972

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Influence of space arrangement of silver nanoparticles in organic photoelectric conversion devices2017

    • Author(s)
      Jing You, Yukina Takahashi, Kwati Leonard, Hiroaki Yonemura, Sunao Yamada
    • Journal Title

      Journal of Photochemistry and Photobiology A: Chemistry

      Volume: 332 Pages: 586-594

    • DOI

      10.1016/j.jphotochem.2016.09.023

    • Related Report
      2016 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] 金属ナノ粒子/p 型半導体界面での新型プラズモン誘起電荷分離を利用した 全固体光電変換セルの開発2020

    • Author(s)
      髙橋 幸奈,村山 太郎,中野 友里花,山田 淳
    • Organizer
      電気化学会第87回大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Nanosystems of Metals and Semiconductors for Analytical and Photoelectrochemical Applications2019

    • Author(s)
      Y. Takahashi
    • Organizer
      International Workshop on Advanced Nanoscience and Nanomaterials 2019 (IWANN2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Development of all-solid-state photoelectric conversion cells based on new type plasmon induced charge separation (PICS) with p-type semiconductors2019

    • Author(s)
      T. Murayama, S. Shingo, S. Yamada, Y. Takahashi
    • Organizer
      International Workshop on Advanced Nanoscience and Nanomaterials 2019 (IWANN2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 金属ナノ粒子の会合状態が局在表面プラズモン共鳴特性に与える効果2019

    • Author(s)
      髙橋幸奈
    • Organizer
      OCU先端光科学シンポジウムーナノフォトニクスが切り拓く分子運動・化学反応制御の探求ー
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Evaluation of plasmon induced charge separation (PICS) with p-type semiconductor for all-solid-state photoelectric cells2019

    • Author(s)
      村山太郎, 新郷翔太, 山田 淳, 髙橋幸奈
    • Organizer
      光化学討論会2019
    • Related Report
      2019 Annual Research Report
  • [Presentation] Development of optimal design of plasmonic metal nanoparticles for practical application2019

    • Author(s)
      Y. Takahashi
    • Organizer
      SPIE Conference 11082: Plasmonics: Design, Materials, Fabrication, Characterization, and Applications XVII
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Plasmonic Properties of Organized Silver Nanoplates on a Substrate for Sensing and Photoelectrical Applications2019

    • Author(s)
      Y. Takahashi
    • Organizer
      Workshop on Advanced Materials and Devices
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 全固体光電変換デバイスによるp型半導体を利用した新型プラズモン誘起電荷分離(PICS)の評価2019

    • Author(s)
      村山太郎, 新郷翔太, 山田淳, 高橋幸奈
    • Organizer
      第56回化学関連支部合同九州大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 新型プラズモン誘起電荷分離を利用した全固体光電変換セルの開発2019

    • Author(s)
      高橋幸奈
    • Organizer
      第16回プラズモニクスシンポジウム
    • Related Report
      2019 Annual Research Report
  • [Presentation] 疎水性金属ナノ粒子を用いた Langmuir-Blodgett 膜の作製2019

    • Author(s)
      高橋幸奈,弥永洋平,石田拓也,山田淳
    • Organizer
      ナノ学会第17回大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 銀ナノ粒子/p型半導体界面での新型プラズモン誘起電荷分離システムの開発2019

    • Author(s)
      髙橋幸奈, 村山太郎, 新郷翔太, 山田 淳
    • Organizer
      電気化学会第86回大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Organization of Silver Nanoplates on a Substrate for Sensing Applications2019

    • Author(s)
      Y. Takahashi
    • Organizer
      Asian International Symposium - Photochemistry -
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Development of plasmon-induced charge separation systems at the interfaces between p-type semiconductors and copper nanostructures2018

    • Author(s)
      K. Kimura, T. Murayama, Y. Takahashi
    • Organizer
      International Workshop on Advanced Nanoscience and Nanomaterials 2018 (IWANN2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of all-solid-state photoelectric conversion devices based on new type plasmon induced charge separation (PICS) with p-type semiconductors2018

    • Author(s)
      T. Murayama, S. Shingo, S. Yamada, Y. Takahashi
    • Organizer
      International Workshop on Advanced Nanoscience and Nanomaterials 2018 (IWANN2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] p型半導体を利用した新型プラズモン誘起電荷分離(PICS)による全固体光電変換デバイスの開発2018

    • Author(s)
      村山太郎, 新郷翔太, 山田 淳, 髙橋幸奈
    • Organizer
      第55回 化学関連支部合同九州大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 棒状および球状金ナノ粒子の疎水化法と単層粒子膜作製法の開発2018

    • Author(s)
      髙橋幸奈, 弥永洋平, 迫敬往, 山田 淳
    • Organizer
      第78回 分析化学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 銀ナノ粒子を用いた全固体プラズモン誘起電荷分離セル2018

    • Author(s)
      村山太郎, 越智亮太, 山田 淳, 髙橋幸奈
    • Organizer
      ナノ学会第16回大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Approaches to Orientation Control of Anisotropic Metal Nanoparticles for Photoelectrochemical and Analytical Applications2018

    • Author(s)
      Y. Takahashi
    • Organizer
      International Workshop on Advanced Nanoscience and Nanomaterials 2018 (IWANN2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] ナノ領域光貯蔵・局在化システムの設計、高性能化と分析科学への展開2018

    • Author(s)
      髙橋幸奈
    • Organizer
      日本分析化学会第67年会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 金属酸化物薄膜が金属ナノ粒子の形状制御に及ぼす効果2018

    • Author(s)
      髙橋幸奈
    • Organizer
      公益社団法人日本セラミックス協会第31回秋季シンポジウム
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 金属ナノ粒子の局在表面プラズモン共鳴を用いた高効率光エネルギー変換デバイスを目指して2018

    • Author(s)
      髙橋幸奈
    • Organizer
      エネルギー・環境・資源問題の解決に繋がる革新的材料創出に向けた光・量子ビーム応用技術調査専門委員会第3 回研究会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Near-infrared photoreactions with Au-TiO2 systems based on plasmon induced charge separation2017

    • Author(s)
      SOTA, Yusuke; TAKAHASHI, Yukina; YAMADA, Sunao
    • Organizer
      2017年光化学討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 疎水性相互作用制御による金ナノ粒子二次元組織化膜の作製と分光特性2017

    • Author(s)
      弥永洋平、迫敬往、石田拓也、高橋幸奈、山田 淳
    • Organizer
      日本分析化学会第66回年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 近赤外光を光源としたプラズモン誘起電荷分離に基づく光エネルギー変換システムの検討2017

    • Author(s)
      髙橋幸奈,曽田祐輔,藤久義幸,石田拓也,山田 淳
    • Organizer
      2017年電気化学秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Improvement in Stabilities and Sensitivities of Silver Nanoplates for Practical Sensing Applications2017

    • Author(s)
      Yukina Takahashi
    • Organizer
      ナノ構造・物性-ナノ機能・応用部会合同シンポジウム
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] センシングデバイスへの応用を志向した平板状銀ナノ粒子単粒子膜の作製2017

    • Author(s)
      高橋幸奈、井手奈都子、弥永洋平、山田 淳
    • Organizer
      第77回分析化学討論会
    • Related Report
      2016 Annual Research Report
  • [Remarks] 先生の森

    • URL

      https://www.kyushu-u.ac.jp/ja/university/professor/takahashi.html

    • Related Report
      2018 Annual Research Report
  • [Remarks] Yukina TAKAHASHI

    • URL

      http://i2cner.kyushu-u.ac.jp/~yukina/

    • Related Report
      2018 Annual Research Report
  • [Funded Workshop] International Workshop on Advanced Nanoscience and Nanomaterials 2018 (IWANN2018)2018

    • Related Report
      2018 Annual Research Report

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Published: 2016-04-21   Modified: 2021-02-19  

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