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Applications of asymmetric plasmonic nanoparticle hybrid systems to ultrafast multiplewave nonlinear nanophotonics

Research Project

Project/Area Number 17H02798
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Optical engineering, Photon science
Research InstitutionShizuoka University

Principal Investigator

Sugita Atsushi  静岡大学, 工学部, 准教授 (20334956)

Co-Investigator(Kenkyū-buntansha) 松尾 淳一  金沢大学, 薬学系, 教授 (50328580)
川田 善正  静岡大学, 電子工学研究所, 教授 (70221900)
Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥17,940,000 (Direct Cost: ¥13,800,000、Indirect Cost: ¥4,140,000)
Fiscal Year 2019: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2018: ¥7,020,000 (Direct Cost: ¥5,400,000、Indirect Cost: ¥1,620,000)
Fiscal Year 2017: ¥8,970,000 (Direct Cost: ¥6,900,000、Indirect Cost: ¥2,070,000)
Keywords非線形光学 / 表面プラズモン / 金属ナノ粒子複合構造 / 金属ナノ粒子 / 超高速分光 / 微小光学 / ナノ光工学 / 応用光学・量子光工学 / 光物性 / 表面・界面物性
Outline of Final Research Achievements

We made researches about nonlinear optics of Au nanoparticle complex structures. In general, the metal nanoparticles for surface plasomo excitation are forbidden for even-order nonlinear susceptibilities because of their centrosymmetric geometries. In the study, we tried obtaining even-order nonlinear susceptibilities by approaching the metal nanoparticles in the close vicinities so as to break the centrosymmetry of the system. It was demonstrated that the SHG signal intensities from the designed nanotrimaric structures was approximately one-magnitude higher than those from the conventional centrosymmetric metal nanoparticle systems.

Academic Significance and Societal Importance of the Research Achievements

複合粒子系における粒子配列を調整することにより、偶数次非線形光学遷移に適した近接場をテーラーメイドに創出するという着想は、先例のない本課題の独自な視点で、実際に作成した金属ナノ粒子複合系を用いてこの点を実証できたことは学術的な価値があると考える。今後、この研究で編み出した非線形ナノ光素子の設計戦略を実用化に向けた各種非線形光学デバイス作成技術へ展開すれば、光工学分野に大きく貢献ができるものと考える。

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • Research Products

    (40 results)

All 2020 2019 2018 2017

All Journal Article (6 results) (of which Peer Reviewed: 5 results,  Open Access: 1 results,  Acknowledgement Compliant: 1 results) Presentation (34 results) (of which Int'l Joint Research: 9 results,  Invited: 1 results)

  • [Journal Article] Second harmonic conversions of surface-plasmon-polariton?enhanced optical fields in nonlinear optics polymer/Ag/glass structures2020

    • Author(s)
      Sugita Atsushi、Kaname Suto、Mochizuki Kannta、Kikuchi Kohei、Ono Atsushi、Inami Wataru、Kawata Yoshimasa
    • Journal Title

      Physical Review B

      Volume: 101 Issue: 4

    • DOI

      10.1103/physrevb.101.045303

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Orientation order of nonelectrically poled FTC-type chromophores in PMMA on SiO2 surfaces2020

    • Author(s)
      Sugita, Atsushi; Tsuruoka, Miwa; Kinoshita, Yuta; Futagami, Yushi; Yoshimura, Tomoyuki; Matsuo, Jun-ichi
    • Journal Title

      Bull. Chem. Soc. Jpn.

      Volume: 93 Issue: 1 Pages: 119-126

    • DOI

      10.1246/bcsj.20190257

    • NAID

      130007784855

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Title: Nonresonant and resonant surface-enhanced Raman scattering of N-ethyl-N-(2-hydroxyethyl)-4-(4-nitrophenylazo) aniline in poly (methyl methacrylate) on Ag films with surface roughness2019

    • Author(s)
      Ayaka Izumi, Kentaro Kumaoka, Masaru Shimomura, Atsushi Sugita
    • Journal Title

      Bulletin of the Chemical Society of Japan

      Volume: - Issue: 8 Pages: 1268-1274

    • DOI

      10.1246/bcsj.20190073

    • NAID

      130007689985

    • Related Report
      2019 Annual Research Report 2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Polarized second harmonic generation spectroscopies from Au nanorods arrayed on SiO2 substrates at localized surface plasmon resonances2017

    • Author(s)
      1.Hirofumi Yogo, Tatsuya Matsui, Shunsuke Nihashi, Takuma Hirabayashi, Wataru Inami, Atsushi Ono, Yoshimasa Kawata, and Atsushi Sugita
    • Journal Title

      The Japanese Journal of Applied Physics

      Volume: 56 Issue: 12 Pages: 122002-122002

    • DOI

      10.7567/jjap.56.122002

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ultramicroscopy2017

    • Author(s)
      2.Yu Masuda, Masashi Kamiya, Atsushi Sugita, Wataru Inami, Yoshimasa Kawata, Hiroko Kominami, Yoichiro Nakanishi
    • Journal Title

      Spatial resolution and cathodoluminescence intensity dependence on acceleration voltage in electron beam excitation assisted optical microscopy using Y2O3:Eu3+ film

      Volume: 182 Pages: 212-215

    • DOI

      10.1016/j.ultramic.2017.07.010

    • Related Report
      2017 Annual Research Report
  • [Journal Article] The Role of Chemisorption for Push-Pull Chromophores on SiO2 Surfaces in Non-Electrically Poling Host-Guest NLO Polymers2017

    • Author(s)
      Atsushi Sugita, Kazuma Ito, Yasuaki Sato, Ryota Suzuki, Kohei Sato, Tetsuo Narumi, Nobuyuki Mase, Yasushi Takano, Tomonori Matsushita, Shigeru Tasaka, and Yoshimasa Kawata
    • Journal Title

      Journal of Photochemistry and Photobiology A: Chemistry

      Volume: 340 Pages: 35-45

    • DOI

      10.1016/j.jphotochem.2017.03.007

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] ドルマン型金ナノ粒子三量体系における超高速応答の粒子間隔依存性2020

    • Author(s)
      杉田篤史、望月寛太、松井大海、小野篤史、居波渉、川田善正、吉澤雅幸
    • Organizer
      第75回日本物理学会年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 金ナノ粒子/NLOポリマー複合系における非線形性増大効果の考察2020

    • Author(s)
      蒔山拓海、青島諒、小野篤史、居波渉、川 善正、杉田篤史
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 金ナノ粒子三量体構造体の第二高調波発生2020

    • Author(s)
      中塚庸靖、小野篤史、川田善正、居波渉、杉田篤史
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] ドルマン型金ナノ粒子構造体のフェムト秒過渡応答の粒子間隔依存性2020

    • Author(s)
      杉田篤史、望月寛太、小野篤史、居波渉、川田善正、吉澤 雅幸
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Nonlinear plasmonics of NLO polymer/Au nanoparticle hybrid Systems2019

    • Author(s)
      1.Atsushi Sugita, Takumi Makiyama, Ryo Aoshima, Atsushi Ono, Wataru Inami, Yoshimasa Kawata
    • Organizer
      Micro + Nanomaetrials, Devices, and Applications, Australian and New Zealand Conferences on Optics+Photonics
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Amplifying conversion efficiencies of SP-enhanced SHG from Ag surface with nonlinear optical polymer films2019

    • Author(s)
      Atsushi Sugita, Kanta Mochizuki, Kohei Kikuchi, Atsushi Ono, Wataru Inami, and Yoshimasa Kawata
    • Organizer
      Plasmonics: Design, Materials, Fabrication, Characterization, and Applications XVII in SPIE Nanoscience + Engineering
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Amplifying SP-enhanced SHG with NLO polymers grown on Ag films2019

    • Author(s)
      Atsushi Sugita, Kanta Mochizuki, Kohei Kikuchi, Atsushi Ono, Wataru Inami, and Yoshimasa Kawata
    • Organizer
      CLEO/Europe-EQEC Conference 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Boosting LSP-enhanced SHG from Au nanoprisms by using NLO polymers2019

    • Author(s)
      Atsushi Sugita, Takumi Makiyama, Hikaru Sato, Atsushi Ono, Wataru Inami, Yoshimasa Kawata
    • Organizer
      CLEO:2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Auナノ粒子/SiO2/Si構造によるSP共鳴SHG現象の干渉増大効果2019

    • Author(s)
      望月寛太、Juodokazis Saulius、小野篤史、居波渉、川田善正、杉田篤史
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 二次元配列金ナノ三角プリズム系におけるSHG現象の粒子密度依存性2019

    • Author(s)
      蒔山拓海、青島諒、小野篤史、居波渉、川田善正、杉田篤史
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 金ナノロッド/金ナノ三角柱状複合構造体の第二高調波発生現象2019

    • Author(s)
      中塚庸靖、奥村功樹、小野篤史、川田善正、居波渉、杉田篤史
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 金ナノディスク系のフェムト秒動力学における偏光依存性2019

    • Author(s)
      杉田篤史、浜田勝平、望月寛太、松井大海、小野篤史、居波渉、吉澤雅幸、川田善正
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Auナノ粒子/SiO2/Si構造の第二高調波発生現象2019

    • Author(s)
      望月寛太、ジュドカジス サウリス、居波渉、川田善正、杉田篤史
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 表面プラズモン共鳴励起した金ナノディスク系におけるフェムト秒緩和現象2019

    • Author(s)
      杉田篤史、望月寛太、浜田勝平、松井大海、小野篤史、居波渉、川田善正、吉澤雅幸
    • Organizer
      2019年日本物理学会秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] ドルマン型金ナノ粒子複合系のフェムト秒時間分解分光2019

    • Author(s)
      杉田篤史、浜田勝平、松井大海、小野篤史、居波渉、川田善正、吉澤雅幸
    • Organizer
      第74回日本物理学会年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] ドルマン型金ナノ粒子複合系の超高速時間分解吸収分光2019

    • Author(s)
      浜田勝平、松井大海、小野篤史、居波渉、川田善正、吉澤雅幸、杉田 篤史
    • Organizer
      2019年応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] FTC非線形光学色素における無電界ポーリング現象に関する研究2018

    • Author(s)
      杉浦真子、菊地康平、木下雄太、吉村智之、松尾淳一、杉田篤史
    • Organizer
      2018年第78回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 一次元・二次元金ナノ粒子配列系表面での有機色素分子のSERS現象2018

    • Author(s)
      泉彩加、熊岡健太郎、岸口光一、二橋俊介、杉田篤史
    • Organizer
      2018年第78回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 金ナノディスク系のフェムト秒時間分解吸収分光2018

    • Author(s)
      浜田勝平、余語宏文、松井大海、小野篤史、居波渉、川田善正、吉澤雅幸、杉田篤史
    • Organizer
      2018年第78回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 非線形光学ポリマー/金ナノ粒子複合系における非線形性の励起波長依存性2018

    • Author(s)
      奥村巧樹、蒔山拓海、佐藤光、小野篤史、居波渉、川田善正、杉田 篤史
    • Organizer
      2018年第78回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 表面プラズモン共鳴励起された金ナノディスクのフェムト秒時間分解吸収分光2018

    • Author(s)
      杉田篤史、余語宏文、浜田勝平、松井大海、小野篤史、居波渉、川田善正、吉澤正幸
    • Organizer
      日本物理学会第73回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Amplifying LSP-enhanced nonlinearities with NLO polymers2018

    • Author(s)
      A. Sugita, K. Kishiguchi, S. Kohei, A. Ono, I. Wataru and Y. Kawata
    • Organizer
      The 15th Conference on near-field optics, nanophotonics and related topics NFO1
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Excitation Light-Induced Anisotropies in LSP-Enhanced SHG from Au Nanoprisms2018

    • Author(s)
      Atsushi Sugita, Hirofumi Yogo, Shohei Hamada, Atsushi Ono and Yoshimasa Kawata
    • Organizer
      CLEO:2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 金ナノ正三角柱における高密度励起条件下でのSHG現象2018

    • Author(s)
      杉田篤史, 余語宏文, 浜田勝平, 小野篤史, 川田善正
    • Organizer
      日本物理学会第73回年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] LSP共鳴励起した非対称金ナノロッド二量体系の二次非線形光学効果2018

    • Author(s)
      2.奥村巧樹、余語宏文、小野篤史、川田善正、居波渉、杉田 篤史
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 非線形光学プッシュ-プル型色素の表面増強ラマン散乱現象2018

    • Author(s)
      泉彩加、熊岡健太郎、岸口光一、佐藤浩平、間瀬暢之、杉田篤史
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Polarization dependent second harmonic generations of equilateral triangular Au nanotriangles at localized surface plasmon resonances2017

    • Author(s)
      1.Atsushi Sugita, Hirofumi Yogo, Atsushi Ono, and Yoshimasa Kawata
    • Organizer
      Plasmonics: Design, Materials, Fabrications, 10346-99, Characterization and Applications XV, SPIE.Optics+Photnics 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 20-fold additional increases in LSP-enhanced SHG of Au nanoparticles with NLO polymers2017

    • Author(s)
      Atsushi Sugita, Tatsuya Matsui, Atsushi Ono, Yoshimasa Kawata
    • Organizer
      CLEO/Europe-EQEC 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] SHG spectroscopy for three-fold rotationally symmetric Au triangular nanoprism at LSP resonances2017

    • Author(s)
      3.Atsushi Sugita, Hirofumi Yogo, Atsushi Ono, and Yoshimasa Kawata,
    • Organizer
      CLEO:2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 非対称金ナノ粒子二量体系の第二高調波発生現象2017

    • Author(s)
      杉田篤史, 奥村功樹, 余語宏文, 小野篤史, 川田善正
    • Organizer
      日本物理学会 2017年秋季大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] SHG自己相関分光による局在表面プラズモン分極の動力学に関する研究2017

    • Author(s)
      余語宏文、小野篤史、川田善正、杉田篤史
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] NLO色素の表面増強ラマン散乱に関する研究2017

    • Author(s)
      泉彩加、熊岡健太郎、岸口光一、佐藤浩平、杉田 篤史
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 非対称金ナノロッド二量体系の第二高調波現象2017

    • Author(s)
      奥村巧樹、余語宏文、小野篤史、川田善正、杉田 篤史
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 表面プラズモン共鳴したNLOポリマー/金ナノ粒子系における二次非線形性増強化機構に関する研究"、7pA-405-9、2017

    • Author(s)
      岸口光一、松井達也、佐藤浩平、小野篤史、下村勝、間瀬暢之、川田善正、杉田篤史
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report

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Published: 2017-04-28   Modified: 2021-02-19  

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