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The interaction between air pollutants and Asian dust

Research Project

Project/Area Number 17K08388
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Environmental and hygienic pharmacy
Research InstitutionKanazawa University

Principal Investigator

Tang Ning  金沢大学, 環日本海域環境研究センター, 准教授 (90372490)

Co-Investigator(Kenkyū-buntansha) 早川 和一  金沢大学, その他部局等, 名誉教授 (40115267)
鳥羽 陽  金沢大学, 薬学系, 准教授 (50313680)
Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2019: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2018: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2017: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywords大気汚染 / 黄砂 / 多環芳香族炭化水素 / 吸着 / 越境輸送 / 大気環境 / 触媒反応
Outline of Final Research Achievements

With the cooperation of Japan, China, and South Korea, we collected air pollutants including PM2.5 at atmospheric monitoring stations in Lanzhou, Beijing, Seoul, and the Noto Peninsula during summer, winter, and Asian dust periods. Then, we analyzed PAHs in PM2.5 and several gaseous pollutants. The results show that the concentration of air pollutants in all regions decreased year by year, which was attributed to the effective control measures adopted by these countries. In the meantime, air pollutants transported to Japan over long distances have also been significantly reduced. In addition, the interaction between PAHs and Kosa particles collected from typical deserts in China was studied in the developed exposure chamber under different conditions (such as acidic and alkaline conditions). The results show that Kosa particles had no substantial effect on the chemical reaction of PAHs.

Academic Significance and Societal Importance of the Research Achievements

本研究で得られたデータより,蘭州の大気汚染実態は初めて明らかにした。同時に,過去の結果も含めて詳細に解析することにより,中国国内のPM2.5の発生,輸送と推移及びそれらを引き起す主要因を総括的に明らかにすることができた。また,本研究の実施により実大気中におけるPAHsの酸化メカニズムと黄砂の寄与を解明するために一歩前進することができた。さらに,本研究で得られた成果は,黄砂飛行ルート上にある東アジア地域の国々の大気汚染対策を進める上で不可欠な科学的知見を提供し,同じく黄砂被害に直面しているアフリカやニュージーランドに価値のある参考データを提供することができた。

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (36 results)

All 2020 2019 2018 2017 Other

All Int'l Joint Research (7 results) Journal Article (18 results) (of which Int'l Joint Research: 16 results,  Peer Reviewed: 17 results,  Open Access: 12 results) Presentation (10 results) (of which Int'l Joint Research: 1 results,  Invited: 1 results) Book (1 results)

  • [Int'l Joint Research] 蘭州大学/中国科学院生態環境研究センター/中国環境科学研究院(中国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] 北京大学(中国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] 韓国外国語大学/ソウル大学(韓国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] 蘭州大学/北京大学/中国科学院 生態環境研究センター(中国)

    • Related Report
      2018 Research-status Report
  • [Int'l Joint Research] 忠北大学校(韓国)

    • Related Report
      2018 Research-status Report
  • [Int'l Joint Research] 蘭州大学/中国科学院生態環境研究センター/中国環境科学研究院(中国)

    • Related Report
      2017 Research-status Report
  • [Int'l Joint Research] 北京大学(中国)

    • Related Report
      2017 Research-status Report
  • [Journal Article] Calculating sources of combustion-derived particulates using 1-nitropyrene and pyrene as markers2020

    • Author(s)
      Hayakawa Kazuichi、Tang Ning、Toriba Akira、Nagato Edward G.
    • Journal Title

      Environmental Pollution

      Volume: in press Pages: 114730-114730

    • DOI

      10.1016/j.envpol.2020.114730

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Comparison of Transcriptomics Changes Induced by TCS and MTCS Exposure in Human Hepatoma HepG2 Cells2020

    • Author(s)
      Li Xiaoqian、Shang Yu、Yao Weiwei、Li Yi、Tang Ning、An Jing、Wei Yongjie
    • Journal Title

      ACS Omega

      Volume: 5 Issue: 19 Pages: 10715-10724

    • DOI

      10.1021/acsomega.0c00075

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Natural aeolian dust particles have no substantial effect on atmospheric polycyclic aromatic hydrocarbons (PAHs): A laboratory study based on naphthalene2020

    • Author(s)
      Zhang Lulu、Zhang Xuan、Xing Wanli、Zhou Quanyu、Yang Lu、Nakatsubo Ryohei、Wei Yongjie、Bi Jianrong、Shima Masayuki、Toriba Akira、Hayakawa Kazuichi、Tang Ning
    • Journal Title

      Environmental Pollution

      Volume: 263 Pages: 114454-114454

    • DOI

      10.1016/j.envpol.2020.114454

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] PM2.5-bound polycyclic aromatic hydrocarbons and nitro-polycyclic aromatic hydrocarbons inside and outside a primary school classroom in Beijing: Concentration, composition, and inhalation cancer risk2020

    • Author(s)
      Zhang Lulu、Morisaki Hiroshi、Wei Yongjie、Li Zhigang、Yang Lu、Zhou Quanyu、Zhang Xuan、Xing Wanli、Hu Min、Shima Masayuki、Toriba Akira、Hayakawa Kazuichi、Tang Ning
    • Journal Title

      Science of The Total Environment

      Volume: 705 Pages: 135840-135840

    • DOI

      10.1016/j.scitotenv.2019.135840

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Characteristics of Polycyclic Aromatic Hydrocarbons (PAHs) and Common Air Pollutants at Wajima, a Remote Background Site in Japan2020

    • Author(s)
      Zhang Xuan、Zhang Lulu、Yang Lu、Zhou Quanyu、Xing Wanli、Toriba Akira、Hayakawa Kazuichi、Wei Yongjie、Tang Ning
    • Journal Title

      International Journal of Environmental Research and Public Health

      Volume: 17 Issue: 3 Pages: 957-957

    • DOI

      10.3390/ijerph17030957

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Characteristics of PM2.5-Bound Polycyclic Aromatic Hydrocarbons and Nitro-Polycyclic Aromatic Hydrocarbons at A Roadside Air Pollution Monitoring Station in Kanazawa, Japan2020

    • Author(s)
      Xing Wanli、Zhang Lulu、Yang Lu、Zhou Quanyu、Zhang Xuan、Toriba Akira、Hayakawa Kazuichi、Tang Ning
    • Journal Title

      International Journal of Environmental Research and Public Health

      Volume: 17 Issue: 3 Pages: 805-805

    • DOI

      10.3390/ijerph17030805

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Long-Term Trends in Urban Atmospheric Polycyclic Aromatic Hydrocarbons and Nitropolycyclic Aromatic Hydrocarbons: China, Russia, and Korea from 1999 to 20142020

    • Author(s)
      Hayakawa Kazuichi、Tang Ning、Nagato Edward、Toriba Akira、Lin Jin-Min、Zhao Lixia、Zhou Zhijun、Qing Wu、Yang Xiaoyang、Mishukov Vassily、Neroda Andrey、Chung Hae-Young
    • Journal Title

      International Journal of Environmental Research and Public Health

      Volume: 17 Issue: 2 Pages: 431-431

    • DOI

      10.3390/ijerph17020431

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Characteristics and health risks of particulate polycyclic aromatic hydrocarbons and nitro-polycyclic aromatic hydrocarbons at urban and suburban elementary schools in Shanghia2019

    • Author(s)
      L. Zhang, T. Tokuda, L. Yang, Q. Zhou, X. Zhang, W. Xing, Q. Wu, Z. Zhou, R. Chen, T. Kameda, A. Toriba, K. Hayakawa, N. Tang
    • Journal Title

      Asian J.Atmos. Environ.

      Volume: 13 Issue: 4 Pages: 266-275

    • DOI

      10.5572/ajae.2019.13.4.266

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Characteristics of air pollutants inside and outside a primary school classroom in Beijing and respiratory health impact on children2019

    • Author(s)
      Zhang Lulu、Morisaki Hiroshi、Wei Yongjie、Li Zhigang、Yang Lu、Zhou Quanyu、Zhang Xuan、Xing Wanli、Hu Min、Shima Masayuki、Toriba Akira、Hayakawa Kazuichi、Tang Ning
    • Journal Title

      Environmental Pollution

      Volume: 255 Pages: 113147-113147

    • DOI

      10.1016/j.envpol.2019.113147

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] The Characteristics of Polycyclic Aromatic Hydrocarbons in Different Emission Source Areas in Shenyang, China2019

    • Author(s)
      Yang Lu、Suzuki Genki、Zhang Lulu、Zhou Quanyu、Zhang Xuan、Xing Wanli、Shima Masayuki、Yoda Yoshiko、Nakatsubo Ryohei、Hiraki Takatoshi、Sun Baijun、Fu Wenhua、Qi Hongye、Hayakawa Kazuichi、Toriba Akira、Tang Ning
    • Journal Title

      International Journal of Environmental Research and Public Health

      Volume: 16 Issue: 16 Pages: 2817-2817

    • DOI

      10.3390/ijerph16162817

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Identification of Long-Range Transported Polycyclic Aromatic Hydrocarbons in Snow at Mt. Tateyama, Japan2018

    • Author(s)
      Hayakawa Kazuichi、Tang Ning、Nagato Edward G.、Toriba Akira、Aoki Kazuma
    • Journal Title

      Aerosol and Air Quality Research

      Volume: 印刷中 Issue: 6 Pages: 1252-1258

    • DOI

      10.4209/aaqr.2018.05.0153

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Characterization and Risk Assessment of Atmospheric PM2.5 and PM10 Particulate-Bound PAHs and NPAHs in Rwanda, Central-East Africa2018

    • Author(s)
      Kalisa Egide、Nagato Edward G.、Bizuru Elias、Lee Kevin C.、Tang Ning、Pointing Stephen B.、Hayakawa Kazuichi、Archer Stephen D. J.、Lacap-Bugler Donnabella C.
    • Journal Title

      Environmental Science & Technology

      Volume: 52 Issue: 21 Pages: 12179-12187

    • DOI

      10.1021/acs.est.8b03219

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] A Comparison of Particulate-Bound Polycyclic Aromatic Hydrocarbons Long-Range Transported from the Asian Continent to the Noto Peninsula and Fukue Island, Japan2018

    • Author(s)
      Yang Lu、Tang Ning、Matsuki Atsushi、Takami Akinori、Hatakeyama Shiro、Kaneyasu Naoki、Nagato Edward G.、Sato Kei、Yoshino Ayako、Hayakawa Kazuichi
    • Journal Title

      Asian Journal of Atmospheric Environment

      Volume: 12 Issue: 4 Pages: 369-376

    • DOI

      10.5572/ajae.2018.12.4.369

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Direct evidence for surface long-lived superoxide radicals photo-generated in TiO2 and other metal oxide suspensions2018

    • Author(s)
      Wang Dabin、Zhao Lixia、Wang Dan、Yan Li、Jing Chuanyong、Zhang Hui、Guo Liang-Hong、Tang Ning
    • Journal Title

      Physical Chemistry Chemical Physics

      Volume: 20 Issue: 28 Pages: 18978-18985

    • DOI

      10.1039/c8cp03081b

    • Related Report
      2018 Research-status Report
  • [Journal Article] Long term trends in atmospheric concentrations of polycyclic aromatic hydrocarbons and nitropolycyclic aromatic hydrocarbons: A study of Japanese cities from 1997 to 20142018

    • Author(s)
      Hayakawa Kazuichi、Tang Ning、Nagato Edward Gou、Toriba Akira、Sakai Shigekatsu、Kano Fumio、Goto Sumio、Endo Osamu、Arashidani Kei-ichi、Kakimoto Hitoshi
    • Journal Title

      Environmental Pollution

      Volume: 233 Pages: 474-482

    • DOI

      10.1016/j.envpol.2017.10.038

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Persistent organic pollutants in red-crowned cranes (Grus japonensis) from Hokkaido, Japan2018

    • Author(s)
      Kakimoto Kensaku、Akutsu Kazuhiko、Nagayoshi Haruna、Konishi Yoshimasa、Kajimura Keiji、Tsukue Naomi、Yoshino Tomoo、Matsumoto Fumio、Nakano Takeshi、Tang Ning、Hayakawa Kazuichi、Toriba Akira
    • Journal Title

      Ecotoxicology and Environmental Safety

      Volume: 147 Pages: 367-372

    • DOI

      10.1016/j.ecoenv.2017.08.060

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Personal inhalation exposure to polycyclic aromatic hydrocarbons and their nitro-derivatives in rural residents in northern Thailand2017

    • Author(s)
      Orakij Walaiporn、Chetiyanukornkul Thaneeya、Chuesaard Thanyarat、Kaganoi Yuichi、Uozaki Waka、Homma Chiharu、Boongla Yaowatat、Tang Ning、Hayakawa Kazuichi、Toriba Akira
    • Journal Title

      Environmental Monitoring and Assessment

      Volume: 189 Issue: 10 Pages: 510-510

    • DOI

      10.1007/s10661-017-6220-z

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Atmospheric behaviors of particulate-bound polycyclic aromatic hydrocarbons and nitropolycyclic aromatic hydrocarbons in Beijing, China from 2004 to 20102017

    • Author(s)
      N. Tang, G. Suzuki, H. Morisaki, T. Tokuda, X. Yang, L. Zhao, J. Lin, T. Kameda, A. Toriba, K. Hayakawa
    • Journal Title

      Atmos. Environ.

      Volume: 152 Pages: 354-361

    • DOI

      10.1016/j.atmosenv.2016.12.056

    • NAID

      120005982986

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] 新規NP法を用いた極東アジア都市の大気中PM,PAH及びNPAH類の発生源比較2020

    • Author(s)
      早川和一,唐寧,鳥羽陽
    • Organizer
      日本薬学会第140年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] アジアンダスト共存下における水相中ナフタレンの転化反応2020

    • Author(s)
      張露露,楊露,周全渝,張セン,ケイ万里,魏永杰,閉建栄,中坪良平,島正之,鳥羽陽,早川和一,唐寧
    • Organizer
      日本薬学会第140年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 東アジア地域の大気中多環芳香族類化合物の環境動態2019

    • Author(s)
      唐寧
    • Organizer
      東北大学(中国)
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Acidity of Atmospheric Aerosol Particles at a remote background site, Japan2019

    • Author(s)
      Zhou, Q.Y., Zhang, L.L., Yang, L., Zhang, X., Xing, W.L., Toriba, A., Hayakawa, K., Tang, N.
    • Organizer
      第60回大気環境学会年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Distribution and health risk of indoor and outdoor particulate polycyclic aromatic hydrocarbons of a school classroom in Beijing, China2019

    • Author(s)
      Tang, N., Zhang, L.L., Morizaki, H., Wei, Y.J., Li, Z.G., Yang, L., Zhou, Q.Y., Zhang, X., Xing, W.L., Hu, M., Shima, M., Toriba, A., Hayakawa, K.
    • Organizer
      Joint International Symposium on Sustainable Development and Environmental issues, KU-INET
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 中国北京の2015年冬季における大気粉じんの奨学生への曝露実態及びそれらの肺機能への影響評価2018

    • Author(s)
      張露露,楊露,周全渝,張セン;,森崎博志,島正之,余田佳子,魏永杰,鳥羽陽,早川和一,唐寧
    • Organizer
      日本薬学会第139年会
    • Related Report
      2018 Research-status Report
  • [Presentation] 輪島における大気汚染物質の特徴2018

    • Author(s)
      張セン;,張露露,楊露,周全渝,鳥羽陽,早川和一,唐寧
    • Organizer
      日本薬学会第139年会
    • Related Report
      2018 Research-status Report
  • [Presentation] 水溶液中における異なるタイプの黄砂のナフタレンに対する吸着挙動2018

    • Author(s)
      張露露,楊露,周全渝,魏永杰,胡敏,趙利霞,閉建栄,早川和一,鳥羽陽,唐寧
    • Organizer
      第59回大気環境学会
    • Related Report
      2018 Research-status Report
  • [Presentation] 能登半島の大気中多環芳香族炭化水素類と反応性ガスとの相関解析2017

    • Author(s)
      唐 寧,長門 豪,楊 露,鶴丸 央,猪股弥生,松木 篤,鳥羽 陽,鈴木 亮,早川和一
    • Organizer
      第58回大気環境学会年会
    • Related Report
      2017 Research-status Report
  • [Presentation] 能登半島における大気中有害化学物質の連続観測2017

    • Author(s)
      唐 寧,楊 露,長門 豪,鶴丸 央,猪股弥生,松木 篤,鳥羽 陽,鈴木 亮,早川和一
    • Organizer
      第58回大気環境学会年会
    • Related Report
      2017 Research-status Report
  • [Book] Polycyclic Aromatic Hydrocarbons-Environmental Behavior and Toxicity in East Asia-2018

    • Author(s)
      Hayakawa et al.
    • Total Pages
      271
    • Publisher
      Springer
    • ISBN
      9789811067754
    • Related Report
      2017 Research-status Report

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Published: 2017-04-28   Modified: 2021-02-19  

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