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Development of paste material with self-propagating exothermic reaction and its application for ecological bonding technology

Research Project

Project/Area Number 16K06138
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Thermal engineering
Research InstitutionKobe City College of Technology

Principal Investigator

Miyake Shugo  神戸市立工業高等専門学校, その他部局等, 准教授 (60743953)

Research Collaborator Namazu Takahiro  
Project Period (FY) 2016-04-01 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥4,940,000 (Direct Cost: ¥3,800,000、Indirect Cost: ¥1,140,000)
Fiscal Year 2018: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2017: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Fiscal Year 2016: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywords自己伝播発熱反応 / 多層構造粉末材 / 高時間分解温度計測 / 熱量測定 / 動的結晶構造解析 / 重ね圧延 / 発熱量測定 / 多層構造粉末 / 高精度温度計測 / 多層金属粉末 / 構造・機能材料 / 金属物性 / 電気・電子材料 / 複合材料・物性 / 熱工学
Outline of Final Research Achievements

In order to utilize energy-saving bonding technology for wiring of electronic devices and metal structure and also as a heat source in special environment such as space and under the sea, we developed metal powder materials with self-propagating exothermic reaction. Using cold-rolling and pulverizing method with aluminium and nickel foils, we succeeded in producing exothermic powder exhibiting very high temperature over 1500°C in 0.1msec. As a result of detailed experiments and analysis, we found that controlling the production conditions of cold-rolling is able to control the exothermic reaction characteristics. Moreover, using this developed powder materials, we also succeeded in joining aluminium foils and copper wire experimentally.

Academic Significance and Societal Importance of the Research Achievements

本研究において開発した発熱粉末材料は,燃焼ではなく化学反応による発熱を示すことから,任意の環境で局所加熱できる事が可能であるだけでなく,不必要なエネルギーを使わずに且つ熱ダメージを最小限にできる有効な技術となりうる可能性を示している.加えてmsecオーダーの極短時間における発熱特性や結晶構造変化を捉える評価技術は,実際の化学反応現象を理解する上で必要不可欠な技術であり,本材料以外にも発展的な利用が期待できる.

Report

(4 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • 2016 Research-status Report
  • Research Products

    (29 results)

All 2019 2018 2017 2016

All Journal Article (5 results) (of which Peer Reviewed: 5 results,  Open Access: 4 results,  Acknowledgement Compliant: 1 results) Presentation (23 results) (of which Int'l Joint Research: 7 results) Book (1 results)

  • [Journal Article] Crystal Structure Analysis of Al / Ni Multilayer Powder during Exothermic Reaction by Synchrotron Radiation X-ray Diffraction Measurement2019

    • Author(s)
      山本 梨乃、三宅 修吾、金築 俊介、生津 資大、後藤 大輝、訓谷 保広、小金澤 智之
    • Journal Title

      Journal of the Japanese Society for Experimental Mechanics

      Volume: 19 Issue: 1 Pages: 30-37

    • DOI

      10.11395/jjsem.19.30

    • NAID

      130007637001

    • ISSN
      1346-4930, 1884-4219
    • Year and Date
      2019-04-22
    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Development of High-Sensitive Calorimeter for Small Amount of Pulverized Material with Self-Propagating Exothermic Reaction2019

    • Author(s)
      三宅 修吾、永井 明里、山田 海斗
    • Journal Title

      Journal of the Japanese Society for Experimental Mechanics

      Volume: 19 Issue: 1 Pages: 19-23

    • DOI

      10.11395/jjsem.19.19

    • NAID

      130007636995

    • ISSN
      1346-4930, 1884-4219
    • Year and Date
      2019-04-22
    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Effect of Free-standing Al/Ni Exothermic Film on Thermal Resistance of Reactively Bonded Solder Joint2019

    • Author(s)
      Kanetsuki Shunsuke、Miyake Shugo、Namazu Takahiro
    • Journal Title

      Sensors and Materials

      Volume: 31 Issue: 3 Pages: 729

    • DOI

      10.18494/SAM.2019.2076

    • ISSN
      0914-4935, 2435-0869
    • Year and Date
      2019-03-08
    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Instantaneous Solder Joining Technique Using Exothermic Reaction of Al/Ni Multilayer Powder2019

    • Author(s)
      Taisei IZUMI, Nagamasa KAMETANI, Shugo MIYAKE , Shunsuke KANETSUKI and Takahiro NAMAZU
    • Journal Title

      Advanced Experimental Mechanics

      Volume: 印刷中

    • NAID

      130007755239

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Temperature behavior of exothermic reaction of Al/Ni multilayer powder materials based on cold-rolling and pulverizing method2017

    • Author(s)
      N. Kametani, T. Izumi, S. Miyake, S. Kanetsuki, and T. Namazu
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 印刷中

    • NAID

      210000147932

    • Related Report
      2016 Research-status Report
    • Peer Reviewed / Open Access / Acknowledgement Compliant
  • [Presentation] Time-resolved X-ray diffraction study of formation of intermetallic compounds in Al/Ni multilayer materials2018

    • Author(s)
      Rino Yamamoto, Taisei Izumi, Sho Nagata, Ryota Wakatsuki, Kai Uozaki, Shugo Miyake, Takahiro Namazu, Shunsuke Kanetsuki, Daiki Goto, Yasuhiro Kuntani, Takumi Nomura, and Tomoyuki Koganezawa
    • Organizer
      13th International Symposium on Advanced Science and Technology in Experimental Mechanics
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Characterization of exothermic reaction of cold-rolled Al/Ni multilayer materials by isothermal calorimetry2018

    • Author(s)
      Akari Nagai, Rino Yamamoto, and Shugo Miyake
    • Organizer
      13th International Symposium on Advanced Science and Technology in Experimental Mechanics
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 圧延率をパラメータとして制御した Al/Ni 多層構造と発熱特性の関係2018

    • Author(s)
      山本梨乃,三宅修吾,金築俊介,生津資大
    • Organizer
      日本機械学会研究発表講演会2018年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 高時分割X線回折法を用いた自己伝播発熱反応の動的結晶構造変化の計測技術2018

    • Author(s)
      三宅修吾,和泉大晟,永田將,山本梨乃,若槻涼太,魚崎海,生津資大,金築俊介,後藤大輝,訓谷保広,野村拓未,小金澤智之
    • Organizer
      日本実験力学会2018年度年次講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Al/Ni多層粉末材料における圧延率が化合物形成と発熱特性に及ぼす影響2018

    • Author(s)
      山本梨乃,三宅修吾,金築俊介,生津貴大
    • Organizer
      日本金属学会2018年春期講演大会
    • Related Report
      2017 Research-status Report
  • [Presentation] Al/Ni 系材料の瞬間発熱反応を熱源に用いたはんだ接合技術の研究2018

    • Author(s)
      和泉大晟, 永田將,三宅修吾, 金築俊介, 生津資大
    • Organizer
      第24回「エレクトロニクスにおけるマイクロ接合・実装技術」シンポジウム
    • Related Report
      2017 Research-status Report
  • [Presentation] 放射測温を用いた金属箔接合部の熱拡散率分布評価2017

    • Author(s)
      永田將,亀谷長諒,和泉大晟,山田海斗,三宅修吾,加藤岳雄,関根誠
    • Organizer
      第31回エレクトロニクス実装学会春季講演大会
    • Place of Presentation
      慶應義塾大学
    • Year and Date
      2017-03-08
    • Related Report
      2016 Research-status Report
  • [Presentation] Al/Ni多層粉末材の発熱反応を用いたバルク金属接合技術の開発2017

    • Author(s)
      和泉大晟, 亀谷長諒,山田海斗,永田將,三宅修吾,金築俊介,生津資大
    • Organizer
      第23回「エレクトロニクスにおけるマイクロ接合・実装技術」シンポジウム
    • Place of Presentation
      パシフィコ横浜
    • Year and Date
      2017-01-31
    • Related Report
      2016 Research-status Report
  • [Presentation] Novel Joining Technique for Aluminum Foils by Using Al/Ni Exothermic Materials as Saving Heat Source2017

    • Author(s)
      Taisei Izumi, Nagamasa Kametani, Shugo Miyake, Shunsuke Kanetsuki, and Takahiro Namazu
    • Organizer
      The 30th International Microprocesses and Nanotechnology Conference (Jeju, Korea)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Effects of Al/Ni Ratio on Exothermic Heat of Cold-Rolled Al/Ni Multilayer Materials2017

    • Author(s)
      Kai UOZAKI, Rino YAMAMOTO, Taisei IZUMI and Shugo MIYAKE,
    • Organizer
      12th International Symposium on Advanced Science and Technology in Experimental Mechanics (ISEM2017-Kanazawa)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] 発熱ペレットの発熱特性に関する研究2017

    • Author(s)
      若槻 涼太, 和泉 大晟, 三宅 修吾
    • Organizer
      第8回マイクロ・ナノ工学シンポジウム
    • Related Report
      2017 Research-status Report
  • [Presentation] 低融点金属を複合した機能性発熱材料の発熱挙動に関する研究2017

    • Author(s)
      和泉 大晟, 若槻 涼太, 三宅 修吾, 金築 俊介, 生津 資大
    • Organizer
      第8回マイクロ・ナノ工学シンポジウム
    • Related Report
      2017 Research-status Report
  • [Presentation] 圧延粉砕法で作製したAl/Ni多層材の発熱特性に関する研究2017

    • Author(s)
      三宅修吾,山田海斗,和泉大晟,金築俊介,生津資大
    • Organizer
      日本金属学会2017年秋期講演大会
    • Related Report
      2017 Research-status Report
  • [Presentation] Ni-Al系瞬間発熱反応を用いた新規熱源における接合技術の研究2017

    • Author(s)
      和泉大晟,亀谷長諒,三宅修吾,吉川卓郎,金築俊介,生津資大
    • Organizer
      日本金属学会2017年秋期講演大会
    • Related Report
      2017 Research-status Report
  • [Presentation] 発熱粉末を用いて局所加熱したアルミ箔接合部の諸特性2017

    • Author(s)
      三宅 修吾,和泉大晟,永田將,金築俊介,生津資大
    • Organizer
      日本機械学会研究発表講演会2017年次大会
    • Related Report
      2017 Research-status Report
  • [Presentation] Al/Ni 瞬間ハンダ接合における発熱反応の自己 伝播性に及ぼす膜厚の影響2017

    • Author(s)
      神谷亮太,金築俊介,桒原晃一,三宅修吾,生津 資大
    • Organizer
      日本機械学会研究発表講演会2017年次大会
    • Related Report
      2017 Research-status Report
  • [Presentation] 瞬間はんだ接合部に及ぼすAlNi多層薄膜の自立化の効果2017

    • Author(s)
      金築俊介,神谷亮太,桒原晃一,訓谷保広,後藤大輝,野村拓未,三宅修吾,生津 資大
    • Organizer
      日本機械学会研究発表講演会2017年次大会
    • Related Report
      2017 Research-status Report
  • [Presentation] 瞬間発熱反応用非接触温度計測技術の開発2017

    • Author(s)
      三宅修吾,和泉大晟
    • Organizer
      日本実験力学会2017年度年次講演会
    • Related Report
      2017 Research-status Report
  • [Presentation] Dependency of Microstructure on Exothermic Characteristics for Al/Ni Multilayer Materials Based on Cold-rolled Method2016

    • Author(s)
      T.Izumi, N.Kametani,S.Miyake,S.Kanetsuki, T.Namazu
    • Organizer
      29th International Microprocesses and Nanotechnology Conference
    • Place of Presentation
      クラウンプラザ京都
    • Year and Date
      2016-11-10
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] 圧延法で作製したAl/Ni多層材の発熱特性と接合技術への可能性検討2016

    • Author(s)
      三宅修吾,金築俊介,生津資大
    • Organizer
      日本機械学会2016年度年次大会
    • Place of Presentation
      九州大学
    • Year and Date
      2016-09-12
    • Related Report
      2016 Research-status Report
  • [Presentation] Study on exothermic reaction in cold-rolled Al/Ni multilayer2016

    • Author(s)
      T.Izumi, N.Kametani,S.Miyake,T.Namazu
    • Organizer
      The 11th International Symposium on Advanced Science and Technology in Experimental Mechanics
    • Place of Presentation
      近畿大学
    • Year and Date
      2016-09-03
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Development of Direct Reaction Calorimeter for Exothermic Materials2016

    • Author(s)
      K.Yamada, S.Nagata, S.Miyake, T.Namazu
    • Organizer
      The 11th International Symposium on Advanced Science and Technology in Experimental Mechanics
    • Place of Presentation
      近畿大学
    • Year and Date
      2016-09-03
    • Related Report
      2016 Research-status Report
    • Int'l Joint Research
  • [Presentation] Al/Ni多層材の反応性と発熱特性に関する研究2016

    • Author(s)
      三宅修吾,和泉大晟,亀谷長諒,永田將,山田海斗
    • Organizer
      日本実験力学会2016年度年次講演会
    • Place of Presentation
      近畿大学
    • Year and Date
      2016-09-03
    • Related Report
      2016 Research-status Report
  • [Book] 伝熱工学の基礎と熱物性測定・熱対策事例2019

    • Author(s)
      三宅修吾他
    • Total Pages
      6
    • Publisher
      株式会社R&D支援センター
    • ISBN
      9784905507314
    • Related Report
      2018 Annual Research Report

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Published: 2016-04-21   Modified: 2020-03-30  

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