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NMR and ESR study of functional materials and biological substances under ultra-high magnetic fields

Research Project

Project/Area Number 17072005
Research Category

Grant-in-Aid for Scientific Research on Priority Areas

Allocation TypeSingle-year Grants
Review Section Science and Engineering
Research InstitutionOkayama University

Principal Investigator

ZHENG Guo-qing  Okayama University, 大学院・自然科学研究科, 教授 (50231444)

Co-Investigator(Kenkyū-buntansha) HAGIWARA Masayuki  大阪大学, 極限量子科学研究センター, 教授 (10221491)
GOTO Takayuki  上智大学, 理工学部, 教授 (90215492)
OTA Hitoshi  神戸大学, 分子フォトサイエンス研究センター, 教授 (70194173)
KUMAGAI Kenichi  北海道大学, 大学院・理学研究科, 教授 (70029560)
Project Period (FY) 2005 – 2009
Project Status Completed (Fiscal Year 2009)
Budget Amount *help
¥104,300,000 (Direct Cost: ¥104,300,000)
Fiscal Year 2009: ¥15,100,000 (Direct Cost: ¥15,100,000)
Fiscal Year 2008: ¥24,100,000 (Direct Cost: ¥24,100,000)
Fiscal Year 2007: ¥24,200,000 (Direct Cost: ¥24,200,000)
Fiscal Year 2006: ¥25,100,000 (Direct Cost: ¥25,100,000)
Fiscal Year 2005: ¥15,800,000 (Direct Cost: ¥15,800,000)
Keywords強磁場 / 磁気共鳴 / 超伝導 / 量子磁性 / 強相関電子系 / NMR / ESR / 磁性体 / タンパク質 / スピン3重項超伝導 / 量子スピン系 / 巨大磁気抵抗 / 強磁性 / 磁化 / 比熱
Research Abstract

The purpose of this project is to develop NMR and ESR techniques for scientific research at pulsed high magnetic fields. We have succeeded, for the first time in the world, in obtaining NMR spectra at pulsed magnetic fields up to 48 T by the spin-echo method. By conducting NMR measurements at static magnetic fields, we were able to reveal the ground state of the high-Tc superconductors, the Magnon excitation of quantum spin system NH_4CuCl_3 and the FFLO state in CeCoIn_5 superconductor. We performed ESR measurements at pulsed fields up to 70 T and studied the magnetic excitations in quantum magnets such as NDMAP, BaCoV_2O_8, Pb_2V_3O_9 and geometrically frustrated magnets NiGa_2S_4 and CuCrO_2, as well as the crystal field effect in Mn-based Myoglobin protein.

Report

(6 results)
  • 2009 Annual Research Report   Final Research Report ( PDF )
  • 2008 Annual Research Report
  • 2007 Annual Research Report
  • 2006 Annual Research Report
  • 2005 Annual Research Report
  • Research Products

    (55 results)

All 2010 2009 2008 2007 2006 2005 Other

All Journal Article (40 results) (of which Peer Reviewed: 22 results) Presentation (10 results) Book (2 results) Remarks (3 results)

  • [Journal Article] Spiral-plane flop probed by ESR in the multiferroic triangular-lattice antiferromagnet CuCrO22010

    • Author(s)
      H. Yamaguchi, S. Ohotomo, S. Kimura, M. Hagiwara, K. Kimurai, T. Kimura, T. Okuda, K. Kindo
    • Journal Title

      Phys. Rev. B 81

    • Related Report
      2009 Final Research Report
  • [Journal Article] Spiral-plane flop probed by ESR in the multiferroic triangular-lattice antiferromagnet CuCr022010

    • Author(s)
      H.Yamaguchi
    • Journal Title

      Phys.Rev.B 81

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin-Echo NMR in Pulsed High Magnetic Fields up to 48 T2009

    • Author(s)
      G. -Q. Zheng, K. Katayama, M. Nishiyama, S. Kawasaki, N. Nishihagi, S. Kimura, M. Hagiwara, K. Kindo:
    • Journal Title

      J. Phys. Soc. Jpn. 78

    • NAID

      130005437954

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Anisotropic spin fluctuations and multiple superconducting gaps in hole-doped Ba0. 7K0. 3Fe2As2: NMR in a single crystal2009

    • Author(s)
      K. Matano, Z. Li, G.L. Sun, D.L. Sun, C.T. Lin, M. Ichioka, G. -Q. Zheng
    • Journal Title

      Europhys. Lett. 87

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Measurement of electron correlations in LixCoO2 (x=0.0-0.35) using 59Co nuclear magnetic resonance and nuclear quadrupole resonance techniques.2009

    • Author(s)
      S. Kawasaki, T. Motohashi, K. Shimada, T. Ono, R. Kanno, M. Karppinen, H. Yamauchi, G. -Q. Zheng
    • Journal Title

      Phys. Rev. B 79

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article]2009

    • Author(s)
      H. Inoue, S. Tani, S. Hosoya, K. Inokuchi, T. Fujiwara, T. Saito, T. Suzuki, A. Oosawa, T. Goto, M. Fujisawa, H. Tanaka, T. Sasaki, S. Awaji, K. Watanabe, N. Kobayashi
    • Journal Title

      Phys. Rev. B 79

    • Related Report
      2009 Final Research Report
  • [Journal Article] Development and Application of High-Frequency ESR up to 55 T.2009

    • Author(s)
      H. Ohta, S. Okubo, N. Souda, M. Tomoo, T. Sakurai, T. Yoshida, E. Ohmichi, M. Fujisawa, H. Tanaka, R. Kato
    • Journal Title

      Appl. Magn. Reson. 35

      Pages: 399-410

    • Related Report
      2009 Final Research Report
  • [Journal Article] High-field multifrequency electron-spin-resonance study of the Haldane magnet Ni(C5H14N2)2N3(PF6)2009

    • Author(s)
      T. Kashiwagi, M. Hagiwara, S. Kimura, Z. Honda, H. Miyazaki, I. Harada, K. Kindo
    • Journal Title

      Phys. Rev. B 79

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Spin-Echo NMR in Pulsed High Magnetic Fields up to 48T2009

    • Author(s)
      G.Q.Zheng
    • Journal Title

      J.Phys.Soc.Jpn. 78

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 63/65Cu-and 35/37Cl-NMR studies of triplet localization in the quantum spin system NH4CuCl32009

    • Author(s)
      H.Inoue
    • Journal Title

      Phys.Rev.B 79

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin-singlet superconductivity with multiple gaps in PrO0. 89F0. 11FeAs.2008

    • Author(s)
      K. Matano, Z.A. Ren, X.L. Dong, L.L. Sun, Z.X. Zhao, G. -Q. Zheng
    • Journal Title

      Europhys. Lett. 83

      Pages: 57001-57001

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] High-field electron spin resonance in the two-dimensional triangular-lattice antiferromagnet NiGa2S42008

    • Author(s)
      H. Yamaguchi, S. Kimura, M. Hagiwara, Y. Nambe, S. Nakatsuji, Y. Maeno, K. Kindo
    • Journal Title

      Phys. Rev. B 78

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Multi-frequency and high-field EPR study of manganese(III) protoporphyrin IX reconstituted myoglobin with an S = 2 integer electron spin.2008

    • Author(s)
      M. Horitani, H. Yashiro, M. Hagiwara, Hiroshi Hori
    • Journal Title

      Journal of Inorganic Biochemistry 102

      Pages: 781-788

    • Related Report
      2009 Final Research Report
  • [Journal Article] Topological effects on magnetic properties of closed and open ring-shaped Cr-based antiferromagnetic nanomagnets2008

    • Author(s)
      Y. Furukawa
    • Journal Title

      Phys. Rev. B 78

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin-singlet superconductivity with multiple gaps in Pr00.89F0.11 FeAs2008

    • Author(s)
      K. Matano
    • Journal Title

      Europhys. Lett. 83

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Longitudinal Spin Density Wave Order in a Quasi-1 D Ising-like Quantum Antiferromagnet2008

    • Author(s)
      S. Kimura
    • Journal Title

      Phys. Rev. Lett. 101

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Novel Ordering of an S=1/2 Quasi-ld Ising -Like Antiferromagnet in Magnetic Field2008

    • Author(s)
      S. Kimura
    • Journal Title

      Phys. Rev. Lett. 10

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin Triplet Superconducting State due to Broken Inversion Symmetry in Li2Pt3B2007

    • Author(s)
      M. Nishiyama, Y. Inada, G. -Q. Zheng
    • Journal Title

      Phys. Rev. Lett. 98

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Local spin moment configuration in the frustrated s = 1/2 Heisenberg triangular antiferromagnet V15 determined by NMR.2007

    • Author(s)
      Y. Furukawa, Y. Nishisaka, K. Kumagai, P. Kogerler, F. Borsa
    • Journal Title

      Phys. Rev. B 75

    • Related Report
      2009 Final Research Report
  • [Journal Article] Field Induced Order to Disorder Transition Driven by a Softening of Spinon Excitation2007

    • Author(s)
      S. Kimura, H. Yashiro, K. Okunishi, M. Hagiwara, Z. He, K. Kindo, T. Taniyama, M. Itoh
    • Journal Title

      Phys. Rev. Lett. 99

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Field induced order to disorder transitiom driven by a softening of spinon excitation2007

    • Author(s)
      S. Kimura
    • Journal Title

      Phys. Rev Lett. 99

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Pressure dependence of the superonducting transition and electron correlations in NaxCoO2*1. 3H2O2007

    • Author(s)
      E. Kusano
    • Journal Title

      Phys. Rev. B 76

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Elliptical hole pockets in the Fermi surfaces of unhydrated and hydrated sodium cobalt oxides2007

    • Author(s)
      J. Laverock
    • Journal Title

      Phys. Rev. B 76

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Local spin moment configuration in the frustrated s=1/2 Heisenberg triangular antiferromagnet V15 ketermined by NMR2007

    • Author(s)
      Y. Furukawa
    • Journal Title

      Phys. Rev. B 75

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Development of higy-pressure. high-field and multifrequency electron spin resonance system2007

    • Author(s)
      T. Sakurai
    • Journal Title

      Rev. Sci. Inst 78

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] NMR study of the vortex slush phase in organic superconductor-(BEDT-TTE)2Cu(NCS)22007

    • Author(s)
      A. Oosawa
    • Journal Title

      Phys. Rev.B 76

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin Triplet Superconducting State due to Broken Inversion Symmetry in Li_2Pt_3B2007

    • Author(s)
      M.Nishiyama
    • Journal Title

      Phys.Rev.Lett. 98

      Pages: 47002-47002

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Field-Induced Ferromagnetic Order and Colossal magnetoresistance in La1. 2Sr1. 8Mn2O7:A 139La NMR Study.2006

    • Author(s)
      Y. Shiotani, J.L. Sarrao, G. -Q. Zheng
    • Journal Title

      Phys. Rev. Lett. 96

      Pages: 57203-57203

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Fulde-Ferrell-Larkin-Ovchinnikov State in a Perpendicular Field of Quasi-Two- Dimensional CeCoIn52006

    • Author(s)
      K. Kumagai, M. Saitoh, T. Oyaizu, Y. Furukawa, S. Takashima, M. Nohara, H. Takagi, Y. Matsuda
    • Journal Title

      Phys. Rev. Lett. Vol.97

    • Related Report
      2009 Final Research Report
  • [Journal Article] Local Spin Moment Distribution in Antiferromagnetic Molecular Rings Probed by NMR2006

    • Author(s)
      E. Micotti, Y. Fururkawa, K. Kumagai, S. Caretta, A. Lascialfari, F. Borsa, G.A. Timco, R.E.P. Winpenny
    • Journal Title

      Phys. Rev. Lett. 97

    • Related Report
      2009 Final Research Report
  • [Journal Article] ESR Measurements on One-dimensional Quantum Ferrimagnets A3Cu3 (PO4)4 with A=Sr and Ca in Submillimeter-wave Region2006

    • Author(s)
      S. Kimura, H. Ishikawa, Y. Inagaki, M. Yoshida, S. Okubo, H. Ohta, H. Nojiri, A.B. Belik, M. Azuma, M. Takano
    • Journal Title

      J. Phys. Soc. Jpn. Vol.75

    • NAID

      210000106334

    • Related Report
      2009 Final Research Report
  • [Journal Article] High Field ESR Study of Three Dimensional Spin Frustrated System MgCr2O42006

    • Author(s)
      M. Yoshida, T. Hirano, Y. Inagaki, S. Okubo, H. Ohta, H. Kikuchi, I. Kagomiya, M. Toki, K. Kohn
    • Journal Title

      J. Phys. Soc. Jpn. Vol.75

    • NAID

      210000106102

    • Related Report
      2009 Final Research Report
  • [Journal Article] Tomonaga-Luttinger Liquid in a Quasi-One-Dimensional S=1 Antiferromagnet Observed by Specific Heat Measurements2006

    • Author(s)
      M.Hagiwara
    • Journal Title

      Phys.Rev.Lett 96

      Pages: 147203-147203

    • Related Report
      2006 Annual Research Report
  • [Journal Article] High Field ESR and Magnetization in Na_2Co_2(C_2O_4)_3(H_2O)_22006

    • Author(s)
      Y.Nakagawa
    • Journal Title

      J. Phys. Soc. Jpn. 75

      Pages: 124708-124708

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Spin Singlet Pairing in the Superconducting State of Na_xCoO_2・1.3H_2O:Evidence from a ^<59>Co Knight Shift in a Single Crystal2006

    • Author(s)
      G.q.Zheng
    • Journal Title

      Phys.Rev.B 73

    • Related Report
      2006 Annual Research Report
  • [Journal Article] High Field ESR Study of Three Dimensional Spin Frustrated System MgCr_2O_42006

    • Author(s)
      M.Yoshida
    • Journal Title

      J.Phys.Soc.Jpn. 75

      Pages: 44709-44709

    • Related Report
      2006 Annual Research Report
  • [Journal Article] ESR Measurements on One-Dimensional Quantum Ferrimagnets A_3CU_3(PO_4)_4 with A=Sr and Ca in Submillimeter-Wave Region2006

    • Author(s)
      S.Kimura
    • Journal Title

      J.Phys.Soc.Jpn. 75

      Pages: 94718-94718

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Field-Induced Ferromagnetic Order and Colossal Magnetoresistance in La_<1.2>Sr_<1.8>Mn_2O_7: A La NMR Study2006

    • Author(s)
      Y.Shiotani
    • Journal Title

      Phys.Rev.Lett. 96

      Pages: 57203-57203

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Crystal structure and properties of phosphate_PbCu_2(PO_4)_2 with spin-singlet ground state2006

    • Author(s)
      A.Belik
    • Journal Title

      Phys.Rev. B 73

      Pages: 24429-24429

    • Related Report
      2005 Annual Research Report
  • [Journal Article] Anomalous Magnetization of Two-Dimensional S=1/2 Frustrated Square-Lattice Antiferromagnet (CuCl)LaNb_2O_72005

    • Author(s)
      H.Kageyama
    • Journal Title

      J.Phys.Soc.Jpn. 74

      Pages: 3155-3155

    • Related Report
      2005 Annual Research Report
  • [Presentation] NMR Study on Strongly Correlated Electron Superconductors under Static and Pulsed Magnetic-Fields up to 48 T2009

    • Author(s)
      G. -Q. Zheng
    • Organizer
      9th International Conference on Research in High Magnetic Fields (RHMF 2009)
    • Place of Presentation
      Dresden, Germany
    • Related Report
      2009 Final Research Report
  • [Presentation] Exotic phases in quantum and frustrated spin systems2009

    • Author(s)
      M. Hagiwara
    • Organizer
      Spin Waves 2009
    • Place of Presentation
      St. Petersburg, Russia
    • Related Report
      2009 Final Research Report
  • [Presentation] NMR Study on Strongly Correlated Electron Superconductors under Static and Pulsed Magnetic-Fields up to 48T2009

    • Author(s)
      G.Q.Zheng
    • Organizer
      9th International Conference on Research in High Magnetic Fields
    • Place of Presentation
      Dresden, Germany
    • Related Report
      2009 Annual Research Report
  • [Presentation] Pairing symmetry of the cobaltate superconductor2008

    • Author(s)
      鄭 国慶
    • Organizer
      American Physical Society March Meeting 2008
    • Place of Presentation
      米国,New Orleans
    • Year and Date
      2008-03-13
    • Related Report
      2007 Annual Research Report
  • [Presentation] Finite Fermi surface in the zero-temperature pseudogap state of the high-Tcsuperconductors2008

    • Author(s)
      鄭 国慶
    • Organizer
      12th Asia Pacific Theoretical Center Winter Workshop
    • Place of Presentation
      韓国、浦項工科大学
    • Year and Date
      2008-01-23
    • Related Report
      2007 Annual Research Report
  • [Presentation] NMR study of transitional-metal-oxide superconductors under static and pulsed high magnetic fields2008

    • Author(s)
      G. -Q. Zheng
    • Organizer
      the Sixth International Conference on Physical Phenomena in High Magnetic Fields (PPHMF-VI)
    • Place of Presentation
      Laulasmaa Resort, Estonia. 招待講演
    • Related Report
      2009 Final Research Report
  • [Presentation] Developments of Multi-Extreme High Frequency ESR Measurements System using a Pulsed Magnetic Field2008

    • Author(s)
      H. Ohta
    • Organizer
      6th Asia Pacific EPR/ESR Symposium 2008
    • Place of Presentation
      Queensland, Australia. 招待講演
    • Related Report
      2009 Final Research Report
  • [Presentation] NMR study of transitional-metal-oxide superconductors under static and pulsed high magnetic fields2008

    • Author(s)
      G.-q. Zheng
    • Organizer
      the Sixth International Conference on Physical Phenomena in Higb Magnetic Fields
    • Place of Presentation
      Laulasmaa Resort, Estoniae
    • Related Report
      2008 Annual Research Report
  • [Presentation] High-field ESR and thermodynamic studies of uniform and bond-alternating S=1 spin chains2006

    • Author(s)
      M. Hagiwara
    • Organizer
      American Physical Society (APS) March Meeting
    • Place of Presentation
      Baltimore, MD, USA招待講演
    • Related Report
      2009 Final Research Report
  • [Presentation] Microscopic Evidence of FFLO State in CeCoIn5 Probed by NMR2005

    • Author(s)
      K. Kumagai
    • Organizer
      International Conference on Strongly Correlated Electron Systems
    • Place of Presentation
      Vienna, Austria招待講演
    • Related Report
      2009 Final Research Report
  • [Book] 超伝導ハンドブック2009

    • Author(s)
      鄭国慶, 他
    • Publisher
      朝倉書店
    • Related Report
      2009 Final Research Report
  • [Book] 超伝導ハンドブック2009

    • Author(s)
      福山秀敏
    • Total Pages
      312
    • Publisher
      朝倉書店
    • Related Report
      2009 Annual Research Report
  • [Remarks]

    • URL

      http://www.physics.okayama-u.ac.jp/zheng_homepage

    • Related Report
      2009 Final Research Report
  • [Remarks]

    • URL

      http://www.physics.okayama-u.ac.jp/zheng.homepage/

    • Related Report
      2008 Annual Research Report
  • [Remarks]

    • URL

      http://www.physics.okayama-u.ac.jp/zheng_homepage/

    • Related Report
      2007 Annual Research Report

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Published: 2005-04-01   Modified: 2018-03-28  

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